Труды сотрудников ИЛ им. В.Н. Сукачева СО РАН

[Text] / J. . Heintzenberg [et al.] // Atmos. Chem. Phys. - 2011. - Vol. 11, Is. 16. - P8703-8719, DOI 10.5194/acp-11-8703-2011. - Cited References: 65. - The Max Planck Society in collaboration with the V. N. Sukachev Institute of Forest established the ZOTTO facility after many years of preparatory fieldwork, planning and massive investments. We thank E.-D. Schulze and M. Heimann (MPI Biogeochemistry), A. A. Onuchin, and S. Verchovetz, (V. N. Sukachev Institute of Forest) for their contributions to the establishment and management of ZOTTO, and Y. Kisilyakhov, A. Tsukanov (V. N. Sukachev Institute of Forest), M. Welling and N. Jurgens (MPI Chemistry), as well as S. Leinert and T. Muller (IfT) for technical support. The ZOTTO project is funded by the Max Plank Society through the International Science and Technology Center (ISTC) partner project #2757p within the framework of the proposal 'Observing and Understanding Biogeochemical Responses to Rapid Climate Changes in Eurasia', and by the German Research Council (DFG). We thank S. Schmidt and K. Kubler (MPI Jena) for their continuous logistic assistance during the experiment. We acknowledge U. Riebel (Technical University of Cottbus, Chair for Particle Technology) for generously sharing his technology of the corona discharge based aerosol neutralizer. We thank A. Wiedensohler (IfT Leipzig) for the fruitful discussions about environmental aerosol charging. . - 17. - ISSN 1680-7316РУБ Meteorology & Atmospheric Sciences

Аннотация: This paper analyses aerosol particle number size distributions, particulate absorption at 570 nm wavelength and carbon monoxide (CO) measured between September 2006 and January 2010 at heights of 50 and 300 m at the Zotino Tall Tower Facility (ZOTTO) in Siberia (60.8 degrees N; 89.35 degrees E). Average number, surface and volume concentrations are broadly comparable to former studies covering shorter observation periods. Fits of multiple lognormal distributions yielded three maxima in probability distribution of geometric mean diameters in the Aitken and accumulation size range and a possible secondary maximum in the nucleation size range below 25 nm. The seasonal cycle of particulate absorption shows maximum concentrations in high winter (December) and minimum concentrations in mid-summer (July). The 90th percentile, however, indicates a secondary maximum in July/August that is likely related to forest fires. The strongly combustion derived CO shows a single winter maximum and a late summer minimum, albeit with a considerably smaller seasonal swing than the particle data due to its longer atmospheric lifetime. Total volume and even more so total number show a more complex seasonal variation with maxima in winter, spring, and summer. A cluster analysis of back trajectories and vertical profiles of the pseudo-potential temperature yielded ten clusters with three levels of particle number concentration: Low concentrations in Arctic air masses (400-500 cm(-3)), mid-level concentrations for zonally advected air masses from westerly directions between 55 degrees and 65 degrees N (600-800 cm(-3)), and high concentrations for air masses advected from the belt of industrial and population centers in Siberia and Kazakhstan (1200 cm(-3)). The observational data is representative for large parts of the troposphere over Siberia and might be particularly useful for the validation of global aerosol transport models.

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Держатели документа:
[Heintzenberg, J.
Birmili, W.
Otto, R.] Leibniz Inst Tropospher Res, D-04318 Leipzig, Germany
[Andreae, M. O.
Mayer, J. -C.
Chi, X.] Max Planck Inst Chem, D-55020 Mainz, Germany
[Panov, A.] Russian Acad Sci, Siberian Branch, VN Sukachev Inst Forest, Krasnoyarsk 660036, Russia

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Heintzenberg, J...; Birmili, W...; Otto, R...; Andreae, M.O.; Mayer, J.C.; Chi, X...; Panov, A...