Рубрики:
BACTERIUM RHODOPSEUDOMONAS-VIRIDIS
PRIMARY CHARGE SEPARATION
AMINO-ACID-SEQUENCE
BACTERIOPHEOPHYTIN
RELAXATION
SUBUNIT
DONOR
MODEL
Кл.слова (ненормированные):
Electron transfer -- External fields -- Fast electron transport -- Initial conditions -- Non equilibrium -- Path-integral -- Perturbation theory -- Photosynthetic reaction center -- Second orders -- Time convolution -- Vibrational modes -- Electron transitions -- Perturbation techniques -- Quantum chemistry -- Photosynthesis
BACTERIUM RHODOPSEUDOMONAS-VIRIDIS
PRIMARY CHARGE SEPARATION
AMINO-ACID-SEQUENCE
BACTERIOPHEOPHYTIN
RELAXATION
SUBUNIT
DONOR
MODEL
Кл.слова (ненормированные):
Electron transfer -- External fields -- Fast electron transport -- Initial conditions -- Non equilibrium -- Path-integral -- Perturbation theory -- Photosynthetic reaction center -- Second orders -- Time convolution -- Vibrational modes -- Electron transitions -- Perturbation techniques -- Quantum chemistry -- Photosynthesis
Аннотация: Creation of electrons or excitons by external fields in a system with initially statistically independent unrelaxed vibrational modes leads to an initial condition term. The contribution of this term in the time convolution generalized master-equation approach is studied in the second order of the perturbation theory in path-integral formalism. The developed approach, applied for the analysis of dynamics in the photosynthetic reaction center, exhibits the key role of the initial condition terms at the primary stage of electron transfer.
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Держатели документа:
[Pudlak, M.
Pincak, R.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia
[Pichugin, K. N.] LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
[Nazmitdinov, R. G.] Univ Illes Balears, Dept Fis, ES-07122 Palma De Mallorca, Spain
[Nazmitdinov, R. G.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia
ИФ СО РАН
Institute of Experimental Physics, Slovak Academy of Sciences, 04353 Kosice, Slovakia
Kirensky Institute of Physics, Akademgorodok 50/38, 660036 Krasnoyarsk, Russian Federation
Departament de Fisica, Universitat de les Illes Balears, ES-07122 Palma de Mallorca, Spain
Bogoliubov Laboratory of Theoretical Physics, Joint Institute for Nuclear Research, 141980 Dubna, Russian Federation
Доп.точки доступа:
Pudlak, M.; Pichugin, K. N.; Пичугин, Константин Николаевич; Nazmitdinov, R. G.; Pincak, R.