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[Text] / A. E. Ershov [et al.] // Appl. Phys. B-Lasers Opt. - 2014. - Vol. 115, Is. 4. - P. 547-560, DOI 10.1007/s00340-013-5636-6. - Cited References: 48. - Authors are thankful to Prof. V. A. Markel (University of Pennsylvania) for supplying program codes for realization of the coupled dipole method for polydisperse metal nanoparticle aggregates. This research was supported by the Russian Academy of Sciences under the Grants 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101); Ministry of Education and Science of Russian Federation under Contract 14.B37.21.0457. . - ISSN 0946-2171. - ISSN 1432-0649РУБ Optics + Physics, Applied

Аннотация: We propose an optodynamical model of interaction of pulsed laser radiation with aggregates of spherical metallic nanoparticles embedded into host media. The model takes into account polydispersity of particles, pair interactions between the particles, dissipation of absorbed energy, heating and melting of the metallic core of particles and of their polymer adsorption layers, and heat exchange between electron and ion components of the particle material as well as heat exchange with the interparticle medium. Temperature dependence of the electron relaxation constant of the particle material and the effect of this dependence on interaction of nanoparticles with laser radiation are first taken into consideration. We study in detail light-induced processes in the simplest resonant domains of multiparticle aggregates consisting of two particles of an arbitrary size in aqueous medium. Optical interparticle forces are realized due to the light-induced dipole interaction. The dipole moment of each particle is calculated by the coupled dipole method (with correction for the effect of higher multipoles). We determined the role of various interrelated factors leading to photomodification of resonant domains and found an essential difference in the photomodification mechanisms between polydisperse and monodisperse nanostructures.

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Держатели документа:
[Ershov, A. E.
Karpov, S. V.
Semina, P. N.] Russian Acad Sci, LV Kirenski Inst Phys, Krasnoyarsk 660036, Russia
[Gavrilyuk, A. P.] Russian Acad Sci, Inst Computat Modeling, Krasnoyarsk 660036, Russia
[Gavrilyuk, A. P.
Karpov, S. V.] Siberian Fed Univ, Krasnoyarsk 660028, Russia
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Доп.точки доступа:
Ershov, A.E.; Gavrilyuk, A.P.; Гаврилюк, Анатолий Петрович; Karpov, S.V.; Semina, P.N.; Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101)]; Ministry of Education and Science of Russian Federation [14.B37.21.0457]