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Low-field electron emission of diamond/pyrocarbon composites / A. V. Karabutov [et al.] // Journal of Vacuum Science and Technology B: Microelectronics and Nanometer Structures. - 2001. - Vol. 19: 13th International Vaccum Microelectronics Conference (14 August 2000 through 17 August 2000, Guangzhou, Is. 3. - P965-970, DOI 10.1116/1.1368669 . - ISSN 1071-1023
Кл.слова (ненормированные):
Carbon nanotubes -- Chemical bonds -- Chemical vapor deposition -- Composite materials -- Diamond films -- Electric conductivity -- Electron emission -- Electron energy levels -- Hysteresis -- Interfaces (materials) -- Raman scattering -- Semiconducting diamonds -- Semiconductor quantum wells -- Transmission electron microscopy -- X ray diffraction analysis -- X ray photoelectron spectroscopy -- Pyrocarbon composites -- Nanostructured materials
Аннотация: The properties of field electron emission for diamond/pyrocarbon nanocomposites produced from diamond particles surrounded by a pyrocarbon matrix were studied. Low-threshold emissions at fields of ?1 V/?m with no activation or hysterisis in the current versus voltage (I/V) behaviour were observed for the materials. Scanning tunneling-field emission microscopy was used to study the mechanisms of low-field electron emission from the composites, and a model based on quantum well effect at the diamond/graphite interface was proposed and discussed.

Scopus
Держатели документа:
General Physics Institute, Vavilova str. 38, Moscow 117942, Russian Federation
Central Research Institute of Materials, Paradnaya str. 8, St. Petersburg 191014, Russian Federation
Institute of Biophysics, Krasnoyarsk 660036, Russian Federation : 660036, Красноярск, Академгородок, д. 50, стр. 50

Доп.точки доступа:
Karabutov, A.V.; Frolov, V.D.; Konov, V.I.; Ralchenko, V.G.; Gordeev, S.K.; Belobrov, P.I.

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Microencapculation of daunorubicin with biodegradable polymer matrix / E. I. Shishatskaya // Antibiotiki i Khimioterapiya. - 2007. - Vol. 52, Is. 9-10. - С. 3-8 . - ISSN 0235-2990
Кл.слова (ненормированные):
Daunorubicin -- Microencapsulation -- Polymer matrix -- antineoplastic antibiotic -- daunorubicin -- polyester -- animal -- article -- Bagg albino mouse -- chemistry -- kinetics -- microcapsule -- mouse -- particle size -- Animals -- Antibiotics, Antineoplastic -- Capsules -- Daunorubicin -- Kinetics -- Mice -- Mice, Inbred BALB C -- Particle Size -- Polyesters -- Animalia
Аннотация: Procedure for microencapsulation providing stable formation of high quality microspheres was designed. Conditions for deposition of the anthracycline antibiotic daunorubicin to polymer matrix were developed and microsheres loaded with various quantities of the drug were prepared. The kinetics of the in vitro and in vivo release of daunorubicin from the microsheres was studied. The rate of the rubomycin release to the medium in vitro (balanced phosphate buffer at 37.8В°C) in a 300-hour experiment directly depended on the quantity of the incorporated drug and averaged 0.81 В· 10 -4 to 2.3 В· 10 -4 mcg/mlВ·h. The experiment on laboratory animals with intraperitoneal administration of the rubomycin microsperes showed that the drug remained in the blood and abdominal liquid for a long time (up to 10 days). Possible control of the quantity of the rubomycin encapsulation to the polymer matrix, no sharp efflux of the drug at the early stages of the observation and low rate of the drug release to the medium allowed to conclude that the use of the biodegradable polymer microsperes as carriers of the high toxic antibiotic providing its prolonged action was prospective.

Scopus
Держатели документа:
Institute of Biophysics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, Russian Federation : 660036, Красноярск, Академгородок, д. 50, стр. 50

Доп.точки доступа:
Shishatskaya, E.I.

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Characterization of polymeric microparticles based on resorbable polyesters of oxyalkanoic acids as a platform for deposition and delivery of drugs / A. V. Goreva [et al.] // Polym. Sci. Ser. A. - 2012. - Vol. 54, Is. 2. - P94-105, DOI 10.1134/S0965545X12020022. - Cited References: 33. - This work was supported by the program for Support of Leading Scientific Schools of the Russian Federation (project no. 11.G34.31.0013.2010, Biotechnology of New Biomaterials) and the program of integrated studies of the Presidium of the Siberian Branch, Russian Academy of Sciences (project no. 93). . - 12. - ISSN 0965-545X

РУБ Polymer Science
Рубрики:
IN-VITRO RELEASE
   POLYHYDROXYBUTYRATE MICROSPHERES
   BLENDS
   RIFAMPICIN
   BIOCOMPATIBILITY
   DEGRADATION
   FORMULATION
   COMPOSITE
   CARRIERS
   MODEL
Аннотация: The effect of the preparation technique (chemical composition of a polymer, type and method of emulsion mixing, and molecular mass of a drug) on the yield, structure, and size of microparticles obtained from resorbable polyesters of microbiological origin, polyhydroxyalkanoates, is studied. It is found that the concentration of the polymer solution and the method of emulsion mixing are the most significant factors affecting the diameter of microparticles based on polyhydroxyalkanoates; the surface structure of particles depends to a higher extent on the chemical composition of the polymer. The family of microparticles from 100-200 nm to 50-70 mu m in diameter is synthesized. It is shown that the rate of drug release from microparticles in vitro into the medium is higher in the case of 3-hydroxybutyrate copolymers with 3-hydroxyvalerate than in the case of the homopolymer of 3-hydroxybutyrate. This parameter increases with the content of 3-hydroxyvalerate units in the copolymer and the porosity and mass fraction of the drug in particles with a decrease in their sizes. For in vitro systems containing a phosphate buffer, variation in the preparation parameters makes it possible to obtain microparticles with various characteristics suitable for deposition of drugs. For microparticles obtained from polyhydroxyalkanoates and having different diameters, the mathematical description of the kinetics of drug release from the polymer matrix is provided.

Держатели документа:
[Goreva, A. V.
Shishatskaya, E. I.
Volova, T. G.] Russian Acad Sci, Siberian Branch, Inst Biophys, Krasnoyarsk 660036, Russia
[Shishatskaya, E. I.
Volova, T. G.] Siberian Fed Univ, Inst Fundamental Biol & Biotechnol, Krasnoyarsk 660041, Russia
[Goreva, A. V.
Sinskey, A. J.] MIT, Cambridge, MA 02139 USA : 660036, Красноярск, Академгородок, д. 50, стр. 50

Доп.точки доступа:
Goreva, A.V.; Shishatskaya, E.I.; Volova, T.G.; Sinskey, A.J.

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Characterization of field emission cathodes with different forms of diamond coatings [Text] / V. V. Zhirnov [et al.] // J. Vac. Sci. Technol. B. - 1999. - Vol. 17: 11th International Vacuum Microelectronics Conference (IVMC 98) (JUL 19-23, 1998, ASHEVILLE, NORTH CAROLINA), Is. 2. - P666-669, DOI 10.1116/1.590614. - Cited References: 9 . - 4. - ISSN 1071-1023

РУБ Engineering, Electrical & Electronic + Nanoscience & Nanotechnology + Physics, Applied
Рубрики:
TIPS
   SILICON
   GROWTH
   ARRAYS
   FILMS
Аннотация: The emission of different, diamond coatings on silicon field emitter. arrays were investigated: chemical vapor deposition diamond, high pressure and high temperature synthetic diamond, and shock-synthesized nanodiamond. Practical emission characteristics such as: emission threshold, maximum current, current stability, and reproducibility were tested. The effects of surface modification, the size of diamond crystallites, and hydrogen plasma treatments were also studied. (C) 1999 American Vacuum Society. [S0734-211X(99)06102-8].

Держатели документа:
Inst Crystallog, Moscow 117333, Russia
Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland
Russian Fed Nucl Ctr, Snezhinsk 456770, Russia
Inst Biophys, Krasnoyarsk 660036, Russia : 660036, Красноярск, Академгородок, д. 50, стр. 50

Доп.точки доступа:
Zhirnov, V.V.; Kuttel, O.M.; Groning, O...; Alimova, A.N.; Detkov, P.Y.; Belobrov, P.I.; Maillard-Schaller, E...; Schlapbach, L...

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Low-field electron emission of diamond/pyrocarbon composites [Text] / A. V. Karabutov [et al.] // J. Vac. Sci. Technol. B. - 2001. - Vol. 19: 13th International Vacuum Microlectronics Conference (AUG 13-17, 2000, GUANGZHOU, PEOPLES R CHINA), Is. 3. - P. 965-970, DOI 10.1116/1.1368669. - Cited References: 31 . - ISSN 1071-1023

РУБ Engineering, Electrical & Electronic + Nanoscience & Nanotechnology + Physics, Applied
Рубрики:
CVD DIAMOND FILMS
   SCANNING-TUNNELING-MICROSCOPY
   AMORPHOUS-CARBON
   COLD-CATHODE
Аннотация: Properties of the field electron emission for diamond/pyrocarbon nanocomposites produced from diamond particles surrounded by an sp(2)-bonded pyrocarbon matrix are considered as functions of a size of diamond particles selected in the range of 5 nm - 5 mum, and of an average thickness of the pyrocarbon shell controlled by the pyrocarbon/diamond mass ratio varied from 0 to 0.5. The low-threshold emission at fields of greater than or equal to1 V/mum with ''no activation/no hysteresis'' I-V behavior was observed for these materials using tungsten tip microprobes as well as a fluorescent screen. A specially designed scanning tunneling-field emission microscope was used for simultaneous mapping of field emission intensity, topography, work function, and electrical resistivity to study the mechanisms of the emission from the composites and well-emitting chemical vapor deposition diamond films. It was found that for both of the materials emission centers are associated with interfaces between diamond and sp2-bonded carbon phases. Possible mechanisms of the low-field electron emission for the diamond/graphite composites including local field enhancement are analyzed. A model of the low-field emission based on quantum well effect at the diamond/graphite interface is proposed and discussed. (C) 2001 American Vacuum Society.

WOS
Держатели документа:
Russian Acad Sci, Inst Gen Phys, Moscow 117942, Russia
Cent Res Inst Mat, St Petersburg, Russia
Russian Acad Sci, Inst Biophys, Krasnoyarsk 660036, Russia
ИБФ СО РАН : 660036, Красноярск, Академгородок, д. 50, стр. 50

Доп.точки доступа:
Karabutov, A.V.; Frolov, V.D.; Konov, V.I.; Ralchenko, V.G.; Gordeev, S.K.; Belobrov, P.I.

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Ni2+-zeolite/ferrosphere and Ni2+-silica/ferrosphere beads for magnetic affinity separation of histidine-tagged proteins / T. A. Vereshchagina [et al.] // Dalton Trans. - 2016. - Vol. 45, Is. 4. - P1582-1592, DOI 10.1039/c5dt03827h . - ISSN 1477-9226
Кл.слова (ненормированные):
Alkalinity -- Amino acids -- Chemical modification -- Fly ash -- Hydrothermal synthesis -- Ion exchange -- Magnetic separation -- Magnetism -- Proteins -- Silica -- Zeolites -- Conventional methods -- Core shell structure -- Green fluorescent protein -- Histidine-tagged proteins -- Hydrothermal treatments -- Magnetic affinity -- Mesoporous Silica -- Sorption capacities -- Nickel
Аннотация: Magnetic Ni2+-zeolite/ferrosphere and Ni2+-silica/ferrosphere beads (Ni-ferrosphere beads - NFB) of a core-shell structure were synthesized starting from coal fly ash ferrospheres having diameters in the range of 0.063-0.050 mm. The strategy of NFB fabrication is an oriented chemical modification of the outer surface preserving the magnetic core of parent beads with the formation of micro-mesoporous coverings. Two routes of ferrosphere modification were realized, such as (i) hydrothermal treatment in an alkaline medium resulting in a NaP zeolite layer and (ii) synthesis of micro-mesoporous silica on the glass surface using conventional methods. Immobilization of Ni2+ ions in the siliceous porous shell of the magnetic beads was carried out via (i) the ion exchange of Na+ for Ni2+ in the zeolite layer or (ii) deposition of NiO clusters in the zeolite and silica pores. The final NFB were tested for affinity in magnetic separation of the histidine-tagged green fluorescent protein (GFP) directly from a cell lysate. Results pointed to the high affinity of the magnetic beads towards the protein in the presence of 10 mM EDTA. The sorption capacity of the ferrosphere-based Ni-beads with respect to GFP was in the range 1.5-5.7 mg cm-3. © The Royal Society of Chemistry.

Scopus,
WOS
Держатели документа:
Institute of Chemistry and Chemical Technology SB RAS, 50/24 Akademgorodok, Krasnoyarsk, Russian Federation
Institute of Biophysics SB RAS, 50/50 Akademgorodok, Krasnoyarsk, Russian Federation
Siberian Federal University, 79 Svobodnyi Avenue, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Vereshchagina, T. A.; Fedorchak, M. A.; Sharonova, O. M.; Fomenko, E. V.; Shishkina, N. N.; Zhizhaev, A. M.; Kudryavtsev, A. N.; Frank, L. A.; Anshits, A. G.

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Detonation Nanodiamond-Assisted Carbon Nanotube Growth by Hot Filament Chemical Vapor Deposition / I. P. Kudarenko [et al.] // Phys. Status Solidi B-Basic Solid State Phys. - 2018. - Vol. 255, Is. 1. - Ст. 1700286, DOI 10.1002/pssb.201700286. - Cited References:28. - The work was supported by RSF project 17-72-10173. . - ISSN 0370-1972. - ISSN 1521-3951

РУБ Physics, Condensed Matter
Рубрики:
DIAMOND
   FILMS
   HFCVD
   FABRICATION
   GRAPHITE
   SCIENCE
   SIZE
   CVD
Кл.слова (ненормированные):
carbon nanotubes -- catalytic growth -- diamond -- hot filament chemical vapor -- deposition -- nanomaterials -- synthesis
Аннотация: Substrates pretreatment in suspensions of a detonation nanodiamond is widely used for nucleation of diamond growth by chemical vapor deposition (CVD). We found that iron inclusions in the nanodiamond provide catalytical growth of carbon nanotubes during CVD in a hot filament reactor (HF CVD). Carbon nanotubes grow in the area between two adjacent Si wafers. The diameters of such obtained nanotubes were in the range of 10-100 nm and the length of the tubes reaches about 10 mu m. The proposed HF CVD method has convincing potential for the fabrication of carbon nanotube coatings on a large surface area.

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Держатели документа:
Moscow MV Lomonosov State Univ, Dept Phys, Moscow 119991, Russia.
Univ Eastern Finland, Dept Phys & Math, Joensuu 80101, Finland.
RAS, Fed Sci Res Ctr Crystallog & Photon, AV Shubnikov Inst Crystallog, Moscow 119333, Russia.
Natl Res Ctr, Kurchatov Inst, Moscow 123182, Russia.
Russian Acad Sci, Krasnoyarsk Sci Ctr SB RAS, Fed Res Ctr, Inst Biophys, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kudarenko, Ilya P.; Malykhin, Sergei A.; Orekhov, Andrey S.; Puzyr, Aleksey P.; Kleshch, Victor I.; Ismagilov, Rinat R.; Obraztsov, Alexander N.; RSF [17-72-10173]

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Preparation, structure and magnetic properties of synthetic ferrihydrite nanoparticles / S. V. Stolyar [et al.] // Journal of Physics: Conference Series : Institute of Physics Publishing, 2018. - Vol. 994: 3rd International School and Workshop on Complex and Magnetic Soft Matter Systems: Structure and Physico - Mechanical Properties, CMSMS 2017 (28 June 2017 through 30 June 2017, ) Conference code: 135760, Is. 1, DOI 10.1088/1742-6596/994/1/012003
Кл.слова (ненормированные):
Magnetic properties -- Mechanical properties -- Nanoparticles -- Powders -- Sols -- Solutions -- Arabinogalactan -- Chemical deposition method -- Fe-ions -- Ferrihydrites -- Metallic state -- Nanoparticle sizes -- Superparamagnetics -- Ultrasonic treatments -- Nanomagnetics
Аннотация: Superparamagnetic ferrihydrite powders with average nanoparticle sizes of 2.5 nm produced by the chemical deposition method. Static and dynamic magnetic properties are measured. As a result of ultrasonic treatment in the cavitation regime of suspensions of ferrihydrite powders in a solution of the albumin protein, the Fe ions are reduced to the metallic state. A sol of ferrihydrite nanoparticles is prepared in an aqueous solution of arabinogalactan polysaccharide. © Published under licence by IOP Publishing Ltd.

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Держатели документа:
Siberian Federal University, Krasnoyarsk, Russian Federation
Kirensky Institute of Physics, SB RAS, Krasnoyarsk, Russian Federation
International Scientific Centre for Organism Extreme States Research Attached Presidium of KSC, SB RAS, Krasnoyarsk, Russian Federation
Institute of Biophysics, SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Stolyar, S. V.; Yaroslavtsev, R. N.; Bayukov, O. A.; Balaev, D. A.; Krasikov, A. A.; Iskhakov, R. S.; Vorotynov, A. M.; Ladygina, V. P.; Purtov, K. V.; Volochaev, M. N.

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Production and characterization of bioaerosols for model validation in spacecraft environment / A. Salmela [et al.] // J. Environ. Sci. - 2018. - Vol. 69. - P227-238, DOI 10.1016/j.jes.2017.10.016. - Cited References:28. - The research leading to these results has received funding from the European Union Seventh Framework Programme (FP/2007-2013) under grant agreement number 263076 within the BIOSMHARS Project (BIO contamination Specific Modeling in Habitats Related to Space). . - ISSN 1001-0742. - ISSN 1878-7320

РУБ Environmental Sciences
Рубрики:
INDOOR AIR
   MICROBIAL-CONTAMINATION
   BUILDING-MATERIALS
   FUNGAL
Кл.слова (ненормированные):
Bioaerosol -- Modeling -- CFD -- Spacecraft -- Fungi -- Bacteria
Аннотация: This study aimed to evaluate the suitability of two bioaerosol generation systems (dry and wet generation) for the aerosolization of microorganisms isolated from the International Space Station, and to calibrate the produced bioaerosols to fulfill the requirements of computational fluid dynamics model (CFD) validation. Concentration, stability, size distribution, agglomeration of generated bioaerosol and deposition of bioaerosols were analyzed. In addition, the dispersion of non-viable particles in the air was studied. Experiments proved that wet generation from microbial suspensions could be used for the production of well-calibrated and stabile bioaerosols for model validation. For the simulation of the natural release of fungal spores, a dry generation method should be used. This study showed that the used CFD model simulated the spread of non-viable particles fairly well. The mathematical deposition model by Lai and Nazaroff could be used to estimate the deposition velocities of bioaerosols on surfaces, although it somewhat underestimated the measured deposition velocities. (c) 2017 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

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Держатели документа:
Univ Eastern Finland, Dept Environm & Biol Sci, POB 1627, FI-70211 Kuopio, Finland.
VTT Ltd, POB 1300, FI-33100 Tampere, Finland.
Belgian Nucl Res Ctr, Microbiol Unit, B-2400 Mol, Belgium.
Inst Med & Physiol Spatiales, BP 74404, F-31405 Toulouse, France.
Inst Biomed Problems, 76-A Khoroshev Skoye Shosse, RU-123007 Moscow, Russia.
RAS, Inst Biophys SB, RU-660036 Krasnoyarsk, Russia.

Доп.точки доступа:
Salmela, Anniina; Kokkonen, Eero; Kulmala, Ilpo; Veijalainen, Anna-Maria; van Houdt, Rob; Leys, Natalie; Berthier, Audrey; Viacheslav, Ilyin; Kharin, Sergey; Morozova, Julia; Tikhomirov, Alexander; Pasanen, Pertti; Van, Rob; European Union [263076]

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10.

РУБ Chemistry, Inorganic & Nuclear + Environmental Sciences
Рубрики:
CS-137
   FOREST
   RADIOCESIUM
   FUNGI
   ACCUMULATION
   ACCIDENT
Кл.слова (ненормированные):
Bioindicators -- biological half-life -- cesium-137 -- effective half-life -- environmental pollution -- isotope ecology -- mushrooms -- nuclear reactors -- radionuclide concentration -- transfer factor
Аннотация: Cs-137 concentrations were measured in mushrooms in an area affected by radioactive discharges of the Mining-and-Chemical Combine (MCC) (Rosatom, Russia) in 2002-2017. The sources of radionuclides in the study sites were global fallouts and waterborne and airborne radioactive discharges of the MCC. The mushroom species Suillus granulatus and S. luteus showed the highest Cs-137 concentrations (140-7100 Bq kg(-1)) for this area. Over the entire monitoring period, no significant change in Cs-137 concentration was observed in the Suillus spp. samples collected from the sites with the aerial deposition of radionuclides. In the floodplain site with the radionuclide deposition from water and air, a significant decrease in the average Cs-137 concentration was observed in the period between 2004 and 2017: a three-fold decrease in Suillus spp. and a nine-fold decrease in Lactarius deliciosus. The effective half-lives of Cs-137 in fruiting bodies of the mushrooms L. deliciosus and Suillus spp. in this site were 3.6 +/- 0.6 and 9.2 +/- 2.7 years, respectively.

WOS
Держатели документа:
Russian Acad Sci, Fed Res Ctr, Inst Biophys, Siberian Branch,Krasnoyarsk Sci Ctr, Krasnoyarsk, Russia.

Доп.точки доступа:
Dementyev, Dmitry; Bolsunovsky, Alexander

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11.

A long-term study of radionuclide concentrations in mushrooms in the 30-km zone around the Mining-and-Chemical Combine (Russia) / D. Dementyev, A. Bolsunovsky // Isot. Environ. Health Stud. - 2020, DOI 10.1080/10256016.2020.1718124 . - Article in press. - ISSN 1025-6016
Кл.слова (ненормированные):
Bioindicators -- biological half-life -- cesium-137 -- effective half-life -- environmental pollution -- isotope ecology -- mushrooms -- nuclear reactors -- radionuclide concentration -- transfer factor
Аннотация: 137Cs concentrations were measured in mushrooms in an area affected by radioactive discharges of the Mining-and-Chemical Combine (MCC) (Rosatom, Russia) in 2002–2017. The sources of radionuclides in the study sites were global fallouts and waterborne and airborne radioactive discharges of the MCC. The mushroom species Suillus granulatus and S. luteus showed the highest 137Cs concentrations (140–7100 Bq kg?1) for this area. Over the entire monitoring period, no significant change in 137Cs concentration was observed in the Suillus spp. samples collected from the sites with the aerial deposition of radionuclides. In the floodplain site with the radionuclide deposition from water and air, a significant decrease in the average 137Cs concentration was observed in the period between 2004 and 2017: a three-fold decrease in Suillus spp. and a nine-fold decrease in Lactarius deliciosus. The effective half-lives of 137Cs in fruiting bodies of the mushrooms L. deliciosus and Suillus spp. in this site were 3.6 ± 0.6 and 9.2 ± 2.7 years, respectively. © 2020, © 2020 Informa UK Limited, trading as Taylor & Francis Group.

Scopus
Держатели документа:
Institute of Biophysics of the Siberian Branch of the Russian Academy of Sciences, Federal Research Center ‘Krasnoyarsk Science Center SB RAS’, Akademgorodok, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Dementyev, D.; Bolsunovsky, A.

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12.

Analysis of interactions between proteins and small-molecule drugs by a biosensor based on a graphene field-effect transistor / S. C. Xu, T. J. Wang, G. F. Liu [et al.] // Sens. Actuator B-Chem. - 2021. - Vol. 326. - Ст. 128991, DOI 10.1016/j.snb.2020.128991. - Cited References:66. - We are grateful for financial support from the Taishan Scholars Program of Shandong Province (tsqn201812104), the Qingchuang Science and Technology Plan of Shandong Province (2019KJJ017 and 2020KJC004), the National Natural Science Foundation of China (61671107, 62071085, 11704059, and 31802309), and the Youth Innovation Team Lead-Education Project of Shandong Educational Committee. . - ISSN 0925-4005

РУБ Chemistry, Analytical + Electrochemistry + Instruments & Instrumentation
Рубрики:
LABEL-FREE DETECTION
CHEMICAL-VAPOR-DEPOSITION
DNA HYBRIDIZATION
Кл.слова (ненормированные):
Single-crystal graphene -- FET -- Binding kinetics -- LMW drugs -- Imatinib
Аннотация: We synthesized large-area single-crystal graphene sheets to use them in biosensors based on field-effect transistors (FET) for quantitative analysis of interaction kinetics and affinity between the imatinib drug and its target protein kinase Abl1. The G-FET biosensor showed an excellent performance and recognized imatinib at as low as 15.5 fM. The biosensor also showed a linear response to the logarithm of imatinib concentration in the 0.1 pM-10 mu M range. This graphene-based FET biosensor (G-FET) was also applied toquantify Abl1 Y253 F mutation and Abl1 dependency on Mg2+ to bind to imatinib in real-time. Results demonstrated in this work clearly showed that the novel G-FET biosensors are very promising to analyze interactions between proteins and low molecular weight drugs.

WOS
Держатели документа:
Dezhou Univ, Inst Biophys, Shandong Key Lab Biophys, Dezhou 253023, Peoples R China.
Fed Res Ctr Krasnoyarsk Sci Ctr SB RAS, Inst Biophys SB RAS, Krasnoyarsk 660036, Russia.
Shandong Normal Univ, Collaborat Innovat Ctr Light Manipulat & Applicat, Jinan 250358, Peoples R China.

Доп.точки доступа:
Xu, Shicai; Wang, Tiejun; Liu, Guofeng; Cao, Zanxia; Frank, Ludmila A.; Jiang, Shouzhen; Zhang, Chao; Li, Zhenhua; Krasitskaya, Vasilisa V.; Li, Qiang; Sha, Yujie; Zhang, Xiumei; Liu, Huilan; Wang, Jihua; Taishan Scholars Program of Shandong Province [tsqn201812104]; Qingchuang Science and Technology Plan of Shandong Province [2019KJJ017, 2020KJC004]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [61671107, 62071085, 11704059, 31802309]; Youth Innovation Team Lead-Education Project of Shandong Educational Committee

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13.

Spatial and temporal variation in Arctic freshwater chemistry-Reflecting climate-induced landscape alterations and a changing template for biodiversity / B. J. Huser, M. N. Futter, D. Bogan [et al.] // Freshw. Biol. - 2020, DOI 10.1111/fwb.13645. - Cited References:98. - Environment and Climate Change Canada; Cumulative Impact Monitoring Program, Government of Northwest Territories . - Article in press. - ISSN 0046-5070. - ISSN 1365-2427

РУБ Ecology + Marine & Freshwater Biology
Рубрики:
DISSOLVED ORGANIC-CARBON
PERMAFROST THAW
CHEMICAL LIMNOLOGY
Кл.слова (ненормированные):
biogeochemistry -- eutrophication -- lakes -- oligotrophication -- rivers
Аннотация: Freshwater chemistry across the circumpolar region was characterised using a pan-Arctic data set from 1,032 lake and 482 river stations. Temporal trends were estimated for Early (1970-1985), Middle (1986-2000), and Late (2001-2015) periods. Spatial patterns were assessed using data collected since 2001. Alkalinity, pH, conductivity, sulfate, chloride, sodium, calcium, and magnesium (major ions) were generally higher in the northern-most Arctic regions than in the Near Arctic (southern-most) region. In particular, spatial patterns in pH, alkalinity, calcium, and magnesium appeared to reflect underlying geology, with more alkaline waters in the High Arctic and Sub Arctic, where sedimentary bedrock dominated. Carbon and nutrients displayed latitudinal trends, with lower levels of dissolved organic carbon (DOC), total nitrogen, and (to a lesser extent) total phosphorus (TP) in the High and Low Arctic than at lower latitudes. Significantly higher nutrient levels were observed in systems impacted by permafrost thaw slumps. Bulk temporal trends indicated that TP was higher during the Late period in the High Arctic, whereas it was lower in the Near Arctic. In contrast, DOC and total nitrogen were both lower during the Late period in the High Arctic sites. Major ion concentrations were higher in the Near, Sub, and Low Arctic during the Late period, but the opposite bulk trend was found in the High Arctic. Significant pan-Arctic temporal trends were detected for all variables, with the most prevalent being negative TP trends in the Near and Sub Arctic, and positive trends in the High and Low Arctic (mean trends ranged from +0.57%/year in the High/Low Arctic to -2.2%/year in the Near Arctic), indicating widespread nutrient enrichment at higher latitudes and oligotrophication at lower latitudes. The divergent P trends across regions may be explained by changes in deposition and climate, causing decreased catchment transport of P in the south (e.g. increased soil binding and trapping in terrestrial vegetation) and increased P availability in the north (deepening of the active layer of the permafrost and soil/sediment sloughing). Other changes in concentrations of major ions and DOC were consistent with projected effects of ongoing climate change. Given the ongoing warming across the Arctic, these region-specific changes are likely to have even greater effects on Arctic water quality, biota, ecosystem function and services, and human well-being in the future.

WOS
Держатели документа:
Swedish Univ Agr Sci, Dept Aquat Sci & Assessment, Box 7050, S-75007 Uppsala, Sweden.
Univ Alaska Anchorage, Alaska Ctr Conservat Sci, Anchorage, AK USA.
Norwegian Water Resources & Energy Directorate, Oslo, Norway.
Univ Oslo, Nat Hist Museum, Oslo, Norway.
Wilfrid Laurier Univ, Cold Regions Res Ctr, Waterloo, ON, Canada.
Russian Acad Sci, Siberian Branch, Inst Biophys, Krasnoyarsk, Russia.
Umea Univ, Climate Impacts Res Ctr, Dept Ecol & Environm Sci, Umea, Sweden.
Queens Univ, Dept Biol, Paleoecol Environm Assessment & Res Lab PEARL, Kingston, ON, Canada.
Norwegian Inst Nat Res, Oslo, Norway.
Univ New Brunswick, Canadian Rivers Inst, Fredericton, NB, Canada.
Univ New Brunswick, Dept Biol, Fredericton, NB, Canada.

Доп.точки доступа:
Huser, Brian J.; Futter, Martyn N.; Bogan, Daniel; Brittain, John E.; Culp, Joseph M.; Goedkoop, Willem; Gribovskaya, Iliada; Karlsson, Jan; Lau, Danny C. P.; Ruhland, Kathleen M.; Schartau, Ann Kristin; Shaftel, Rebecca; Smol, John P.; Vrede, Tobias; Lento, Jennifer; Environment and Climate Change Canada; Cumulative Impact Monitoring Program, Government of Northwest Territories

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14.

Spatial and temporal variation in Arctic freshwater chemistry—Reflecting climate-induced landscape alterations and a changing template for biodiversity / B. J. Huser, M. N. Futter, D. Bogan [et al.] // Freshw. Biol. - 2020, DOI 10.1111/fwb.13645 . - Article in press. - ISSN 0046-5070
Кл.слова (ненормированные):
biogeochemistry -- eutrophication -- lakes -- oligotrophication -- rivers
Аннотация: Freshwater chemistry across the circumpolar region was characterised using a pan-Arctic data set from 1,032 lake and 482 river stations. Temporal trends were estimated for Early (1970–1985), Middle (1986–2000), and Late (2001–2015) periods. Spatial patterns were assessed using data collected since 2001. Alkalinity, pH, conductivity, sulfate, chloride, sodium, calcium, and magnesium (major ions) were generally higher in the northern-most Arctic regions than in the Near Arctic (southern-most) region. In particular, spatial patterns in pH, alkalinity, calcium, and magnesium appeared to reflect underlying geology, with more alkaline waters in the High Arctic and Sub Arctic, where sedimentary bedrock dominated. Carbon and nutrients displayed latitudinal trends, with lower levels of dissolved organic carbon (DOC), total nitrogen, and (to a lesser extent) total phosphorus (TP) in the High and Low Arctic than at lower latitudes. Significantly higher nutrient levels were observed in systems impacted by permafrost thaw slumps. Bulk temporal trends indicated that TP was higher during the Late period in the High Arctic, whereas it was lower in the Near Arctic. In contrast, DOC and total nitrogen were both lower during the Late period in the High Arctic sites. Major ion concentrations were higher in the Near, Sub, and Low Arctic during the Late period, but the opposite bulk trend was found in the High Arctic. Significant pan-Arctic temporal trends were detected for all variables, with the most prevalent being negative TP trends in the Near and Sub Arctic, and positive trends in the High and Low Arctic (mean trends ranged from +0.57%/year in the High/Low Arctic to ?2.2%/year in the Near Arctic), indicating widespread nutrient enrichment at higher latitudes and oligotrophication at lower latitudes. The divergent P trends across regions may be explained by changes in deposition and climate, causing decreased catchment transport of P in the south (e.g. increased soil binding and trapping in terrestrial vegetation) and increased P availability in the north (deepening of the active layer of the permafrost and soil/sediment sloughing). Other changes in concentrations of major ions and DOC were consistent with projected effects of ongoing climate change. Given the ongoing warming across the Arctic, these region-specific changes are likely to have even greater effects on Arctic water quality, biota, ecosystem function and services, and human well-being in the future. © 2020 The Authors. Freshwater Biology published by John Wiley & Sons Ltd.

Scopus
Держатели документа:
Department of Aquatic Sciences and Assessment, Swedish University of Agricultural Sciences, Uppsala, Sweden
Alaska Center for Conservation Science, University of Alaska Anchorage, Anchorage, AK, United States
Norwegian Water Resources & Energy Directorate, Oslo, Norway
Natural History Museum, University of Oslo, Oslo, Norway
Cold Regions Research Centre, Wilfrid Laurier University, Waterloo, ON, Canada
Institute of Biophysics, Siberian Branch of Russian Academy of Sciences, Krasnoyarsk, Russian Federation
Department of Ecology and Environmental Science, Climate Impacts Research Centre, Umea University, Abisko, Sweden
Paleoecological Environmental Assessment and Research Laboratory (PEARL), Department of Biology, Queen’s University, Kingston, ON, Canada
Norwegian Institute for Nature Research, Oslo, Norway
Canadian Rivers Institute and Department of Biology, University of New Brunswick, Fredericton, NB, Canada

Доп.точки доступа:
Huser, B. J.; Futter, M. N.; Bogan, D.; Brittain, J. E.; Culp, J. M.; Goedkoop, W.; Gribovskaya, I.; Karlsson, J.; Lau, D. C.P.; Ruhland, K. M.; Schartau, A. K.; Shaftel, R.; Smol, J. P.; Vrede, T.; Lento, J.

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15.

Winter atmospheric nutrient and pollutant deposition on Western Sayan Mountain lakes (Siberia) / D. Diaz-De-Quijano, A. Vladimirovich Ageev, E. Anatolevna Ivanova, O. Valerevna Anishchenko // Biogeosciences. - 2021. - Vol. 18, Is. 5. - P1601-1618, DOI 10.5194/bg-18-1601-2021 . - ISSN 1726-4170
Аннотация: The world map of anthropogenic atmospheric nitrogen deposition and its effects on natural ecosystems is not described with equal precision everywhere. In this paper, we report atmospheric nutrient, sulfate and spheroidal carbonaceous particle (SCP) deposition rates, based on snowpack analyses of a formerly unexplored Siberian mountain region. Then, we discuss their potential effects on lake phytoplankton biomass limitation. We estimate that the nutrient depositions observed in the late-season snowpack (4016 mgNO3-Nm2 and 0.580.13 mg TP-Pm2; TP for total phosphorous) would correspond to yearly depositions lower than 11971 mgNO3-Nm2 yr1 and higher than 1.710.91 mg TP-Pm2 yr1. These yearly deposition estimates would approximately fit the predictions of global deposition models and correspond to the very low nutrient deposition range, although they are still higher than world background values. In spite of the fact that such a low atmospheric nitrogen deposition rate would be enough to induce nitrogen limitation in unproductive mountain lakes, phosphorus deposition was also extremely low, and the resulting lake water N: P ratio was unaffected by atmospheric nutrient deposition. In the end, the studied lakes' phytoplankton appeared to be split between phosphorus and nitrogen limitation. We conclude that these pristine lakes are fragile sensitive systems exposed to the predicted climate warming, increased winter precipitation, enhanced forest fires and shifts in anthropogenic nitrogen emissions that could finally couple their water chemistry to that of atmospheric nutrient deposition and unlock temperature-inhibited responses of phytoplankton to nutrient shifts. © Author(s) 2021. This work is distributed under the Creative Commons Attribution 4.0 License.

Scopus
Держатели документа:
Siberian Federal University, 79, Svobondyi prospekt, Krasnoyarsk, Krasnoyarsk Krai, 660041, Russian Federation
Institute of Biophysics, Siberian Branch Russian Academy of Sciences, 50/50, Akademgorodok, Krasnoyarsk, Krasnoyarsk Krai, 660036, Russian Federation

Доп.точки доступа:
Diaz-De-Quijano, D.; Vladimirovich Ageev, A.; Anatolevna Ivanova, E.; Valerevna Anishchenko, O.

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16.

Winter atmospheric nutrient and pollutant deposition on Western Sayan Mountain lakes (Siberia) / DQD Diaz, A. V. Ageev, E. A. Ivanova, O. V. Anishchenko // Biogeosciences. - 2021. - Vol. 18, Is. 5. - P1601-1618, DOI 10.5194/bg-18-1601-2021. - Cited References:86. - This research has been supported by the Russian Foundation for Basic Research (grant no. 20-04-00960) and the Ministry of Science and Higher Education of the Russian Federation (postdoctoral program project no. 5-100, grant no. FSRZ-2020-0014). . - ISSN 1726-4170. - ISSN 1726-4189

РУБ Ecology + Geosciences, Multidisciplinary
Рубрики:
FLY-ASH PARTICLES
NITROGEN DEPOSITION
PHOSPHORUS DEPOSITION
Аннотация: The world map of anthropogenic atmospheric nitrogen deposition and its effects on natural ecosystems is not described with equal precision everywhere. In this paper, we report atmospheric nutrient, sulfate and spheroidal carbonaceous particle (SCP) deposition rates, based on snowpack analyses of a formerly unexplored Siberian mountain region. Then, we discuss their potential effects on lake phytoplankton biomass limitation. We estimate that the nutrient depositions observed in the late-season snowpack (40 +/- 16 mgNO(3)-Nm(-2) and 0.58 +/- 0.13 mg TP-Pm-2; TP for total phosphorous) would correspond to yearly depositions lower than 119 +/- 71 mgNO(3)-Nm(-2) yr(-1) and higher than 1.71 +/- 0.91 mg TP-Pm-2 yr(-1). These yearly deposition estimates would approximately fit the predictions of global deposition models and correspond to the very low nutrient deposition range, although they are still higher than world background values. In spite of the fact that such a low atmospheric nitrogen deposition rate would be enough to induce nitrogen limitation in unproductive mountain lakes, phosphorus deposition was also extremely low, and the resulting lake water N: P ratio was unaffected by atmospheric nutrient deposition. In the end, the studied lakes' phytoplankton appeared to be split between phosphorus and nitrogen limitation. We conclude that these pristine lakes are fragile sensitive systems exposed to the predicted climate warming, increased winter precipitation, enhanced forest fires and shifts in anthropogenic nitrogen emissions that could finally couple their water chemistry to that of atmospheric nutrient deposition and unlock temperature-inhibited responses of phytoplankton to nutrient shifts.

WOS
Держатели документа:
Siberian Fed Univ, 79 Svobondyi Prospekt, Krasnoyarsk 660041, Krasnoyarsk Kra, Russia.
Russian Acad Sci, Siberian Branch, Inst Biophys, 50-50 Akademgorodok, Krasnoyarsk 660041, Krasnoyarsk Kra, Russia.

Доп.точки доступа:
Diaz, A. V.; Ageev, Aleksander Vladimirovich; Ivanova, Elena Anatolevna; Anishchenko, Olesia Valerevna; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [20-04-00960]; Ministry of Science and Higher Education of the Russian Federation [5-100, FSRZ-2020-0014]

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17.

18.

Single-Crystal Diamond Needle Fabrication Using Hot-Filament Chemical Vapor Deposition / R. Ismagilov, S. Malykhin, A. Puzyr [et al.] // Materials. - 2021. - Vol. 14, Is. 9. - Ст. 2320, DOI 10.3390/ma14092320. - Cited References:32. - This work was supported by the Russian Science Foundation (project no. 19-79-00203) and by the Russian Foundation for Basic Research (grant no. 18-29-19071, in part for PL and Raman inspection). . - ISSN 1996-1944

РУБ Chemistry, Physical + Materials Science, Multidisciplinary + Metallurgy &

Кл.слова (ненормированные):
thin films -- diamond needles -- chemical vapor deposition -- hot-filament -- CVD -- large-scale synthesis
Аннотация: Single-crystal diamonds in the form of micrometer-scale pyramids were produced using a combination of hot-filament (HF) chemical vapor deposition (CVD) and thermal oxidation processes. The diamond pyramids were compared here with similar ones that were manufactured using plasma-enhanced (PE) CVD. The similarities revealed in the morphology, Raman, and photoluminescent characteristics of the needles obtained using the hot-filament and plasma-enhanced CVD are discussed in connection with the diamond film growth mechanism. This work demonstrated that the HF CVD method has convincing potential for the fabrication of single-crystal diamond needles in the form of regularly shaped pyramids on a large surface area, even on non-conducting substrates. The experimental results demonstrated the ability for the mass production of the single-crystal needle-like diamonds, which is important for their practical application.

WOS
Держатели документа:
Moscow MV Lomonosov State Univ, Dept Phys, Moscow 119991, Russia.
Univ Eastern Finland, Dept Phys & Math, Joensuu 80101, Finland.
Russian Acad Sci, Lebedev Phys Inst, Div Solid State Phys, Moscow 119991, Russia.
Russian Acad Sci, RAS, Inst Biophys, Fed Res Ctr,Krasnoyarsk Sci Ctr SB, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Ismagilov, Rinat; Malykhin, Sergei; Puzyr, Aleksey; Loginov, Artem; Kleshch, Victor; Obraztsov, Alexander; Russian Science FoundationRussian Science Foundation (RSF) [19-79-00203]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [18-29-19071]

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19.

SEASONAL VARIABILITY OF SEDIMENTATION FLOWS IN SALT MEROMICTIC LAKE SHIRA (KHAKASSIA) / V. V. Babich, A. V. Darin, I. A. Kalugin [и др.] // Bull. Tomsk Polytech. Univ.-Geo Assets Eng. - 2021. - Vol. 332, Is. 12. - С. 22-34, DOI 10.18799/24131830/2021/12/3178. - Cited References:29. - The work was carried out on state assignment of IGM SB RAS, supported by the Ministry of Science and Higher Education of the Russian Federation, with partial support of the RFBR - grant 21-54-52001 (setting of traps, sampling) and grant 19-05-50046 (micro-XRF-SR). . - ISSN 2500-1019. - ISSN 2413-1830

РУБ Engineering, Geological
Рубрики:
CENTRAL TIBETAN PLATEAU
NAM-CO
VARVE
Кл.слова (ненормированные):
Bottom sediments -- sedimentation traps -- salt lakes -- micro-XRF -- synchrotron radiation -- regression analysis
Аннотация: The relevance of the work is caused by the need to study seasonal variations in the volume and composition of sedimentation flows in modern lakes and their relationship with weather and climatic factors, which can serve as a basis for reconstructing climatic changes in the past. The main aim: to assess seasonal changes in the mass, velocity and chemical composition of sedimentary material entering Lake Shira on the basis of generalization and analysis of the results of multiyear annual monitoring of the material of sedimentation traps incubated in the lake. Object of the study was the drainless, slightly saline meromictic lake Shira, located in the steppe intermontane depression on the territory of the Republic of Khakassia. Methods: long-term seasonal monitoring of sedimentary material forming bottom sediments using sedimentation traps incubated in the lake; study of the obtained material for a wide range of parameters (biological, hydrochemical, lithological-geochemical, granulometric, etc.) by various conventional methods, including the method of X-ray fluorescence microanalysis on synchrotron radiation beams (XRF-SI), adapted for the study of bottom samples; computer statistical analysis of the data obtained (multiple regression method, cross-correlation analysis, etc.) in order to identify the relationship between regional temperatures and the chemical composition of the deposited material with the construction of a regression model. Results. Based on the study of the amount and elemental composition of the sedimentary material of the seasonal bottom traps of Lake Shira, collected for 2012-2017, a dynamic model of the seasonal influx of sedimentary flows in lakes of this landscape-geochemical type was formulated. It has been established that the most intensive sedimentation of the material occurs in the summer-autumn period, less - in the winter-spring period. At the same time, in spring, the accumulation of allochthonous (terrigenous) aleurite material, supplied with flood waters, predominates; in the summer-autumn period, simultaneously with the deposition of clastogenic pelitic material, biogenic and chemogenic materials are accumulated in sediments in large quantities. In winter, clastogenic and biogenic processes of sedimentation practically stop, only chemogenic sedimentation of carbonates is observed. It was established that the sedimentation of allochthonous material entering the reservoir occurs during two-three months, which indicates a certain inertness of sedimentation. The presence of a stable relationship between the mass and chemical composition of terrigenous material entering the lake with the regional temperature of the near-surface air, which is one of the main regulators of the water balance of the reservoir, is shown.

WOS
Держатели документа:
Russian Acad Sci, Siberian Branch, Sobolev Inst Geol & Mineral, 3 Academician Koptyug Ave, Novosibirsk 360090, Russia.
Inst Biophys SB RAS, 50 Akad Gorodok, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Babich, Valery V.; Darin, Andrey, V; Kalugin, Ivan A.; Markovich, Tatyana, I; Zykov, Viktor V.; Rogozin, Denis Yu; Ministry of Science and Higher Education of the Russian Federation; RFBRRussian Foundation for Basic Research (RFBR) [21-54-52001, 19-05-50046]

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