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Magnetic ordering of NdFe3(BO3)(4) studied by infrared absorption spectroscopy / E. P. Chukalina [et al.] // Phys. Lett. A. - 2004. - Vol. 322, Is. 3-4. - P. 239-243, DOI 10.1016/j.physleta.2003.12.062. - Cited References: 8 . - ISSN 0375-9601

РУБ Physics, Multidisciplinary
Рубрики:
CRYSTALS
Кл.слова (ненормированные):
ferroborates -- Fourier-transform spectroscopy -- magnetic ordering -- Ferroborates -- Fourier-transform spectroscopy -- Magnetic ordering -- iron -- neodymium -- absorption spectroscopy -- article -- electronics -- infrared spectroscopy -- magnetism -- molecular interaction -- molecular physics -- temperature
Аннотация: We report the first measurements of the optical spectra of NdFe3(BO3)(4), a promising material for optoelectronics. Exchange splitting of Nd3+ spectral lines due to magnetic interactions in a magnetically ordered state was observed. The temperature dependences of the exchange splitting and of the linewidth point to the temperature T-c 33 +/- 1K of the magnetic ordering in both iron and neodymium. magnetic subsystems. 2004 Elsevier B.V. All rights reserved.

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Держатели документа:
Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Region, Russia
RAS, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, Russian Academy of Sciences, 142190 Troitsk, Moscow Region, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch of RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Chukalina, E. P.; Kuritsin, D. Y.; Popova, M. N.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Kharlamova, S. A.; Temerov, V. L.; Темеров, Владислав Леонидович
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Cascade of phase transitions in GdFe3(BO3)(4) / R. Z. Levitin [et al.] // JETP Letters. - 2004. - Vol. 79, Is. 9. - P. 423-426, DOI 10.1134/1.1776236. - Cited References: 8 . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
CRYSTALS
ND
Аннотация: Cascade of phase transitions in GdFe3(BO3)(4) at 156, 37, and 9 K has been detected by specific heat measurements and further studied by Raman scattering and Nd3+ spectroscopic probe method. A weakly first-order structural phase transition at 156 K is followed by a second-order antiferromagnetic ordering phase transition at 37 K and a first-order spin-reorientational phase transition at 9 K. (C) 2004 MAIK "Nauka / Interperiodica".

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Держатели документа:
Moscow MV Lomonosov State Univ, Fac Phys, Moscow 119992, Russia
Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Region, Russia
Univ Groningen, Ctr Mat Sci, NL-9747 AG Groningen, Netherlands
Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН

Доп.точки доступа:
Levitin, R. Z.; Popova, E. A.; Chtsherbov, R. M.; Vasiliev, A. N.; Popova, M. N.; Chukalina, E. P.; Klimin, S. A.; van Loosdrecht, PHM; Fausti, D.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич
}
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Chukalina, E. P.
Spectroscopic study of magnetic phase transitions in NdxGd1-xFe3(BO3)(4) / E. P. Chukalina, L. N. Bezmaternykh // Phys. Solid State. - 2005. - Vol. 47: 12th Feofilov Workshop on Spectroscopy of Crystal Activated by Rare-Earth and Transition-Metal Ions (SEP 22-25, 2004, Yekaterinburg, RUSSIA), Is. 8. - P. 1528-1531, DOI 10.1134/1.2014507. - Cited References: 10 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
CRYSTALS
ND
Аннотация: Magnetic ordering and spin reorientation in iron borates NdxGd1 - xFe3(BO3)(4) (x = 0.01, 0.04, 0.25, 1.0) are studied using a rare-earth spectroscopic probe. (c) 2005 Pleiades Publishing, Inc.

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Держатели документа:
Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Oblast, Russia
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, Moscow oblast, 142190, Russian Federation
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Bezmaternykh, L. N.; Безматерных, Леонард Николаевич
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Optical spectra, crystal-field parameters, and magnetic susceptibility of multiferroic NdFe3(BO3)(4) / M. N. Popova [et al.] // Phys. Rev. B. - 2007. - Vol. 75, Is. 22. - Ст. 224435, DOI 10.1103/PhysRevB.75.224435. - Cited References: 22 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
IRON BORATE GDFE3(BO3)(4)
   CRYSTALLIZATION
   SPECTROSCOPY
   LASER
   ND3+
Аннотация: We report high-resolution optical absorption spectra for NdFe3(BO3)(4) trigonal single crystal, which is known to exhibit a giant magnetoelectric effect below the temperature of magnetic ordering T-N=33 K. The analysis of the temperature-dependent polarized spectra reveals the energies and, in some cases, symmetries and exchange splittings of Nd3+ 84 Kramers doublets. We perform crystal-field calculations starting from the exchange-charge model, obtain a set of six real crystal-field parameters, and calculate wave functions and magnetic g factors. In particular, the values g(perpendicular to)=2.385 and g(parallel to)=1.376 were found for the Nd3+ ground-state doublet. We obtain B-loc=7.88 T and parallel to J(FN)parallel to=0.48 K for the values of the local effective magnetic field at liquid-helium temperatures at the Nd3+ site and the Nd-Fe exchange integral, respectively, using the experimentally measured Nd3+ ground-state splitting of 8.8 cm(-1). To check the reliability of our set of crystal-field parameters, we model the magnetic susceptibility data from literature. A dimer containing two nearest-neighbor iron ions in the spiral chain is considered to partly account for quasi-one-dimensional properties of iron borates, and then the mean-field approximation is used. The results of calculations with the exchange parameters for Fe3+ ions J(nn)=-6.25 K (intrachain interactions) and J(nnn)=-1.92 K (interchain interactions) obtained from fitting agree well with the experimental data.

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Держатели документа:
Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Region, Russia
Kazan VI Lenin State Univ, Kazan 420008, Russia
Ecole Natl Super Chim Paris, CNRS, UMR7574, Lab Chim Appl & Etat Solide, F-75231 Paris, France
Moscow MV Lomonosov State Univ, Fac Phys, Moscow 119992, Russia
RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, Russian Academy of Sciences, 142190 Troitsk, Russian Federation
Kazan State University, 420008 Kazan, Russian Federation
Laboratoire de Chimie Applique'e de l'E Tat Solide, CNRS-UMR7574, ENSCP, 11, Rue Pierre et Marie Curie, F-75231 Paris Cedex 05, France
Physics Faculty, Moscow State University, 119992 Moscow, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch of RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Popova, M. N.; Chukalina, E. P.; Stanislavchuk, T. N.; Malkin, B. Z.; Zakirov, A. R.; Antic-Fidancev, E.; Popova, E. A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Temerov, V. L.; Темеров, Владислав Леонидович
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Investigation of the iron borates DyFe3(BO3)(4) and HoFe3(BO3)(4) by the method of Er3+ spectroscopic probe / T. N. Stanislavchuk [et al.] // Phys. Lett. A. - 2007. - Vol. 368, Is. 5. - P. 408-411, DOI 10.1016/j.physleta.2007.04.044. - Cited References: 16 . - ISSN 0375-9601

РУБ Physics, Multidisciplinary
Рубрики:
GDFE3(BO3)(4)
CRYSTALS
Кл.слова (ненормированные):
rare-earth iron borates -- magnetic ordering -- optical spectroscopy -- Magnetic ordering -- Optical spectroscopy -- Rare-earth iron borates
Аннотация: Temperature-dependent high-resolution optical spectra of the Er3+ probe ion in DyFe3(BO3)(4) and HoFe3(BO3)(4) are reported. The data provide the temperature of magnetic ordering and direction of the Fe3+ magnetic moments. Both compounds order magnetically at T-N = 39 +/- 1K. The magnetic structure of DyFe3(BO3)(4) is of the easy-axis type, while that of HoFe3(BO3)(4) is of the easy-plane type. The role of anisotropic interactions between the iron and the rare-earth subsystems is discussed. (c) 2007 Elsevier B.V. All rights reserved.

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Держатели документа:
Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Region, Russia
LV Kirenskii Inst Phys, RAS, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, Russian Academy of Sciences, 142190 Troitsk, Moscow region, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch, RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Stanislavchuk, T. N.; Chukalina, E. P.; Popova, M. N.; Bezmaternykh, L. N.; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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Spectroscopic Study of the Mag netic Ordering in SmFe3(BO3)4 [Text] / Chukalina E.P.Popova M.N. [et al.] // Physics Letters A. - 2010. - Vol. 374. - P1790-1792

Доп.точки доступа:
Chukalina, E.P.; Popova, M.N.; Bezmaternykh, L.N.; Gudim, I.A.
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Spectroscopic study of the magnetic ordering in SmFe3(BO3)(4) / E. P. Chukalina [et al.] // Phys. Lett. A. - 2010. - Vol. 374, Is. 15-16. - P. 1790-1792, DOI 10.1016/j.physleta.2010.02.018. - Cited References: 20. - The authors thank B.Z. Malkin and S.A. Klinnin for helpful discussions and K.N. Boldyrev for participating in some low-temperatures measurements. This work was supported in part by the Russian Foundation for Basic Research (grants Nos. 10-02-01071 and 10-02-00765), and by the Russian Academy of Sciences under the Programs for Basic Research. . - ISSN 0375-9601

РУБ Physics, Multidisciplinary
Рубрики:
IRON BORATE GDFE3(BO3)(4)
SINGLE-CRYSTAL
DYFE3(BO3)(4)
Кл.слова (ненормированные):
Rare-earth iron borates -- Magnetic ordering -- Optical spectroscopy -- Magnetic ordering -- Optical spectroscopy -- Rare-earth iron borates
Аннотация: SmFe3(BO3)(4) belongs to the family of rare-earth RFe3(BO3)(4) multiferroics. We present the first measurements of the optical spectra of SmFe3(BO3)(4) (on single crystals) and report the data on the crystal-field levels and their symmetries for the ground multiplet H-6(5/2) [0 (Gamma(4)). 135 (Gamma(56)), and 220 (Gamma(4)) cm(-1)] and on the ground-state exchange splitting (13.2 cm(-1) at 1.7 K), important to interpret the magnetic, magnetoelectric, and thermodynamic properties of this compound. The observed exchange splitting of the Sm3+ Kramers doublets manifests the magnetic ordering in SmFe3(BO3)(4) at 32 +/- 1 K. From a comparison of the temperature-dependent spectra of the Sm3+ ion in SmFe3(BO3)(4) and in Nd-Gd mixed iron borate where the magnetic spin reorientation has been found earlier, we suggest the easy-plane arrangement of the Fe spins in SmFe3(BO3)(4). The samarium iron borate preserves the R32 (D-3(7)) crystal structure at all the investigated temperatures (down to 1.7 K). (C) 2010 Elsevier B.V. All rights reserved.

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Держатели документа:
[Chukalina, E. P.
Popova, M. N.] RAS, Inst Spect, Troitsk 142190, Moscow Region, Russia
[Bezmaternykh, L. N.
Gudim, I. A.] RAS, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, RAS, 5, Fizicheskaya str, 142190 Troitsk, Moscow region, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch, RAS, 660036 Krasnoyarsk, Russian Federation

Доп.точки доступа:
Chukalina, E. P.; Popova, M. N.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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Crystal field and exchange interactions in the SmFe3(BO3)4 multiferroic / M. N. Popova [et al.] // J. Exp. Theor. Phys. - 2014. - Vol. 118, Is. 1. - P. 111-123, DOI 10.1134/S1063776114010142. - Cited References: 22. - This work was supported by the Russian Foundation for Basic Research (project no. 13-02-00787) and the basic research program Quantum Mesoscopic and Disordered Structures of the Presidium of the Russian Academy of Sciences. . - ISSN 1063-7761. - ISSN 1090-6509

РУБ Physics, Multidisciplinary

Аннотация: The optical spectra of oriented SmFe3(BO3)4 single crystals are studied in the region of the f-f transitions in the Sm3+ ion by Fourier spectroscopy. The energies, the symmetry properties, and the exchange splittings of the Stark sublevels of the ground and 17 excited multiplets of the Sm3+ ion in a crystal field of symmetry D 3 are determined from the measured temperature dependences of polarized-radiation absorption spectra. The parameters of the crystal field acting on samarium ions and the parameters of the exchange interaction between Sm3+ and Fe3+ ions are found. The anisotropy of the effective exchange interaction is shown to be substantially stronger than the magnetic anisotropy, due to a strong crystal-field-induced mixing of the ground and excited multiplets.

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Публикация на русском языке Исследование кристаллического поля и обменных взаимодействий в мультиферроике SmFe3( BO3)4 [Текст] / М. Н. Попова [и др.] // Журн. эксперим. и теор. физ. : Наука, 2014. - Т. 145 Вып. 1. - С. 128-142

Держатели документа:
Russian Acad Sci, Inst Spect, Moscow 142190, Russia
Kazan Privolzhsky Fed Univ, Kazan 420008, Russia
State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Oblast, Russia
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Popova, M. N.; Chukalina, E. P.; Malkin, B. Z.; Erofeev, D. A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Russian Foundation for Basic Research [13-02-00787]; basic research program Quantum Mesoscopic and Disordered Structures of the Presidium of the Russian Academy of Sciences
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Improving one’s understanding of magnetic properties of SmFe3(BO3)4 by means of spectroscopic data [Текст] / E. P. Chukalina [et al.] // Moscow int. Symp. on Magnet. (MISM-2014) : Book of abstracts. - 2014. - Ст. 30PO-M-22. - P. 279 . - ISBN 978-5-91978-025-0

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Доп.точки доступа:
Chukalina, E. P.; Malkin, B. Z.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Popova, M. N.; Moscow International Symposium on Magnetism(6 ; 2014 ; 29 June-3 July ; Moscow); Московский государственный университет им. М.В. Ломоносова
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10.

Spectroscopy of f-f transitions, crystal-field calculations, and magnetic and quadrupole helix chirality in DyFe3(BO3)4 / M. N. Popova [et al.]. - Electronic text data // ArXiv. - 2016. - Ст. 1611.07092. - Cited References: 47. - This work was supported by the Russian Science Foundation (Grant No14-12-01033). I. A. G. thanks L. N. Bezmaternykh for useful comments concerning the crystal growth and the Russian Foundation for Basic Research for a financial support under Grant No 14-02-00307a.
Аннотация: Recently, quadrupole helix chirality and its domain structure was observed in resonant x-ray diffraction experiments on DyFe3(BO3)4 using circularly polarized x rays [T. Usui et al., Nature Materials 13, 611 (2014)]. We show that this effect can be explained quantitatively by calculating the quadrupole moments of the Dy3+ ions induced by the low-symmetry (C2) crystal-field (CF) component. In this work, the CF parameters for the Dy3+ ions in the P3121 (P3221) phase of DyFe3(BO3)4 are obtained from CF calculations based on the analysis of high-resolution temperature-dependent optical spectroscopy data. We also consider the helix chirality of the single-site magnetic susceptibility tensors of the Dy3+ ions in the paramagnetic P3121 (P3221) phase and suggest a neutron diffraction experiment to reveal it.

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Держатели документа:
Institute of Spectroscopy, Russian Academy of Sciences, 108840 Moscow, Troitsk, Russia
Department of Physics, New Jersey Institute of Technology, 07102 Newark, New Jersey, USA
Kazan Federal University, 420008 Kazan, Russia
Kirensky Institute of Physics, Siberian Branch of RAS, 660036 Krasnoyarsk, Russia

Доп.точки доступа:
Popova, M. N.; Chukalina, E. P.; Boldyrev, K. N.; Stanislavchuk, T. N.; Malkin, B. Z.; Gudim, I. A.; Гудим, Ирина Анатольевна
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