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Optical absorption and luminescence of Tm3+ and Yb3+ ions in huntite structure / Malakhovskii A.V., Edelman I.S., Sokolov A.E., Sukhachov A.L., Temerov V.L., Gnatchenko S.L., Kachur I.S., Piryatinskaya V.G., Valiev U.V. // Республиканская конференция «Оптические методы в современной физике», Ташкент, Узбекистан, 2008, с. 33-35

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Edelman, I. S.; Эдельман, Ирина Самсоновна; Sokolov, A. Е.; Соколов, Алексей Эдуардович; Sukhachev, A. L.; Сухачев, Александр Леонидович; Temerov, V. L.; Темеров, Владислав Леонидович; Gnatchenko, S. L.; Kachur, I. S.; Piryatinskaya, V. G.; Valiev, U. V.
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Malakhovskii, A. V.
Nature of magnetic circular dichroism and absorption spectra of f-f transitions in Na0.4Ho0.6F2.2 single crystal / A. V. Malakhovskii, V. V. Sokolov, D. N. Karimov // Chem. Phys. - 2024. - Vol. 581. - Ст. 112257, DOI 10.1016/j.chemphys.2024.112257. - Cited References: 25 . - ISSN 0301-0104. - ISSN 1873-4421
Кл.слова (ненормированные):
Magnetic circular dichroism -- f-f transitions -- Fluoride crystals -- Ho ions
Аннотация: We present first study of magnetic circular dichroism (MCD) spectra of Ho3+ ion in C4v local symmetry, which it has in fluorite Na0.4Ho0.6F2.2. Optical absorption and MCD spectra were studied in this single crystal in the region of 5I8> 5F3, 5F2, 3K8 and 5G5 transitions in the temperature range 3.6–––90 K. It was revealed, that number of transitions observed in the MCD and absorption spectra coincides with the number of transitions only from the doublet E state to singlet excited states. The E-E type transitions are not active in MCD, but they are not observed in the absorption spectra either. Paramagnetic magneto-optical activities (MOA) of the absorption bands and their temperature dependences were measured and interpreted with the help of the theory based on the nature of f-f transitions allowance. The MCD spectra were also analyzed in approximation of the J,±MJ wave functions of the free atom. It was shown in particular, that the lowest initial state of the transitions observed at T ˃ 10 K had MJ = 7, but this is not the lowest state of the holmium ion in the crystal. A little lower there is a quasi-doublet with MJ = 8 and, accordingly, with a higher magneto-optical activity of transitions from it. However, the intensity of transitions from this state is low.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, 660036 Krasnoyarsk, Russian Federation
Federal Scientific Research Centre «Crystallography and Photonics» of Russian Academy of Sciences, Leninskiy Prospekt 59, 119333 Moscow, Russia

Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Karimov, D.N.; Малаховский, Александр Валентинович
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Transformation of 5I8→5F5 Ho absorption band in Ho0.75Nd0.25Fe3(BO3)4 crystal during spin-reorientation transition / A. V. Malakhovskii, A. L. Sukhachev, V. V. Sokolov [et al.] // Phys. B: Condens. Matter. - 2023. - Vol. 654. - Ст. 414706, DOI 10.1016/j.physb.2023.414706. - Cited References: 17 . - ISSN 0921-4526. - ISSN 1873-2135
Кл.слова (ненормированные):
Optical f-f transitions -- Magnetic reorientation transition -- Local properties in the optically excited states
Аннотация: Polarized absorption spectra of crystal Ho0.75Nd0.25Fe3(BO3)4 in the region of the 5I8→5F5 absorption band of Ho ions were investigated depending on temperature in the range of 5–20 K. Absorption spectra are decomposed into components of the Lorentz form. The spin-reorientation phase transition was detected at 6.9 K. The observed line position shifts during the reorientation transition were different for different lines, which indicated different local magnetic anisotropy of the Ho ion in its excited states. Significant changes in absorption line intensities as a function of temperature were observed during the reorientation transition and above. These were explained as a consequence of the change in even components of the local crystal field in excited states. These components mix the closely spaced 4f states. Distortion of local symmetry in the ground state was detected at one of the electron transitions.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Sukhachev, A. L.; Сухачев, Александр Леонидович; Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Kuchesheva-Titova, V. R.; Кучешева-Титова, Вероника Романовна
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Спектры поглощения кристалла HOAl3(BO3)4 в области переходов 5I8→5F3 и 5F2 / В. В. Соколов, А. В. Малаховский, А. Л. Сухачев, И. А. Гудим // Невская фотоника-2023 : материалы Всероссийской научной конференции с международным участием. - СПб., 2023. - С. 257. - Библиогр.: 3

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Держатели документа:
Институт физики им. Л.В. Киренского СО РАН

Доп.точки доступа:
Соколов, В. В.; Малаховский, Александр Валентинович; Malakhovskii, A. V.; Сухачев, Александр Леонидович; Sukhachev, A. L.; Гудим, Ирина Анатольевна; Gudim, I. A.; "Невская фотоника-2023", Всероссийская научная конференция с международным участием(1 ; 2023 ; 9-13 окт. ; Санкт-Петербург); Университет ИТМО
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Magnetic circular dichroism of f-f transitions in multiferroic antiferromagnet Ho0.75Nd0.25Fe3(BO3)4 / A. V. Malakhovskii, V. V. Sokolov, A. L. Sukhachev, I. A. Gudim // International conference "Functional materials" : book of abstracts / ed. V. N. Berzhansky ; org. com. S. G. Ovchinnikov [et al.]. - Simferopol, 2023. - P. 100-101. - Cited References: 2

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Держатели документа:
Kirensky Institute of Physics, FRC KSC SB RAS,

Доп.точки доступа:
Berzhansky, V. N. \ed.\; Бержанский, Владимир Наумович; Ovchinnikov, S. G. \org. com.\; Овчинников, Сергей Геннадьевич; Malakhovskii, A. V.; Малаховский, Александр Валентинович; Sokolov, V. V.; Соколов, Валерий Владимирович; Sukhachev, A. L.; Сухачев, Александр Леонидович; Gudim, I. A.; Гудим, Ирина Анатольевна; "Functional materials", International conference(2023 ; Oct. 2-6 ; Crimea, Foros); Крымский федеральный университет имени В.И. Вернадского
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Magnetic circular dichroism and absorption of a HoAl3(BO3)4 crystal in the region of 5I8 → 5I3 and 5F2 transitions / V. V. Sokolov, A. V. Malakhovskii, A. L. Sukhachev, I. A. Gudim // VIII Euro-Asian symposium "Trends in magnetism" (EASTMAG-2022) : Book of abstracts / program com. S. G. Ovchinnikov [et al.]. - 2022. - Vol. 1, Sect. : Magnetotransport, magnetooptics and magnetophotonics. - Ст. D.P16. - P. 470-471. - Cited References: 4 . - ISBN 978-5-94469-051-7

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russia

Доп.точки доступа:
Ovchinnikov, S. G. \program com.\; Овчинников, Сергей Геннадьевич; Sokolov, V. V.; Соколов, Валерий Владимирович; Malakhovskii, A. V.; Малаховский, Александр Валентинович; Sukhachev, A. L.; Сухачев, Александр Леонидович; Gudim, I. A.; Гудим, Ирина Анатольевна; Российская академия наук; Физико-технический институт им. Е.К. Завойского ФИЦ Казанского научного центра РАН; Казанский (Приволжский) федеральный университет; Euro-Asian Symposium "Trends in MAGnetism"(8 ; 2022 ; Aug. ; 22-26 ; Kazan); "Trends in MAGnetism", Euro-Asian Symposium(8 ; 2022 ; Aug. ; 22-26 ; Kazan)
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Erratum to: Comparison of the absorption spectra of Nd3+ ions in the NdFe3(BO3)4, Nd0.5Gd0.5Fe3(BO3)4, and Ho0.75Nd0.25Fe3(BO3)4 crystals (Physics of the Solid State, (2021), 63, 1, (113-121), 10.1134/S1063783421010200) / A. L. Sukhachev, A. V. Malakhovskii, C. S. Nelson [et al.] // Phys. Solid State. - 2021. - Vol. 63, Is. 3. - P. 511, DOI 10.1134/S1063783421030203 . - ISSN 1063-7834
Аннотация: Section Funding should read as follows: The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project No. 19-42-240003 “Influence of the local environment on magnetooptical properties of f-f transitions in rare-earth aluminum and iron borates” and the Russian Foundation for Basic Research, project No. 19-02-00034.

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Держатели документа:
Kirensky Institute of Physics, FRC KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, N.Y. 11973, United States

Доп.точки доступа:
Sukhachev, A. L.; Сухачев, Александр Леонидович; Malakhovskii, A. V.; Малаховский, Александр Валентинович; Nelson, C. S.; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович
}
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Magnetic linear dichroism and features of the local magnetic structure of HoFe3(BO3)4 single crystal in 5F2 and 5F3 excited states of Ho3+ ion / A. V. Malakhovskii, S. L. Gnatchenko, I. S. Kachur [et al.] // J. Magn. Magn. Mater. - 2021. - Vol. 536. - Ст. 168106, DOI 10.1016/j.jmmm.2021.168106. - Cited References: 22. - A.V. Malakhovskii acknowledges the financing of the reported study by the Russian Foundation for Basic Researches grant 19-02-00034 and by the Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project: number 19-42-240003 “Influence of the local environment on magneto-optical properties of f-f transitions in rare-earth aluminum and iron borates” . - ISSN 0304-8853
Кл.слова (ненормированные):
Magnetic linear dichroism -- F-f transitions -- Excited states -- Local magnetic properties
Аннотация: We measured spectra of magnetic linear dichroism (MLD) of 5I8 → 5F2, 5F3 transitions in the basal plane of the HoFe3(BO3)4 single crystal in the light propagated along the trigonal c-axis at temperature 2 K as a function of magnetic field 0 – 65 kOe directed along a and b axes. The substantial anisotropy of the MLD in the basal plane was revealed. The anisotropy of the MLD is strongly different for different electron transitions, that is, the MLD is mainly connected with the excited electron states. Transformations of the MLD spectra permitted us to retrace variations of the Ho ion magnetic moment orientation in different excited electron states as a function of the magnetic field. It was shown that in the excited states the local Ho magnetic moments do not reveal reorientation transitions synchronously with that of the Fe-sublattice. A small splitting of the ground doublet of the Ho3+ ion was observed during certain electron transitions. This means that during these electron transitions the local crystal field can change not only in the excited but in the ground state as well.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
B. Verkin Institute for Low Temperature Physics and Engineering, National Academy of Sciences of Ukraine, Kharkov, 61103, Ukraine

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Gnatchenko, S. L.; Kachur, I. S.; Piryatinskaya, V. G.; Gudim, I. A.; Гудим, Ирина Анатольевна
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Malakhovskii, A. V.
Magnetic circular dichroism of 5I8→ 5F3, 5F2 and 3K8 transitions in Na0.4Ho0.6F2.2 single crystal / A. V. Malakhovskii, V. V. Sokolov, D. N. Karimov // Opt. Mater. - 2021. - Vol. 114. - Ст. 110953, DOI 10.1016/j.optmat.2021.110953. - Cited References: 23. - A.V. Malakhovskii and V.V. Sokolov acknowledge the financing of the reported study by the Russian Foundation for Basic Researches grant 19-02-00034 and by the Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project: number 19-42-240003 “Influence of the local environment on magneto-optical properties of f-f transitions in rare-earth aluminum and iron borates.” D.N. Karimov acknowledges the financing support by the Ministry of Science and Higher Education of Russia within the State assignment FSRC «Crystallography and Photonics» of Russian Academy of Sciences . - ISSN 0925-3467
Кл.слова (ненормированные):
Magnetic circular dichroism -- f-f transitions -- Fluoride crystals Ho3+ ions
Аннотация: We measured optical absorption and magnetic circular dichroism spectra of Na0.4Ho0.6F2.2 single crystal in the region of 5I8→ 5F3, 5F2 and 3K8 transitions in Ho3+ ion at 90 K and room temperature. Paramagnetic magneto-optical activities (MOA) of the transitions were found for these two temperatures and compared with the theory based on the nature of f-f transitions allowance. It was shown that nature of allowance of three considered transitions is different. The MCD spectra were also analyzed in approximation of the |J, ±MJ› wave functions of the free atom and using concept of the crystal quantum number. Using this concept and experimental paramagnetic MOA, we found that MJeff = 2.1 for the initial state of the 5I8→ 5F3 transition.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Federal Scientific Research Centre «Crystallography and Photonics» of Russian Academy of Sciences, Leninskiy Prospekt 59, Moscow, 119333, Russian Federation

Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Karimov, D. N.; Малаховский, Александр Валентинович
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10.

Comparison of the absorption spectra of Nd3+ ions in the NdFe3(BO3)4, Nd0.5Gd0.5Fe3(BO3)4, and Ho0.75Nd0.25Fe3(BO3)4 crystals / A. L. Sukhachev, A. V. Malakhovskii, C. S. Nelson [et al.] // Phys. Solid State. - 2021. - Vol. 63, Is. 1. - P. 113-121, DOI 10.1134/S1063783421010200. - Cited References: 21. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project: number 19-42-240003 “Influence of the local en-vironment on magneto-optical properties of f–f transitions in rare-earth aluminum and iron borates” . - ISSN 1063-7834
Кл.слова (ненормированные):
neodymium -- hantite-structure ferroborates -- f–f electronic transitions -- structural transition
Аннотация: The polarized optical absorption spectra in the region of a series of the f–f transitions of Nd3+ ions in the Ho0.75Nd0.25Fe3(BO3)4, Nd0.5Gd0.5Fe3(BO3)4, and NdFe3(BO3)4 crystals at 90 K have been compared. The spectral features related to the difference in the local environment of Nd3+ ions in these crystals have been established. In the region of the transition 4I9/2 → 4G5/2 + 2G7/2 of Nd3+ ions in the Ho0.75Nd0.25Fe3(BO3)4 crystal, the appearance of some absorption lines at the structural transition R32 → P3121 around ~200 K due to the local symmetry variation has been found. The intensity of these lines smoothly increases with a decrease in temperature from the transition point. The temperature dependence of the lattice parameters of the Ho0.75Nd0.25Fe3(BO3)4 crystal has been measured. It has been found that, at the transition temperature, the lattice parameter a changes stepwise, which is indicative of the occurrence of a first-order phase transition. The lattice parameter c changes smoothly.

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Публикация на русском языке Сравнение спектров поглощения ионов Nd3+ в кристаллах NdFe3(BO3)4, Nd0.5Gd0.5Fe3(BO3)4 и Ho0.75Nd0.25Fe3(BO3)4 [Текст] / А. Л. Сухачев, А. В. Малаховский, C. S. Nelson [и др.] // Физ. тверд. тела. - 2021. - Т. 63 Вып. 1. - С. 111-119

Держатели документа:
Kirensky Institute of Physics, FRC KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY 11973, United States

Доп.точки доступа:
Sukhachev, A. L.; Сухачев, Александр Леонидович; Malakhovskii, A. V.; Малаховский, Александр Валентинович; Nelson, C. S.; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович
}
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