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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Balaev D. A., Semenov S. V., Pochekutov M. A.
Заглавие : Anisotropy of the magnetoresistance hysteresis in the granular superconductor Y-Ba-Cu-O at different magnetic-field and transport-current orientations
Место публикации : J. Appl. Phys.: American Institute of Physics, 2017. - Vol. 122, Is. 12. - Ст.123902. - ISSN 00218979 (ISSN), DOI 10.1063/1.4986253
Примечания : Cited References: 45. - This study was supported by the Russian Foundation for Basic Research, Government of the Krasnoyarsk Territory, Krasnoyarsk Region Science and Technology Support Fund to the research project No. 16-48-243018.
Ключевые слова (''Своб.индексиров.''): anisotropy--high temperature superconductors--hysteresis--magnetic fields--magnetic flux--magnetism--magnetoresistance--different-magnetic fields--external magnetic field--granular superconductors--macroscopic transport--magnetic flux compression--magneto transport properties--model representation--transport currents--superconducting materials
Аннотация: Dissipation in granular high-temperature superconductors (HTSs) during the passage of macroscopic transport current j is mainly determined by carrier tunneling through intergrain boundaries (Josephson junctions). In the presence of external magnetic field H, it is necessary to take into account the significant magnetic flux compression, which can lead to the situation when the effective field Beff in the intergrain boundaries exceeds the external field by an order of magnitude. This is observed as a wide hysteresis of the field dependence of magnetoresistance R(H). In this study, we investigate the R(H) hysteresis evolution in granular 1-2-3 HTSs in different j-H orientations. The magnetic flux compression significantly affects the magnetoresistance and its hysteresis for both perpendicular (H ⊥ j) and parallel (H ∥ j) orientations. The obtained experimental data on the R(H) hysteresis at the arbitrary angles θ = ∠H, j are explained using the approach developed for describing the magnetoresistance hysteresis in granular HTSs with regard to the magnetic flux compression and the model representations proposed by Daghero et al. [Phys. Rev. B 66(13), 11478 (2002)]. A concept of the effective field in the intergrain medium explains the well-known anisotropy of the magnetotransport properties of granular HTSs.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Коржнева, Ксения Евгеньевна, Исаенко Л. И., Елисеев, Александр Павлович, Молокеев, Максим Сергеевич
Заглавие : Экспериментальное исследование процессов кристаллизации K2Ba(NO3)4 из раствор-расплава
Место публикации : Фундамент. пробл. совр. материаловед. - 2018. - Т. 15, № 1. - С. 11-15. - ISSN 1811-1416, DOI 10.25712/ASTU.1811-1416.2018.01.001
Примечания : Библиогр.: 7. - Работа выполнена в рамках государственного задания, проект № 0330 - 2016 - 0008 и при поддержке Российского фонда фундаментальных исследований (грант № 18-32-00359).
Ключевые слова (''Своб.индексиров.''): рост из раствор-расплава--двойные соединения--нецентросимметричные кристаллы k2ba(no3)4--рентгенофазовый и термический анализы--оптическое пропускание--growth from solution-melt--double compounds--noncentrosymmetrical crystals k2ba(no3)4--x-ray diffraction and thermal analysis--optical transmittance
Аннотация: С развитием технологий неуклонно возрастает потребность в высокоэффективных функциональных материалах. Поэтому все более важной и актуальной становится задача разработки принципов и алгоритмов поиска этих материалов. В настоящее время системы двойных нитратов привлекают внимание исследователей тем, что в этой группе существуют двойные соединения с нецентросимметричной структурой, которые рассматриваются как перспективные нелинейные материалы для коротковолнового диапазона. В результате проведенных ранее исследований из водных растворов были получены кристаллы K2Ba(NO3)4. Было выявлено, что K2Ba(NO3)4 при температуре 197,3 оС разлагается на KNO3 и Ba(NO3)2. Из-за большого количества дефектов (дендриты, зарастание основными гранями роста) оптическое качество этих кристаллов оказалось невысоким. Что обусловило необходимость поиска новых методик выращивания, обеспечивающих получение качественных оптически прозрачных кристаллов. Поэтому нами исследовались процессы кристаллизации K2Ba(NO3)4 из раствор-расплава. Подобран растворитель состава LiNO3-CsNO3-KNO3 с температурой эвтектик ниже температуры разложения двойного соединения. Выращены прозрачные кристаллы K2Ba(NO3)4 размером до 0,7 мм, определена их структура, показано отсутствие у них центра симметрии. На данных кристаллах были сняты спектры оптического пропускания. Исследование двух спектров данного соединения выращенного разными методами показало, что кристаллы, полученные из водных растворов, прозрачен от 0,25 мкм до 2,2 мкм, при этом наблюдается пик поглощения с максимум 0,3 мкм. Кристаллы, выращенные методом из раствор-расплава, прозрачны от 0,3 мкм до 2,2 мкм. Ширина запрещенной зоны составляет около 5 эВ.With the development of technology, the need for highly efficient functional materials is steadily increasing. Therefore, the developing of principles and algorithms for these materials' search becomes more and more important and actual. Currently systems of double nitrates attract researchers attention due to the double compounds with a noncentrosymmetric structure which are considered as promising nonlinear materials for the short-wave range. As a result of previous studies K2Ba(NO3)4 crystals were obtained from aqueous solutions. It was found that K2Ba(NO3)4 decomposes on KNO3 and Ba(NO3)2 at the temperature of 197.3 oC. Due to the large amount of defects (dendrites, overgrowing by the main growth facets), the optical quality of these crystals was not high. This necessitated the search for new growth techniques that provide the production of high-quality optically transparent crystals. Therefore, we investigated the processes of crystallization of K2Ba(NO3)4 from a solution-melt. A solvent of the LiNO3-CsNO3-KNO3 composition with a eutectic temperature below the decomposition temperature of the double compound was chosen. Transparent crystals of K2Ba(NO3)4 up to 0.7 mm in size were grown, their structure was determined, and the absence of center of symmetry was shown. The optical transmission spectra were investigated on these crystals. The study of two spectra of this compound grown by different methods showed that crystals obtained from aqueous solutions are transparent from 0.25 μm to 2.2 μm, with an absorption peak with a maximum of 0.3 μm. Crystals grown by the solution-melt method are transparent from 0.3 μm to 2.2 μm. The width of the band gap is about 5 eV.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhou Z., Zhang N., Chen J., Zhou X., Molokeev M. S., Guo C.
Заглавие : The Vis-NIR multicolor emitting phosphor Ba4Gd3Na3(PO4)6F2: Eu2+, Pr3+ for LED towards plant growth
Место публикации : J. Ind. Eng. Chem. - 2018. - Vol. 65. - P.411-417. - ISSN 1226086X (ISSN), DOI 10.1016/j.jiec.2018.05.014
Примечания : Cited References: 36. - This work was supported by National Natural Science Foundation of China (No. 11704312, 11274251), Research Fund for the Doctoral Program of Higher Education of China (RFDP) (No.20136101110017), Foundation of Key Laboratory of Photoelectric Technology in Shaanxi Province (15JS101).
Ключевые слова (''Своб.индексиров.''): phosphor--plant growth--leds--energy transfer
Аннотация: Photosynthesis process is the basic for plant growth, which needs energy from the light. The pigments of chlorophyll a, b and bacteriochlorophyll are responsible for the absorption of light, in which blue, red and near-infrared (NIR) light directly or indirectly promote the plant growth and enhancement of nurtiments. It is important for plant to support absorbable light, and phosphhor-converted light emitting diodes (pc-LEDs) are low-cost, energy-saving and enviromental friendly devices for plant growth. To develop a phosphor with emission covering the blue, red and NIR, a series of phosphors Ba4Gd3Na3(PO4)6F2: Eu2+, Pr3+ with blue, red and NIR multi-emitting were prepared. Their emissions not only match well with the absorption spectra of pigments in the plant, but also could be excited by near ultraviolet (n-UV) LED chip. The crystal structure of host Ba4Gd3Na3(PO4)6F2 was refined from the XRD data and three different crystallographic sites occupied by Eu2+ were determined through low temperature photoluminescence spectra. The energy transfer from Eu2+ to Pr3+ ions was also discussed in detail. Results indicated that the multi-emitting Ba4Gd3Na3(PO4)6F2: Eu2+, Pr3+ can serve as a phosphor candidate for plant growth LEDs.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Velikanov D. A., Rabinovich K. S., Samoilenko L. L.
Заглавие : Magnetic properties of Ba2Cu3O4Cl2
Коллективы : Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium, Институт физики им. Л.В. Киренского Сибирского отделения РАН
Место публикации : VI Euro-Asian Symposium "Trends in MAGnetism" (EASTMAG-2016): abstracts/ ed.: O. A. Maksimova, R. D. Ivantsov. - Krasnoyarsk: KIP RAS SB, 2016. - Ст.P2.16. - P.158. - ISBN 978-5-904603-06-9 (Шифр -478014040)
Примечания : References: 4
Ключевые слова (''Своб.индексиров.''): layered cuprate--magnetic moment--coercivity--remanence--weak ferromagnet
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Velikanov D. A., Rabinovich K. S., Samoilenko L. L.
Заглавие : Magnetic properties of Ba2Cu3O4Cl2
Коллективы : "Магнитные материалы. Новые технологии", Байкальская международная конференция, "Magnetic materials. New tecnologies", Baikal International Conference, Байкальская международная конференция "Магнитные материалы. Новые технологии", Иркутский государственный университет
Место публикации : Магнитные материалы. Новые технологии: тез. докл. VII Байкал. Междунар. конф./ Иркутский гос. ун-т. - Иркутск, 2016. - P.224. - ISBN 978-591-345-152-1: тез. докл. VII Байкал. Междунар. конф. BICMM-2016/ "Magnetic materials. New tecnologies", Baikal International Conference (7 ; 2016 ; Aug. ; 22–26 ; Listvyanka, Irkutsk region), Иркутский гос. ун-т; чл. прогр. ком.: Р. С. Исхаков, С. С. Аплеснин, С. Г. Овчинников. - ISBN 978-591-345-152-1
Примечания : Библиогр.: 5 назв. - The work was supported by Russian Foundation for Basic Research. Project 16-03-00256
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Atuchin V. V., Molokeev M. S., Park, Hee Kook, Lee, Beom Hyun, Won, Dong Min, Oh, Won-Chun, Lim, Chang Sung
Заглавие : Microwave sol-gel derived MMoO4 (M=Ba,Cs,Sr) nanoparticles doped with Er/Yb, Ho/Yb, Ho/Yb/Tm and their upconversion photoluminescence properties for biomedical applications
Коллективы : International Conference on Multifunctional Materials and Application
Место публикации : The 10th International conference on multifunctional materials and application. - 2016. - Ст.43-P. - P.76
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shtarev D. S., Shtareva, A., V, Kevorkyants R., Rudakova, A., V, Molokeev M. S., Bakiev, T., V, Bulanin K. M., Ryabchuk V. K., Serpone N.
Заглавие : Materials synthesis, characterization and DFT calculations of the visible-light-active perovskite-like barium bismuthate Ba1.264(4)Bi1.971(4)O4 photocatalyst
Коллективы : Russian Science FoundationRussian Science Foundation (RSF) [19-73-10013]; Saint-Petersburg State University [39054581]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [18-03-00855]
Место публикации : J. Mater. Chem. C. - 2020. - Vol. 8, Is. 10. - P.3509-3519. - ISSN 2050-7526, DOI 10.1039/c9tc06457e. - ISSN 2050-7534(eISSN)
Примечания : Cited References: 42. - The current research was kindly funded by a grant from the Russian Science Foundation (project No. 19-73-10013). R. K., A. V. R., V. K. R. and T. V. B. acknowledge financial support from Saint-Petersburg State University (Pure ID 39054581). A. V. R. thanks the Russian Foundation for Basic Research for a Grant No. 18-03-00855 that supported studies into the photoinduced hydrophilicity of the bismuthate. The authors are further grateful to the staff of the Khabarovsk Innovation and Analytical Center of the Yu. A. Kosygin Institute of Tectonics and Geophysics of the Far Eastern Branch of the Russian Academy of Sciences, and the Resource Centers of the Research Park at the Saint-Petersburg State University: (i) the Center for Diagnostics of Functional Materials for Medicine, Pharmacology and Nanoelectronics, (ii) the Center for Physical Methods of Surface Investigation, (iii) the Center for Optical and Laser Materials Research, and the laboratories of (iv) Nanotechnology and (v) Nanophotonics for their valuable assistance in carrying out the research and in providing the needed equipment. One of us (N.S.) is grateful to Prof. Angelo Albini and the staff of the PhotoGreen Laboratory at the University of Pavia, Italy, for their continued hospitality.
Предметные рубрики: OXIDE
NIO/SRBI2O4
SPECTRA
DRIVEN
CO2
LA
Аннотация: A perovskite-like barium bismuthate of the BaBi2O4 class, Ba1.264(4)Bi1.971(4)O4, has been prepared by solid-state synthesis and subsequently characterized by a number of experimental techniques (XPS, DRS, SEM, EDX and Raman spectroscopy), as well as by a DFT computational approach using the GGA Perdew–Burke–Ernzerhof (PBE) density functional to determine the energy band structure. XRD peaks were indexed to a rhombohedral cell (R[3 with combining macron]m) with parameters close to Ba0.156Bi0.844O1.422 (i.e., to Ba0.439Bi2.374O4), which upon Rietveld refinement gave Ba1.264(4)Bi1.971(4)O4. The Bi–O bond lengths determined from this refinement (1.86 and 2.31 Å) accorded with the bond lengths estimated from Raman spectra (1.97 and 2.26 Å). DFT calculations revealed the bismuthate to display two bandgaps that correspond to lower-energy indirect (2.28 eV) and to higher-energy direct (2.36 eV) electronic transitions in good agreement with the experimental bandgaps of 2.26 eV and 2.43 eV, respectively, from Tauc plots of DRS spectra. Relative to the indirect bandgap energy of 2.26 eV, the energies of the valence band and of the conduction band were, respectively, +1.14 eV and −1.12 eV. The photoactivity of Ba1.264(4)Bi1.971(4)O4 was examined toward the photoreduction of the greenhouse gas CO2 in aqueous media photoelectrochemically yielding alcohols and alkanes, while in the gas phase in an infrared cell reactor the products were carbon monoxide and alkanes.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhang, Guangqing, Molokeev M. S., Ma, Qianchao, Yang, Xuening, Han, Shuiquan, Chen, Q.i., Zhong, Binnian, Ma, Bin
Заглавие : Structural analysis and optical temperature sensing performance of Eu3+-doped Ba3In(PO4)3
Место публикации : CrystEngComm. - 2020. - Vol. 22, Is. 35. - P.5809-5817. - ISSN 1466-8033, DOI 10.1039/d0ce00997k
Примечания : Cited References: 52. - This work was supported by the National Natural Science Foundation of China (Grant No. 51802172) and the Qinghai Provincial Natural Science Foundation for Young Scholars (No. 2018-ZJ-957Q)
Предметные рубрики: FLUORESCENCE INTENSITY RATIO
UP-CONVERSION EMISSIONS
RARE-EARTH IONS
Аннотация: Eu3+-Doped Ba3In(PO4)3 was synthesized through a high-temperature solid-phase method. According to the structure refinement based on X-ray diffraction and density functional theory, the crystal and energy band structures of Ba3In(1−x)(PO4)3:xEu3+ were studied and analyzed in detail. The effect of Eu3+ doping concentrations on emission was studied at an excitation wavelength of 393 nm. For the material Ba3In(1−x)(PO4)3:xEu3+(x = 0.01–0.30), the optimal doping level is confirmed to be 0.18. Due to the thermal quenching differences of Eu3+ at the 5D0 and 5D1 energy levels, and based on the temperature-variable fluorescence intensity ratio between emission peaks, the optical temperature measurement performance of this material in the temperature range from 298.15 K to 623.15 K was characterized, and the maximum absolute and relative sensor sensitivities (Sa and Sr) were determined to be 0.1002 K−1 and 4.058%, respectively. With temperature as the only variable, the color of the phosphor changes from red to yellow light with rising temperature. Besides, Sa and Sr values of this phosphor are comparable to other sensing materials. The results indicate that Eu3+-doped Ba3In(PO4)3 phosphors have great potential to be applied in optical temperature sensing.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yang, Zhiyu, Zhou, Yayun, Qiao, Jianwei, Molokeev M. S., Xia, Zhiguo
Заглавие : Rapid synthesis of red-emitting Sr2Sc0.5Ga1.5O5:Eu2+ phosphors and the tunable photoluminescence via Sr/Ba substitution
Место публикации : Adv. Opt. Mater. - 2021. - Vol. 9. Is. 16. - Ст.2100131. - ISSN 2195-1071, DOI 10.1002/adom.202100131
Примечания : Cited References: 44. - Z.Y. and Y.Z. contributed equally to this work. This research was supported by the National Natural Science Foundations of China (Grant Nos. 51972118 and 51961145101), International Cooperation Project of National Key Research and Development Program of China (No. 2021YFE0105700), Guangzhou Science & Technology Project (No. 202007020005), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (No. 2017BT01x137). This work was also funded by RFBR according to the research Project No. 19-52-80003
Предметные рубрики: LUMINESCENCE PROPERTIES
THERMAL-STABILITY
EU2+
GREEN
EU3+
SR
Аннотация: Discovering new Eu2+-doped red-emitting phosphors in oxide-based materials is a challenge for white light-emitting diode (WLED) applications. Herein, a highly efficient high-frequency induction heating method is employed to rapidly prepare the red-emitting Sr2Sc0.5Ga1.5O5:Eu2+ phosphors peaking at 614 nm and exhibiting a high photoluminescence quantum yield of 78.4% under the excitation of 440 nm. The structural and spectral analyses suggest that Eu2+ ions tend to enter the [Sc1/Ga1O6] and [Ga2O6] polyhedrons with small coordination numbers, leading to the broadband red emission originated from large crystal field splitting of Eu2+ 5d level. The chemical substitution of Ba in the Sr site enhances the thermal stability and helps to the photoluminescence tuning from 614 to 728 nm in SrBaSc0.5Ga1.5O5:Eu2+. The WLED device fabricated by blending the red Sr1.7Ba0.3Sc0.5Ga1.5O5:Eu2+ and yellow Y3(Al, Ga)5O12:Ce3+ phosphors shows a high color-rendering index (Ra = 91.1), and low color-correlated temperature (CCT = 4750 K). This study aims to provide a new synthesis method and design principle for guiding the development of Eu2+-doped oxide-based red phosphors with low preparation cost; moreover, the photoluminescence tuning strategy via cation substitutions is essential to achieve tunable emission, even the near-infrared luminescence.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Xiang J., Zheng J., Zhou Z., Suo H., Zhao X., Zhou X., Zhang N., Molokeev M. S., Guo C.
Заглавие : Enhancement of red emission and site analysis in Eu2+ doped new-type structure Ba3CaK(PO4)3 for plant growth white LEDs
Место публикации : Chem. Eng. J. - 2019. - Vol. 356. - P.236-244. - ISSN 13858947 (ISSN) , DOI 10.1016/j.cej.2018.09.036
Примечания : Cited References: 42. - This work was supported by National Natural Science Foundation of China (No. 11704312 , 51672215 , 11274251 ), Research Fund for the Doctoral Program of Higher Education of China (RFDP) (No. 20136101110017) and by RFBR (17-52-53031).
Ключевые слова (''Своб.индексиров.''): phosphor--ba3cak(po4)3--sites-dependent photoluminescence--plant growth--white leds
Аннотация: A novel compound Ba3CaK(PO4)3 (BCKP) with new-type structure was synthesized and its structure was determined by X-ray diffraction Rietveld refinement, in which crystal structure consists of Ba1O9, Ba2O12, Ba3O9, CaO8 and KO10 polyhedra, that's five cationic sites. As a phosphor host, Eu2+ doped BCKP emits cold white light with about 90% quantum efficiency (QE) through entering different cationic sites. Based on the results of refinement, three Eu2+ luminescence centers in sites Ca, Ba2 and K were clearly assigned in Eu2+ solely doped BCKP by the time-resolved emission spectra (TRES), Van Uitert equation, but the emissions of Eu2+ at Ba1 and Ba3 sites are not easy to be determined for the same coordination number (CN). According to their different spatial distribution of the coordinated atoms, the first-principles calculation was used to compute the d orbital splitting energy of Eu2+ ions in Ba1 and Ba3 sites to accurately distinguish the ambiguous luminescence centers. In order to meet the requirement of plant growth spectra, Mn2+ was introduced into BCKP: Eu2+ to enhance the red component of spectra, which not only perfectly match with the absorption spectra of carotenoid and chlorophyll-b, but also LEDs fabricated through combining 365 nm near ultraviolet (n-UV) chip with BCKP: Eu2+, Mn2+ phosphor exhibit excellent parameters including high color rendering index (Ra) (92), excellent correlated color temperature (CCT) (4486 K) and outstanding QE up to 65%. Results confirmed that BCKP: Eu2+/Mn2+ phosphor with great potential applications in white LEDs and plant growth.
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