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Автор(ы) : Yang, Zhiyu, Zhou, Yayun, Qiao, Jianwei, Molokeev M. S., Xia, Zhiguo
Заглавие : Rapid synthesis of red-emitting Sr2Sc0.5Ga1.5O5:Eu2+ phosphors and the tunable photoluminescence via Sr/Ba substitution
Место публикации : Adv. Opt. Mater. - 2021. - Vol. 9. Is. 16. - Ст.2100131. - ISSN 2195-1071, DOI 10.1002/adom.202100131
Примечания : Cited References: 44. - Z.Y. and Y.Z. contributed equally to this work. This research was supported by the National Natural Science Foundations of China (Grant Nos. 51972118 and 51961145101), International Cooperation Project of National Key Research and Development Program of China (No. 2021YFE0105700), Guangzhou Science & Technology Project (No. 202007020005), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (No. 2017BT01x137). This work was also funded by RFBR according to the research Project No. 19-52-80003
Предметные рубрики: LUMINESCENCE PROPERTIES
THERMAL-STABILITY
EU2+
GREEN
EU3+
SR
Аннотация: Discovering new Eu2+-doped red-emitting phosphors in oxide-based materials is a challenge for white light-emitting diode (WLED) applications. Herein, a highly efficient high-frequency induction heating method is employed to rapidly prepare the red-emitting Sr2Sc0.5Ga1.5O5:Eu2+ phosphors peaking at 614 nm and exhibiting a high photoluminescence quantum yield of 78.4% under the excitation of 440 nm. The structural and spectral analyses suggest that Eu2+ ions tend to enter the [Sc1/Ga1O6] and [Ga2O6] polyhedrons with small coordination numbers, leading to the broadband red emission originated from large crystal field splitting of Eu2+ 5d level. The chemical substitution of Ba in the Sr site enhances the thermal stability and helps to the photoluminescence tuning from 614 to 728 nm in SrBaSc0.5Ga1.5O5:Eu2+. The WLED device fabricated by blending the red Sr1.7Ba0.3Sc0.5Ga1.5O5:Eu2+ and yellow Y3(Al, Ga)5O12:Ce3+ phosphors shows a high color-rendering index (Ra = 91.1), and low color-correlated temperature (CCT = 4750 K). This study aims to provide a new synthesis method and design principle for guiding the development of Eu2+-doped oxide-based red phosphors with low preparation cost; moreover, the photoluminescence tuning strategy via cation substitutions is essential to achieve tunable emission, even the near-infrared luminescence.
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