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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gorev M. V., Bogdanov E. V., Flerov I. N., Voronov V. N., Laptev Y. V.
Заглавие : Barocaloric effect and phase transitions in oxyfluorides Rb2KTiOF5 and (NH4)2NbO5F
Коллективы : Воронежский государственный технический университет, Российская академия наук, International Seminar on ferroelastic physics (6; 2009 ; Sept. 22-25; Voronezh), Международный семинар по физике сегнетоэластиков (6(11); 2009 ; 22-25 сент.; Воронеж)
Место публикации : The 6th International Seminar on Ferroelastic Physics: abstract book. - Voronezh, 2009. - P.22
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Fokina V. D., Flerov I. N., Molokeev M. S., Pogoreltsev E. I., Bogdanov E. V., Laptev Y. V.
Заглавие : Effect of central cation substitutionon the properties and phase transitions in (NH4)3Me(O2)2F4 oxyfluorides
Коллективы : Воронежский государственный технический университет, Российская академия наук, International Seminar on ferroelastic physics (6; 2009 ; Sept. 22-25; Voronezh), Международный семинар по физике сегнетоэластиков (6(11); 2009 ; 22-25 сент.; Воронеж)
Место публикации : The 6th International Seminar on Ferroelastic Physics: abstract book. - Voronezh, 2009. - P.5
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Kolesnikova E. M., Sofronova S. N.
Заглавие : Nonempirical calculation lattice dynamics of oxyfluorides A2KWO3F3 (A= Cs, K, Rb)
Коллективы : Russia/CIS/Baltic/Japan Symposium on Ferroelectricity
Место публикации : Abstracts of the 10th Russia/CIS/Baltic/Japan Symposium on Ferroelectricity. - 2010. - P.171
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Flerov I. N., Gorev M. V., Fokina V. D., Bovina A. F., Bogdanov E. V., Pogoreltsev E. I., Laptash N. M.
Заглавие : Disorder and phase transitions in oxyfluoride (NH4)(3)Ta(O-2)(2)F-4
Место публикации : J. Fluor. Chem. - 2011. - Vol. 132, Is. 10. - P.713-718. - ISSN 0022-1139, DOI 10.1016/j.jfluchem.2011.05.012
Примечания : Cited Reference Count: 19. - Гранты: This work was supported by the Council on Grants from the President of the Russian Federation for the Support of Leading Scientific Schools of the Russian Federation (NSh-4645.2010.2).Финансирующая организация: Council on Grants from the President of the Russian Federation for the Support of Leading Scientific Schools of the Russian Federation [NSh-4645.2010.2]
Предметные рубрики: HEAT-CAPACITY
COMPLEXES
RB2KTIOF5
FLUORIDES
CRYOLITE
Ключевые слова (''Своб.индексиров.''): cubic oxyfluorides--structural disorder--phase transitions--entropy--permittivity--pressure effect--cubic oxyfluorides--entropy--permittivity--phase transitions--pressure effect--structural disorder
Аннотация: Calorimetric, X-ray, dielectric and DTA under pressure measurements have been performed on oxyfluoride (NH4)(3)Ta(O-2)(2)F-4. The succession of nonferroelectric phase transitions was found associated with the order-disorder processes. The comparative analysis tantalate with related niobate has revealed the important role of the central atom in the physical properties behavior, mechanism of structural distortions and barocaloric effect in oxyfluorides with the eight-coordinated anionic polyhedra. (C) 2011 Elsevier By. All rights reserved.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vtyurin A.N., Gerasimova J.V., Krylov A.S., Ivanenko A.A., Shestakov N.P., Laptash N.M., Voyt E.I.
Заглавие : Vibrational spectroscopy of alkaline tungsten oxyfluoride crystals: structure, lattice dynamics, ordering processes, and phase transitions
Место публикации : J. Raman Spectrosc. - MALDEN: WILEY-BLACKWELL, 2010. - Vol. 41, Is. 12. - С. 1784-1791. - DEC. - ISSN 0377-0486, DOI 10.1002/jrs.2637
Примечания : Cited Reference Count: 13. - Гранты: We would like to thank Prof. Igor Flerov for fruitful discussion. Technical assistance of Victor Ouskin is highly appreciated. This work has been supported by the Russian Foundation for Basic Researches, grant no. 08-02-00066-a.Финансирующая организация: Russian Foundation for Basic Researches [08-02-00066-a]
Предметные рубрики:
Ключевые слова (''Своб.индексиров.''): raman scattering--infrared absorption--alcaline tungsten oxyfluorides--phase transitions--alcaline tungsten oxyfluorides--infrared absorption--phasetransitions--raman scattering
Аннотация: Raman scattering (RS) and infrared absorption (IR) of ammonium oxyfluoride crystals (NH(4))(3)WO(3)F(3), (NH(4))(2)KWO(3)F(3), and Cs(2)(NH(4))WO(3)F(3) are compared. Conformation of the WO(3)F(3) octahedral groups has been established; anomalies have been found close to the transition temperatures in the internal vibrational regions of ammonium and WO(3)F(3) groups. The phase transition in (NH(4))(3)WO(3)F(3) is associated mostly with the ordering of octahedral groups and formation of W-O center dot center dot center dot H-N hydrogen bonds. In (NH(4))(2)KWO(3)F(3) crystal, the transition is not related to the ordering processes; CS(2)(NH(4))WO(3)F(3) retains its disordered structure down to 10 K. Copyright (C) 2010 John Wiley & Sons, Ltd.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Kolesnikova E.M., Sofronova S.N.
Заглавие : The nonemperical calculations of the lattice dynamics of the oxyfluorides A2KW03F3 (A=Cs, Rb, K)
Коллективы : European Meeting on Ferroelectricity
Место публикации : 12th European Meeting on Ferroelectricity: Abstracts. - 2011. - Ст.Pl-26
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Flerov I.N., Gorev M.V.
Заглавие : Barocaloric and piezocaloric effects in some ferroelectric and fer- roelastic oxyfluorides
Коллективы : European Meeting on Ferroelectricity
Место публикации : 12th European Meeting on Ferroelectricity: Abstracts. - 2011. - Ст.9A-20
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krylov A. S., Laptash N. M., Vtyurin A. N., Krylova S. N.
Заглавие : Phase transitions in (NH4)2MoO2F4 crystal
Коллективы : International Symposium on Two-Dimensional Correlation Spectroscopy
Место публикации : J. Mol. Struct.: Elsevier Science, 2016. - Vol. 1124, Special Issue: Novel developments and applications of two-dimensional correlation spectroscopy — A festschrift in honor of professor Isao Noda. - P.125-130. - ISSN 0022-2860, DOI 10.1016/j.molstruc.2016.03.009. - ISSN 1872-8014(eISSN)
Примечания : Cited References:17
Предметные рубрики: OXYFLUORIDE
(NH4)2WO2F4
DISORDER
DIAGRAMS
Ключевые слова (''Своб.индексиров.''): phase transitions--raman high-pressure--two-dimensional correlations--oxyfluorides
Аннотация: The mechanisms of temperature and high pressure phase transitions have been studied by Raman spectroscopy. Room temperature (295 K) experiments under high hydrostatic pressure up to 3.6 GPa for (NH4)(2) MoO2 F-4 have been carried out. Experimental data indicates a phase transition into a new high-pressure phase for (NH4)(2) MoO2 F-4 at 1.2 GPa. This phase transition is related to the ordering anion octahedron groups [MoO2 F-4](2) and is not associated with ammonium group. Raman spectra of small non-oriented crystals ranging from 10 to 350 K have been observed. The experiment shows anion groups [MoO2 F-4](2-) and ammonium in high temperature phase are disordered. The phase transition at T-1 = 269.8 K is of the first-order, close to the tricritical point. The first temperature phase transition is related to the ordering anion octahedron groups [MoO2 F-4](2-). Second phase transitions T-2 = 180 K are associated with the ordering of ammonium. The data presented within this study demonstrate that 2D correlation analysis combined with traditional Raman spectroscopy are powerful tool to study phase transitions in the crystals. (C) 2016 Elsevier B.V. All rights reserved.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Flerov I. N., Gorev M. V., Mikhaleva E. A., Kartashev A. V., Bondarev V. S.
Заглавие : Caloric Effects in Some Ferroelectric and Ferroelastic Fluorides, Oxyfluorides and Oxides
Коллективы : Russia/CIS/Baltic/Japan Symposium on Ferroelectricity, International Workshop on Relaxor Ferroelectrics
Место публикации : Joint 13th Russia/CIS/Baltic/Japan Symp. on Ferroelectricity and Int. Workshop on Relaxor Ferroelectrics (RCBJSF-IWRF 2016): book of abstracts. - 2016. - Ст.Invite-6
Примечания : References: 4. - The reported study was partially supported by RFBR, research project No. 15-02-02009 a
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bogdanov E. V., Mel'nikova S. V., Pogoreltsev E. I., Molokeev M. S., Flerov I. N.
Заглавие : The structure and phase transitions in oxyfluoride (ND4)2MoO2F4
Место публикации : Solid State Sci.: Elsevier, 2016. - Vol. 61. - P.155-160. - ISSN 12932558 (ISSN), DOI 10.1016/j.solidstatesciences.2016.08.012
Примечания : Cited References: 18. - The authors are grateful to A.G. Kocharova for the synthesis and deuteration of the samples, and to A.A. Sukhovsky and Y.N. Ivanov for the execution of NMR studies to determine the degree of sample deuteration.This study was partially supported by Russian Foundation for Basic Research, project No. 16–32–00201 mol_а.
Ключевые слова (''Своб.индексиров.''): deuterium--heavy water--single crystals--x ray analysis--crystal phasis--deuterations--distorted phasis--oxyfluorides--polarization optics--scanning microcalorimetry--tricritical point--molybdenum oxide
Аннотация: Single crystals of (ND4)2MoO2F4 containing 95% deuterium were produced by repeated recrystallization of (NH4)2MoO2F4 in heavy water. The effect of deuteration on the parameters of successive phase transitions was investigated by differential scanning microcalorimetry and polarization optics. X-ray analysis of the original and distorted phases was performed. It was found that deuteration does not change the sequence of crystal phases typical for (NH4)2MoO2F4, but leads to a shift in the phase transition Cmcm Pnma towards the tricritical point. The mechanism of phase transitions in (ND4)2MoO2F4 was associated with both the ordering and the displacement of atoms. © 2016 Elsevier Masson SAS
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Flerov I. N., Gorev M. V., Bogdanov E. V., Laptash N. M.
Заглавие : Barocaloric effect in ferroelastic fluorides and oxyfluorides
Место публикации : Ferroelectrics: Taylor and Francis, 2016. - Vol. 500, Is. 1. - P.153-163. - ISSN 00150193 (ISSN), DOI 10.1080/00150193.2016.1214525
Примечания : Библиогр.: 33. - The reported study was partially supported by the Russian Foundation for Basic Research (RFBR), research project No. 15-02-02009 a.
Ключевые слова (''Своб.индексиров.''): phase transition--fluorides--oxyfluorides--thermal properties--barocaloric effect
Аннотация: Using the data about the temperature - pressure phase diagram and the phase transition entropy at ambient and high pressure, intensive and extensive barocaloric effects were analyzed in the region of single and successive order-disorder phase transitions in fluorides and oxyfluorides with the elpasolites-cryolite structure. It was found that hydrostatic as well as chemical pressure are the effective tools to change the entropy of compounds with disordered ionic groups or atoms in structure and to realize the significant intensive and extensive barocaloric effects comparable with the values of baro- and magnetocaloric effects, characteristic for materials, considered as promising solid refrigerants. © 2016 Taylor & Francis Group, LLC.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bogdanov E. V., Pogoreltsev E. I., Kartashev A. V., Gorev M. V., Molokeev M. S., Mel'nikova S. V., Flerov I. N., Laptash N. M.
Заглавие : Thermodynamic properties of vanadium oxypentafluoride (IV) (NH4)3VOF5
Место публикации : Phys. Solid State. - 2020. - Vol. 62, Is. 7. - P.1271-1279. - ISSN 10637834 (ISSN), DOI 10.1134/S1063783420070057
Примечания : Cited References: 17. - This study was supported by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory, and the Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activity, project no. 18-42-243003 “Effect of Deuteration on Orientational Ordering and Phase Transitions in Ammonium Fluorine-Oxygen Vanadates”
Аннотация: The (NH4)3VOF5 crystals have been synthesized and their homogeneity and single-phase structure has been established by the X-ray diffraction, energy dispersive spectroscopy, and X-ray photoelectron spectroscopy studies. The investigations of the temperature dependences of specific heat, entropy, strain, and pressure susceptibility show the occurrence of three phase transitions caused by the structural transformations in the (NH4)3VOF5 crystals. The T–p phase diagram shows the temperature limits of stability of the crystalline phases implemented in (NH4)3VOF5. The optical and dielectric studies disclose the ferroelastic nature of the phase transitions. An analysis of the experimental data together with the data on the isostructural (NH4)3VO2F4 crystal makes it possible to distinguish the physical properties of oxyfluorides containing vanadium of different valences (IV and V).
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13.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Flerov I. N., Gorev M. V., Bogdanov E. V.
Заглавие : Complex fluorides and oxyfluorides: successive ferroelastic phase transitions and barocaloric effect
Коллективы : International Symposium on Solid State Chemistry for Applications and Sustainable Development, Sustainable Industrial Processing Summit and Exhibition, FLOGEN Stars Outreach
Место публикации : Tressaud Int. Symp. on Solid State Chem. for Applications and Sustainable Dev.: program. - 2019. - Ст.ChemistryFriPM106. - P.103
Примечания : Cited References: 4
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14.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gorev M. V., Bogdanov E. V., Flerov I. N.
Заглавие : Fluorides and oxyfluorides: successive ferroelastic phase transitions and barocaloric effect
Коллективы : Fall Meeting, European Materials Research Society, European Materials Research Society, Warsaw University of Technology
Место публикации : E-MRS fall meeting: conference programme. - 2019. - С. E.P.2
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bogdanov E. V., Bondarev V. S., Gorev M. V., Molokeev M. S., Flerov I. N.
Заглавие : Effect of deuteration on phase transitions in (NH4)3VOF5
Место публикации : Phys. Solid State. - 2022. - Vol. 64, Is. 3. - P.394-399. - ISSN 10637834 (ISSN), DOI 10.21883/PSS.2022.03.53195.237. - ISSN 10906460 (eISSN)
Примечания : Библиогр.: 26
Аннотация: The (ND4)3VOF5 crystal was grown with a high degree of deuteration (D≈92%). Structural and thermophysical studies have been carried out, the parameters of phase transitions have been determined. It was found that the deuteration of the ammonium cation in (NH4)3VOF5 led to a change in the chemical pressure, which was accompanied by an increase in the unit cell volume and an increase in the phase transition temperatures. The baric coefficients dTi/dp were determined and the phase T−p diagram (ND4)3VOF5 was constructed. A decrease in the temperature stability of the initial cubic phase Fm3¯m in (ND4)3VOF5, as well as a wedging out of the intermediate monoclinic phase at a lower pressure as compared to (NH4)3VOF5, was found.
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16.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vtyurin A. N., Krylov A. S., Gerasimova J. V., Ivanenko A. A., Shestakov N. P., Laptash N. M., Voit E. I.
Заглавие : Structure and ordering processes in A2BWO3F3 oxyfluorides studied by vibrational spectroscopy
Коллективы : "Advanced inorganic fluorides", International Siberian workshop
Место публикации : Advanced inorganic fluorides: the Third International Siberian workshop Intersibfluorine - 2008, September 01-06, 2008, Vladivostok, Russia : proceedings of ISIF-2008. - Vladivostok, 2008. - p.71-74. - ISBN 978-5-98128-036-8
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17.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Fokina V. D., Laptash N. M., Flerov I. N.
Заглавие : Oxyfluorides with Elpasolite-Cryolite Structure as Materials of Fundamental and Practical Interests
Коллективы : "Advanced inorganic fluorides", International Siberian workshop
Место публикации : Advanced inorganic fluorides: the Third International Siberian workshop Intersibfluorine - 2008, September 01-06, 2008, Vladivostok, Russia : proceedings of ISIF-2008. - Vladivostok, 2008. - p.29-30. - ISBN 978-5-98128-036-8
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18.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Flerov I. N.
Заглавие : Ferroelectric and ferroelastic phase transitions in some oxyfluorides A2AMOxF6-x with elpasolite-cryolite structure
Коллективы : Russia/CIS/Baltic/Japan Symposium on Ferroelectricity
Место публикации : 9th Russai/CIS/Baltic/Japan symposium on ferroelectricity: abstracts book : June 15-19, 2008, Vilnius, Lithuania. - p.113
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Flerov I. N., Gorev M. V., Bogdanov E. V., Laptash N. M.
Заглавие : The role of chemical pressure in the formation of the structure and barocaloric properties of complex fluorides and oxyfluorides
Колич.характеристики :14 с
Место публикации : Crystallogr. Rep. - 2023. - Vol. 68, Is. 5. - P.765-778. - ISSN 10637745 (ISSN), DOI 10.1134/S1063774523600485. - ISSN 1562689X (eISSN)
Примечания : Cited References: 67
Аннотация: The role of chemical pressure as an effective tool in the processes of formation of initial and distorted (as a result of structural transformations) phases, thermodynamic properties, and direct and inverse barocaloric effects in some complex oxyfluorides and fluorides with octahedral, tetrahedral, and spherical anion and cation groups in the structure has been studied. It is found that, due to the small temperature hysteresis and high baric sensitivity of materials, the maximum values of absolute and integral barocaloric characteristics can be implemented at low pressures. Correspondingly, the temperature range of reversibility of thermodynamic cycles based on fluorides/oxyfluorides as solid-state coolants can be expanded.
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20.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vasil'ev A. D., Flerov I. N., Gorev M. V., Molokeev M. S., Vasiliev A. D., Laptash N. M.
Заглавие : Effect of cationic substitution on ferroelectric and ferroelastic phase transitions in oxyfluorides A2A?WO3F3 (A, A?: K, NH4, Cs)
Место публикации : Ferroelectrics: 8th Russia/CIS/Baltic/Japan Symposium on Ferroelectricity, RCBJSF-8/ sponsors: Murata Science Foundation ; (2006 ; 15.05 - 19.05). - Tsukuba: Gordon and Breach Science Publishers, 2007. - 347. - С. 60-64. - DOI 10.1080/00150190601187039 (Шифр 15049374)
ГРНТИ : 29.19
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