Библиотека института физики им. Л.В. Киренского СО РАН

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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vtyurin A. N., Krylov A. S., Voronov V. N., Oreshonkov A. S., Krylova S. N.
Заглавие : Structural phase transitions in elpasolite-like fluorides comprising rare earth elements – Raman scattering study
Коллективы : Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Scanning Probe Microscopy, International Conference, Russia-China Workshop on Dielectric and Ferroelectric Materials, "Functional Imaging of Nanomaterials", International Youth Conference
Место публикации : 3th Int. Conf. "Scanning Probe Microscopy". 4th Russia-China Workshop on Dielectric and Ferroel. Mater. (SPM-2019-RCWDFM). Int. Youth Conf. "Functional Imaging of Nanomaterials": Abstract book of joint int. conf. - 2019. - P.29. - ISBN 978-5-9500624-2-1
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Krylov A. S., Senkovska I., Bon V., Kaske S., Slysareva E. A., Krylova S. N., Vtyurin A. N.
Заглавие : Raman spectroscopy study of the switchable phases metal-organic frameworks DUT-8(Ni)
Коллективы : Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Scanning Probe Microscopy, International Conference, Russia-China Workshop on Dielectric and Ferroelectric Materials, "Functional Imaging of Nanomaterials", International Youth Conference
Место публикации : 3th Int. Conf. "Scanning Probe Microscopy". 4th Russia-China Workshop on Dielectric and Ferroel. Mater. (SPM-2019-RCWDFM). Int. Youth Conf. "Functional Imaging of Nanomaterials": Abstract book of joint int. conf. - 2019. - Ст.P60. - P.186. - ISBN 978-5-9500624-2-1
Примечания : Cited References: 3. - Acknowledgments: I.S.,V.B., S.K. thank the DFG for financial support (FOR 2433); A.K., S.K., A.V. thank the Russian Foundation for Basic Research for financial support (18-02-00754)
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gnezdilov V., Pashkevich Yu., Kurnosov V., Zhuravlev O. V., Wulferding D., Lemmens P., Kazak N. V., Knyazev Yu. V., Ovchinnikov S. G.
Заглавие : Magnetic and structural correlations in the warwickite Mn2OBO3
Место публикации : Физ. низких температур. - 2019. - Т. 45, Вып. 9: Спеціальний випуск (Частина II) До 100-річчя з дня народження Б.І. Вєркіна. - С.1223-1230. - ISSN 01326414 (ISSN); Fiz. Nizk. Temp.
Примечания : Cited References: 28
Аннотация: We report a Raman scattering study of single-crystalline homometallic oxyborate Mn2OBO3, a compound realizing a one-dimensional ribbon-structure. Phonon excitations as a function of temperature and light polarization are compared to lattice dynamical calculations, giving evidence for a strong coupling between lattice and magnetic degrees of freedom. Furthermore, a broader feature with a distinct structure emerges at low temperatures. Based on our theoretical analysis, we assign this signal to specific two-magnon scattering processes related to high energy flat-band magnon branches.Досліджено раманівське розсіювання в монокристалі гомометалічного оксиборату Mn2OBO3 — сполуки, в якій реалізується одномірна стрічкова структура. Температурна та поляризаційна залежності фононних збуджень у порівнянні з розрахунками динаміки ґратки свідчать про сильний зв’язок між ґратковими та магнітними ступенями свободи. Широка спектральна особливість з виразною структурою виникає, крім того, при низьких температурах. Ґрунтуючись на теоретичному аналізі, цей сигнал віднесено до специфічних процесів двомагнонного розсіювання, що пов’язаний з високо-енергетичними магнонними вітками з «плоскою» дисперсією.Исследовано рамановское рассеяние в монокристалле гомометаллического оксибората Mn2OBO3 — соединения, в котором реализуется одномерная ленточная структура. Температурная и поляризационная зависимость фононных возбуждений в сравнении с расчетами динамики решетки свидетельствуют о сильной связи между решеточными и магнитными степенями свободы. Широкая спектральная особенность с отчетливой структурой возникает, кроме того, при низких температурах. Основываясь на теоретическом анализе, этот сигнал отнесен к специфическим процессам двухмагнонного рассеяния, связанным с высокоэнергетическими магнонными ветвями с «плоской» дисперсией.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lim, Chang Sung, Aleksandrovsky A. S., Atuchin V. V., Molokeev M. S., Oreshonkov A. S.
Заглавие : Microwave sol-gel synthesis, microstructural and spectroscopic properties of scheelite-type ternary molybdate upconversion phosphor NaPbLa(MoO4)3:Er3+/Yb3+
Место публикации : J. Alloys Compd. - 2020. - Vol. 826. - Ст.152095. - ISSN 0925-8388 (ISSN), DOI 10.1016/j.jallcom.2019.152095. - ISSN 1873-4669 (eISSN)
Примечания : Cited References: 53. - This research was supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science, ICT and Future Planning (2018R1D1A1A09082321). This study was supported by the Russian Science Foundation (19-42-02003, in part of conceptualization). Also, this study was supported by RFBR (18-32-20011, 18-03-00750).
Аннотация: New ternary molybdate NaPbLa(1-x-y)(MoO4)3:xEr3+,yYb3+ (x = y = 0, x = 0.05 and y = 0.35, 0.4, 0.45 and 0.5) phosphors were successfully fabricated by the MSG (microwave sol-gel) method, and the microstructural and spectroscopic properties were characterized. The crystal structure of NaPbLa(MoO4)3 (NPLM) was defined by Rietveld analysis in space group I41/a with unit cell parameters a = 5.3735(2) and c = 11.8668(4) Å, V = 342.65(3) Å3, Z = 4 (RB = 6.64%). The unit cell volume of NaPbLa(MoO4)3 (NPLM) was intermediate between those of NaLa(MoO4)2 and PbMoO4. Under the 980 nm excitation, upconverted yellowish-green emissions at transitions from 2H11/2 and 4S3/2 were observed. No concentration quenching in the subsystem of donor ions at the content up to 50 at.% and no cross-relaxation losses in the subsystem of acceptor ions at the concentrations as high as 5 at. % were verified. The individual chromaticity points for the NaPbLa(MoO4)3:Er3+,Yb3+ phosphors, corresponding to the equal-energy point in the standard CIE diagram, revealed yellowish-green emissions.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Krylova S. N., Vtyurin A. N., Krylov A. S., Wei X., Chen W.
Заглавие : Raman scattering study of SrTiO3: Bi ceramics with higher (x = 0.16) bismuth content
Коллективы : Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Scanning Probe Microscopy, International Conference, Russia-China Workshop on Dielectric and Ferroelectric Materials, "Functional Imaging of Nanomaterials", International Youth Conference
Место публикации : 3th Int. Conf. "Scanning Probe Microscopy". 4th Russia-China Workshop on Dielectric and Ferroel. Mater. (SPM-2019-RCWDFM). Int. Youth Conf. "Functional Imaging of Nanomaterials": Abstract book of joint int. conf. - 2019. - Ст.P62. - P.188. - ISBN 978-5-9500624-2-1
Примечания : Cited References: 2
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Krylov A. S., Senkovska I., Bon V., Kaske S., Slysareva E. A., Krylova S. N., Vtyurin A. N.
Заглавие : Switchable phases of metal-organic frameworks DUT-8(Ni): Raman spectroscopy study
Коллективы : IEEE International Symposium on Applications of Ferroelectrics, International Conference on ElectroCeramics, European Meeting on Ferroelectricity, International Workshop on PiezoMEMS, Piezoresponse Force Microscopy Workshop
Место публикации : Joint Conference of the IEEE ISAF, EMF, ICE, IWPM and PFM: Abstract book. - 2019. - P.408
Примечания : Cited References: 3. - I.S.,V.B., S.K. thank the DFG for financial support (FOR 2433); A.K., S.K., A.V. thank the Russian Foundation for Basic Research for financial support (18-02-00754)
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Вид документа : Статья из сборника (выпуск продолж. издания)
Шифр издания :
Автор(ы) : Tripathy A., Gautam K., Dey K., Ahad A., Gudim I. A., Sathe V. G., Shukla D. K.
Заглавие : Dielectric and Raman spectroscopy measurements across structural phase transition in multiferroic HoFe3(BO3)4 single crystal
Коллективы : International Conference on Advanced Materials
Место публикации : AIP Conf. Proc. - 2019. - Vol. 2162: International Conference on Advanced Materials, ICAM 2019. - Ст.020062. - , DOI 10.1063/1.5130272
Примечания : Cited References: 10. - DKS acknowledges support from the DST, New Delhi, India through the grant no INI/RUS/RFBR/P-269 (Indo Russian project). K.G. thanks, Council of Scientific and Industrial Research, New Delhi, India, for support in the form of SRF.
Аннотация: We report on findings in the HoFe3(BO3)4 single crystal across structural phase transition by the dielectric and Raman spectroscopic measurements. In most of the compounds of RFe3(BO3)4 (R=La-Lu) family low temperature P3121 structure is introduced through structural phase transition (from space group R32). Temperature dependent dielectric measurements on the HoFe3(BO3)4 crystal depicts a step like feature at the structural phase transition at ?366 K. The Raman spectroscopy study also confirms the structural transition around this temperature. A clear signature of structural transition is reflected in the Raman spectra, mainly in the frequency range (200-400 cm-1). Appearance of new Raman modes below the transition temperature also indicates that the transition is from a high symmetry phase to a low symmetry phase.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vtyurin A. N., Gerasimova Y. V., Krylov A. S., Laptash N. M., Krylova S. N.
Заглавие : Cubic to cubic phase transition in (NH4)3SnF7 ferroelastic crystal– Raman scattering study
Коллективы : Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Scanning Probe Microscopy, International Conference, Russia-China Workshop on Dielectric and Ferroelectric Materials, "Functional Imaging of Nanomaterials", International Youth Conference
Место публикации : 3th Int. Conf. "Scanning Probe Microscopy". 4th Russia-China Workshop on Dielectric and Ferroel. Mater. (SPM-2019-RCWDFM). Int. Youth Conf. "Functional Imaging of Nanomaterials": Abstract book of joint int. conf. - 2019. - Ст.P182. - P.285. - ISBN 978-5-9500624-2-1
Примечания : Cited References: 1. - This work was supported by Russian Foundation for Basic Research (Grant N 17-02-00920)
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vtyurin A. N., Krylov A. S., Krylova S. N., Wei, Xiaoyong, Feng, Yujun, Xu, Ran, Zhao, Tian
Заглавие : Dumping soft modes in Raman spectra of antiferroelectric (Pb-La)(Zr-Sn-Ti)O3 ceramics
Коллективы : IEEE International Symposium on Applications of Ferroelectrics, International Conference on ElectroCeramics, European Meeting on Ferroelectricity, International Workshop on PiezoMEMS, Piezoresponse Force Microscopy Workshop
Место публикации : Joint Conference of the IEEE ISAF, EMF, ICE, IWPM and PFM: Abstract book. - 2019. - P.694
Примечания : Cited References: 3
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vyunishev A. M., Myslivets S. A., Fokin V. A., Volochaev M. N., Smolyarova T. E., Radionov N. V., Zaitsev A. I., Arkhipkin V. G., Chirkin A. S.
Заглавие : Dual wavelength Talbot self-imaging using facet patterned nonlinear crystals
Коллективы : Russian Science Foundation (RSF) [19-12-00203]
Место публикации : Opt. Lett. - 2019. - Vol. 44, Is. 15. - P.3761-3764. - ISSN 0146-9592, DOI 10.1364/OL.44.003761. - ISSN 1539-4794(eISSN)
Примечания : Cited References: 19. - Russian Science Foundation (RSF) (19-12-00203).
Предметные рубрики: RAMAN-NATH DIFFRACTION
LITHOGRAPHY
FIELD
Аннотация: A method for functional patterning of facets of a nonlinear crystal using focused ion beam milling has been developed. The near-field diffraction on periodic gratings has been experimentally and theoretically studied. The periodicity of the structure enables Talbot self-imaging at the fundamental and second-harmonic frequencies simultaneously. Spatial interference patterns for both harmonic frequencies are individual ones, which can enable the higher-accuracy optical testing, coupling the radiation at both frequencies, and wavelength-division demultiplexing. The impact of the aperture effect on a Talbot carpet is discussed.
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Atuchin V. V., Aleksandrovsky A. S., Bazarov B. G., Bazarova J. G., Chimitova, Olga D., Denisenko, Yuriy G., Gavrilova T. A., Krylov A. S., Maximovskiy, Eugene A., Molokeev M. S., Oreshonkov A. S., Pugachev, Alexey M., Surovtsev, Nikolay V.
Заглавие : Exploration of structural, vibrational and spectroscopic properties of self-activated orthorhombic double molybdate RbEu(MoO4)2 with isolated MoO4 units
Коллективы : RFBR [16-52-48010, 17-52-53031, 18-03-00557]; Ministry of Science and Higher Education of the Russian Federation [0339-2016-0007]; Act 211 Government of the Russian Federation [02.A03.21.0011]; Ministry of Education and Science of the Russian Federation [4.1346.2017/4.6]
Место публикации : J. Alloy. Compd. - 2019. - Vol. 785. - P.692-697. - ISSN 0925-8388, DOI 10.1016/j.jallcom.2019.01.013. - ISSN 1873-4669(eISSN)
Примечания : Cited References: 42. - The reported study was funded by RFBR according to research projects 16-52-48010, 17-52-53031 and 18-03-00557. Besides, this study was supported by the Ministry of Science and Higher Education of the Russian Federation (project 0339-2016-0007). The work was supported by Act 211 Government of the Russian Federation, contract No 02.A03.21.0011. Additionally, the work was partially supported by the Ministry of Education and Science of the Russian Federation (4.1346.2017/4.6).
Предметные рубрики: MORPHOLOGY-CONTROLLED SYNTHESIS
LUMINESCENCE PROPERTIES
Ключевые слова (''Своб.индексиров.''): rubidium europium molybdate--solid state reaction--rietveld refinement--dsc--raman luminescence
Аннотация: RbEu(MoO4)2 is synthesized by the two-step solid state reaction method. The crystal structure of RbEu(MoO4)2 is defined by Rietveld analysis in space group Pbcn with cell parameters a = 5.13502(5), b = 18.8581(2) and c = 8.12849(7) Å, V = 787.13(1) Å3, Z = 4 (RB = 0.86%). This molybdate possesses its phase transition at 817 K and melts at 1250 K. The Raman spectra were measured with the excitation at λ = 1064 and 514.5 nm. The photoluminescence spectrum is evaluated under the excitation at 514.5 nm. The absolute domination of hypersensitive 5D0→7F2 transition is observed. The ultranarrow 5D0→7F0 transition in RbEu(MoO4)2 is positioned at 580.2 nm being 0.2 nm blue shifted, with respect to that in Eu2(MoO4)3.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zaytseva I. V., Pugachev A. M., Okotrub K. A., Surovtsev N. V., Mikerin S. L., Krylov A. S.
Заглавие : Residual mechanical stresses in pressure treated BaTiO3 powder
Коллективы : RFBR [17-32-5009, 18-02-00399, AAAA-A17-117052410033-9]
Место публикации : Ceram. Int. - 2019. - Vol. 45, Is. 9. - P.12455-12460. - ISSN 0272-8842, DOI 10.1016/j.ceramint.2019.03.179. - ISSN 1873-3956(eISSN)
Примечания : Cited References: 33. - The reported study was funded by RFBR according to the research projects No. 17-32-5009, 18-02-00399 and State assignment No AAAA-A17-117052410033-9. The experiments were performed in the multiple-access center "High-Resolution Spectroscopy of Gases and Condensed Matter" in IA&E SBRAS (Novosibirsk, Russia) and Center for Common Use of the Krasnoyarsk Scientific Center, SBRAS (Krasnoyarsk, Russia).
Предметные рубрики: DIELECTRIC-PROPERTIES
PHASE-TRANSITION
DIAMOND ANVILS
RAMAN
Ключевые слова (''Своб.индексиров.''): residual mechanical stress--raman spectroscopy--high non-hydrostatic pressure--temperature treatment--residual pressure--batio3 ceramics
Аннотация: Here we present Raman spectroscopy approach to monitor the spatial distribution and the magnitude of the residual mechanical stresses in ceramic after non-hydrostatic pressure treatments. The residual pressure can be found from the E-phonon line shift (∼307 cm−1) in the Raman spectra. The relationship between the non-hydrostatic pressure (up to 11 GPa) and the shift of this line has been established. It is demonstrated that the change in the Raman line position (1332 cm−1) of the diamond anvil can be used for monitoring of applied non-hydrostatic pressures. A linear dependence of residual mechanical stresses on the applied pressures is found. Micro-Raman spectroscopy shows that the residual mechanical stresses are distributed fairly uniformly in the studied BaTiO3 samples at the micron scale. In the future, the proposed Raman technique can be used for monitoring the quality of produced BaTiO3 ceramics.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Tanwar, Manushree, Yogi, Priyanka, Lambora, Simran, Mishra, Suryakant, Saxena, Shailendra K., Sagdeo, Pankaj R., Krylov A. S., Kumar, Rajesh
Заглавие : Generalisation of phonon confinement model for interpretation of Raman line-shape from nano-silicon
Место публикации : Adv. Mater. Process. Technol. - 2018. - Vol. 4, Is. 2. - P.227-233. - ISSN 2374-068X, DOI 10.1080/2374068X.2017.1413527
Примечания : Cited References: 32. - This work was supported by the Department of Science and Technology (DST), Government of India; Science and Engineering Research Board.
Ключевые слова (''Своб.индексиров.''): silicon nanomaterial--raman line-shape--phonon--quantum confinement
Аннотация: A comparative analysis of two Raman line-shape functions has been carried out to validate the true representation of experimentally observed Raman scattering data for semiconducting nanomaterials. A modified form of already existing phonon confinement model (PCM) incorporates two basic considerations, phonon momentum conservation and shift in zone centre phonon frequency. After incorporation of the above mentioned two factors, a rather symmetric Raman line-shape is generated which is in contrary to the usual asymmetric Raman line-shapes obtained from nanostructured semiconductor. By fitting an experimentally observed Raman scattering data from silicon nanostructures, prepared by metal induced etching, it can be established that the Raman line-shape obtained within the framework of PCM is a true representative Raman line-shape of sufficiently low dimensions semiconductors.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Dubrovskiy A. A., Balaev D. A., Krasikov A. A., Yakushhkin S. S., Kirillov V. L., Martyanov O. N.
Заглавие : Magnetodielectric effect in a metamaterial consisting of xerogel with embedded ε-Fe2O3 iron oxide nanoparticles
Коллективы : Russian Science Foundation [17-12-01111]
Место публикации : Solid State Commun. - 2019. - Vol. 289. - P.27-29. - ISSN 0038-1098, DOI 10.1016/j.ssc.2018.11.020. - ISSN 1879-2766(eISSN)
Примечания : Cited References: 30. - This work was supported by the Russian Science Foundation, project no. 17-12-01111.
Предметные рубрики: MAGNETIC-PROPERTIES
HIGH-TEMPERATURE
PHASE
RAMAN
Аннотация: The ε-Fe2O3 iron oxide is a fairly rare polymorphic modification, which only exists in the form of nanoparticles embedded, as a rule, into a silica gel matrix. This magnetically ordered iron oxide, which exhibits a significant room-temperature coercivity, is a ferroelectric; therefore, the magnetoelectric and magnetodielectric properties of this material evoke keen interest. In this work, we investigate the magnetodielectric (MD) effect in a metamaterial consisting of xerogel SiO2 with embedded ε-Fe2O3 nanoparticles 9 nm in size on average in a concentration of 20 mass.%. This bulk material exhibits the MD effect in a wide temperature range. The temperature behavior of the permittivity is related to the magnetic state of the ε-Fe2O3 oxide, which undergoes the magnetic transition from the magnetically hard to magnetically soft phase in the temperature range of 80–150 K, indicating the interplay of the ε-Fe2O3 magnetic and charge subsystems.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krylov A. S., Vtyurin A. N., Voronov V. N., Krylova S. N.
Заглавие : Phase transitions in Rb2KLuF6 crystal
Коллективы : Russia/CIS/Baltic/Japan Symposium on Ferroelectricity
Место публикации : Ferroelectrics: Proceedings of the Joint International Symposium : [May 14–18, 2018, St. Petersburg, Russia]. - 2019. - Vol. 538, Is. 1. - P.28-34. - ISSN 00150193 (ISSN), DOI 10.1080/00150193.2019.1569982
Примечания : Cited References: 15. - This work was partly supported by Russian Foundation for Basic Research Grant no 16-02-00102, 18-02-00754.
Предметные рубрики: Phase Transitions and Critical Phenomena
Аннотация: The Raman spectra of Rb2KLuF6 elpasolite crystal have been studied in a wide temperature range, including two phase transitions: from the cubic phase to the tetragonal phase and then to the monoclinic phase. The results of an analysis of the temperature dependences of the parameters of spectral lines are in good agreement with the thermodynamic data on the phase transitions. The analysis of Raman spectra shows that the transition from cubic to tetragonal phase is a second-order transition and the transition from the tetragonal to the monoclinic phase is a weak first-order transition.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gerasimova J. V., Abramova G. M., Zhandun V. S., Vtyurin A. N.
Заглавие : Magnon mode in α-MnS Raman spectrum
Место публикации : J. Raman Spectrosc. - 2019. - Vol. 50, Is. 10. - P.1572–1575. - ISSN 03770486 (ISSN) , DOI 10.1002/jrs.5640
Примечания : Cited References: 19. - The authors are grateful to Prof. B. Kolesov and M. Molokeev for his help with experimental data.
Аннотация: Raman spectra of manganese monosulphide (α-MnS) with NaCl structure in the temperature range 5–300 К are presented. A new peak at 22 cm–1 has been found at low temperatures. The temperature dependence of this peak made possible to attribute it to the magnon mode at k = 0. This is in good agreement with the magnon wavenumber calculated with Munich SPRKKR-package.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vtyurin A. N., Krylov A. S., Krylova S. N., Oreshonkov A. S., Wei X., Feng Y., Xu R., Zhao T.
Заглавие : Soft modes condensation in Raman spectra of (Pb-La)(Zr-Sn-Ti)O3 ceramics
Место публикации : J. Adv. Dielectr. - 2019. - Vol. 9, Is. 3. - Ст.1950024. - ISSN 2010135X (ISSN), DOI 10.1142/S2010135X19500243
Примечания : Cited References: 11
Аннотация: Low frequency Raman spectra of (Pb0.97La0.02)(Zr0.864Sn0.04Ti0.096)O3 ceramic samples have been studied near cubic to antiferroelectric phase transition at about 200 °C. A set of low frequency soft modes were observed restoring below the transition point, in addition to the known one above 100cm-1. These modes show strong damping anomalies at the transition point that supposes considerable intermode interactions via dampings. © 2019 The Author(s).
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krylov A. S., Vtyurin A. N., Voronov V. N., Krylova S. N.
Заглавие : Manifestations of Structural Phase Transitions in a Rb2KLuF6 Crystal in Its Raman Spectra
Коллективы : Russian Foundation for Basic Research [16-02-00102, 18-02-00754]
Место публикации : Opt. Spectrosc. - 2019. - Vol. 126, Is. 4. - P.341-345. - ISSN 0030-400X, DOI 10.1134/S0030400X1904012X. - ISSN 1562-6911(eISSN)
Примечания : Cited References: 27. - This work was supported by the Russian Foundation for Basic Research, project nos. 16-02-00102, 18-02-00754.
Предметные рубрики: SCATTERING
ELPASOLITES
LUMINESCENCE
TRANSFORMATIONS
FLUORIDES
Аннотация: The Raman spectra of an Rb2KLuF6 crystal are studied in the temperature range from 8 to 375 K, which includes two phase transitions: one of which proceeds from a cubic to a tetragonal phase, while the other transition takes place from a tetragonal to a monoclinic phase. An analysis of the temperature dependences of parameters of spectral lines shows that the former transition is of the second kind, while the latter transition is of the first kind, close to the tricritical point. It is shown that the structural phase transitions in the Rb2KLuF6 double perovskite are not associated with disordering. The former transition is associated with rotations of LuF6 octahedra around the fourth-order axis, while the latter transition is related with rotations of octahedra and displacements of rubidium ions.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mishra S., Yogi P., Chaudhary A., Pathak D. K., Saxena S. K., Krylov A. S., Sagdeo P. R., Kumar R.
Заглавие : Understanding perceived color through gradual spectroscopic variations in electrochromism
Коллективы : Department of Science and Technology (DST), Govt. of India; MHRD; CSIR (Govt. of India); DST under FIST scheme [SR/FST/PSI-225/2016]
Место публикации : Indian J. Phys. - 2019. - Vol. 93, Is. 7. - P.927-933. - ISSN 0973-1458, DOI 10.1007/s12648-018-1353-7. - ISSN 0974-9845(eISSN)
Примечания : Cited References: 34. - Authors acknowledge financial support from the Department of Science and Technology (DST), Govt. of India. Authors are thankful to Dr. K. V. Adarsh (IISER Bhopal) for Raman measurements. Authors thank Prof. V.D. Vankar (IIT Delhi) for useful discussions. Authors (AC and DKP) are thankful to MHRD and CSIR (Govt. of India), respectively, for providing fellowships. Support received from DST under FIST scheme (grant number: SR/FST/PSI-225/2016) is also acknowledged.
Предметные рубрики: 3 REDOX FORMS
TUNGSTEN-OXIDE
RAMAN-SPECTRA
VIOLOGEN
SALTS
Аннотация: A bias-dependent in situ Raman scattering and UV–Vis absorption spectroscopic change has been correlated with the corresponding color change of an electrochromic device in an attempt to explain how to understand the relationship between actual perceived color and its absorption/transmittance spectra. For this, the bias across an electrochromic device was increased gradually, rather than abruptly turning ON and OFF, to see subtle variations in Raman and absorption spectra due to bias. Raman scattering establishes that viologen changes its oxidation state reversibly between two redox species (EV2+ to EV+•) as a result of bias-induced dynamic redox process. A gradual variation in Raman and absorption spectra, which shows maximum absorption corresponding to the yellow light, accompanies similar variation in color change of the device as visible by naked eye. These spectroscopic results are correlated with the perceived blue color, in the reflected light, by the eye to understand the actual reason behind this. Maximum absorption of yellow light by the device resulting in blue appearance has been explained using the concept of additive and subtractive primary colors.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ivantsov R. D., Ivanova O. S., Zharkov S. M., Molokeev M. S., Krylov A. S., Gudim I. A., Edelman I. S.
Заглавие : Magnetic circular dichroism in the canted antiferromagnet α-Fe2O3: bulk single crystal and nanocrystals
Место публикации : J. Magn. Magn. Mater. - 2020. - Vol. 498. - Ст.166208. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2019.166208. - ISSN 1873-4766 (eISSN)
Примечания : Cited References: 60. - The authors thank S.L. Sukhachev for help in conducting absorption experiments and S.G. Ovchinnikov for fruitful discussions. The work is supported by Russian Academy of Sciences in the frame of the Project № 0356-2017-0030.
Аннотация: Hematite, α-Fe2O3, is a canted antiferromagnet with the Neel temperature of 960 K. The Morin transition, which occurs when the temperature is lowered to ∼260 K, when the magnetic moments of the sublattices become strictly antiparallel to each other and the resulting magnetic moment disappears, is a characteristic feature of this compound. Detailed investigations are presented here of the magneto-optical effects in the α-Fe2O3 nanoparticles in the transmitted light and in the α-Fe2O3 single crystal in the reflected light. Two types of magneto-optic features were revealed in the magnetic circular dichroism (MCD) spectrum. Some of them described by the Gauss line shape were associated with one-ion d-d transitions. Others were described by the S-shaped line with the inflection points corresponding to the absorption maxima. Last features were assigned to the pair exciton-magnon transitions. An exceptionally strong S-shaped line at 2.0-2.5 eV appeared to be a unique feature of α-Fe2O3 distinguishing it from other iron oxide compounds. The origin of the high effectiveness of the pair exciton-magnon interaction giving rise to this strong S-shaped feature in the MCD spectrum of α-Fe2O3 is discussed.
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