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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pyatnov M. V., Bikbaev R. G., Timofeev I. V., Ryzhkov I. I., Vetrov S. Ya., Shabanov V. F.
Заглавие : Broadband Tamm plasmons in chirped photonic crystals for light-induced water splitting
Место публикации : Nanomaterials. - 2022. - Vol. 12, Is. 6. - Ст.928. - ISSN 20794991 (ISSN), DOI 10.3390/nano12060928
Примечания : Cited References: 41
Аннотация: An electrode of a light-induced cell for water splitting based on a broadband Tamm plasmon polariton localized at the interface between a thin TiN layer and a chirped photonic crystal has been developed. To facilitate the injection of hot electrons from the metal layer by decreasing the Schottky barrier, a thin n-Si film is embedded between the metal layer and multilayer mirror. The chipping of a multilayer mirror provides a large band gap and, as a result, leads to an increase in the integral absorption from 52 to 60 percent in the wavelength range from 700 to 1400 nm. It was shown that the photoresponsivity of the device is 32.1 mA/W, and solar to hydrogen efficiency is 3.95%.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zos’ko, Nikolay A., Aleksandrovsky A. S., Kenova, Tatyana, Gerasimova, Marina A., Maksimov, Nikolay G., Taran, Oxana P.
Заглавие : Cyclic voltammetry as an activation method of TiO2 nanotube arrays for improvement of photoelectrochemical water splitting performance
Колич.характеристики :11 с
Место публикации : ChemPhotoChem. - 2023. - Vol. 7, Is. 9. - Ст.e202300100. - ISSN 23670932 (eISSN), DOI 10.1002/cptc.202300100
Примечания : Cited References: 36. - The authors express their gratitude to A. M. Zhizhaev for the microscopy and XRD analysis and V. F. Shabanov for the fruitful discussionThis work was conducted within the framework of the budget project FWES-2021-0023 for Institute of Chemistry and Chemical Technology SB RAS using the equipment of Krasnoyarsk Regional Research Equipment Centre of SB RAS
Аннотация: A facile and eco-friendly method for activating anodic TiO2 nanotubes (TNTs) by cyclic voltammetry (CV) is proposed, and photoelectrochemical properties of CV-activated TNTs are compared with those of non-activated TNTs and of TNTs activated by hydrogen-thermal reduction. EPR and luminescence studies show that the pristine samples demonstrate rather large content of paramagnetic and luminescing defects, while hydrogenation and CV-activation lead to the different type of rearrangement of defects. TNTs activated by CV-Na2SO4 demonstrate significantly improved photocurrent density (2.25 mA cm-2) in comparison with that of the hydrogen treated and pristine ones (0.93 mA cm-2 and 0.31 mA cm-2) under NUV-irradiation at 0.2 V (RHE). Enhanced photoactivity of Na2SO4-activated TNTs correlates with higher luminescence quantum yield, lowest paramagnetic defects content and larger decay time of the luminescence. Thus, a decrease in the content of defects is an important factor that reduces the non-radiative recombination of charge carriers. The activation-induced redistribution of surface and bulk defects in nanotubes explains the increased photoelectrochemical activity of TiO2-based anodes. Cyclic voltammetry has been proved to be a reliable method to increase the efficiency of TNTs in PEC water splitting.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Sukhanova, Ekaterina V., Sagatov, Nursultan E., Oreshonkov A. S., Gavryushkin, Pavel N., Popov, Zakhar I.
Заглавие : Halogen-doped Chevrel phase Janus monolayers for photocatalytic water splitting
Место публикации : Nanomaterials. - 2023. - Vol. 13, Is. 2. - Ст.368. - ISSN 20794991 (eISSN), DOI 10.3390/nano13020368
Примечания : Cited References: 85. - The authors acknowledge financial support from the Russian Science Foundation (no. 21-73-20183)
Аннотация: Chevrel non-van der Waals crystals are promising candidates for the fabrication of novel 2D materials due to their versatile crystal structure formed by covalently bonded (Mo6X8) clusters (X–chalcogen atom). Here, we present a comprehensive theoretical study of the stability and properties of Mo-based Janus 2D structures with Chevrel structures consisting of chalcogen and halogen atoms via density functional theory calculations. Based on the analysis performed, we determined that the S2Mo3I2 monolayer is the most promising structure for overall photocatalytic water-splitting application due to its appropriate band alignment and its ability to absorb visible light. The modulated Raman spectra for the representative structures can serve as a blueprint for future experimental verification of the proposed structures.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Malakhovskii A. V., Gnatchenko S. L., Kachur I. S., Piryatinskaya V. G., Sukhachev A. L., Temerov V. L.
Заглавие : Influence of magnetic ordering on electronic structure of Tb3+ ion in TbFe3(BO3)(4) crystal
Разночтения заглавия :авие SCOPUS: Influence of magnetic ordering on electronic structure of Tb 3+ ion in TbFe 3(BO 3) 4 crystal
Место публикации : Eur. Phys. J. B: SPRINGER, 2011. - Vol. 80, Is. 1. - P1-10. - ISSN 1434-6028, DOI 10.1140/epjb/e2011-10806-x
Примечания : Cited References: 28. - The work was supported by the Russian Foundation for Basic Researches grant No. 09-02-00171-a, and by OFN RAS Program 2.3.3.1.
Ключевые слова (''Своб.индексиров.''): abrupt change--absorption lines--crystal-field splitting--equilibrium geometries--exchange fields--excited electronic state--external magnetic field--ion environment--local environments--magnetic ordering--magnetic ordering temperatures--magnetically ordered state--optical absorption spectrum--singlet state--structural phase transition--sub-lattices--temperature intervals--temperature variation--absorption--crystal orientation--electric excitation--electronic structure--ground state--ions--light absorption--magnetic fields--magnetic moments--excited states
Аннотация: Optical absorption spectra of trigonal crystal TbFe3(BO3)(4) have been studied in the region of F-7(6) - D-5(4) transition in Tb3+ ion depending on temperature (2-220 K) and on magnetic field (0-60 kOe). Splitting of the Tb3+ excited states, both under the influence of the external magnetic field and effective exchange field of the Fe-sublattice, have been determined. Land, factors of the excited states have been found. Stepwise splitting of one of the absorption lines has been discovered in the region of the Fe-sublattice magnetic ordering temperature. This is shown to be due to the abrupt change of equilibrium geometry of the local Tb3+ ion environment only in the excited state of the Tb3+ ion. In general, the magnetic ordering is accompanied by temperature variations of the Tb3+ local environment in the excited states. The crystal field splitting components have been identified. In particular, it has been shown that the ground state (in D (3) symmetry approximation) consists of two close singlet states of A (1) and A (2) type, which are split and magnetized by effective exchange field of the Fe-sublattice. Orientations of magnetic moments of the excited electronic states relative to that of the ground state have been experimentally determined in the magnetically ordered state of the crystal. A pronounced shift of one of absorption lines has been observed in the vicinity of the TbFe3(BO3)(4) structural phase transition. The temperature interval of coexistence of the phases is about 3 K.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Val'kov V. V., Korovushkin M. M.
Заглавие : Lower subband splitting and superconductivity of 2D Hubbard fermions with strong intersite correlations
Коллективы : International Symposium "Nanophysics and Nanoelectronics-2011" (March 2011; Nizhni Novgorod)
Место публикации : Bull. Russ. Acad. Sci. Phys.: Allerton Press, 2012. - Vol. 76, Is. 2. - P.133-135. - ISSN 1062-8738, DOI 10.3103/S1062873812020074
Примечания : Cited References: 6. - This study was supported by Quantum Physics of Condensed Matter program of the Presidium of the Russian Academy of Sciences; the Russian Foundation for Basic Research, project np. 10-02-00251; the federal target program Scientists and Science Teachers of an Innovate Russia, 2009-2013; the Siberian Branch of the Russian Academy of Sciences, complex integration project no. 53; RF Presidential Grant MK-1300.2011.2; and the Siberian Branch of the Russian Academy of Sciences' Lavrent'ev Competition for Young Scientists.
Ключевые слова (''Своб.индексиров.''): coulomb correlations--doping levels--electron structures--fermi state--hubbard--intersite correlation--mean-square fluctuations--spectral intensity--split-off band--subbands--natural sciences
Аннотация: The effect of the strong intersite Coulomb correlations on the formation of an electron structure in the Shubin-Vonsowsky model in the regime of strong one-site correlations is studied. The results reveal a split-off band of the Fermi states. The spectral intensity of this band grows with the enhancement of the doping level and is determined by the mean-square fluctuation of occupation numbers. This changes the structure of the electron density of states qualitatively. © 2012 Allerton Press, Inc.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zvezdin A. K., Kadomtseva A. M., Popov Y. F., Vorob'ev G. P., Pyatakov A. P., Ivanov V. Y., Kuz'menko A. M., Mukhin A. A., Bezmaternykh L. N., Gudim I. A.
Заглавие : Magnetic anisotropy and magnetoelectric properties of Tb1-x Er (x) Fe-3(BO3)(4) ferroborates
Коллективы : Russian Foundation for Basic Research [07-02-00580]
Разночтения заглавия :авие SCOPUS: Magnetic anisotropy and magnetoelectric properties of Tb1 - X Er xFe3(BO3)4 ferroborates
Место публикации : J. Exp. Theor. Phys. - 2009. - Vol. 109, Is. 1. - P.68-73. - ISSN 1063-7761, DOI 10.1134/S1063776109070097
Примечания : Cited References: 18. - This study was supported by the Russian Foundation for Basic Research (project no. 07-02-00580).
Предметные рубрики: GDFE3(BO3)(4)
Ключевые слова (''Своб.индексиров.''): competing exchange--complex compositions--critical fields--electric polarization--er concentrations--exchange splitting--ferroborates--g factors--magnetoelectric properties--nonmonotonic--simple model--spin-flop transitions--composite micromechanics--erbium--ions--magnetic anisotropy--magnetostriction--magnetostrictive devices--phase transitions--polarization--spin dynamics--terbium alloys--single crystals
Аннотация: Magnetic and magnetoelectric properties of ferroborate single crystals with complex composition (Tb1 - x Er (x) Fe-3(BO3)(4), x = 0, 0.75) and with competing exchange Tb-Fe and Er-Fe interactions are investigated. Jumps in electric polarization, magnetostriction, and magnetization are observed as a result of spin-flop transitions, as well as a considerable decrease in the critical field upon an increase in the Er concentration, in a field H (c) parallel to the c axis. The observed behavior of phase-transition fields is analyzed and explained using a simple model taking into account anisotropy in g factors and exchange splitting of funda-mental doublets of the easy-axis Tb3+ ion and easy-plane Er3+ ion. It is established that magnetoelectric and magnetostriction anomalies under spin-flop transitions are mainly controlled by the Tb subsystem. The Tb subsystem makes a nonmonotonic contribution Delta P (a) (H (a) , T) to polarization along the a axis: the value of Delta P (a) reverses its sign and increases with temperature due to the contribution from the excited states of the Tb3+ ion.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M., Rumyantsev V. G.
Заглавие : Manifestations of the higher moments of the orientation distribution function of molecules in the spectral properties of an impurity nematic
Место публикации : J. Exp. Theor. Phys.: AMER INST PHYSICS, 2004. - Vol. 98, Is. 6. - P1146-1151. - ISSN 1063-7761, DOI 10.1134/1.1777627
Примечания : Cited References: 15
Предметные рубрики: LIQUID-CRYSTAL
SCATTERING
PHASES
MATRIX
ORDER
DYES
Ключевые слова (''Своб.индексиров.''): absorption--band structure--impurities--molecular dynamics--polarization--spectrum analysis--distribution function--local field parameters--splitting--temperature dependence--nematic liquid crystals
Аннотация: The polarized electronic absorption spectra, orientation ordering, and the special local field features were studied for push-pull linear dye molecules with strong donor-acceptor electronic conjugation of terminal fragments in the matrix of a nematic liquid crystal. The temperature-induced inversion of the sign of the splitting of polarized impurity absorption bands was observed. This effect was shown to be caused by the statistical character of orientation ordering of impurity molecules and manifestation of the higher moments of the orientation distribution function. The dependence of local field parameters (Lorentz tensor components) of impurity molecules on their orientation ordering was established. This dependence was used to reproduce the temperature dependence of the orientation order parameter of the matrix. (C) 2004 MAIK "Nauka / Interperiodica".
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popov M. A., Zavislyak I. V., Movchan N. N., Gudim, I. A., Srinivasan G.
Заглавие : Mode splitting in 37-42 GHz barium hexaferrite resonator: Theory and device applications
Место публикации : IEEE Trans. Magn.: IEEE-Institute Electrical and Electronics Engineers, 2014. - Vol. 50, Is. 6. - Ст.4004507. - ISSN 0018-9464, DOI 10.1109/TMAG.2014.2298498. - ISSN 1941-0069
Примечания : Cited References: 34
Предметные рубрики: MILLIMETER-WAVE APPLICATIONS
GUIDE JUNCTION CIRCULATORS
FERRITE
MICROWAVE
PROPAGATION
CYLINDERS
Ключевые слова (''Своб.индексиров.''): dielectric resonance--ferromagnetic resonance (fmr)--hexagonal ferrite--isolator--phase shifter
Аннотация: Dielectric resonances in the 37-42 GHz frequency band in the single crystal barium hexaferrite that occur well below the ferromagnetic resonance (FMR) have been investigated. Sample dimensions have been chosen so that the mode frequency is lower than the spin-wave excitation (in this case, the natural domain resonance) frequency. Such dielectric mode frequencies, being a function of both permittivity and permeability, are magnetic field H tunable. Here, we report on below-FMR magnetodielectric resonance (MDR) axially magnetized barium hexaferrites and their H-tuning characteristics. Our studies reveal H-tuning by up to 2.5 GHz and the tuning is the largest when the ferrite is in a magnetically unsaturated state. A theory for the MDR is presented and a fairly good agreement between experimental data and theory has been obtained. Tunable millimeter wave phase shifters and isolators utilizing the below-FMR dielectric resonances have been demonstrated.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Sukhanova E.V., Sagatov N., Oreshonkov A. S., Gavryushkin P.N., Popov Z.I.
Заглавие : Novel Janus 2D structures of XMoY (X, Y = O, S, Se, Te) composition for solar hydrogen production
Место публикации : Int. J. Hydrog. Energy. - 2023. - Vol. 48, Is. 38. - P.14226-14237. - ISSN 03603199 (ISSN), DOI 10.1016/j.ijhydene.2022.12.286. - ISSN 18793487 (eISSN)
Примечания : Cited References: 97. - The authors acknowledge financial support from Russian Science Foundation (№ 21-73-20183). The authors are grateful to the Joint Supercomputer Center of the Russian Academy of Sciences and to the Information Technology Centre of Novosibirsk State University for providing access to the cluster computational resources
Аннотация: The successful fabrication of H-phase Janus transition metal dichalcogenides (TMDs) has received considerable interest due to its great potential in photocatalytic applications. Here, new A′-XMoY (X/Y = O, S, Se, Te) Janus-type structures belonging to the family of TMDs were theoretically investigated for the first time in terms of photocatalytic water splitting via DFT calculations. For all compounds, the Raman spectra were calculated. The SMoO, SeMoO, SMoSe, SMoTe and SeMoTe compounds are dynamically stable and are semiconductors. Among all considered structures SMoTe is the most promising candidate for solar hydrogen production because valence and conduction bands perfectly engulf the redox potentials of water at both neutral and acidic media, opposite to SMoSe, SMoO, SeMoO suitable only in the acidic media, and SeMoTe – in the neutral media. Moreover, A′-SMoTe demonstrates the outstanding values of the solar-to-hydrogen (STH) conversion efficiencies of 54.0 and 67.1 for neutral and acidic media.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vetrov S.Ya., Pankin P. S., Timofeev I. V.
Заглавие : Peculiarities of spectral properties of a one-dimensional photonic crystal with an anisotropic defect layer of the nanocomposite with resonant dispersion
Коллективы : SB RAS programme [43, 101, 24.29]; Russian Foundation for Basic Research [14-02-31248]; Government Programme of the Ministry of Education and Science of the Russian Federation [1276]; RF President's Grants Council [MK-250.2013.2]; NSCT-SB RAS joint project
Место публикации : Quantum Electron.: Turpion, 2014. - Vol. 44, Is. 9. - P.881-884. - ISSN 1063-7818, DOI 10.1070/QE2014v044n09ABEH015473. - ISSN 1468-4799
Примечания : Cited References: 22. - The work was partially supported by the SB RAS programme (Grant Nos 43, 101 and 24.29); the Russian Foundation for Basic Research (Grant No. 14-02-31248); the Government Programme of the Ministry of Education and Science of the Russian Federation (Project No. 1276); RF President's Grants Council for the State Support to Young Russian Scientists (No. MK-250.2013.2); and NSCT-SB RAS joint project.
Предметные рубрики: MODE
GLASS
Ключевые слова (''Своб.индексиров.''): transmission spectrum--splitting of the defect mode--plasmon resonance--nanocomposite
Аннотация: We have studied the spectral properties of a one-dimensional photonic crystal with a structure defect that represents an anisotropic nanocomposite layer sandwiched between two multi-layer dielectric mirrors. The nanocomposite consists of metallic nanoscale inclusions of orientationally ordered spheroidal shape, dispersed in a transparent matrix, and is characterised by an effective resonant permittivity. Each of the two orthogonal polarisations of probe radiation corresponds to a particular plasmon resonant frequency of the nanocomposite. The problem of calculating the transmittance spectrum of the waves with s- and p-polarisations for such structures is solved. Spectral manifestation of splitting of the defect mode depending on the structure parameters and volumetric fraction of the nanospheroids is studied. The essential dependence of the position of maxima of the defect modes in the bandgap of the photonic crystal and their splitting on the incidence angle, polarisation, and the ratio of lengths of the polar and equatorial semi-axes of the spheroidal nanoparticles is shown.
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