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K2(l-x)Rb2xA12B207, 0x0.75: nonlinear optical borates [Text] / V. G. Grossman, B. G. Bazarov, V. V. Atuchin [et al.] // International Conference on Minerals and Materials / International Conference on Minerals and Materials (2011 ; Sep. ; 29-30, ; Ulaanbaatar, Mongolia). - 2011. - P90-92

https://www.sites.google.com/site/mmcem2011/abstracts

Доп.точки доступа:
Grossman, V.G.; Bazarov, B.G.; Atuchin, V.V.; Molokeev, M.S.; Bazarova, J.G.; Gavrilova, T.A.; International Conference on Minerals and Materials(2011 ; Sep. ; 29-30, ; Ulaanbaatar, Mongolia)
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    Anisotropy of the electromechanical characteristics of SH-waves and Lamb waves in yttrium aluminum borate single crystals / P. P. Turchin, S. I. Burkov, V. I. Turchin [et al.] // J. Sib. Fed. Univ. Math. Phys. - 2022. - Vol. 15, Is. 1. - P. 80-87 ; Журн. СФУ. Матем. и физика, DOI 10.17516/1997-1397-2022-15-1-80-87. - Cited References: 24. - The study was carried out within the framework of the state assignment of the Ministry of Science and Higher Education of the Russian Federation (research project code FSRZ-2020-0011) . - ISSN 1997-1397. - ISSN 2313-6022
   Перевод заглавия: Анизотропия и электромеханические характеристики SH-волн и волн Лэмба в монокристаллах иттриевого алюмобората

РУБ Mathematics

Кл.слова (ненормированные):
surface acoustic, SH and Lamb waves -- piezoelectrics -- multiferroics -- yttrium aluminum borates -- поверхностные акустические, SH- и Лэмба волны -- пьезоэлектрики -- мультиферроики -- алюмоборат иттрия
Аннотация: The anisotropy of the electromechanical properties of SH-waves and Lamb waves in yttrium aluminum borates, which are nonmagnetic representatives of the RMe3(BO3)4 single crystals family (where R=Y, La-Lu; M=Fe, Al, Cr, Ga, Sc) with unique properties of magnetoelectrics and multiferroics, has been studied. In the process of the numerical simulation of the acoustic waves characteristics, the values of linear electromechanical constants of YAl3(BO3)4 single crystals, previously measured by ultrasonic pulse echo and quasi-static methods, have been used.
Исследована анизотропия электромеханичеких характеристик SH-волн и волн Лэмба в иттриевых алюмоборатах, которые являются немагнитным представителем семейства монокри- сталлов RMe3(BO3)4 (где R=Y, La-Lu; M=Fe, Al, Cr, Ga, Sc) с уникальными свойствами магнитоэлектриков и мультиферроиков. При численном моделировании характеристик акустических волн использованы значения линейных электромеханических постоянных монокристаллов YAl3(BO3)4, измеренных ранее ультразвуковым эхо-импульсным и квазистатическим методами.

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Держатели документа:
Siberian Fed Univ, Krasnoyarsk, Russia.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk, Russia.

Доп.точки доступа:
Turchin, Pavel P.; Турчин, Павел Петрович; Burkov, S. I.; Turchin, Vladimir, I; Pletnev, Oleg N.; Chulkova, Marina Yu; Nechepuryshina, Anastasia G.; Ministry of Science and Higher Education of the Russian Federation [FSRZ-2020-0011]

}
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Temperature- and field-induced magnetic transitions in the cobalt-containing borates / N. V. Kazak, N. A. Bel’skaya, Yu. V. Knyazev [et al.] // International conference "Functional materials" : book of abstracts / ed. V. N. Berzhansky ; org. com. S. G. Ovchinnikov [et al.]. - Simferopol, 2021. - P. 31. - Библиогр.: 5 назв. - This work has been financed by the Russian Foundation for Basic Research (project no.20-02-00559).

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Доп.точки доступа:
Berzhansky, V. N. \ed.\; Бержанский, Владимир Наумович; Ovchinnikov, S. G. \org. com.\; Овчинников, Сергей Геннадьевич; Kazak, N. V.; Казак, Наталья Валерьевна; Bel’skaya, N. A.; Knyazev, Yu. V.; Князев, Юрий Владимирович; Molokeev, M. S.; Молокеев, Максим Сергеевич; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Yumashev, V. V.; Gavrilkin, S. Yu.; Ovchinnikov, S. G.; "Functional materials", International conference(2021 ; Oct. 4-8 ; Alushta, Russia); Крымский федеральный университет имени В.И. Вернадского
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    Synthesis and growth of rare earth borates NaSrR(BO3)2 (R = Ho-Lu, Y, Sc) / A. B. Kuznetsov, K. A. Kokh, N. Sagatov [et al.] // Inorg. Chem. - 2022. - Vol. 61, Is. 19. - P. 7497-7505, DOI 10.1021/acs.inorgchem.2c00596. - Cited References: 51 . - ISSN 0020-1669
   Перевод заглавия: Синтез и рост редкоземельных боратов NaSrR(BO3)2 (R = Ho-Lu, Y, Sc)
Аннотация: NaSrR(BO3)2 (R = Ho-Lu, Y, Sc) compounds were obtained for the first time. Their structures exhibit disordered positions of Sr2+ and Na+ atoms while RO6 polyhedra are connected through the BO3 groups. Large distances between R atoms and high transparency in the range of 250-900 nm make them promising for phosphor applications. A pathway to obtain single crystals was shown by growing NaSrY(BO3)2 and NaSrYb(BO3)2 by the top seeded solution growth method with Na2O-B2O3-NaF flux.

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Держатели документа:
Sobolev Institute Of Geology And Mineralogy Sb Ras, Novosibirsk, 630090, Russian Federation
Novosibirsk State University, Novosibirsk, 630090, Russian Federation
Kemerovo State University, Kemerovo, 650000, Russian Federation
Kirensky Institute Of Physics, Siberian Branch, Russian Academy Of Sciences, Krasnoyarsk, 660036, Russian Federation
Tomsk State University, Tomsk, 634050, Russian Federation
Al-Farabi Kazakh National University, Center Of Physical-Chemical Methods Of Research And Analysis, Almaty, 050040, Kazakhstan

Доп.точки доступа:
Kuznetsov, A. B.; Kokh, K. A.; Sagatov, N.; Gavryushkin, P. N.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Svetlichnyi, V. A.; Lapin, I. N.; Kononova, N. G.; Shevchenko, V. S.; Bolatov, A.; Uralbekov, B.; Goreiavcheva, A. A.; Kokh, A. E.
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Magnetic order, spontaneous polarization, and magnetoelectric effect in rare earth iron borates: Ho1−xNdxFe3(BO3)4 [Text] / B. Lorenz, R. P. Chaudhury [et al.] // Bull. Amer. Phys. Soc. - 2010. - Vol. 55, Namb. 2. - Ст. BAPS.2010.MAR.Q36.6

Материалы конференции

Доп.точки доступа:
Lorenz, B.; Chaudhury, R.P.; Sun, Y. Y.; dela Cruz, C. R.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Temerov, V. L.; Темеров, Владислав Леонидович; Chu, C. W.; APS March Meeting(2010 ; March 15-19 ; Portland, Oregon); American Physical Society March Meeting(2010 ; March 15-19)
}
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Structural peculiarities of bismuth-containing RFe3(BO3)4 (R = Ho, Y, Sm, Nd) / E. Smirnova, O. Alekseeva, A. Dudka [et al.] // Acta Crystallogr. A. - 2021. - Vol. 77, Supplement. - P. C1237-C1237, DOI 10.1107/S0108767321084749. - Cited References: 4. - This work was performed using the equipment of the Shared Research Center FSRC 'Crystallography and Photonics' RAS and was supported by the Ministry of Science and Higher Education within the State assignment FSRC 'Crystallography and Photonics' RAS . - ISSN 2053-2733

РУБ Chemistry, Multidisciplinary + Crystallography

Кл.слова (ненормированные):
phase transition -- single crystals -- multiferroics -- rare-earth iron borates -- X-ray structure analysis -- EDS spectroscopy -- Mossbauer spectroscopy -- characteristic temperatures

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Держатели документа:
FSRC Crystallog & Photon RAS, Leninskiy Prospekt 59, Moscow 119333, Russia.
RAS, Kirensky Inst Phys, Siberian Branch, Akad Gorodok 50, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Smirnova, E.; Alekseeva, O. A.; Dudka, A. P.; Verin, I. A.; Artemov, V. V.; Артемов Владимир В.; Khmelenin, D. N.; Gudim, I. A.; Гудим, Ирина Анатольевна; Frolov, K. V.; Lyubutin, I. S.; Ministry of Science and Higher Education within the State assignment FSRC 'Crystallography and Photonics' RAS; Congress of the International Union of Crystallography(25 ; 14-22 August 2021 ; Prague, Czech Republic)
}
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    Synthesis, structure and properties of K2(1-x)Rb2xAl2B2O7 and Cs1.39Tl0.61Al2B2O7 borates as the basis for preparing new oxide materials / V. G. Grossman [et al.] // Lett. Mater. - 2019. - Vol. 9, Is. 1. - P. 86-90 ; Письма о материалах, DOI 10.22226/2410-3535-2019-1-86-90. - Cited References:22. - The research was carried out within the state assignment of FASO of Russia (Theme No 0339-2016-0007). . - ISSN 2218-5046. - ISSN 2410-3535
   Перевод заглавия: Синтез, структура и свойства боратов K2(1-x)Rb2xAl2B2O7 и Cs1.39Tl0.61Al2B2O7 как основа получения новых оксидных материалов

РУБ Materials Science, Multidisciplinary
Рубрики:
OPTICAL-PROPERTIES
   CRYSTAL-STRUCTURE
   K2Al2B2O7
   GROWTH
Кл.слова (ненормированные):
borate -- solid-phase synthesis -- optical properties -- борат -- твердофазный синтез -- оптические свойства
Аннотация: With the development of technology, the need for highly efficient functional materials is steadily increasing. Currently, borates attract the attention of researchers, as they are promising nonlinear materials. Potassium rubidium aluminum borate based on potassium aluminum borate (trigonal syngony, space group P321, Z = 3) was obtained by solid-phase synthesis. The individuality and purity of the borates were confirmed by X-ray diffraction. Analysis of differential scanning calorimetry and thermogravimetric method for K2(1‑x)Rb2xAl2B2O7 (x = 0.1– 0.8) was performed in the temperature range of 25–1075°С. Potassium rubidium borates decompose in the temperature range of 900 –1000°C. Differential scanning calorimetry, dielectric loss tangent, and second-harmonic generation data revealed phase transitions for K0.6Rb1.4Al2B2O7. A significant SHG effect was found at room temperature for K0.6Rb1.4Al2B2O7 (Q = 70). Then the SHG effect increases to Q = 85 at a temperature of 645°C and remains constant with a further increase in temperature. The new triple borate Cs1.39Tl0.61Al2B2O7 was synthesized by the solid-phase synthesis, and its crystallographic parameters were obtained by the Rietveld method. This borate crystallizes in the monoclinic space group P21 / c with the unit cell parameters: Z = 2, a = 6.6669(3) Å, b = 7.2991(3) Å , c = 9.3589(4) Å , β =116.6795(18)°, V = 406.94(3) Å 3. The structure can be considered to be built up from the nearly planar [Al2B2O10] rings, which are composed of two AlO4 tetrahedra and two BO3 triangles, connected, alternately to each other by corner-sharing.
С развитием технологии потребность в высокоэффективных функциональных материалах растет. В настоящее время бораты привлекают внимание исследователей, поскольку они являются перспективными нелинейными материалами. Твердофазным синтезом получены бораты K2(1-x)Rb2xAl2B2O7 (x = 0.1–0.8) на основе калий-алюминиевого бората (тригональная сингония, пространственная группа P321, Z = 3). Индивидуальность и чистота боратов подтверждена рентгеновской дифракцией. Анализ дифференциально-сканирующей калориметрией и термогравиметрическим методом для K2(1-x)Rb2xAl2B2O7 (x = 0.1–0.8) был проведен в интервале температур 25–1075 ºС. Калий-рубидиевые бораты разлагаются в интервале температур 900–1000 °C. Дифференциальной сканирующей калориметрией, диэлектрическими измерениями и методом генерации второй оптической гармоники выявлены фазовые переходы для K0.6Rb1.4Al2B2O7. Значительный ГВГ-эффект был обнаружен при комнатной температуре для K0.6Rb1.4Al2B2O7 (Q = 70). Эффект генерации второй гармоники возрастает до Q = 85 при температуре 645 °C и остается постоянным при дальнейшем увеличении температуры. Новый тройной борат Cs1.39Tl0.61Al2B2O7 был синтезирован методом твердофазного синтеза, а его кристаллографические параметры были получены с помощью метода Ритвельда. Этот борат кристаллизуется в моноклинной пространственной группе P21/c с параметрами элементарной ячейки: Z = 2, a = 6.6669 (3) Å, b = 7.2991 (3) Å, c = 9.3589 (4) Å, β = 116.6795 (18)º, V = 406.94 (3) Å3. Структуру можно представить в виде почти плоских колец [Al2B2O10], которые состоят из двух тетраэдров AlO4 и двух BO3 треугольников, соединенных попеременно друг с другом посредством вершин.

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Держатели документа:
RAS, Baikal Inst Nat Management, Siberian Branch, 6 Sakhyanova St, Ulan Ude 670047, Russia.
Lomonosov Moscow State Univ, GSP 1,1-3 Leninskie Gory, Moscow 119991, Russia.
RAS, Siberian Branch, Kirensky Inst Phys, Fed Res Ctr KSC, 50-38 Akademgorodok, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, 82 Svobodniy Av, Krasnoyarsk 660041, Russia.

Доп.точки доступа:
Grossman, V. G.; Гроссман В. Г.; Bazarov, B. G.; Базаров Б. Г.; Stefanovich, S. Y.; Стефанович С. Ю.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Bazarova, J. G.; Базарова Ж. Г.; [0339-2016-0007]

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    Zero linear compressibility in nondense borates with a "Lu-Ban stool"-like structure / X. X. Jiang [et al.] // Adv. Mater. - 2018. - Vol. 30, Is. 32. - Ст. 1801313, DOI 10.1002/adma.201801313. - Cited References: 28. - X.J., Y.Y., and M.M. contributed equally to this work. The authors acknowledge Zhuohong Yin for useful discussions. This work was supported by the National Scientific Foundations of China (Grant Nos. 11474292, 51702330, 11611530680, 91622118, and 91622124), Russian Foundation for Basic Research (Grant No. 17-52-53031), the Special Foundation of the Director of Technical Institute of Physics and Chemistry (TIPC), the China "863" project (No. 2015AA034203), key project of Beijing Synchrotron Radiation Facility and the Youth Innovation Promotion Association, CAS (outstanding member for Z.L. and Grant No. 2017035 for X.J.). . - ISSN 0935-9648. - ISSN 1521-4095
   Перевод заглавия: Нулевое тепловое расширение в неплотных боратах со структурой типа "стула Лю Бана"

РУБ Chemistry, Multidisciplinary + Chemistry, Physical + Nanoscience & Nanotechnology + Materials Science, Multidisciplinary + Physics, Applied + Physics, Condensed Matter
Рубрики:
MECHANICAL METAMATERIALS
   PRESSURE
   METABORATE
   STRENGTH
Кл.слова (ненормированные):
borates -- "Lu-Ban stool"-like structure -- ultraviolet transparency -- zero -- linear compressibility
Аннотация: Discovering materials that exhibit zero linear compressibility (ZLC) behavior under hydrostatic pressure is extremely difficult. To date, only a handful of ZLC materials have been found, and almost all of them are ultrahard materials with densified structures. Here, to explore ZLC in nondense materials, a structural model analogous to the structure of the “Lu‐Ban stool,” a product of traditional Chinese woodworking invented 2500 years ago, is proposed. The application of this model to borates leads to the discovery of ZLC in AEB2O4 (AE = Ca and Sr) with the unique “Lu‐Ban stool”‐like structure, which can obtain a subtle mechanical balance between pressure‐induced expansion and contraction effects. Coupled with the very wide ultraviolet transparent windows, the ZLC behavior of AEB2O4 may result in some unique but important applications. The applications of the “Lu‐Ban stool” model open a new route for pursuing ZLC materials in nondense structural systems.

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Держатели документа:
Chinese Acad Sci, Tech Inst Phys & Chem, Beijing 100190, Peoples R China.
Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Lab Crystal Phys, Krasnoyarsk 660036, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Chinese Acad Sci, Fujian Inst Res Struct Matter, Fuzhou 350002, Fujian, Peoples R China.
Univ Bonn, Mulliken Ctr Theoret Chem, Inst Phys & Theoret Chem, D-53115 Bonn, Germany.
China Univ Geosci, State Key Lab Geol Proc & Mineral Resources, Wuhan 430074, Peoples R China.
Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China.
Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China.
Huazhong Univ Sci & Technol, Wuhan Natl High Magnet Field Ctr, Wuhan 430074, Peoples R China.
Tianjin Univ Technol, Inst Funct Crystals, Tianjin 300384, Peoples R China.

Доп.точки доступа:
Jiang, Xingxing; Yang, Y.i.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Gong, Pifu; Liang, Fei; Wang, Shuaihua; Liu, Lei; Wu, Xiang; Li, Xiaodong; Li, Yanchun; Wu, Shaofan; Li, Wei; Wu, Yicheng; Lin, Zheshuai
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Crystal structure, phase transition and structural deformations in iron borate (Y0.95Bi0.05)Fe3(BO3)4 in the temperature range 90–500 K / E. S. Smirnova [et al.] // Acta Crystallogr. B. - 2018. - Vol. 74. - P. 226-238, DOI 10.1107/S2052520618002962. - Cited References:27. - The following funding is acknowledged: Russian Foundation for Basic Research (award No. 17-02-00766) and Federal Agency of Scientific Organizations (Agreement No 007-GZ/Ch3363/26). . - ISSN 2052-5206

РУБ Chemistry, Multidisciplinary + Crystallography
Рубрики:
HIGH-PRESSURES
   GDFE3(BO3)4
   SPECTROSCOPY
   IFEFFIT
Кл.слова (ненормированные):
rare-earth iron borates -- crystal structure -- structural phase transition -- structural deformations
Аннотация: An accurate X-ray diffraction study of (Y0.95Bi0.05)Fe3(BO3)4 single crystals in the temperature range 90–500 K was performed on a laboratory diffractometer and used synchrotron radiation. It was established that the crystal undergoes a diffuse structural phase transition in the temperature range 350–380 K. The complexity of localization of such a transition over temperature was overcome by means of special analysis of systematic extinction reflections by symmetry. The transition temperature can be considered to be Tstr ≃ 370 K. The crystal has a trigonal structure in the space group P3121 at temperatures of 90–370 K, and it has a trigonal structure in the space group R32 at 375–500 K. There is one type of chain formed by the FeO6 octahedra along the c axis in the R32 phase. When going into the P3121 phase, two types of nonequivalent chains arise, in which Fe atoms are separated from the Y atoms by a different distance. Upon lowering the temperature from 500 to 90 K, a distortion of the Y(Bi)O6, FeO6, B(2,3)O3 coordination polyhedra is observed. The distances between atoms in helical Fe chains and Fe—O—Fe angles change non-uniformly. A sharp jump in the equivalent isotropic displacement parameters of O1 and O2 atoms within the Fe—Fe chains and fluctuations of the equivalent isotropic displacement parameters of B2 and B3 atoms were observed in the region of structural transition as well as noticeable elongation of O1, O2, B2, B3, Fe1, Fe2 atomic displacement ellipsoids. It was established that the helices of electron density formed by Fe, O1 and O2 atoms may be structural elements determining chirality, optical activity and multiferroicity of rare-earth iron borates. Compression and stretching of these helices account for the symmetry change and for the manifestation of a number of properties, whose geometry is controlled by an indirect exchange interaction between iron cations that compete with the thermal motion of atoms in the structure. Structural analysis detected these changes as variations of a number of structural characteristics in the c unit-cell direction, that is, the direction of the helices. Structural results for the local surrounding of the atoms in (Y0.95Bi0.05)Fe3(BO3)4 were confirmed by EXAFS and Mössbauer spectroscopies.

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Держатели документа:
Russian Acad Sci, Fed Sci Res Ctr Crystallog & Photon, Shubnikov Inst Crystallog, Moscow 119333, Russia.
Natl Res Ctr, Kurchatov Inst, Moscow 123182, Russia.
Russian Acad Sci, Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Smirnova, Ekaterina S.; Alekseeva, Olga A.; Dudka, Alexander P.; Artemov, V. V.; Zubavichus, Yan V.; Gudim, I. A.; Гудим, Ирина Анатольевна; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Frolov, Kirill V.; Lyubutin, Igor S.; Russian Foundation for Basic Research [17-02-00766]; Federal Agency of Scientific Organizations [007-GZ/Ch3363/26]
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10.

Electronic band structures of NdFe3(BO3)4 and NdGa3(BO3)4 crystals: ab initio calculations / S. Krylova, I. Gudim, A. Aleksandrovsky [et al.] // Ferroelectrics. - 2021. - Vol. 575, Is. 1. - P. 11-17, DOI 10.1080/00150193.2021.1888219. - Cited References: 27. - This work was supported by the Russian Foundation for Basic Research Grant No. 20-42-240009 . - ISSN 0015-0193. - ISSN 1563-5112

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
HOFE3(BO3)4
   TEMPERATURE
   SPECTRA
   GROWTH
Кл.слова (ненормированные):
Borates -- ab initio calculation -- electronic bands -- crystal structure
Аннотация: NdFe3(BO3)4 and NdGa3(BO3)4 crystals are of great interest due to their physical properties. For example, NdFe3(BO3)4 crystal demonstrates magnetodielectric and magnetopiezoelectric effects, and NdGa3(BO3)4 crystal possesses luminescent and nonlinear optical properties. In this work, the properties of these materials are calculated by the plane-wave pseudo-potential method based on density functional theory. The structures of the crystals are optimized. The electronic structure of NdFe3(BO3)4 and NdGa3(BO3)4 are calculated.

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Держатели документа:
Kirensky Inst Phys FRC KSC SB RAS, Krasnoyarsk, Russia.
Siberian Fed Univ, Krasnoyarsk, Russia.

Доп.точки доступа:
Krylova, S. N.; Крылова, Светлана Николаевна; Gudim, I. A.; Гудим, Ирина Анатольевна; Aleksandrovsky, A. S.; Александровский, Александр Сергеевич; Vtyurin, A. N.; Втюрин, Александр Николаевич; Krylov, A. S.; Крылов, Александр Сергеевич; Russian Foundation for Basic Research GrantRussian Foundation for Basic Research (RFBR) [20-42-240009]
}
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11.

Sofronova, S. N.
Super-Superexchange Influence on Magnetic Ordering in Ni3B2O6 Kotoite / S. N. Sofronova, I. I. Nazarenko // Phys. Status Solidi B. - 2019. - Vol. 256, Is. 10. - Ст. 1900060, DOI 10.1002/pssb.201900060. - Cited References: 22. - The study was carried out with the financial support of the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory, the Krasnoyarsk Regional Science Foundation as part of a research project: “Low-dimensional and frustrated magnetism in nickel oxyborates and manganites with the substitution of manganese by Yang-Teller ions,” No. 18-42-240007. . - ISSN 0370-1972
Кл.слова (ненормированные):
borates -- computational physics -- crystal structure -- density functional theory -- dow dimensional structures -- magnetic materials -- solid solutions
Аннотация: Using ab initio software package WIEN2k, the calculations of electronic propertiesand of the energies of various magnetically ordered structures are carried out and possible mechanisms of magnetic ordering are analyzed in Ni3B2O6. The superexchange (Ni-O-Ni) and super-superexchange interactions (Ni-O-B-O-Ni) are calculated, a magnetic ordering model is proposed.

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Держатели документа:
Kirensky Institute of Physics of Federal Research Center KSC Siberian Branch Russian Academy of Sciences, Akademgorodok, 50, Building No. 38, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Nazarenko, I. I.; Назаренко, Илья Иванович; Софронова, Светлана Николаевна
}
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12.

Comparing the magnetic and magnetoelectric properties of the SmFe3(BO3)4 ferroborate single crystals grown using different solvents / E. Eremin [et al.] // J. Cryst. Growth. - 2019. - Vol. 518. - P. 1-4, DOI 10.1016/j.jcrysgro.2019.04.017. - Cited References: 17. - This study was supported by the Russian Foundation for Basic Research (RFBR) according to the research projects No. 18-02-00696_a and RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Region Science and Technology Support Fund by project No. 18-42-240011 p_a. . - ISSN 0022-0248. - ISSN 1873-5002

РУБ Crystallography + Materials Science, Multidisciplinary + Physics, Applied
Рубрики:
POLARIZATION
FEATURES
Кл.слова (ненормированные):
Impurities -- Growth from solutions -- Single crystal growth -- Borates -- Ferroelectric materials -- Magnetic materials
Аннотация: SmFe3(BO3)4 single crystals have been grown from the bismuth trimolybdate and lithium tungstate-based melt–solutions. Samarium ferroborate single crystals were grown first from the lithium–tungstate flux. The magnetic and magnetoelectric properties of the synthesized crystals have been compared. It is shown that the SmFe3(BO3)4 ferroborate grown from the bismuth trimolybdate-based melt–solution contains impurities of Bi3+ ions (∼5% at.), which replace Sm3+ ions, while the SmFe3(BO3)4, ferroborate grown from the lithium tungstate-based melt–solution contains minor or zero amounts of such impurities. The magnetoelectric and magnetodielectric effects with the Bi3+ admixture appeared 1.5× stronger than in SmFe3(BO3)4; this is probably due to twinning.

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Держатели документа:
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.

Доп.точки доступа:
Eremin, E. V.; Еремин, Евгений Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович; Smolyakov, D. A.; Смоляков, Дмитрий Александрович; Molokeev, M. S.; Молокеев, Максим Сергеевич; Russian Foundation for Basic Research (RFBR) [18-02-00696_a]; RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Region Science and Technology Support Fund [18-42-240011 p_a]
}
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13.

Crystal structure dynamics of RFe3(BO3)4 single crystals in the temperature range 25–500 K / O. A. Alekseeva, E. S. Smirnova, K. V. Frolov [et al.] // Crystals. - 2022. - Vol. 12, Is. 9. - Ст. 1203, DOI 10.3390/cryst12091203. - Cited References: 67. - This research was funded by the Ministry of Science and Higher Education within the State assignment FSRC ‘Crystallography and Photonics’ RAS 075-01025-22-00 . - ISSN 2073-4352
Кл.слова (ненормированные):
rare-earth iron borates -- low-temperature X-ray diffraction -- single crystals -- structural distortions -- temperature structural dynamics -- exchange and super-exchange interaction -- Mossbauer spectroscopy
Аннотация: The multiferroic RFe3(BO3)4 family is characterized by diverse magnetic, magnetoelectric, and magnetoelastic properties, the fundamental aspects of which are essential for modern electronics. The present research, using single-crystal X-ray diffraction (XRD) and Mossbauer spectroscopy (MS) in the temperature range of 25–500 K, aimed to analyze the influence of local atomic coordination on magnetoelectric properties and exchange and super-exchange interactions in RFe3(BO3)4. Low-temperature, single-crystal XRD data of the magnetically ordered phase of RFe3(BO3)4 at 25 K, which were obtained for the first time, were supplemented with data obtained at higher temperatures, making it possible to draw conclusions about the mechanism of the structural dynamics. It was shown that, in structures with R = Gd, Ho, and Y (low-temperature space group P3121), a shift in oxygen atoms (O2, second coordination sphere of R atoms) was accompanied by rotation of the B2O3 triangle toward R atoms at low temperatures, and by different rearrangements in iron chains of two types, in contrast to Nd and Sm iron borates (space group R32). These rearrangements in the structures of space group P3121 affected the exchange and super-exchange paths at low temperatures. The MS results confirm the influence of the distant environment of atoms on the magnetoelectric properties of rare-earth iron borates at low temperatures.

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Держатели документа:
Shubnikov Institute of Crystallography of Federal Scientific Research Centre ‘Crystallography and Photonics’, Russian Academy of Sciences, Moscow, 119333, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Alekseeva, O. A.; Smirnova, E. S.; Frolov, K. V.; Lyubutina, M. V.; Lyubutin, I. S.; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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14.

Terahertz spectroscopy of magnetoelectric HoAl3(BO3)4 / A. M. Kuzmenko, V. Yu. Ivanov, A. Yu. Tikhanovsky [et al.] // Opt. Spectrosc. - 2023. - Vol. 131, Is. 6. - P. 409-414, DOI 10.1134/S0030400X23020121. - Cited References: 18. - This study was partially financially supported by the Russian Science Foundation (project 16-12-10531) . - ISSN 0030-400X. - ISSN 1562-6911
Кл.слова (ненормированные):
Terahertz spectroscopy -- rare earth aluminum borates -- multiferroics -- electron transitions
Аннотация: Experimental and theoretical study of submillimeter (terahertz) spectroscopic and magnetic properties of the rare-earth aluminum borate HoAl3(BO3)4 were performed at temperatures 3–300K. In the transmittance spectra a number of resonance lines were detected at frequencies 2–35 cm–1 for different radiation polarizations. These modes were identified as transitions between the lower levels of the ground multiplet of the Ho3+ ion split by the crystal field, including both transitions from the ground state to the excited ones and transitions between the excited states. The established excitation conditions of the observed modes and the simulation of the spectra made it possible to separate the magnetic and electric dipole transitions and to determine the energies of the corresponding states, their symmetry, and the matrix elements of the transitions. Low-frequency lines that do not fit into the established picture of the electron states of Ho3+ were also found; these lines, apparently, correspond to the ions with the distorted by defects local symmetry of the crystal field.

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Публикация на русском языке Терагерцовая спектроскопия магнитоэлектрика HoAl3(BO3)4 [Текст] / А. М. Кузьменко, В. Ю. Иванов, А. Ю. Тихановский [и др.]. - 6 с. // Опт. и спектроскоп. - 2022. - Т. 130 Вып. 1. - С. 59-64

Держатели документа:
Prokhorov Institute of General Physics, Russian Academy of Sciences, 119991, Moscow, Russia
Institute of Solid State Physics, Vienna University of Technology, 1040, Vienna, Austria
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, 660036, Krasnoyarsk, Russia

Доп.точки доступа:
Kuzmenko, A. M.; Ivanov, V. Yu.; Tikhanovsky, A. Yu.; Pimenov, A. G.; Shuvaev, A. M.; Gudim, I. A.; Гудим, Ирина Анатольевна; Mukhin, A. A.
}
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15.

Terahertz spectroscopy of magnetoelectric HoAl3(BO3)4 / A. M. Kuzmenko, V. Yu. Ivanov, A. Yu. Tikhanovskii A. Yu. [et al.] // Opt. Spectrosc. - 2022. - Vol. 130, Is. 1. - P. 54-59, DOI 10.21883/EOS.2022.01.52987.33-21. - Cited References: 18. - This study was partially financially supported by the Russian Science Foundation (project 16-12-10531) . - ISSN 0030-400X. - ISSN 1562-6911
Кл.слова (ненормированные):
terahertz spectroscopy -- rare earth aluminum borates -- multiferroics -- electron transitions
Аннотация: Experimental and theoretical study of submillimeter (terahertz) spectroscopic and magnetic properties of the rare-earth aluminum borate HoAl3(BO3)4 were performed at temperatures 3–300 K. In the transmittance spectra a number of resonance lines were detected at frequencies 2–35 cm-1 for different radiation polarizations. These modes were identified as transitions between the lower levels of the ground multiplet of the Ho3+ ion split by the crystal field, including both transitions from the ground state to the excited ones and transitions between the excited states. The established excitation conditions of the observed modes and the simulation of the spectra made it possible to separate the magnetic and electric dipole transitions and to determine the energies of the corresponding states, their symmetry, and the matrix elements of the transitions. Low-frequency lines that do not fit into the established picture of the electron states of Ho3+ were also found; these lines, apparently, correspond to the ions with the distorted by defects local symmetry of the crystal field.

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Держатели документа:
Prokhorov General Physics Institute of the Russian Academy of Sciences, Moscow, Russia
Institute of Solid State Physics, Vienna University of Technology, Vienna, Austria
Kirensky Institute of Physics, Federal Research Center KSC SB, Russian Academy of Sciences, Krasnoyarsk, Russia

Доп.точки доступа:
Kuzmenko, A. M.; Ivanov, V. Yu.; Tikhanovskii A. Yu., A. Yu.; Pimenov, A.; Shuvaev, A.; Gudim, I. A.; Гудим, Ирина Анатольевна; Mukhin, A. A.
}
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16.

Crystal structure of bismuth-containing samarium iron–aluminium borates Sm1−xBixFe3−yAly(BO3)4 (x = 0.05–0.07, y = 0–0.28) in the temperature range of 25–500 K / E. S. Smirnova, O. A. Alekseeva, V. V. Artemov [et al.] // Crystals. - 2023. - Vol. 13, Is. 7. - Ст. 1128, DOI 10.3390/cryst13071128. - Cited References: 59. - This work was supported by the Russian Science Foundation (project No 23-22-00286) . - ISSN 2073-4352
Кл.слова (ненормированные):
rare-earth iron–aluminium borates -- solid solutions -- low-temperature X-ray diffraction -- single crystals -- temperature structural dynamics -- negative thermal expansion
Аннотация: Structural features of new mixed bismuth-containing samarium iron–aluminium borate single crystals Sm1−xBixFe3−yAly(BO3)4 (x = 0.05–0.07, y = 0–0.28) were studied using X-ray diffraction analysis based on aluminium content and temperature in the range 25–500 K. The crystals were grown using the solution-in-melt technique with Bi2Mo3O12 in a flux. The composition of the single crystals was analyzed using energy-dispersive X-ray fluorescence and energy-dispersive X-ray elemental analysis. Temperature dependencies of Sm1−xBixFe3−yAly(BO3)4 unit-cell parameters were studied. Negative thermal expansion was identified below 100 K and represented by characteristic surfaces of the thermal expansion tensor. (Sm,Bi)–O, (Sm,Bi)–(Fe,Al), (Fe,Al)–(Fe,Al), and (Fe,Al)–O interatomic distances decreased with the addition of aluminium atoms. An increase in the (Fe,Al)–(Fe,Al) intrachain bond length at low temperatures in the magnetically ordered state weakened this bond, whereas a decrease in the (Fe,Al)–(Fe,Al) interchain distance strengthened super-exchange paths between different chains. It was found that the addition of aluminium atoms influenced interatomic distances in Sm1−xBixFe3−yAly(BO3)4 much more than lowering the temperature from 293 K to 25 K. The effect of aluminium doping on magnetoelectric properties and structural symmetry of rare-earth iron borates is also discussed.

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Держатели документа:
Shubnikov Institute of Crystallography of Federal Scientific Research Centre ‘Crystallography and Photonics’, Russian Academy of Sciences, Moscow 119333, Russia
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Smirnova, E. S.; Alekseeva, O. A.; Artemov, V. V.; Sorokin, T. A.; Khmelenin, D. N.; Sidorova, E. V.; Frolov, K. V.; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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17.

Synthesis, structure and magnetic properties of monoclinic lanthanum-chromium borate LaCr3(BO3)4 / E. A. Volkova, M. S. Platunov, A. M. Antipin [et al.] // J. Alloys Compd. - 2024. - Vol. 994. - Ст. 174683, DOI 10.1016/j.jallcom.2024.174683. - Cited References: 38. - Single crystal X-ray analysis was carried out within the State assignment NRC "Kurchatov institute" (research contribution of A.M.A.). The research contribution of M.S.P. was partially supported by the Ministry of Science and Higher Education of the Russian Federation within the governmental assignment for Synchrotron radiation facility "SKIF", Boreskov Institute of Catalysis (project FWUR-2024–0040) . - ISSN 0925-8388. - ISSN 1873-4669
Кл.слова (ненормированные):
Borates -- Flux growth -- Crystal structure -- Differential scanning calorimetry -- Powder X-ray diffraction -- IR spectroscopy -- Antiferromagnet
Аннотация: Single crystals of LaCr3(BO3)4 were synthesized through spontaneous nucleation from a K2Mo3O10 flux melt. The crystal structure was determined using single-crystal X-ray diffraction (XRD) at temperatures of 293 K and 85 K. LaCr-borate crystallizes in the monoclinic C2/c space group with unit cell parameters a = 7.47980(5) Å, b = 9.55180(7) Å, c = 11.48330(8) Å, β= 104.0060(6)°, V = 796.04(1) Å3 (for C1, T = 293 K), and a = 7.47380(5) Å, b = 9.55520(7) Å, c = 11.47100(8) Å, β = 103.9330(6)°, V = 795.08(1) Å3 (for C2, T = 85 K), each with Z = 4. The temperature dependence of the unit cell parameters, including the monoclinic angle (β) and the unit cell volume (V), was investigated over the range of 85–293 K. No structural phase transitions were observed in the low-temperature region down to 85 K. Differential scanning calorimetry (DSC) measurements revealed no high-temperature phase transitions between 50 and 1350°C. Infrared (IR) spectroscopy confirmed the monoclinic structure of LaCr3(BO3)4 crystals, revealing characteristic absorption bands, including the lowest frequency mode associated with the translational vibrations of the La3+ ion.

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Держатели документа:
Faculty of Geology, Lomonosov Moscow State University, Moscow, Russian Federation
Synchrotron radiation facility SKIF, Boreskov Institute of Catalysis SB RAS, Kol’tsovo, Russian Federation
Shubnikov Institute of Crystallography, Complex "Crystallography and Photonics", NRC "Kurchatov institute", Moscow, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Institute of Engineering Physics and Radio Electronics, Siberian Federal University, Krasnoyarsk, Russian Federation
Melnikov Research Institute of Comprehensive Exploitation of Mineral Resources of the Russian Academy of Sciences, Moscow, Russian Federation

Доп.точки доступа:
Volkova, E. A.; Platunov, M. S.; Платунов, Михаил Сергеевич; Antipin, A. M.; Alpanova, R. R.; Dubrovskiy, A. A.; Дубровский, Андрей Александрович; Pyastolova, Yu. V.; Пястолова, Юлия Валентиновна; Podobraznyh, A. D.; Kosorukov, V. L.; Koporulina, E. V.; Maltsev, V. V.
}
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18.

Features of the melt–solution synthesis of the TbCr3(BO3)4 single crystals / I. A. Gudim, N. V. Mikhashenok, A. D. Vasiliev [et al.] // J. Cryst. Growth. - 2024. - Vol. 637-638. - Ст. 127716, DOI 10.1016/j.jcrysgro.2024.127716. - Cited References: 22. - The authors thank A.V. Zamkov for assistance in preparing the samples for the conoscopic study. The characterization and examination of the samples were performed at the Center for Collective Use, Krasnoyarsk Scientific Center, Siberian Branch of the Russian Academy of Sciences. - This study was supported in part by the Russian Science Foundation and the Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activity, project no. 22-12-20019 . - ISSN 0022-0248. - ISSN 1873-5002
Кл.слова (ненормированные):
Growth from melt-solution -- Single crystal growth -- Cromium borates -- Rare-earth compounds -- Oxides -- Magnetic materials
Аннотация: The phase formation of terbium chromoborate TbCr3(BO3)4 in the bismuth trimolybdate and lithium tungstate melt–solutions has been studied. The absence of the terbium chromoborate trigonal phase in the bismuth trimolybdate-based system at all component ratios has been shown. The component ratio in the lithium tungstate-based system has been found at which the TbCr3(BO3)4 trigonal crystals are formed at temperatures above 1100 °C; below this temperature, the monoclinic phase dominates. The structural and magnetic properties of the grown crystals have been studied. It has been established that the trigonal and monoclinic TbCr3(BO3)4 crystals synthesized from the lithium tungstate-based solvent exhibit identical magnetic properties. At the same time, a significant difference of the magnetic properties of the single crystals synthesized from the bismuth molybdate melt–solution has been observed. This difference has been attributed to the effect of Bi3+ ions that partially replace Tb3+ ions.

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Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036 Russia

Доп.точки доступа:
Gudim, I. A.; Гудим, Ирина Анатольевна; Mikhashenok, N. V.; Михашенок, Наталья Владимировна; Vasiliev, A. D.; Васильев, Александр Дмитриевич; Melnikova, S. V.; Мельникова, Светлана Владимировна; Pavlovskii, M. S.; Павловский, Максим Сергеевич; Skorobogatov, S. A.; Скоробогатов, Станислав Алексеевич; Pankrats, A. I.; Панкрац, Анатолий Иванович
}
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19.

Chukalina, E. P.
Study of the magnetic properties of neodymium and samarium iron borates by the method of erbium spectroscopic probe / E. P. Chukalina, A. Jablunovskis, I. A. Gudim // Opt. Spectrosc. - 2023. - Vol. 131, Is. 8. - P. 630-636, DOI 10.1134/S0030400X23060024. - Cited References: 30. - This paper was carried out under financial support of the Russian Science Foundation (grant № 19-12-00413) . - ISSN 0030-400X. - ISSN 1562-6911
Кл.слова (ненормированные):
multiferroics -- optical spectroscopy -- crystals with rare earths -- Kramers ions
Аннотация: Iron borates NdFe3(BO3)4 and SmFe3 (BO3)4 activated with 1% erbium, with ahuntite structure (space symmetry group R32) were investigated by the method of erbium spectroscopic probe. From an analysis of the temperature dependence of the transmission spectra in the region of the 4I15/2 → 4113/2 transition in the Er3+ ion, it was found that both studied compounds order antiferromagnetically at TN ≈ 33 K into an easy-plane magnetic structure. No other phase transitions were found.

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Публикация на русском языке Чукалина Е. П. Исследование магнитных свойств ферроборатов неодима и самария методом спектроскопического эрбиевого зонда [Текст] / Е. П. Чукалина, А. Яблуновский, И. А. Гудим // Опт. и спектроскоп. - 2022. - Т. 130 Вып. 1. - С. 104-110

Держатели документа:
Institute of Spectroscopy, Russian Academy of Sciences, 108840, Troitsk, Moscow, Russia
Moscow Institute of Physics and Technology (National Research University), 141701, Dolgoprudny, Moscow oblast, Russia
Kirensky Institute of Physics, Federal Research Center KSC SB, Russian Academy of Sciences, 660036, Krasnoyarsk, Russia

Доп.точки доступа:
Jablunovskis, A.; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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20.

Crystal growth of ReCa3Mn3O3(BO3)4 (Re = Gd, Y) gaudefroyite: Phase sequence and equilibrium study in multi-component fluxes / E. Moshkina, N. Belskaya, Z. Bashleev [et al.] // J. Cryst. Growth. - 2022. - Vol. 600. - Ст. 126917, DOI 10.1016/j.jcrysgro.2022.126917. - Cited References: 32. - The study was supported by the Russian Science Foundation (grant No. 21-72-00130). The X-ray, and EDX data were obtained using the analytical equipment of the Krasnoyarsk Regional Center of Research Equipment of the Federal Research Center “Krasnoyarsk Science Center SB RAS” . - ISSN 0022-0248
Кл.слова (ненормированные):
Phase equilibria -- Growth from solutions -- Borates -- Gaudefroyites
Аннотация: The work is aimed at studying the crystallization of ReCa3Mn3O3(BO3)4 (Re = Gd, Y) borates with the gaudefroyite structure in different flux systems. Gaudefroyites are promising materials in the field of spin ice and magnetocaloric effect. The study has been performed on systems based on the following solvents: Bi2Mo3O12-Na2B4O7-B2O3, Bi2O3-Na2B4O7-B2O3, Bi2O3-BaO-Na2B4O7-B2O3, Li2WO4-Li2O-B2O3. The influence of the solvent components on the sequence of high-temperature crystallizing phases has been studied. The feature of Mo- and W-containing fluxes consisting in the formation of stable chemical bonds of the M2+Mo(W)O4 (M = Ca, Mn) molybdate or tungstate types has been revealed which prevents the formation of gaudefroyite type bonds. An approach has been suggested for changing the sequence of the crystallizing phases which consists in the super saturation of molybdate (tungstate) bonds by Na+ or Li+ cations up to the formation of delafossite-type bonds (Li(Na)-Mn-O phase) with higher manganese valence states Mn3+ and Mn4+. The optimization of the growth conditions of ReCa3(MnO)3(BO3)4 (Re = Gd, Y) gaudefroyite crystals has allowed one to obtain single crystal samples with the size up to 0.8 × 0.8 × 5 mm3. The structural characterization and chemical composition of all the obtained phases are also presented.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Ioffe Institute, Saint Petersburg, 194021, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Research and Development Department, Kemerovo State University, Kemerovo, 650000, Russian Federation
Institute of Chemistry and Chemical Technology, Federal Research Center KSC SB RAS, Krasnoyarsk, 660049, Russian Federation
Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian State University of Science and Technologies, Krasnoyarsk, 660037, Russian Federation

Доп.точки доступа:
Moshkina, E. M.; Мошкина, Евгения Михайловна; Belskaya, N.; Bashleev, Z.; Башлеев, Зоригто Егорович; Molokeev, M. S.; Молокеев, Максим Сергеевич; Soloviev, L.; Shabanova, K.
}
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