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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kostikov D. A., Krakhalev M. N., Prishchepa O. O., Zyryanov V. Ya.
Заглавие : Electrically induced structural transformations of a chiral nematic under tangential-conical boundary conditions
Колич.характеристики :10 с
Место публикации : Molecules. - 2023. - Vol. 28, Is. 23. - Ст.7842. - ISSN 14203049 (eISSN), DOI 10.3390/molecules28237842
Примечания : Cited References: 30
Аннотация: In this study, structural transformations induced by an electric field in the chiral nematic under tangential-conical boundary conditions have been considered. The composition influence of the orienting polymer films on the director tilt angles, the formation of orientational structures in the LC layer, as well as the electro-optical response and relaxation processes have been studied. It has been shown that the poly(tert-butyl methacrylate) concentration change in the orienting polymer mixture allows for smoothly controlling the director tilt angle without fixing its azimuthal orientation rigidly.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Паршин, Александр Михайлович, Гуняков, Владимир Алексеевич, Зырянов, Виктор Яковлевич, Шабанов, Василий Филиппович
Заглавие : Структура и оптические свойства самоорганизованных ансамблей нематических доменов на поверхности поликарбоната
Место публикации : Жидк. крист. и их практич. использ. - 2022. - Т. 22, № 1. - С. 84-88. - ISSN 19913966 (ISSN), DOI 10.18083/LCAppl.2022.1.84; Liq. Cryst. Appl. - ISSN 24999644 (eISSN); Zidk. Krist. Prakt. Ispol'z.
Примечания : Библиогр.: 9
Аннотация: Рассмотрено структурное упорядочение самоорганизованных ансамблей нематических доменов с радиально-планарной конфигурацией, формирующихся на поверхности поликарбоната. Под влиянием теплового, упругого, электрического или магнитного полей структура доменов трансформируется в радиально-гомеотропную. При переориентации директора в данных структурах наблюдаются интерференционные осцилляции проходящего света с большой глубиной модуляции в отсутствие поляризаторов, что позволяет оценивать их как перспективный материал для оптических модуляторов.The structural ordering of self-organized ensembles of nematic domains (SEND) with a radial-planar configuration, which are formed on the polycarbonate surface, is considered. The domain structure is transformed into radialhomeotropic one under the influence of a thermal, elastic, electric or magnetic fields. Interference oscillations of transmitted light with a large modulation depth are observed in the absence of polarizers, when the director is reoriented in these structures, which makes it possible to evaluate them as a promising material for optical modulators.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Сутормин, Виталий Сергеевич, Крахалев, Михаил Николаевич, Прищепа, Оксана Олеговна, Зырянов, Виктор Яковлевич
Заглавие : Ориентационный переход в слое нематика с гомеотропно-коническими граничными условиями, индуцированный ионной модификацией поверхностного сцепления
Место публикации : Жидк. крист. и их практич. использ. - 2022. - Т. 22, № 3. - С. 105-110. - ISSN 1991-3966 (ISSN), DOI 10.18083/LCAppl.2022.3.105; Liq. Cryst. Appl. - ISSN 2499-9644 (eISSN)
Примечания : Библиогр.: 4. - В.С. Сутормин, М.Н. Крахалев и О.О. Прищепа благодарят за поддержку грант РФФИ, Правительства Красноярского края и Красноярского краевого фонда науки в рамках научного проекта № 20-42-240007
Аннотация: Исследована трансформация ориентационной структуры в слое нематика с гомеотропно-коническими граничными условиями, индуцированная электроуправляемой ионной модификацией поверхностного сцепления. Обнаружено, что изменение азимутального угла директора на подложке с коническим сцеплением возможно осуществить путем модификации граничных условий на второй подложке.The transformation of the orientational structure induced by the electrically controlled ionic modification of surface anchoring in the nematic layer with homeotropic-conical boundary conditions has been considered. It has been found that the change in the azimuthal angle of director at the substrate with conical anchoring can be realized by modification of boundary conditions at the second substrate.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gardymova A. P., Krakhalev M. N., Zyryanov V. Ya., Gruzdenko A. A., Alekseev A. A., Rudyak V. Yu.
Заглавие : Polymer dispersed cholesteric liquid crystals with a toroidal director configuration under an electric field
Место публикации : Polymers. - 2021. - Vol. 13, Is. 5. - Ст.732. - P.1-11. - ISSN 20734360 (ISSN), DOI 10.3390/polym13050732
Примечания : Cited References: 49. - This research was funded by Russian Science Foundation, Grant No. 20-72-10038
Аннотация: The electro-optical properties of polymer dispersed liquid crystal (PDLC) films are highly dependent on the features of the contained liquid crystal (LC) droplets. Cholesteric LC droplets with homeotropic boundaries can form several topologically different orientational structures, including ones with single and more point defects, layer-like, and axisymmetric twisted toroidal structures. These structures are very sensitive to an applied electric field. In this work, we have demonstrated experimentally and by computer simulations that twisted toroidal droplets reveal strong structural response to the electric field. In turn, this leads to vivid changes in the optical texture in crossed polarizers. The response of droplets of different sizes were found to be equivalent in terms of dimensionless parameters. In addition, the explanation of this phenomenon showed a comparison of theoretical and experimental structural response curves aids to determine the shape of the droplet. Finally, we demonstrated that the addition of a dichroic dye allows such films to be used as optical filters with adjustable color even without polarizers.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kostikov D. A., Krakhalev M. N., Prishchepa O. O., Zyryanov V. Ya.
Заглавие : Nematic structures under conical anchoring at various director tilt angles specified by polymethacrylate compositions
Коллективы : Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science [20-42-240007]
Место публикации : Polymers. - 2021. - Vol. 13, Is. 17. - Ст.2993. - ISSN 2073-4360(eISSN), DOI 10.3390/polym13172993
Примечания : Cited References: 49. - Mikhail N. Krakhalev and Oxana O. Prishchepa acknowledge financial support from Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science (No 20-42-240007)
Предметные рубрики: LIQUID-CRYSTAL
PRETILT ANGLE
ALIGNMENT LAYERS
SURFACE
INTERFACE
Аннотация: Dependence of the director tilt angle of nematic liquid crystal (LC) under conical anchoring from the two-component polymer mixture composition has been studied. We varied the ratio of poly(isobutyl methacrylate) (PiBMA), which specifies a conical anchoring for the nematic liquid crystal LN-396, and poly(methylmethacrylate) (PMMA) assigning a tangential alignment for the same nematic. An oblique incidence light technique to determine a tilt angle has been used. It has been shown that the tilt angle increases from 0∘ to 47.7∘ when PiBMA:PMMA ratio changes in the range 30:70 to 100:0. The specific optical textures viewed under the polarizing microscope and proper orientational structures have been considered for various compositions of the polymer films. An electric field action on the formed orientational structures has been investigated. The obtained results are promising for the application in various electro-optical LC devices with a conical anchoring in which the director tilt angle is a crucial parameter: a controlled diffraction gratings, an electrically operated achromatic rotators of linear light polarization, etc.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krinitsin, Pavel, Yelisseyev, Alexander, Jiang, Xingxing, Isaenko, Lyudmila, Molokeev M. S., Lin, Zheshuai, Pugachev, Alexey
Заглавие : Growth, Structure, and Optical Properties of Nonlinear LiGa0.55In0.45Te2 Single Crystals
Коллективы : Russian Foundation of Basic Research [15-02-03408a, 17-45-540775r_a, 17-52-53031]; national scientific foundations of China [11474292, 51702330, 11611530680, 91622118, 91622124]; special foundation of the director of Technical Institute of Physics and Chemistry (TIPC); China "863" project [2015AA034203]; Youth Innovation Promotion Association, CAS [2017035]; [0330-2016-0008]
Место публикации : Cryst. Growth Des. - 2019. - Vol. 19, Is. 3. - P.1805-1814. - ISSN 1528-7483, DOI 10.1021/acs.cgd.8b01788. - ISSN 1528-7505(eISSN)
Примечания : Cited References: 43. - This work was supported by state assignment project #0330-2016-0008 and partially by the Russian Foundation of Basic Research (Grant Nos. 15-02-03408a, 17-45-540775r_a, and 17-52-53031), national scientific foundations of China (Grant Nos. 11474292, 51702330, 11611530680, 91622118, and 91622124), the special foundation of the director of Technical Institute of Physics and Chemistry (TIPC), the China "863" project (No. 2015AA034203) and the Youth Innovation Promotion Association, CAS (outstanding member for Z.L. and Grant 2017035 for X.J.). Some part of the experiments was performed in the multiple-access center "High-Resolution Spectroscopy of Gases and Condensed Matter" at the IA&E SBRAS (Novosibirsk, Russia). The authors are grateful to N. F. Beisel from the Analytical laboratory of the Nikolaev Institute of Inorganic Chemistry SB RAS for atomic-emission spectral analysis of the studied crystals.
Предметные рубрики: PHASE-MATCHING PROPERTIES
ELECTRONIC-STRUCTURE
MID-IR
Аннотация: In search of new nonlinear optical crystals for the mid-IR range, we grew single crystals of LiGa0.55In0.45Te2 (LGITe) of optical quality; its structure was established, and the spectroscopic properties were studied. LGITe crystallizes in a tetragonal chalcopyrite-like (I4̅2d) structure at 667 ± 5 °C. Crystals are transparent in the 0.76–14.8 μm spectral region with some absorption bands related to OH/H2O and Ge–O vibrations. Analysis of the Tauc plots showed that LGITe is a direct band gap semiconductor with the band gap Eg = 1.837 eV at 300 K. The Raman spectrum for LGITe is very similar to that for LiGaTe2: the most intense band A1 near 120 cm–1 corresponds to the Li–Te vibration. DFT calculations were carried out for the first time to simulate the energy band structure (band gap ∼1.67 eV), density of states (DOS), birefringence (0.049 at 2 μm), and nonlinear susceptibility (d14 = d36 = −48.73 pm/V). For ternary LiInTe2 these parameters are Δn = 0.007 and d14 = d36 = −61.4 pm/V, respectively. The calculated optical properties indicate that LiGa0.55In0.45Te2 is a promising mid-IR nonlinear optical crystal with nonlinear parameters higher than those of LiGaTe2.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krakhalev M. N., Sutormin V. S., Prishchepa O. O., Kuz'menok N. M., Mikhalyonok S. G., Bezborodov V. S., Zyryanov V. Ya.
Заглавие : Anionic-cationic surfactant mixture providing the electrically controlled homeotropic surface anchoring of liquid crystals
Коллективы : International conference on Hole Burning, Single Molecule, and Related Spectroscopies: Science and Applications - 2018 , Belarusian Republican Foundation for Fundamental Research [X16P-110]; Russian Foundation for Basic Research (RFBR) [16-53-00073]; RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science [18-42-243006]
Место публикации : J. Mol. Liq. - 2019. - Vol. 282: Suzdal Conference (2018, Suzdal, RUSSIA). - P.57-62. - ISSN 0167-7322, DOI 10.1016/j.molliq.2019.02.132. - ISSN 1873-3166(eISSN)
Примечания : Cited References: 30. - The reported study was supported by the Belarusian Republican Foundation for Fundamental Research (project No X16P-110) and Russian Foundation for Basic Research (RFBR) (project No 16-53-00073). Mikhail N. Krakhalev and Vitaly S. Sutormin acknowledge financial support from RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science (project No 18-42-243006).
Предметные рубрики: IONIC MODIFICATION
TRANSITION
DROPLETS
CONFIGURATION
LAYER
Аннотация: In search of a substance able to function as an anionic surfactant applied for the electrically-induced anchoring transitions in liquid crystals, the compound 4-heptyloxybenzoate benzyl dodecyldimethylammonium (HOBBDDA) has been synthesized. Its orienting influence on nematic liquid crystal 4-pentyl-4'-cyanobiphenyl (5CB) has been tested. HOBBDDA dissolved up to 1.4%in 50 droplets dispersed in polymer film does not change the tangential surface anchoring inherent to polyvinyl alcohol matrix used. Homeotropic surface anchoring is realized if the HOBBDDA content exceeds 1.7%. The molecules of the surfactant in 5CB dissociate into anions and cations. The anions modify the surface anchoring under the action of DC electric field both in the normal and inverse mode. The mixture of HOBBDDA and cetyltrimethylammonium bromide can function as a binary ionic cationic surfactant which significantly expands the prospects for using the ionic-surfactant method to control liquid crystal materials. (C) 2019 Elsevier B.V. All rights reserved.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Krakhalev M. N., Prishchepa O. O., Sutormin V. S., Bikbaev R. G., Timofeev I. V., Zyryanov V. Ya.
Заглавие : Director configurations in cholesteric layer with tangential-conical boundary conditions
Коллективы : European Conference on Liquid Crystals
Место публикации : 15th Eur. Conf. Liq. Cryst. (ECLC): conf. progr. - 2019. - Ст.PC-06
Примечания : Cited References: 2
Материалы конференции,
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krakhalev M. N., Bikbaev R. G., Sutormin V. S., Timofeev I. V., Zyryanov V. Ya.
Заглавие : Nematic and Cholesteric Liquid Crystal Structures in Cells with Tangential-Conical Boundary Conditions
Коллективы : Russian Science Foundation [18-72-10036]
Место публикации : Crystals. - 2019. - Vol. 9, Is. 5. - Ст.249. - ISSN 2073-4352, DOI 10.3390/cryst9050249
Примечания : Cited References: 43. - This work was supported by the Russian Science Foundation (No. 18-72-10036).
Предметные рубрики: TRANSITION
GRATINGS
Аннотация: Orientational structures formed in nematic and cholesteric layers with tangential-conical boundary conditions have been investigated. LC cells with one substrate specifying the conical surface anchoring and another substrate specifying the tangential one have been considered. The director configurations and topological defects have been identified analyzing the texture patterns obtained by polarizing microscope in comparison with the structures and optical textures calculated by free energy minimization procedure of director field and finite-difference time-domain method, respectively. The domains, periodic structures and two-dimensional defects proper to the LC cells with tangential-conical anchoring have been studied depending on the layer thickness and cholesteric pitch.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yelisseyev A. P., Molokeev M. S., Jiang, Xingxing, Krinitsin P. G., Isaenko L. I., Lin, Zheshuai
Заглавие : Structure and optical properties of the Li2In2GeSe6 crystal
Коллективы : Russian Foundation of Basic Research [15-02-03408a, 17-45-540775r_a, 17-52-53031]; National Scientific Foundations of China [11474292, 51702330, 11611530680, 91622118, 91622124]; special foundation of the director of Technical Institute of Physics and Chemistry (TIPC); China "863" project [2015AA034203]; Youth Innovation Promotion Association, CAS [2017035]; [0330-2016-0008]
Место публикации : J. Phys. Chem. C. - 2018. - Vol. 122, Is. 30. - P.17413-17422. - ISSN 1932-7447, DOI 10.1021/acs.jpcc.8b02799
Примечания : Cited References: 49. - This work was supported by state assignment project #0330-2016-0008 and partly by the Russian Foundation of Basic Research (grants nos. 15-02-03408a, 17-45-540775r_a, and 17-52-53031), National Scientific Foundations of China (grants 11474292, 51702330, 11611530680, 91622118, and 91622124), the special foundation of the director of Technical Institute of Physics and Chemistry (TIPC), the China "863" project (no. 2015AA034203), and the Youth Innovation Promotion Association, CAS (outstanding member for Z.L. and grant 2017035 for X.J.).
Предметные рубрики: PHASE-MATCHING PROPERTIES
TEMPERATURE-DEPENDENCE
ELECTRONIC-STRUCTURE
Аннотация: Intense search for new nonlinear optical crystals for the mid-infrared region is in progress, and Li-containing quaternary chalcogenides are expected to improve transparency range, stability, phase-matching conditions, and other parameters in comparison with commercially available AgGaS2, AgGaSe2, and ZnGeP2. Single crystals of Li2In2GeSe6 up to 8 mm in size were obtained by the Bridgman- Stockbarger growth technique, and their high quality was confirmed by exciton luminescence. A monoclinic structure and direct band-to-band electronic transitions were established, and the thermal expansion was shown to be virtually isotropic. Defect-related absorption and luminescence were revealed, and the way to lower them was suggested. The electronic structure, density of states, and some optical properties were calculated from the first principles for Li2In2GeSe6. The calculated nonlinear coefficients and rather large birefringence indicate a strong phase-matching ability. These investigations demonstrate that Li2In2GeSe6 is a promising mid-infrared nonlinear optical crystal.
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