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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Wang, Yuanjing, Tang, Wenyu, Zhang, Chuang, Molokeev M. S., Ming, Hong, Zhou, Yayun, Peng, Shuai, Song, Enhai, Zhang, Qinyuan
Заглавие : Structure-based machine learning enables discovery of Mn4+-activated red-light fluorides for ultrawide-gamut mini-light-emitting diodes
Колич.характеристики :11 с
Место публикации : Adv. Funct. Mater. - 2024. - Vol. 34, Is. 14. - Ст.2313490. - ISSN 1616301X (ISSN), DOI 10.1002/adfm.202313490. - ISSN 16163028 (eISSN)
Примечания : Cited References: 61. - This research was financially supported by the National Key R& D Program of China (Grant No. 2022YFB3503800) and the National Natural Science Foundation of China (Grant Nos. 52202170 and 52322208). This research was supported by the Tyumen Oblast Government, as part of the West-Siberian Interregional Science and Education Center's project No. 89-DON (3)
Аннотация: Mn4+-activated fluorides with a saturated red color and sharp line emission are ideal for applications in the light-emitting diodes (LEDs) backlight for displays. However, the emissions attributed to 2E→4A2 parity and spin-forbidden transitions limit the design and adjustments of emission wavelength and chromaticity coordinates. Herein, machine learning algorithms are used to build a wavelength-prediction model for Mn4+-activated fluorides. The model precisely identifies the key structural features that affect wavelengths and discovers target materials. The predicted candidate Cs2NaAlF6:Mn4+ (CNAF) with a long-wavelength zero-phonon-line emission at 628 nm exhibits a redshift in comparison with other reported Mn4+-activated fluorides and commercial K2SiF6:Mn4+, but maintains narrow spectral emission with full-width half maximum (FWHM) of 11.2 nm. The redshift and narrow spectra result in a color purity of 99.7% and Commission Internationale de L'Eclairage (CIE) chromaticity coordinate of (0.7032,0.2967) that is close to the pure red-light point of Recommendation BT. 2020 (Rec. 2020). Moreover, CNAF is prepared as a transparent red-light film, and the device fabricated using the blue-light mini-LEDs, green quantum-dot film, and CNAF film exhibits a wide color-gamut of 121.5% National Television Standards Committee (NTSC) or 90.6% Rec. 2020, suggesting that CNAF has potential for wide-color-gamut displays.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ming H., Zhou Ya., Molokeev M. S., Zhang Ch., Huang L., Wang Yu., Sun H.-T., Song E., Zhang Q.
Заглавие : Machine-learning-driven discovery of Mn4+-doped red-emitting fluorides with short excited-state lifetime and high efficiency for mini light-emitting dIode displays
Колич.характеристики :11 с
Место публикации : ACS Mater. Lett. - 2024. - Vol. 6. - P.1790-1800. - ISSN 26394979 (eISSN), DOI 10.1021/acsmaterialslett.4c00263
Примечания : Cited References: 39. - This work was financially supported by the National Key Research and Development Program of China (No. 2022YFB3503800), National Natural Science Foundation of China (Grants Nos. 52202170 and 52322208), Natural Science Foundation of Guangdong Province (No. 2022A1515140032) and Distinguished Youth Foundation of Guangdong Scientific Committee (No. 2023B1515020059). This work was also supported by the Tyumen Oblast Government, as part of the West-Siberian Interregional Science and Education Center’s Project No. 89-DON (3). H. Ming acknowledges the fellowship support from the China Scholarship Council (CSC No. 202206150038)
Аннотация: The discovery of high-efficiency Mn4+-activated fluoride red phosphors with short excited-state lifetimes (ESLs) is urgent and crucial for high-quality, wide-color-gamut display applications. However, it is still a great challenge to design target phosphors with both short ESL and high luminescence efficiency. Herein, we propose an efficient machine learning approach based on a small dataset to establish the ESL prediction model, thereby facilitating the discovery of new Mn4+-activated fluorides with short ESLs. Such a model can not only accurately predict the ESLs of Mn4+ in fluorides but also quantify the impact of structure features on ESLs, therefore elucidating the “structure-lifetime” correlations. Guided by the correlations, two new Mn4+-doped tetramethylammonium (TMA)-based hybrid fluorides (TMA)2BF6:Mn4+ (B = Sn or Hf) with both short ESLs (τ ≤ 3.7 ms) and high quantum efficiencies (internal QEs ˃ 92%, external QEs ˃ 55%) have been discovered successfully. A prototype displayer with excellent performance (∼124% National Television Standards Committee (NTSC) color gamut) is assembled by employing a (TMA)2SnF6:Mn4+-based white Mini-LED backlight module, demonstrating its practical prospects in high-quality displays. This work not only brings promising candidates for Mn4+-doped fluoride phosphors but also provides a valuable reference for accelerating the discovery of new promising phosphors.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Chen J., Zou X., Li W., Zhang H., Zhang X., Molokeev M. S., Liu Y., Lei B.
Заглавие : Strategy to construct high thermal-stability narrow-band green-emitting Si-CDs@MAs phosphor for wide-color-gamut backlight displays
Место публикации : Adv. Opt. Mater. - 2022. - Vol. 10, Is. 21. - Ст.2200851. - ISSN 21951071 (ISSN), DOI 10.1002/adom.202200851
Примечания : Cited References: 47. - The work was supported by the Ministry of Science and Technology of China (No. G2021030022L), the Guangdong Provincial Special Fund for Modern Agriculture Industry Technology Innovation Teams (No. 2021KJ122), the National Natural Science Foundations of China (No. 52102042), the Independent Research and Development Projects of Maoming Laboratory (No. 2021ZZ004), the Key Realm R&D Program of Guangdong Province (No. 2021B0707010003), the Guangzhou Science & Technology Project (Nos. 202007020005 and 202103000059), the Guangdong Provincial Science and Technology Project (Nos. 2021A0505050006 and 2022A1515010229), and the Project of GDUPS (2018) for B.L.
Аннотация: Developing innovative narrow-band green-emitting phosphors featuring low thermal quenching and eco-friendliness for white light-emitting diode (WLED) backlights is a pivotal challenge. Benefitting from narrowband and low toxicity of green-emitting silanized carbon dots (Si-CDs), an efficient confinement and protection strategy through embedding Si-CDs in mesoporous aluminas (MAs) is proposed to construct MAs and Si-CDs composites (Si-CDs@MAs) with superior luminescence properties. Si-CDs@MAs phosphor exhibits green emission at 526 nm with narrow full width at half maximum of 51 nm, zero-thermal quenching even up to 423 K (104.1%@423 K of the emission peak intensity at 298 K), and the internal quantum efficiency of 64.46%. Compared with broad-band yellow-emitting solid-state Si-CDs (S-Si-CDs), the thermal stability, photostability, and water stability of Si-CDs@MAs phosphor are remarkably improved due to surface protection. The WLED backlight is fabricated with optimized Si-CDs@MAs phosphor, which shows high luminous efficacy of 117.43 lm W?1 and wide color gamut (107% NTSC). Furthermore, this work provides the design principles of realizing stable narrow-band solid-state fluorescence carbon dots, suggesting its great potential for wide-color-gamut display application.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhou G., Ren Q., Molokeev M. S., Zhou Y., Zhang J., Zhang X. -M.
Заглавие : Unraveling the ultrafast self-assembly and photoluminescence in zero-dimensional Mn2+-based halides with narrow-band green emissions
Место публикации : ACS Appl. Electron. Mater. - 2021. - Vol. 3, Is. 9. - P.4144-4150. - ISSN 26376113 (ISSN), DOI 10.1021/acsaelm.1c00606
Примечания : Cited References: 37. - This work is supported by the Natural Science Foundation of China (no. 21871167) and the 1331 project of Shanxi Province and funded by RFBR according to the research project no. 19-52-80003
Аннотация: The discovery of narrow-band luminescent materials remains an immense challenge to optimize the performance of white light-emitting diodes (LEDs). So far, the zero-dimensional (0D) Mn2+-based halides with near-unity narrow-band emissions have emerged as a class of promising phosphors in solid-state displays, but the related large-scale synthesis strategies have not been proposed and evaluated. Herein, we report an in situ synthetic process of 0D Mn2+-based halides and utilize (C20H20P)2MnBr4 as a case to investigate the photoluminescence characteristics and the structural essence of ultrafast self-assembly. The bright green emission peak at 523 nm with a full width at half maximum of 48 nm for (C20H20P)2MnBr4 is attributed to the d–d transition (4T1–6A1) of tetrahedrally coordinated [MnBr4]2– centers, and the fabricated white LED device shows a wide color gamut of 103.7% National Television System Committee (NTSC) standard. Remarkably, the experimental and theoretical results indicate that there are hydrogen bonding of C–H···Br and weak van der Waals interactions between [C20H20P]+ and [MnBr4]2–, resulting in the root for the realization of ultrafast self-assembly in 0D Mn2+-based halides. This work reveals a feasible and general synthesis method for preparing 0D Mn2+-based halides, thereby providing a possibility for their industrial application in solid-state displays.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Qiao J., Zhou Y., Molokeev M. S., Zhang Q., Xia Z.
Заглавие : Narrow bandwidth luminescence in Sr2Li(Al,Ga)O4:Eu2+ by selective site occupancy engineering for high definition displays
Место публикации : Laser Photon. Rev. - 2021. - Vol. 15, Is. 11. - Ст.2100392. - ISSN 18638880 (ISSN), DOI 10.1002/lpor.202100392
Примечания : Cited References: 39. - J.Q. and Y.Z. contributed equally to this work. This research was supported by the National Natural Science Foundation of China (grant nos. 51972118 and 51961145101), International Cooperation Project of National Key Research and Development Program of China (2021YFE0105700), Guangzhou Science & Technology Project (202007020005), the State Key Laboratory of Luminescent Materials and Devices (Skllmd-2021-09), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01×137). This work is also funded by RFBR according to the research project no. 19-52-80003
Аннотация: It remains a critical challenge to develop narrow-band emitters for wide color gamut displays. Herein, it is designed by the selective site occupancy engineering and an unprecedented narrow-band green-emitting phosphor is prepared through chemical substitution. By introducing Ga3+ ions into Sr2LiAlO4:Eu2+ phosphor, the distribution of Eu2+ ions in Sr1 and Sr2 sites is effectively controlled, and only one type of luminescent centers Eu2+(Sr1) is remained in Sr2LiAl0.6Ga0.4O4:Eu2+ due to the compression effect of Sr2O8 polyhedra. Sr2LiAl0.6Ga0.4O4:Eu2+ phosphor presents an extremely narrow-band green emission centered at 512 nm with a full-width at half-maximum of only 40 nm. The wide color gamut (107% National Television System Committee) of the as-fabricated white liquid crystal displays and the vivid figures captured from the projector demonstrate the potential application of narrow-band emitter for wide-color gamut displays. This work provides the design principles of realizing narrow-band emission by selective site occupancy engineering and can set the stage for the exploring of Eu2+-activated phosphor for high definition displays.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Loiko V. A., Zyryanov V. Ya., Konkolovich A. V., Miskevich A. A., Prishchepa O. O., Shabanov A. V., Krakhalev M. N.
Заглавие : Spectral dependences of transmittance and polarizing ability of stretched PDLC films with homogeneous and inhomogeneous interface anchoring
Коллективы : EuroDisplay international conference, Society for Information Displays, Белорусский государственный университет информатики и радиоэлектроники
Место публикации : EuroDisplay 2019: book of abstracts of International conference. - 2019. - Ст.O-9. - P.25
Примечания : Cited References: 2
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Krakhalev M. N., Prishchepa O. O., Feyzer K. A., Sutormin V. S., Loiko V. A., Konkolovich A. V., Miskevich A. A., Zyryanov V. Ya.
Заглавие : Electro-optical response of PDLC films with conical boundary conditions
Коллективы : EuroDisplay international conference, Society for Information Displays, Белорусский государственный университет информатики и радиоэлектроники
Место публикации : EuroDisplay 2019: book of abstracts of International conference. - 2019. - Ст.O-31. - P.63
Примечания : Cited References: 3
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Sutormin V. S., Krakhalev M. N., Timofeev I. V., Bikbaev R. G., Prishchepa O. O., Zyryanov V. Ya.
Заглавие : Polarization characteristics of light passed through a cholesteric layer with tangential-conical boundary conditions
Коллективы : EuroDisplay international conference, Society for Information Displays, Белорусский государственный университет информатики и радиоэлектроники
Место публикации : EuroDisplay 2019: book of abstracts of International conference. - 2019. - Ст.O-4. - P.20
Примечания : Cited References: 2
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Кузьменок Н. М., Михалёнок С. Г., Орёл А. С., Безбородов В. С., Крахалев, Михаил Николаевич, Сутормин, Виталий Сергеевич, Прищепа, Оксана Олеговна, Зырянов, Виктор Яковлевич
Заглавие : Синтез и исследование анизотропных солей аммония для создания жидкокристаллических материалов и устройств с варьируемым поверхностным сцеплением
Место публикации : Жидк. кристаллы и их практич. использ. - 2018. - Т. 18, № 4. - С. 27-39. - ISSN 1991-3966, DOI 10.18083/LCAppl.2018.4.27; Liq. Cryst. Appl.
Примечания : Библиогр.: 13. - Работа выполнена частично при поддержке БРФФИ (грант № X16P-110) и РФФИ (грант № 16-53-00073).
Ключевые слова (''Своб.индексиров.''): жидкокристаллические материалы--ионные сурфактанты--амины--кватернизация--электрооптические устройства--дисплеи--liquid crystals--ionic surfactants--amines--quaternization--electro-optical devices--displays
Аннотация: Получены разнообразные анизотропные четвертичные соли аммония, характеризующиеся специфическим взаимодействием с границей раздела и способные к формированию различных ориентационных структур жидкокристаллического слоя. Показано, что данные соли перспективны для создания более совершенных ЖК-композиций с поверхностным сцеплением, обусловленным ионными сурфактантами, а результаты исследований представляют несомненный интерес для разработчиков новых жидкокристаллических материалов и электрооптических устройств на их основе.Various anisotropic quaternary ammonium salts characterized by a specific interaction with the interface and capable to form various orientational structures of liquid crystal layer, have been prepared. It has been shown that these salts are promising materials for creation of advanced LC compositions with surface anchoring caused by ionic surfactants. The obtained results are of undoubted interest for the developers of new liquid crystal materials and electro-optical devices based on them.
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10.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Loiko V. A., Konkolovich A. V., Krakhalev M. N., Miskevich A. A., Prishchepa O. O., Zyryanov V. Ya.
Заглавие : Development of scattering media optics methods to calculate optical properties of polymer dispersed liquid crystal films
Коллективы : EuroDisplay conference, Society for Information Displays, Institute of Physics
Место публикации : EuroDisplay 2017: Abstract book. - 2017. - P.27-28
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