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Antiferromagnetic resonance and phase diagrams of gadolinium ferroborate GdFe3(BO3)(4) / A. I. Pankrats [et al.] // J. Exp. Theor. Phys. - 2004. - Vol. 99, Is. 4. - P. 766-775, DOI 10.1134/1.1826168. - Cited References: 16 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary

Кл.слова (ненормированные):
Anisotropy -- Antiferromagnetic materials -- Antiferromagnetism -- Phase diagrams -- Resonance -- Single crystals -- Antiferromagnetic resonance -- Antiferromagnets -- Crystal axis -- Transition fields -- Gadolinium compounds
Аннотация: Antiferromagnetic resonance in single crystals of rhombohedral gadolinium ferroborate GdFe3(BO3)(4) was studied. The frequency-field dependences of antiferromagnetic resonance over the frequency range 26-70 GHz and the temperature dependences of resonance parameters for magnetic fields oriented along the crystal axis and in the basal plane were determined. It was found that the iron subsystem, which can be treated as a two-sublattice antiferromagnet with anisotropy of the easy-plane type, experienced ordering at T = 38 K. At temperatures below 20 K, the gadolinium subsystem with the opposite anisotropy sign strongly influenced the anisotropic properties of the crystal. This resulted in a spontaneous spin-reorientation transition from the easy-plane to the easy-axis state at 10 K. Below 10 K, magnetic field-induced transitions between the states were observed. Experimental phase diagrams on the temperature-magnetic field plane were constructed for fields oriented along the crystal axis and in the basal plane. A simple model was used to calculate the critical transition fields. The results were in close agreement with the experimental values measured at T = 4.2 K for both field orientations. (C) 2004 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, Siberian Div, Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Pankrats, A. I.; Панкрац, Анатолий Иванович; Petrakovskii, G. A.; Петраковский, Герман Антонович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Bayukov, O. A.; Баюков, Олег Артемьевич
}
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Antiferromagnetic resonance in ferroborate NdFe3(BO3)(4) / M. I. Kobets, K. G. Dergachev, E. N. Khatsko [et al.] // Physica B. - 2011. - Vol. 406, Is. 18. - P. 3430-3435, DOI 10.1016/j.physb.2011.06.014. - Cited Reference Count: 19 . - SEP 15. - ISSN 0921-4526. - ISSN 1873-2135
Рубрики:
Physics, Condensed Matter
Кл.слова (ненормированные):
antiferromagnet -- resonance -- multiferroics -- commensurate-incommensurate phase
Аннотация: The AFMR spectra of the NdFe3(BO3)(4) crystal are measured in a wide range of frequencies and temperatures. It is found that by the type of its magnetic anisotropy the compound is an easy-plane antiferromagnet with a weak anisotropy in the basal plane. The effective magnetic parameters are determined: anisotropy fields H-a1 = 1.14 kOe and H-a2 = 60 kOe and magnetic excitation gaps Delta v(1) = 101.9 GHz and Delta v(2) = 23.8 GHz. It is shown that commensurate-incommensurate phase transition causes a shift in resonance field and a considerable change in absorption line width. At temperatures below 4.2 K nonlinear regimes of AFMR excitation at low microwave power levels are observed. (C) 2009 Elsevier B.V. All rights reserved.

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Держатели документа:
Natl Acad Sci, B Verkin Inst Low Temp Phys & Engn, UA-61103 Kharkov, Ukraine;
L V Kirensky Inst Phys SB RAS, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Kobets, M.I.; Dergachev, K.G.; Khatsko, E.N.; Gnatchenko, S.L.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Temerov, V. L.; Темеров, Владислав Леонидович
}
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Comparing the magnetic and magnetoelectric properties of the SmFe3(BO3)4 ferroborate single crystals grown using different solvents / E. Eremin [et al.] // J. Cryst. Growth. - 2019. - Vol. 518. - P. 1-4, DOI 10.1016/j.jcrysgro.2019.04.017. - Cited References: 17. - This study was supported by the Russian Foundation for Basic Research (RFBR) according to the research projects No. 18-02-00696_a and RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Region Science and Technology Support Fund by project No. 18-42-240011 p_a. . - ISSN 0022-0248. - ISSN 1873-5002

РУБ Crystallography + Materials Science, Multidisciplinary + Physics, Applied
Рубрики:
POLARIZATION
FEATURES
Кл.слова (ненормированные):
Impurities -- Growth from solutions -- Single crystal growth -- Borates -- Ferroelectric materials -- Magnetic materials
Аннотация: SmFe3(BO3)4 single crystals have been grown from the bismuth trimolybdate and lithium tungstate-based melt–solutions. Samarium ferroborate single crystals were grown first from the lithium–tungstate flux. The magnetic and magnetoelectric properties of the synthesized crystals have been compared. It is shown that the SmFe3(BO3)4 ferroborate grown from the bismuth trimolybdate-based melt–solution contains impurities of Bi3+ ions (∼5% at.), which replace Sm3+ ions, while the SmFe3(BO3)4, ferroborate grown from the lithium tungstate-based melt–solution contains minor or zero amounts of such impurities. The magnetoelectric and magnetodielectric effects with the Bi3+ admixture appeared 1.5× stronger than in SmFe3(BO3)4; this is probably due to twinning.

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Держатели документа:
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.

Доп.точки доступа:
Eremin, E. V.; Еремин, Евгений Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович; Smolyakov, D. A.; Смоляков, Дмитрий Александрович; Molokeev, M. S.; Молокеев, Максим Сергеевич; Russian Foundation for Basic Research (RFBR) [18-02-00696_a]; RFBR, Government of Krasnoyarsk Territory, Krasnoyarsk Region Science and Technology Support Fund [18-42-240011 p_a]
}
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    Dynamics of structural and magnetic phase transitions in ferroborate YFe3(BO3)4 / K. V. Frolov [et al.] // J. Alloys Compd. - 2018. - Vol. 748. - P. 989-994, DOI 10.1016/j.jallcom.2018.03.243. - Cited References: 58. - We thank Dr. A.P. Dudka for help in the low temperature XRD measurements and Dr. D.Yu. Chernyshov for help in the synchrotron XRD measurements. This study was supported by the Federal Agency of Scientific Organizations (Agreement No 007-ГЗ/Ч3363/26 ) in parts of energy-dispersive X-ray microanalysis, high-temperature XRD, and Mossbauer measurements, by the Russian Foundation for Basic Research (project #17-02-00766а ) in parts of low-temperature XRD and Mossbauer measurements, Russian Ministry of Education and Science and performed using the equipment of the Shared Research Center of the Shubnikov Institute of Crystallography of FSRC “Crystallography and Photonics” RAS. . - ISSN 0925-8388
   Перевод заглавия: Динамика структурных и магнитных фазовых переходов в ферроборате YFe3(BO3)4
Кл.слова (ненормированные):
Multiferroics -- Rare-earth compounds -- X-ray diffraction -- Mossbauer spectroscopy -- Crystal structure
Аннотация: X-ray analysis of the YFe3(BO3)4 single crystal revealed different behavior of parameters of the crystal cell with an increase in temperature from 25 to 500 K. The parameters a and b initially increase monotonically and then rise sharply in the range between 360 and 380 K, which corresponds to the structural phase transition. The parameter c initially decreases linearly upon heating and then begins to increase, passing through a minimum at 90 K. In the interval of 200–500 K the parameter c grows linearly and does not undergo anomalies at the structural phase transition. The results of Mössbauer measurements at 57Fe nuclei in the paramagnetic phase of YFe3(BO3)4 correlate well with the XRD data, but they do not separate the two structural states of iron ions Fe1 and Fe2 arising in the P3121 phase during the structural phase transition. The temperature of the magnetic phase transition TN = 39.42(16) K is established, below which the iron ions form a 3D magnetic order of the Heisenberg type. The calculated “Mössbauer” Debye temperature ΘM = 340(2) K turned out to be three times lower than the Debye temperature of the entire crystal lattice TD = 1020 K. Mössbauer data indicate a weak bonding between the helicoidal chains of iron and the rest of the crystal lattice.
Рентгеновский анализ монокристалла YFe3(bo3-серии)4 выявил различие в поведении параметров кристаллической ячейки с увеличением температуры от 25 до 500 к. Параметры a и b сначала монотонно возрастают, а затем резко поднимется в диапазон между 360 и 380 К, что соответствует структурному фазовому переходу. Параметр c сначала линейно уменьшается при нагревании, а затем начинает возрастать, проходя через минимум при 90 K. В интервале 200-500 K параметр c растет линейно и не претерпевает аномалий при структурном фазовом переходе. Результаты Мёсбауэровской спектроскопии ядер 57Fe в парамагнитной фазе в YFe3(BO3)4 коррелируют с РСА, но они не разделяют двух структурных состояний ионов железа Fe1 и Fe2, возникающие в фазе P3121 в процессе структурного перехода. Установили температуру магнитного фазового перехода TN= 39.42(16) К, в результате которого ионы железа образуют 3D магнитный порядок типа Гейзенберга. Рассчитанная по Мёссбауэру Дебаевская температура QM= 340(2) K оказалась в три раза ниже температуры Дебая внутри кристаллической решетки TD= 1020 K. Данные Мёсбауэра указывают на слабую связь между геликоидальными цепочками железной и остальных кристаллических решеток.

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Держатели документа:
Shubnikov Institute of Crystallography of FSRC “Crystallography and Photonics” RAS, Moscow, Russian Federation
Kirensky Institute of Physics, Siberian Branch of Russian Academy of Sciences, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Frolov, K. V.; Lyubutin, I. S.; Alekseeva, O. A.; Smirnova, E. S.; Verin, I. A.; Temerov, V. L.; Темеров, Владислав Леонидович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Artemov, V. V.; Dmitrieva, T. V.
}
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Gavrichkov, V. A.
Effect of optical f - f excitations on the Nd-Fe exchange interaction in Nd ferroborate with multiferroic properties / V. A. Gavrichkov, A. V. Malakhovskii, S. G. Ovchinnikov // Phys. Rev. B. - 2021. - Vol. 104, Is. 6. - Ст. 064445, DOI 10.1103/PhysRevB.104.064445. - Cited References: 28. - The reported study was supported by the RFBR Grant 19-02-00034. V.A.G. is also grateful to the Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, and Krasnoyarsk Regional Fund of Science according to the research project "Studies of superexchange and electron-phonon interactions in correlated systems as a basis for searching for promising functional materials" No. 20-42-240016 . - ISSN 2469-9950. - ISSN 2469-9969

РУБ Materials Science, Multidisciplinary + Physics, Applied + Physics, Condensed Matter
Рубрики:
LOCAL MAGNETIC-PROPERTIES
SINGLE-CRYSTAL
EXCITED-STATES
Аннотация: We considered the effect of optical pumping at the f−f transitions frequency on d−f superexchange in the rare-earth antiferromagnetic ferroborate Nd0.5Gd0.5Fe3(BO3)4 between Nd3+ ions in the excited states of the 4G5/2, 2G7/2, and Fe3+ in the ground state 6A1. In the ferroborate, d−f superexchange is directly related to the strong magnetoelectric coupling observed in the ground state of the material. We show that under optical pumping at the frequency of f−f transitions 4I9/2↔(4G5/2+2G7/2) in the Nd3+ ion, the nature of the d−f interaction changes to FM. The phenomena can be explained by the occupation of the excited Nd3+ “spin pure” states with spin 1/2, or their mixing to the optically excited states with spin 3/2 due to the spin-orbit interaction. Near optically excited ions Nd3+, magnetic frustrations change from FM ordering under the d−f AFM interaction to AFM ordering under the FM interaction in the basal hexagonal plane.

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Держатели документа:
Kirensky Inst Phys, Akademgorodok 50,Bld 38, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Гавричков, Владимир Александрович; RFBRRussian Foundation for Basic Research (RFBR) [19-02-00034]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Krasnoyarsk Regional Fund of Science [20-42-240016]; Government of Krasnoyarsk Territory
}
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Electron transport in FeBO3 ferroborate at ultrahigh pressures / I. A. Troyan [et al.] // JETP Letters. - 2012. - Vol. 94, Is. 10. - P. 748-752, DOI 10.1134/S0021364011220115. - Cited References: 22. - This work was supported by the Russian Foundation for Basic Research (project nos. 09-02-01527-a, 09-02-00127-a, 09-02-00171-a, 11-02-00291-a, and 11-02-00636-a), by the Ministry of Education and Science of the Russian Federation (state contract nos. 16.518.11.7021 and MK-5632.2010.2), and by the Division of Physical Sciences, Russian Academy of Sciences (program "Strong Electron Correlations"). . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
MAGNETIC COLLAPSE
TRANSITION
STATE
Аннотация: The electrical resistance of FeBO3 crystals at high and ultrahigh pressures (up to 198 GPa) and low temperatures has been measured using diamond anvil cells. It has found that in the high-pressure phase, 46 GPa ‹ P‹ 100 GPa, the activation energy E-ac decreases gradually from 0.55 to 0.3 eV according to a linear law. Its extrapolation to zero gives an estimated value of about 210 GPa for the pressure at which complete metallization is expected. However, above 100 GPa, the linear E-ac(P) dependence smoothly transforms to a nonlinear one. At the same time, the temperature dependence of the electrical resistance at fixed pressure significantly deviates from the Arrhenius activation law and does not obey the Mott law for the hopping conductivity. Experimental data demonstrate the dependence of the activation energy E-ac both on pressure and temperature. At T = 0, the gap tends to zero. Theoretical analysis shows that the decrease in E-ac upon cooling can be interpreted in terms of the transition of the low-spin FeBO3 phase to the magnetically ordered (anti-ferromagnetic) state.

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Публикация на русском языке Транспортные свойства ферро-бората FeBO3 при сверхвысоких давлениях [Текст] / И. А. Троян [и др.] // Письма в Журн. эксперим. и теор. физ. : Наука, 2011. - Т. 94 Вып. 10. - С. 811-815

Держатели документа:
[Troyan, I. A.
Gavrilyuk, A. G.
Lyubutin, I. S.] Russian Acad Sci, Shubnikov Inst Crystallog, Moscow 119333, Russia
[Troyan, I. A.] Max Planck Inst Chem, D-55020 Mainz, Germany
[Gavrilyuk, A. G.] Russian Acad Sci, Inst Nucl Res, Troitsk 142190, Moscow Region, Russia
[Ovchinnikov, S. G.
Kazak, N. V.] Russian Acad Sci, Siberian Branch, Kirensky Inst Phys, Krasnoyarsk 660036, Russia
[Ovchinnikov, S. G.] Siberian Fed Univ, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Troyan, I. A.; Gavrilyuk, A. G.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Lyubutin, I. S.; Kazak, N. V.; Казак, Наталья Валерьевна
}
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Features of magnetoelastic properties of yttrium ferroborate at low temperatures / G. A. Zvyagina [и др.] // First International Workshop Novel Trends in Physics of Ferroics. [[b]]NTPF-2014[[/b]], July 4-6, 2014, St. Petersburg, Russia : Book of abstracts. - 2014. - P59

Материалы конференции

Доп.точки доступа:
Zvyagina, G. A.; Zhekov, K. R.; Bilych, I. V.; Zvyagin, A. A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович; International Workshop Novel Trends in Physics of Ferroics (1 ; July 4-6 ; St. Petersburg, Russia)
}
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Giant gigahertz optical activity in multiferroic ferroborate / A. M. Kuzmenko [et al.] // Phys. Rev. B. - 2014. - Vol. 89, Is. 17. - Ст. 174407, DOI 10.1103/PhysRevB.89.174407. - Cited References: 35. - This work was supported by the Russian Foundation for Basic Researches (Grants No. 12-02-01261 and No. 12-02-31461 mol) and by the Austrian Science Funds (Grants No. I815-N16 and No. W1243). . - ISSN 1098-0121. - ISSN 1550-235X
Рубрики:
RFE3(BO3)4
Аннотация: In contrast to the well-studied multiferroic manganites with a spiral structure, the electric polarization in multiferroic borates is induced within a collinear antiferromagnetic structure and can easily be switched by small static fields. Because of specific symmetry conditions, the static and dynamic properties in borates are directly connected, which leads to giant magnetoelectric and magnetodielectric effects. Here we prove experimentally that the giant magnetodielectric effect in samarium ferroborate, SmFe3(BO3)4, is of intrinsic origin and is caused by an unusually large electromagnon situated in the microwave range. This electromagnon reveals a strong optical activity exceeding 120 degrees of polarization rotation in a millimeter thick sample.
В отличие от хорошо изученных мультиферроиков манганитов со спиральной структуры, электрическая поляризация в мультиферроиков боратов индуцируется в коллинеарной антиферромагнитной структуре и может легко переключаться небольшими статическими полями. Из-за специфических условий симметрии, статические и динамические свойства боратов непосредственно связаны, что приводит к гигантским магнитоэлектрическому и магнитодиэлектрическому эффектам. Здесь мы экспериментально доказываем, что гигантский магнитодиэлектрический эффект в самариевом ферробората, SmFe3 (BO3) 4, имеет самостоятельное происхождение и вызван необычно большим электромагноном, расположеным в микроволновом диапазоне. Это электромагнон показывает сильную оптическую активность, более 120 градусов вращения поляризации в миллиметровом образце.

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Держатели документа:
Russian Acad Sci, Prokhorov Gen Phys Inst, Moscow 119991, Russia
Vienna Univ Technol, Inst Solid State Phys, A-1040 Vienna, Austria
RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Kuzmenko, A. M.; Кузьменко А. М.; Shuvaev, A.; Dziom, V.; Pimenov, A.; Schiebl, M.; Mukhin, A. A.; Ivanov, V. Yu.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Russian Foundation for Basic Researches [12-02-01261, 12-02-31461 mol]; Austrian Science Funds [I815-N16, W1243]
}
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Titova, Veronika.
Growth of single crystals of trigonal ferroborate Ho0,5Nd0,5Fe3(BO3)4 with the huntite structure depending on the crystallochemical growth conditions / V. R. Titova, I. A. Gudim // Химия, физика, биология, математика: теоретические и прикладные исследования : сб. статей по материалам XXXIV междун. науч.-практич. конф. - 2020. - Т. 3 (24). - P. 123-129

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Источник статьи
Держатели документа:
Kirensky Institute of Physics
Sibirian Federal University

Доп.точки доступа:
Gudim, I. A.; Гудим, Ирина Анатольевна; Химия, физика, биология, математика: теоретические и прикладные исследования, международная научно-практическая конференция(34 ; 2020 ; 17 марта ; Москва)
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10.

Infrared absorption spectrum of HoFe3(BO3)4 crystal / S. N. Sofronova [et al.] // Vib. Spectrosc. - 2014. - Vol. 72. - P. 20-25, DOI 10.1016/j.vibspec.2014.02.005. - Cited References: 18. - The work was partially supported by the RFBR through Grants No. 13-02-00825 and 13-02-98041, SS-4828.2012.2. . - ISSN 0924-2031. - ISSN 1873-3697

РУБ Chemistry, Analytical + Chemistry, Physical + Spectroscopy
Рубрики:
MAGNETOELASTIC INTERACTIONS
IRON
GDFE3(BO3)4
Кл.слова (ненормированные):
Holmium ferroborate -- Infrared absorption
Аннотация: Infrared (IR) absorption spectra of HoFe3(BO3)4 crystal have been obtained in spectral range 30–7000 cm−1 at temperatures from 4 to 423 K. Vibrational frequencies have been simulated with ‘Lady’ software package both for high-temperature and low-temperature phases. The experimental spectra have been analyzed on the basis of calculated data, and interpreted within the framework of internal vibrations of ionic complexes of HoFe3(BO3)4 crystal lattice. The spectral range under study was observed to have no Davydov splitting of internal vibrational modes due to unit cell multiplication. No effects of magnetic ordering on the IR spectra of the crystal under study were observed in the low-temperature range.

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Держатели документа:
Kirensky Inst Phys SB RAS, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660079, Russia

Доп.точки доступа:
Sofronova, S. N.; Софронова, Светлана Николаевна; Gerasimova, Y. V.; Герасимова, Юлия Валентиновна; Vtyurin, A. N.; Втюрин, Александр Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Shestakov, N. P.; Шестаков, Николай Петрович; Ivanenko, A. A.; Иваненко, Александр Анатольевич; RFBR [13-02-00825, 13-02-98041, SS-4828.2012.2]
}
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