Библиотека института физики им. Л.В. Киренского СО РАН

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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov Yu. S., Dudnikov V. A., Vereshchagin S. N., Volochaev M. N., Gavrilkin S. Y., Tsvetkov A. Y.
Заглавие : Order–disorder transition in the Dy0.2Sr0.8CoO3-δ rare-earth cobalt oxide solid solutions: Structural and thermoelectric properties
Место публикации : J. Eur. Ceram. Soc. - 2020. - Vol. 40, Is. 15. - P.5559-5565. - ISSN 09552219 (ISSN), DOI 10.1016/j.jeurceramsoc.2020.06.066
Примечания : Cited References: 29. - This study was supported by the Russian Science Foundation, project no. 19-72-00097
Аннотация: By the example of the Dy0.2Sr0.8CoO3-δ compound undergoing an order–disorder phase transition with increasing temperature, we demonstrate a significant dependence of the kinetic properties on the morphology of the internal spatially inhomogeneous structure, which forms in the sample depending on the rate of its transition from the high-temperature disordered cubic phase to the ground tetragonal ordered phase upon cooling. The results of transmission electron microscopy visualization of the spatially inhomogeneous state in the Dy0.2Sr0.8CoO3-δ ceramic samples are presented and compared with the X-ray diffraction data.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mikhaleva E. A., Gorev M. V., Bondarev V. S., Bogdanov E. V., Flerov I. N.
Заглавие : Comparative analysis of elastocaloric and barocaloric effects in single-crystal and ceramic ferroelectric (NH4)2SO4
Место публикации : Scripta Mater. - 2021. - Vol. 191. - P.149-154. - ISSN 13596462 (ISSN), DOI 10.1016/j.scriptamat.2020.09.030
Примечания : Cited References: 47. - The reported study was supported by the Russian Science Foundation (project no. 19-72-00023 ). X-ray and dilatometric data were obtained using the equipment of Krasnoyarsk Regional Center of Research Equipment of Federal Research Center “Krasnoyarsk Science Center SB RAS”
Аннотация: We report the influence of anisotropy and texture on elasto(ElCE)- and baro(BCE)-caloric effects in single-crystal and ceramic (NH4)2SO4. Inverse extensive and intensive ElCE in ceramics, (ΔSElCE)cer = 87 J/kg·K; ΔTAD = - 11.6 K), as well as in a single crystal along the ferroelectric axis a, (ΔSElCE)a = 115 J/kg·K; (ΔTAD)a = - 16 K, significantly exceed BCE, ΔSBCE = 75 J/kg·K; ΔTAD = - 9.8 K, even at low pressure ~ 0.3 GPa. Caloric parameters of ammonium sulphate are comparable with those for promising solid-state refrigerants.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gerasimova Y.V., Oreshonkov A. S., Laptash N. M., Krylov A. S., Aliev A. R., Roginskii E. M.
Заглавие : Raman scattering and phase transitions in (NH4)3TiF7
Место публикации : J. Raman Spectrosc. - 2018. - Vol. 49, Is. 7. - P.1230-1235. - ISSN 03770486 (ISSN), DOI 10.1002/jrs.5374
Примечания : Cited References: 18
Ключевые слова (''Своб.индексиров.''): (nh4)3tif7--lattice dynamics--order–disorder--reconstructive phase transition--symmetry lowering
Аннотация: Raman spectra of (NH4)3TiF7 within spectral range 10–3,400 cm−1 at temperatures 8–370 K are recorded, which revealed 2 phase transitions at temperatures T1 = 355 K and T2 = 283 K. First principles calculations of lattice dynamics and assignment of the observed lines to specific vibrational types are performed. The first phase transition is classified as an “order–disorder” one. Manifestation of 97 cm−1 vibration (mixed translational [NH4 + F7]) evidences the creation of the hydrogen bond between ammonium group and free fluorine atom, indicating to reconstructive type of phase transition an T2 = 283 K. The emergence of a large number of vibrational lines in Raman spectra at low temperatures proves symmetry lowering of NH4 tetrahedra with the simultaneous ordering of TiF6 octahedra.
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Вид документа : Статья из журнала
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Автор(ы) : Gorev M. V., Mikhaleva E. A., Flerov I. N., Bogdanov E. V.
Заглавие : Conventional and inverse barocaloric effects in ferroelectric NH4HSO4
Место публикации : J. Alloys Compd. - 2019. - Vol. 806. - P.1047-1051. - ISSN 09258388 (ISSN), DOI 10.1016/j.jallcom.2019.07.273
Примечания : Cited References: 22
Аннотация: In this study, the conventional and inverse barocaloric effects (BCE) in ferroelectric NH4HSO4 are reported. Maximum extensive and intensive BCE near order–disorder phase transition can be achieved at low pressure p≤0.1 GPa. Large thermal expansion of the crystal lattice plays a very important role in the developing conventional BCE and conversation between BCE of different sign in the narrow temperature range.
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