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1.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Aplesnin S. S., Udod L. V., Sitnikov M. N., Velikanov D. A., Gorev M. V., Molokeev M. S., Galyas A. I., Yanushkevich K. I.
Заглавие
: Magnetic and electrical properties of bismuth cobaltite Bi24(CoBi)O40 with charge ordering
Место публикации
: Phys. Solid State. - 2012. - Vol. 54, Is. 10. - P.2005-2014. - ISSN 1063-7834,
DOI
10.1134/S106378341210006X
Примечания
: Cited References: 22. - This study was supported by the Russian Foundation for Basic Research (project nos. 09-02-92001-NNS_a, 12-02-00125-a, and 11-02-98004-r_sibir'_a)
Предметные рубрики:
Thermoelectric-power
Co3O4
Conductivity
Transition
Аннотация:
The compound Bi24(CoBi)O40 has been synthesized using the solid-phase reaction method. The temperature and field dependences of the magnetic moment in the temperature range 4 K T 300 K and the temperature dependences of the EPR line width and g-factor at temperatures 80 K T 300 K have been investigated. The electrical resistivity and thermoelectric power have been measured in the temperature range 100 K T 1000 K. The activation energy has been determined and the crossover of the thermoelectric power from the phonon mechanism to the electron mechanism with variations in the temperature has been observed. The thermal expansion coefficient of the samples has been measured in the temperature range 300 K T 1000 K and the qualitative agreement with the temperature behavior of the electrical resistivity has been achieved. The electrical and structural properties of the compound have been explained in the framework of the model of the electronic-structure transition with inclusion of the exchange and Coulomb interactions between electrons and the electron-phonon interaction.
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2.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Korshunov M. M., Efremov D. V., Golubov A. A., Dolgov O. V.
Заглавие
: Unexpected impact of magnetic disorder on multiband superconductivity
Коллективы
: Dynasty Foundation; ICFPM; Ministry of Education and Science of the Russian Federation [14Y26.31.0007]; RFBR [12-02-31534, 13-02-01395]; Leading Scientific Schools of the Russian Federation [NSh-2886.2014.2]; DFG [1458]; EU-Japan
Место публикации
: Phys. Rev. B: American Physical Society, 2014. - Vol. 90, Is. 13. - ISSN 1098-0121,
DOI
10.1103/PhysRevB.90.134517. - ISSN 1550-235X
Примечания
: Cited References: 41. - The authors are grateful to S.-L. Drechsler, P.J. Hirschfeld, K. Kikoin, and S.G. Ovchinnikov for useful discussions. We acknowledge partial support by the Dynasty Foundation and ICFPM (MMK), the Ministry of Education and Science of the Russian Federation (Grant No. 14Y26.31.0007), RFBR (Grant Nos. 12-02-31534 and 13-02-01395), President Grant for Government Support of the Leading Scientific Schools of the Russian Federation (NSh-2886.2014.2), DFG Priority Program 1458, and FP7 EU-Japan program IRON SEA.
Предметные рубрики:
HIGH-TEMPERATURE SUPERCONDUCTIVITY
PARAMAGNETIC IMPURITIES
IRON
CONDUCTIVITY
ALLOYS
Аннотация:
We analyze how the magnetic disorder affects the properties of the two-band s± and s++ models, which are the subject of discussions regarding iron-based superconductors and other multiband systems like MgB2. We show that there are several cases when the transition temperature Tc is not fully suppressed by magnetic impurities in contrast to the Abrikosov-Gor'kov theory, but a saturation of Tc takes place in the regime of strong disorder. These cases are: (1) the purely interband impurity scattering and (2) the unitary scattering limit. We show that in the former case the s± gap is preserved, while the s++ state transforms into the s± state with increasing magnetic disorder. For case (2), the gap structure remains intact.
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3.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Belyaev B. A., Drokin N. A.
Заглавие
: Impedance spectroscopy investigation of electrophysical characteristics of the electrode-liquid crystal interface
Коллективы
: Siberian Branch of the Russian Academy of Sciences [109]
Место публикации
: Phys. Solid State: MAIK Nauka-Interperiodica / Springer, 2015. - Vol. 57, Is. 1. - P.181-187. - ISSN 1063,
DOI
10.1134/S1063783415010060. - ISSN 10906460(eISSN)
Примечания
: Cited References:22. - This study was supported by the Siberian Branch of the Russian Academyof Sciences (integration project no. 109).
Предметные рубрики:
DIELECTRIC-PROPERTIES
CONDUCTIVITY
Аннотация:
The behavior of frequency dependences of the impedance of a capacitive measuring cell with a liquid crystal has been investigated in the frequency range from 10−1 to 105 Hz. A method for determining electrophysical characteristics of the liquid crystal in the bulk and at the liquid crystal-metal electrode interface has been proposed and tested for liquid crystals of the alkyl cyanobiphenyl series, which are doped with ionic surfactants. The method is based on the use of an equivalent electrical circuit, which makes it possible to approximate the impedance spectra with the required accuracy, and also on the determination of the frequency at the singular point in the impedance spectra, at which the reactive component of the electric current flowing through the liquid-crystal cell is negligible compared to the active component.
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4.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Aver'yanov E. M.
Заглавие
: Effective refractive index of a two-dimensional polycrystal
Место публикации
: JETP Letters. - 2015. - Vol. 101, Is. 10. - P.685-689. - ISSN 0021-3640,
DOI
10.1134/S0021364015100033
Примечания
: Cited References: 28
Предметные рубрики:
SPECTROSCOPIC ELLIPSOMETRY
CONJUGATED POLYMERS
LOCAL-FIELD
FILMS
CONDUCTIVITY
POLYFLUORENE
ANISOTROPY
DISPERSION
MEDIA
Аннотация:
A relation of the effective refractive index of a two-dimensional polycrystalline dielectric film in the transparency region to the refractive indices n1 and n2 of crystallites at the positions of axes 1 and 2, respectively, of refraction ellipsoids of the crystallites in the plane of the film has been obtained. This relation and the relation L* = (L1 + L2)/2 between the components of the Lorentz tensors for the film and crystallites have been confirmed by comparison with experimental data for conjugate-polymer films with uniaxial domains.
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5.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Aplesnin S. S., Romanova O. B., Янушкевич, Казимир Иосифович
Заглавие
: Magnetoresistance effect in anion-substituted manganese chalcogenides
Место публикации
: Phys. Status Solidi B. - 2015. - Vol. 252, Is. 8. - P.1792-1798. - ISSN 0370,
DOI
10.1002/pssb.201451607. - ISSN 15213951 (eISSN)
Примечания
: Cited References: 35. - This study was supported by the official assignment no. 114090470016.
Предметные рубрики:
MAGNETIC-PROPERTIES
ELECTRONIC-STRUCTURE
SOLID-SOLUTIONS
MnTe
MnSe
CONDUCTIVITY
TRANSITION
Ключевые слова
(''Своб.индексиров.''): electron tunneling--magnetic properties--magnetoresistance--semiconductors
Аннотация:
The electric and magnetic properties of anion-substituted antiferromagnetic MnSe1-xTex (0.1≤x≤0.4) semiconductors in the 77-700K temperature range and magnetic fields under 1T are studied. In the MnSe1-xTex solid solutions, negative magnetoresistance in the vicinity of the Néel temperature for x=0.1 and for composition with x=0.2 in the paramagnetic range below 270K is revealed. A dependence of the magnetic susceptibility versus the prehistory of the samples is found. The model of localized spin-polarized electrons with the localization radius depending on the magnetic field is proposed for x=0.1. In the paramagnetic range, the negative magnetoresistance and the behavior of magnetic moment are a result of orbital glass formation.
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6.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Petrov M. I., Balaev D. A., Gokhfel'd D. M., Shaikhutdinov K. A.
Заглавие
: Andreev reflection in natural grain boundaries of polycrystalline high-T-c superconductor La1.85Sr0.15CuO4
Разночтения заглавия
:авие SCOPUS: Andreev reflection in natural grain boundaries of polycrystalline high-Tc superconductor La1.85Sr0.15CuO 4
Место публикации
: Phys. Solid State: AMER INST PHYSICS, 2003. - Vol. 45, Is. 7. - P1219-1222. - ISSN 1063-7834,
DOI
10.1134/1.1594233
Примечания
: Cited References: 30
Предметные рубрики:
CURRENT-VOLTAGE CHARACTERISTICS
WEAK LINKS
CHARGE-TRANSPORT
JUNCTIONS
CONDUCTIVITY
HYSTERESIS
COMPOSITES
SCATTERING
Аннотация:
The temperature evolution of the current-voltage characteristic (CVC) of a "break junction" with metal-type
conductivity
on the polycrystalline La1.85Sr0.15CuO4 high-temperature superconductor is investigated. The CVC exhibits gap peculiarities and hysteresis, which is observed in the region of negative differential resistance. The experimental results are described well in terms of the Kummel-Gunsenheimer-Nicolsky theory for an S-N-S junction (S is a superconductor, N is a normal metal) this theory takes into account multiple Andreev reflection of quasiparticles. It is shown that the shape of the CVC and the existence and the shape of hysteresis are determined by the ratio of "long" and "short" grain boundaries in the polycrystal under investigation. (C) 2003 MAIK "Nauka / Interperiodica".
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7.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Shalaev V. M., Poliakov E. Y., Markel V. A.
Заглавие
: Small-particle composites .2. Nonlinear optical properties
Место публикации
: Phys. Rev. B: AMERICAN PHYSICAL SOC, 1996. - Vol. 53, Is. 5. - P2437-2449. - ISSN 0163-1829,
DOI
10.1103/PhysRevB.53.2437
Примечания
: Cited References: 45
Предметные рубрики:
FRACTAL CLUSTERS
RAMAN-SCATTERING
SUSCEPTIBILITY
CONDUCTIVITY
EXCITATIONS
COLLOIDS
LIGHT
Аннотация:
Strong fluctuations of local fields may result in very large optical nonlinearities in small-particle composites. Enhancement associated with particle clustering is found for a number of optical processes, including four-wave mixing (FWM), third-harmonic generation (THG), Raman scattering, and nonlinear refraction and absorption in Kerr media. Field fluctuations and optical nonlinear susceptibilities are especially large in fractal clusters. The enhancement of optical processes is expressed in terms of the resonant linear absorption by collective dipolar eigenmodes in a cluster, and quality factors, q, of the modes (q much greater than 1). It is shown that the susceptibility of a composite material consisting of random small-particle clusters is proportional to q(3) for Raman scattering and the Kerr optical nonlinearity, and to q(4) and q(6) for THG and FWM, respectively. For all of these processes, a spectral dependence of the effective susceptibility is found. Broad-scale numerical simulations of the optical response in small-particle composites are performed to complement the theory. The simulations are in reasonable agreement with available experimental data.
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8.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Gorev M. V., Flerov I. N., Sciau P., Guillemet-Fritsch S.
Заглавие
: Thermal expansion of (Ba1-x La (x) )Ti1-x/4O3 solid solutions
Коллективы
: Russian Foundation for Basic Research [07-02-00069]; Russian Federation [NSh-1011.2008.2]
Разночтения заглавия
:авие SCOPUS: Thermal expansion of (Ba1 - X la x )Ti 1 - X/4O3 solid solutions
Место публикации
: Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2009. - Vol. 51, Is. 4. - P790-796. - ISSN 1063-7834,
DOI
10.1134/S106378340904026X
Примечания
: Cited References: 22. - This work was supported by the Russian Foundation for Basic Research (project no. 07-02-00069) and the Council on Grants from the President of the Russian Federation for the Support of Leading Scientific Schools of the Russian Federation (grant NSh-1011.2008.2).
Предметные рубрики:
CERAMICS
BATIO3
BA(TI1-XZRX)O-3
FERROELECTRICS
CONDUCTIVITY
BEHAVIOR
SYSTEM
PHASE
HEAT
Аннотация:
Deformation and the thermal expansion coefficient of ceramic samples of (Ba1 - x La (x) )Ti1 - x/4O3 solid solutions (x = 0, 0.026, 0.036, 0.054) were studied in the temperature range 120-700 K. Based on an analysis of the data obtained, the temperature-composition phase diagram is refined, and the temperature dependence of the polarization is calculated. The results are discussed in combination with the dielectric measurement data.
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9.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Gorev M. V., Bondarev V. S., Flerov I. N., Maglione M., Simon A., Sciau P., Boulos M., Guillemet-Fritsch S.
Заглавие
: Thermal expansion, polarization and phase diagrams of Ba1-yBi2y/3Ti1-xZrxO3 and Ba1-yLayTi1-y/4O3 compounds
Коллективы
: Russian Foundation for Basic Research [07-02-00069]; Council on Grants from the President of the Russian Federation for Support of Leading Scientific Schools [NSh-1011.2008.2]
Разночтения заглавия
:авие SCOPUS: Thermal expansion, polarization and phase diagrams of Ba 1-yBi2y/3Ti1-xZrxO3 and Ba1-yLayTi1-y/4O3 compounds
Место публикации
: J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2009. - Vol. 21, Is. 7. - Ст.75902. - С. P. - ISSN 0953-8984,
DOI
10.1088/0953-8984/21/7/075902
Примечания
: Cited References: 28. - This work was supported by the Russian Foundation for Basic Research ( project no. 07-02-00069) and the Council on Grants from the President of the Russian Federation for Support of Leading Scientific Schools ( project no. NSh-1011.2008.2).
Предметные рубрики:
HEAT-CAPACITY
CERAMICS
BA(TI1-XZRX)O-3
FERROELECTRICS
BEHAVIOR
BATIO3
BATI0.65ZR0.35O3
CONDUCTIVITY
PEROVSKITES
CHEMISTRY
Ключевые слова
(''Своб.индексиров.''): barium--dielectric properties--lanthanum--phase diagrams--polarization--thermal stress--zirconium--ceramic compositions--root mean squares--temperature ranges--temperature-dependent measurements--thermal expansion co-efficient--thermal-expansion properties--thermal expansion
Аннотация:
The thermal expansion properties of the ceramic compositions Ba1-yLayTi1-y/4O3 (y = 0.0, 0.026, 0.036, 0.054) and Ba1-yBi2y/3Ti1-xZrxO3 (y = 0.10; x = 0.0, 0.04, 0.05, 0.10, 0.15) were determined in the temperature range 120-700 K. We report the temperature- dependent measurements of the strain, thermal expansion coefficient and the magnitude of root mean square polarization. The results obtained are discussed together with the data on the structure and dielectric properties.
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10.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Oreshonkov A. S., Roginskii E. M., Krylov A. S., Ershov A. A., Voronov V. N.
Заглавие
: Structural, electronic and vibrational properties of LaF3 according to density functional theory and Raman spectroscopy
Коллективы
: RFBR [17-52-53031, 16-02-00102]; Ministry of Education and Science of the Russian Federation; Krasnoyarsky regional fund of scientific support and scientific-technical activity
Место публикации
: J. Phys.: Condens. Matter. - 2018. - Vol. 30, Is. 25. - Ст.255901. - ISSN 0953-8984,
DOI
10.1088/1361-648X/aac452. - ISSN 1361-648X(eISSN)
Примечания
: Cited References: 39. - The reported study was funded by RFBR according to the research project No. 17-52-53031 and 16-02-00102. It was partially supported by the Ministry of Education and Science of the Russian Federation and the 'Krasnoyarsky regional fund of scientific support and scientific-technical activity'. The computations were performed using facilities of the Computational Centre of the Research Park of St. Petersburg State University.
Предметные рубрики:
CRYSTAL-STRUCTURE
NEUTRON-DIFFRACTION
NANOPARTICLES
CONDUCTIVITY
Ключевые слова
(''Своб.индексиров.''): laf3--tysonite structure--dft--electronic structure--lattice vibrations--raman spectroscopy
Аннотация:
Crystal structure of LaF3 single crystal is refined in tysonite-type trigonal unit cell P c1 using density functional theory calculations and Raman spectroscopy. It is shown that trigonal structure with P c1 space group is more energy-efficient than hexagonal structure with space group P63 cm. Simulated Raman spectra obtained using LDA approximation is in much better agreement with experimental data than that obtained with PBE and PBEsol functionals of GGA. The calculated frequency value of silent mode B 2 in case of hexagonal structure P63 cm was found to be imaginary (unstable mode), thus the energy surface obtains negative curvature with respect to the corresponding normal coordinates of the mode which leads to instability of the hexagonal structure in harmonic approximation. The A 1g line at 214 cm−1 in Raman spectra of LaF3 related to the translation of F2 ions along c axis can be connected with F2 ionic
conductivity
.
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11.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Aplesnin S. S., Romanova O. B., Sitnikov M. N., Kretinin V. V., Galyas, A., I, Yanushkevich, K., I
Заглавие
: The alternating-sign magnetoresistance of polycrystalline manganese chalcogenide films
Коллективы
: Russian Foundation for Basic Research (RFBR) [18-52-00009 Bel_a, 18-32-00079 mol_a, 18-42-240001 r_a]; [3.5743.2017/6.7]
Место публикации
: Semicond. Sci. Technol. - 2018. - Vol. 33, Is. 8. - Ст.085006. - ISSN 0268-1242,
DOI
10.1088/1361-6641/aace44. - ISSN 1361-6641(eISSN)
Примечания
: Cited References: 33. - The reported study was funded by Russian Foundation for Basic Research (RFBR) according to the research project No 18-52-00009 Bel_a; No 18-32-00079 mol_a; No 18-42-240001 r_a; the state order No 3.5743.2017/6.7.
Предметные рубрики:
NEUTRON-SCATTERING
SURFACE-STATES
MNTE
CONDUCTIVITY
MECHANISM
Ключевые слова
(''Своб.индексиров.''): polycrystalline films--magnetoresistance--impedance--polaron--magnetic--properties--thermoelectric
Аннотация:
The correlation between the dc and ac electrical resistance and the structural, magnetic, and thermoelectric properties of polycrystalline MnSe1−X Te Х (0.3 ≤ X ≤ 0.4) manganese chalcogenide films in the temperature range of 80–400 K has been investigated. Inhomogeneous electronic states and transitions between them accompanied by structural lattice deformations have been found at temperatures including the Neel temperature region. The magnetic susceptibility maximum above the Neel temperature in a magnetic field of 8.6 kOe has been observed. Temperature ranges of the coexistence of two types of electrically inhomogeneous states have been established by impedance spectroscopy in the frequency range of 0.1–1000 kHz and the change of the hopping
conductivity
for diffusion one accompanied by the magnetic susceptibility minimum has been found. The magnetoresistance in magnetic fields of up to 12 kОе has been established. It has been revealed that the thermopower and magnetoresistance change its sign upon heating. The experimental data are explained using a spin polaron model with the localization of polarons and formation of the electron phase-separation. The alternation of magnetoresistance in sign is attributed to the ferromagnetic orbital ordering of electrons and the negative magnetoresistance is explained by suppression of spin fluctuations in a magnetic field.
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12.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Knyazev Yu. V., Shishkina N. N., Bayukov O. A., Kirik N. P., Solovyov L. A., Zhizhaev A. M., Rabchevsky E. V., Anshits A. G.
Заглавие
: Cation Distribution in the Composite Materials of the CaFe2O4-α-Fe2O3 Series
Коллективы
: Russian Foundation for Basic Research; Government of the Krasnoyarsk Krai; Krasnoyarsk Regional Science Foundation [18-42-243011]; UMNIK program
Место публикации
: J. Struct. Chem. - 2019. - Vol. 60, Is. 5. - P.763-771. - ISSN 0022-4766,
DOI
10.1134/S0022476619050081. - ISSN 1573-8779(eISSN)
Примечания
: Cited References: 25. - The study was performed with the financial support of the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Krai, the Krasnoyarsk Regional Science Foundation within the project No. 18-42-243011 "The effect of the composition and the defective structure of CaFe2O4 based "core-shell" composite materials on their electronic and catalytic properties" and the UMNIK program.
Предметные рубрики:
PD/P-TYPE CAFE2O4
OXYGEN
CONDUCTIVITY
Аннотация:
Structured composite materials CaFe2O4-α-Fe2O3 (α-Fe2O3 content is 2–82 wt.%) are obtained with the method of solid-phase synthesis at 1000 °C. The phase composition of the samples is studied using powder X-ray diffraction. It is shown that the content of CaFe2O4 and α-Fe2O3 phases changes linearly, depending on the composition of the starting material. The scanning electron microscopy data indicate the formation of a two-phase system α-Fe2O3-CaFe2O4. The Mössbauer spectroscopy data at room temperature testify the formation of cationic iron vacancies in the CaFe2O4 crystal structure in the absence of α-Fe2O3 structural defects. Cationic vacancies can be formed during the synthesis in the atmosphere of air.
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13.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Markevich I. A., Drokin N. A., Selyutin G. E.
Заглавие
: Impedance Spectroscopy Study of a Polymer Composite with Carbon Nanotubes in Contact with an Electrolyte
Место публикации
: Tech. Phys. - 2019. - Vol. 64, Is. 9. - P.1324-1329. - ISSN 1063-7842,
DOI
10.1134/S1063784219090093. - ISSN 1090-6525(eISSN)
Примечания
: Cited References: 14
Предметные рубрики:
BEHAVIOR
CONDUCTIVITY
RELAXATION
Аннотация:
The measured frequency dependence of the electric impedance of a composite based on ultra-high molecular weight polyethylene reinforced with carbon nanotubes in contact with an electrolyte is presented. The behavior of the active and reactive impedance components, permittivity, and
conductivity
in the frequency range from 0.1 Hz to 120 MHz is analyzed. An equivalent electric circuit simulating the dispersion of the impedance of the polymer composite making contact with the electrolyte is proposed. The formation of a double electric layer at the interface between the polymer composite and electrolyte layer is demonstrated and the electrical characteristics of this layer are determined.
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14.
Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Dudnikov V. A., Orlov Yu. S., Solovyov, Leonid A., Vereshchagin, Sergey N., Gavrilkin, Sergey Yu., Tsvetkov, Alexey Yu., Velikanov D. A., Gorev M. V., Novikov, Sergey V., Ovchinnikov S. G.
Заглавие
: Effect of multiplicity fluctuation in cobalt ions on crystal structure, magnetic and electrical properties of NdCoO3 and SmCoO3
Коллективы
: Russian Science FoundationRussian Science Foundation (RSF) [18-02-00022]
Место публикации
: Molecules. - 2020. - Vol. 25, Is. 6. - Ст.1301. - ISSN 1420-3049(eISSN),
DOI
10.3390/molecules25061301
Примечания
: Cited References: 56. - This work is supported by the Russian Science Foundation grant 18-02-00022.
Предметные рубрики:
SPIN-STATE TRANSITIONS
CO3+ ION
CONDUCTIVITY
TEMPERATURE
BEHAVIOR
Аннотация:
The structural, magnetic, electrical, and dilatation properties of the rare-earth NdCoO3 and SmCoO3 cobaltites were investigated. Their comparative analysis was carried out and the effect of multiplicity fluctuations on physical properties of the studied cobaltites was considered. Correlations between the spin state change of cobalt ions and the temperature dependence anomalies of the lattice parameters, magnetic susceptibility, volume thermal expansion coefficient, and electrical resistance have been revealed. A comparison of the results with well-studied GdCoO3 allows one to single out both the general tendencies inherent in all rare-earth cobaltites taking into account the lanthanide contraction and peculiar properties of the samples containing Nd and Sm.
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Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Dudnikov V. A., Fedorov A. S., Orlov Yu. S., Solovyov L. A., Vereshchagin S. N., Gavrilkin, S. Yu, Tsvetkov, A. Yu, Gorev M. V., Novikov, S., V, Ovchinnikov S. G.
Заглавие
: Thermoelectric properties of the SmCoO3 and NdCoO3 cobalt oxides
Коллективы
: Russian Science FoundationRussian Science Foundation (RSF) [16-13-00060]
Место публикации
: Ceram. Int. - 2020. - Vol. 46, Is. 11. - P.17987-17991. - ISSN 0272-8842,
DOI
10.1016/j.ceramint.2020.04.113. - ISSN 1873-3956(eISSN)
Примечания
: Cited References: 41. - This study was supported by the Russian Science Foundation, project no. 16-13-00060.
Предметные рубрики:
MAGNETIC-PROPERTIES
SPIN
CONDUCTIVITY
TRANSITIONS
LACOO3
SITE
Аннотация:
The thermoelectric properties of the NdCoO3 and SmCoO3 rare-earth cobalt oxides with a perovskite structure have been investigated in a wide temperature range. It is shown that, in the low-temperature region, the thermal
conductivity
of the compounds has a sharp maximum and the electrical
conductivity
of the samples increases with temperature, whereas the Seebeck coefficient behaves nonmonotonically with increasing temperature. The SmCoO3 oxide is characterized by the positive thermopower over the entire investigated range with a sharp growth in the low-temperature region, attaining the maximum value (S ≈ 1000 μV/K) near room temperature, and a further decrease. It has been established that, in the NdCoO3 oxide, the Seebeck coefficient changes its sign, which was rarely observed in the La-based compounds and is atypical of the undoped rare-earth cobalt oxides. The thermopower maximum obtained at a temperature of 450 K is 400 μV/K. The regions of the fastest growth of the thermoelectric power factor correspond to the anomalies caused by the spin transition of Со3+ ions and the dielectric–metal transition.
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Вид документа
: Статья из журнала
Шифр издания
:
Автор(ы)
: Orlov Yu. S., Vereshchagin S. N., Novikov, S., V, Burkov A. T., Borus A. A., Sitnikov, M., V, Solovyov L. A., Volochaev M. N., Dudnikov V. A.
Заглавие
: Effect of mechanical activation on the thermoelectric properties of Sr1-xSmxTiO3 ceramics
Коллективы
: Russian Science FoundationRussian Science Foundation (RSF) [19-72-00097]
Место публикации
: Ceram. Int. - 2021. - Vol. 47, Is. 20. - P.28992-28999. - ISSN 0272-8842,
DOI
10.1016/j.ceramint.2021.07.060. - ISSN 1873-3956(eISSN)
Примечания
: Cited References: 31. - This study was supported by the Russian Science Foundation, project no. 19-72-00097
Предметные рубрики:
SRTIO3
LA
MICROSTRUCTURE
CONDUCTIVITY
PERFORMANCE
FIGURE
MERIT
Аннотация:
The Sr1-xSmxTiO3 (х = 0.025, 0.05, 0.075, 0.1, 0.2) strontium titanate solid solutions were prepared from oxides and carbonates using a conventional ceramic technology based on the mechanochemical activation. The electrical
conductivity
and Seebeck coefficient of the synthesized compounds were measured in the temperature range from 300 to 800 K. We found that the properties of the samples significantly depend on the preliminary mechanochemical activation. The thermoelectric power factor attains maximum value in the hydrogen reduced samples with concentration of х = 0.05 and 0.075 obtained from nanoparticles: 5.5 μW/(cm · K2) for Sr0.95Sm0.05TiO3 (580 K) and 4.10 μW/(cm · K2) for Sr0.925Sm0.075TiO3 (650 K). An increase in the annealing temperature of mechanically activated samples leads to an even greater increase in electrical
conductivity
and power factor: 9.2 μW/(cm · K2) for Sr0.925Sm0.075TiO3 (650 K).
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