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Sadreev, A. F.
Phase transitions in a system of CH3(CH2)(n-1) self-assembled on the Au(111) crystal surface / A. F. Sadreev, Y. V. Sukhinin // Phys. Rev. B. - 1996. - Vol. 54, Is. 24. - P. 17966-17973, DOI 10.1103/PhysRevB.54.17966. - Cited References: 44 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
ORGANIZED MOLECULAR ASSEMBLIES
   ALKYL THIOL MONOLAYERS
   STRUCTURAL CHARACTERIZATION
   DYNAMICS SIMULATION
   DEVILS STAIRCASE
   GOLD SURFACES
   FILMS
   MODEL
   CHAIN
   DIFFRACTION
Аннотация: The n-alkanethiols CH3(CH2)(n-1) on the crystal surface of gold (111) are considered. Couplings between atoms (C, H) of the n-alkanethiols were modelled by the Morse potential, and couplings between the n-alkanethiols and the crystal surface were modelled by 12-3 potentials. Because of symmetry Z(2) of the n-alkanethiols in a tilted state, the system can be reduced to the Ising model on the triangular lattice, the phase diagram of which can be explicitly considered. Depending on the choice of the coupling parameters, the ordered state of the system may form an incommensurate or 2X1 superstructure. The temperatures of the phase transition, equilibrium tilting, twisting, and azimuthal angles are found to depend on the Morse coupling constants.

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Доп.точки доступа:
Sukhinin, Y. V.; Садреев, Алмаз Фаттахович
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Multilayer composite epitaxial CuCo single crystals / E. S. Mushailov [et al.] // JETP Letters. - 2000. - Vol. 71, Is. 5. - P. 195-197, DOI 10.1134/1.568313. - Cited References: 10 . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
SUPERLATTICES
DIFFRACTION
FILMS
Аннотация: The ion-plasma spraying method was used to synthesize new phases of metastable atomic-ordered layered CuCo single crystals and single crystals of CucCo1 - c solid solutions via epitaxial layer-by-layer crystallization, and some of their physical properties were studied. (C) 2000 MAIK "Nauka/Interperiodica".

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Держатели документа:
Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Krasnoyarsk State Univ, Krasnoyarsk 660049, Russia
Russian Acad Sci, Siberian Div, Inst Chem & Chem Technol, Krasnoyarsk, Russia
ИФ СО РАН
ИХХТ СО РАН

Доп.точки доступа:
Mushailov, E. S.; Kim, P. D.; Ким, Пётр Дементьевич; Turpanov, I. A.; Турпанов, Игорь Александрович; Bondarenko, G. V.; Бондаренко, Геннадий Васильевич; Bondarenko, G. N.; Бондаренко, Галина Николаевна; Mishina, S. E.
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Heat capacity of the PbFe1/2Ta1/2O3 perovskite-like compound / M. V. Gorev [et al.] // Phys. Solid State. - 2004. - Vol. 46, Is. 3. - P. 521-525, DOI 10.1134/1.1687872. - Cited References: 26 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
SINGLE-CRYSTALS
   PBFE0.5TA0.5O3
   FERROELECTRICS
   DIFFRACTION
   NIOBATE
   GROWTH
Аннотация: The heat capacity C-p(T) of the complex perovskite PbFe1/2Ta1/2O3 has been studied using adiabatic calorimetry in the temperature range 150-370 K. Three diffuse anomalies in C-p(T) are found to exist at temperatures T-d approximate to 350 K, T-m approximate to 250-300 K, and T-c approximate to 205 K. The anomalous and the lattice contribution to the heat capacity are separated, and the change in the entropy is determined. The results of the study are discussed jointly with the data on the structure and physical properties of the compound. (C) 2004 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
CNRS, CEMES, F-31055 Toulouse, France
INFM, I-090124 Cagliari, Italy
Dipartimento Fis, I-090124 Cagliari, Italy
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation
CEMES-CNRS, 29 Rue Jeanne Marvig, Toulouse, 31055, France
Inst. Naz. di Fisica della Materia, Dipartimento di Fisica, Monserrato (Cagliari), 090124, Italy

Доп.точки доступа:
Gorev, M. V.; Горев, Михаил Васильевич; Flerov, I. N.; Флёров, Игорь Николаевич; Bondarev, V. S.; Бондарев, Виталий Сергеевич; Sciau, P.; Lehmann, A. G.
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Heat capacity, structural disorder, and the phase transition in cryolite (NH4)(3)Ti(O-2)F-5 / I. N. Flerov [et al.] // Phys. Solid State. - 2006. - Vol. 48, Is. 8. - P. 1559-1567, DOI 10.1134/S1063783406080221. - Cited References: 18 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
PEROVSKITE-LIKE OXYFLUORIDES
   CRYSTAL-STRUCTURES
   (NH4)(3)TIOF5
   (NH4)(3)WO3F3
   DIFFRACTION
Аннотация: The heat capacity, T-p phase diagrams, and unit cell parameters of cryolite (NH4)(3)Ti(O-2)F-5 were studied over a wide temperature range. A phase transition was found near 226 K, and its thermodynamic characteristics and their dependence on the crystallization conditions were determined. The coordinates and thermal parameters of atoms in the Fm3m phase were refined. An analysis of the electron density distribution and the transition entropy showed that the mechanism of the structural transition involves, above all, rotation of the Ti(O-2)F-5 octahedra. Possible models of disordering of tetrahedral ammonium groups are considered.

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Держатели документа:
Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Russian Acad Sci, Inst Chem, Far E Div, Vladivostok 690022, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation
Institute of Chemistry, Far East Division, Russian Academy of Sciences, pr. Stoletiya Vladivostoka 159, Vladivostok, 690022, Russian Federation

Доп.точки доступа:
Flerov, I. N.; Флёров, Игорь Николаевич; Gorev, M. V.; Горев, Михаил Васильевич; Fokina, V. D.; Фокина, Валентина Дмитриевна; Molokeev, M. S.; Молокеев, Максим Сергеевич; Vasil'ev, A. D.; Васильев, Александр Дмитриевич; Bovina, A. F.; Бовина, Ася Федоровна; Laptash, N. M.
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Simultaneous antiferromagnetic Fe3+ and Nd3+ ordering in NdFe3((BO3)-B-11)(4) / P. . Fischer [et al.] // J. Phys.: Condens. Matter. - 2006. - Vol. 18, Is. 34. - P. 7975-7989, DOI 10.1088/0953-8984/18/34/010. - Cited References: 20 . - ISSN 0953-8984

РУБ Physics, Condensed Matter
Рубрики:
PHASE-TRANSITION
   DIFFRACTION
   CRYSTALS
   GDFE3(BO3)(4)
   SINQ
Кл.слова (ненормированные):
Iron compounds -- Magnetic moments -- Magnetization -- Neodymium compounds -- Neutron diffraction -- Vectors -- Crystal-field effects -- Free ion moment -- Specific heat measurements -- Symmetry analysis -- Antiferromagnetic materials
Аннотация: By means of magnetic susceptibility and specific heat measurements, x-ray and unpolarized neutron diffraction investigations on powder and single-crystal samples, simultaneous long-range antiferromagnetic Fe and Nd ordering in NdFe3((BO3)-B-11)(4) with R32 chemical structure has been found at temperatures below T-N = 30.5(5) K down to 1.6 K. At temperatures down to 19 K the propagation vector is k(hex) = [0, 0, 3/2] and becomes slightly incommensurate at lower temperatures. Combined with symmetry analysis, best powder neutron profile fits are obtained with magnetic spiral configurations with the magnetic moments oriented parallel to the hexagonal basal plane according to the irreducible representations tau(3) in the commensurate case. This is in agreement with the easy directions of magnetization perpendicular to the c-axis as determined by magnetic susceptibility measurements. At 1.6 K the magnetic Fe moment amounts to 4.9 mu(B) B close to the free ion moment of Fe3+. The magnetic Nd3+ moment saturates presumably due to crystal-field effects at 2.7 mu(B).

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Держатели документа:
ETH, Neutron Scattering Lab, CH-5232 Villigen, Switzerland
Paul Scherrer Inst, CH-5232 Villigen, Switzerland
Tech Univ Munich, Dept Phys, D-85748 Garching, Germany
RAS, SB, Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
Laboratory for Neutron Scattering, ETH Zurich, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
Physik Department E21, TU Munchen, D-85748 Garching, Germany
Institute of Physics SB RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Fischer, P.; Pomjakushin, V.; Sheptyakov, D.; Keller, L.; Janoschek, M.; Roessli, B.; Schefer, J.; Petrakovskii, G. A.; Петраковский, Герман Антонович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Temerov, V. L.; Темеров, Владислав Леонидович; Velikanov, D. A.; Великанов, Дмитрий Анатольевич
}
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Mechanism and nature of phase transitions in the (NH4)(3)MoO3F3 oxyfluoride / I. N. Flerov [et al.] // Phys. Solid State. - 2008. - Vol. 50, Is. 3. - P. 515-524, DOI 10.1134/S1063783408030219. - Cited References: 13 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
(NH4)(2)WO2F4
DIFFRACTION
CS
Аннотация: The temperature dependences of the heat capacity, the unit cell parameter, and the permittivity for the (NH4)(3)MoO3F3 cryolite (space group Fm (3) over barm) are investigated. It is revealed that the compound undergoes ferroelectric and ferroelastic structural phase transitions at temperatures of 297 and 205 K, respectively. The mechanism of structural distortions is discussed in terms of the entropy parameters, pressure-temperature phase diagrams, and electron density maps for critical atoms. An analysis is made of the influence of the cation size and shape on the phase transitions in oxyfluorides of the general formula A(2)A'MO3F3 (A,A' = NH4, K; M = Mo, W).

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Держатели документа:
[Flerov, I. N.
Fokina, V. D.
Bovina, A. F.
Bogdanov, E. V.
Molokeev, M. S.
Kocharova, A. G.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
[Pogorel'tsev, E. I.] Siberian Fed Univ, Polytech Inst, Krasnoyarsk 660074, Russia
[Laptash, N. M.] Russian Acad Sci, Inst Chem, Far E Div, Vladivostok 690022, Russia
ИФ СО РАН

Доп.точки доступа:
Flerov, I. N.; Флёров, Игорь Николаевич; Fokina, V. D.; Фокина, Валентина Дмитриевна; Bovina, A. F.; Бовина, Ася Федоровна; Bogdanov, E. V.; Богданов, Евгений Витальевич; Molokeev, M. S.; Молокеев, Максим Сергеевич; Kocharova, A. G.; Кочарова, Алла Георгиевна; Pogorel'tsev, E. I.; Laptash, N. M.
}
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    Phase transitions and thermodynamic properties of (NH4)(3)VO2F4 cryolite / V. D. Fokina [et al.] // Solid State Sci. - 2009. - Vol. 11, Is. 4. - P. 836-840, DOI 10.1016/j.solidstatesciences.2008.11.004. - Cited Reference Count: 17. - Гранты: The authors are grateful to Dr. SM. Mel'nikova for the permission to use the unpublished results.; This work was supported by the Russian Foundation for Basic Research (project 06-02-16102). - Финансирующая организация: Russian Foundation for Basic Research [06-02-16102] . - ISSN 1293-2558
Рубрики:
PEROVSKITE-LIKE OXYFLUORIDES
   (NH4)(3)TIOF5
   CS
   (NH4)(3)WO3F3
   DIFFRACTION
   (NH4)3VO2F4
   ELPASOLITE
   METALS
   RB
Кл.слова (ненормированные):
Oxyfluorides -- Phase transition -- Calorimetry -- Phase diagram -- Ferroelectricity -- Calorimetry -- Ferroelectricity -- Oxyfluorides -- Phase diagram -- Phase transition -- Calorimetry -- Ferroelectricity -- Halide minerals -- Phase diagrams -- Sugar (sucrose) -- Thermodynamic properties -- Calorimetric measurements -- Cubic phase -- First-order phase transitions -- Heat capacities -- Oxyfluorides -- Phase transition temperatures -- Pressure dependences -- Structural transformations -- Temperature ranges -- Phase transitions
Аннотация: Calorimetric measurements performed in a wide temperature range on (NH4)(3)VO2F4 have shown the presence of four heat capacity anomalies at T-1 = 438 K, T-2 = 244 K, T-3 = 210.2 K, T-4 = 205.1 K associated with the first order phase transitions. In accordance with the permittivity behavior, the structural transformations are of nonferroelectric nature. Pressure dependence of the phase transition temperatures has been studied by DTA under pressure. The entropy of phase transitions is analyzed mainly in the framework of the orientational disordering of NH4+ and VO2F43- ions in a cubic phase. (C) 2008 Elsevier Masson SAS. All rights reserved.

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Держатели документа:
RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660074, Russia

Доп.точки доступа:
Fokina, V. D.; Фокина, Валентина Дмитриевна; Gorev, M. V.; Горев, Михаил Васильевич; Kocharova, A. G.; Кочарова, Алла Георгиевна; Flerov, I. N.; Флёров, Игорь Николаевич; Pogoreltsev, E.I.
}
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Calorimetric and dielectric studies of the (NH4)(2)MoO2F4 oxyfluoride / V. D. Fokina [et al.] // Phys. Solid State. - 2010. - Vol. 52, Is. 1. - P. 158-166, DOI 10.1134/S1063783410010282. - Cited References: 22. - This study was supported by the Russian Foundation for Basic Research ( project no. 09-02-00062). . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
PHASE-TRANSITIONS
   (NH4)(2)WO2F4
   DIFFRACTION
   MECHANISM
   CRYSTALS
Аннотация: The temperature dependences of the heat capacity, dielectric properties, and response to an external pressure and an electric field for the (NH4)(2)MoO2F4 oxyfluoride (space group Cmcm, Z = 4) have been studied. A comparative analysis of the data on the entropy of phase transitions, p-T phase diagrams, permittivity, and anomalous heat capacity in combination with the results of previous studies of the related compounds (NH4)(2)WO2F4 and (ND4)(2)WO2F4 has made it possible to establish that both [MO2F4](2-) anions and ammonium groups play a substantial role in the mechanism and nature of the structural transformations.

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Держатели документа:
[Fokina, V. D.
Bogdanov, E. V.
Bondarev, V. S.
Flerov, I. N.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[Fokina, V. D.
Pogorel'tsev, E. I.
Bondarev, V. S.
Flerov, I. N.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
[Laptash, N. M.] Russian Acad Sci, Far Eastern Branch, Inst Chem, Vladivostok 690022, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50, Krasnoyarsk 660036, Russian Federation
Siberian Federal University, pr. Svobody 79, Krasnoyarsk 660041, Russian Federation
Institute of Chemistry, Far Eastern Branch, Russian Academy of Sciences, pr. Stoletiya Vladivostoka 159, Vladivostok 690022, Russian Federation

Доп.точки доступа:
Fokina, V. D.; Фокина, Валентина Дмитриевна; Bogdanov, E. V.; Богданов, Евгений Витальевич; Pogorel'tsev, E. I.; Bondarev, V. S.; Бондарев, Виталий Сергеевич; Flerov, I. N.; Флёров, Игорь Николаевич; Laptash, N. M.
}
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Nonresonant x-ray magnetic scattering on rare-earth iron borates RFe3(BO3)(4) / J. E. Hamann-Borrero [et al.] // Phys. Rev. B. - 2010. - Vol. 82, Is. 9. - Ст. 94411, DOI 10.1103/PhysRevB.82.094411. - Cited References: 38. - This work was supported by the Deustche Forschungsgemeinschaft, through the Forschergruppe FOR520 (Grant No. HE3439/6) and HASYLAB at the Feyerherm from HMI Berlin and specially to Jorg Strempfer from HASYLAB at DESY in Hamburg for valuable discussions. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
SINGLE-CRYSTALS
   CROSS-SECTION
   GDFE3(BO3)(4)
   NDFE3(BO3)(4)
   DIFFRACTION
   MNF2
Аннотация: Hard x-ray scattering experiments with a photon energy of 100 keV were performed as a function of temperature and applied magnetic field on selected compounds of the RFe3(BO3)4 family. The results show the presence of several diffraction features, in particular, nonresonant magnetic reflections in the magnetically ordered phase and structural reflections that violate the diffraction conditions for the low-temperature phase P3(1)21 of the rare-earth iron borates. The temperature and field dependence of the magnetic superlattice reflections corroborate the magnetic structures of the borate compounds obtained by neutron diffraction. The detailed analysis of the intensity and scattering cross section of the magnetic reflection reveals details of the magnetic structure of these materials such as the spin domain structure of NdFe3(BO3)(4) and GdFe3(BO3)(4). Furthermore we find that the correlation length of the magnetic domains is around 100 angstrom for all the compounds and that the Fe moments are rotated 53 degrees +/- 3 degrees off from the hexagonal basal plane in GdFe3(BO3)(4).

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Держатели документа:
[Hamann-Borrero, J. E.
Philipp, M.
Kataeva, O.
Geck, J.
Klingeler, R.
Buechner, B.
Hess, C.] IFW Dresden, Leibniz Inst Solid State & Mat Res, D-01171 Dresden, Germany
[Kataeva, O.] Russian Acad Sci, AE Arbuzov Organ & Phys Chem Inst, Kazan 420088, Russia
[Zimmermann, M. V.] Deutsch Elektronen Synchrotron DESY, Hamburger Synchrotronstrahlungslabor HASYLAB, D-22603 Hamburg, Germany
[Klingeler, R.] Univ Heidelberg, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany
[Vasiliev, A.] Moscow MV Lomonosov State Univ, Fac Phys, Low Temp Phys Dept, Moscow 119992, Russia
[Bezmaternykh, L.] Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Leibniz Institute for Solid State and Materials Research, IFW Dresden, 01171 Dresden, Germany
A. E. Arbuzov Institute of Organic and Physical Chemistry, Russian Academy of Sciences, Arbuzov Str. 8, Kazan 420088, Russian Federation
Hamburger Synchrotronstrahlungslabor (HASYLAB), Deutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22603 Hamburg, Germany
Kirchhoff Institute for Physics, University of Heidelberg, Im Neuenheimer Feld 227, D-69120 Heidelberg, Germany
Low Temperature Physics Department, Faculty of Physics, Moscow State University, Moscow 119992, Russian Federation
L. V. Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Krasnoyarsk 660,0,36, Russian Federation

Доп.точки доступа:
Hamann-Borrero, J. E.; Philipp, M.; Kataeva, O.; Zimmermann, M. V.; Geck, J.; Klingeler, R.; Vasiliev, A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Buchner, B.; Hess, C.
}
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10.

Structural and electronic parameters of ferroelectric K3WO3F3 / V. V. Atuchin [et al.] // Solid State Commun. - 2010. - Vol. 150, Is. 43-44. - P. 2085-2088, DOI 10.1016/j.ssc.2010.09.023. - Cited References: 34. - This study was partly supported by RFBR (Grant 09-02-00062) and SB RAS (Grant 34). . - ISSN 0038-1098

РУБ Physics, Condensed Matter
Рубрики:
CORE-LEVEL SPECTROSCOPY
   PHASE-TRANSITIONS
   RHEED ANALYSIS
   SURFACE
   OXYFLUORIDE
   ELPASOLITE
   (NH4)(2)KWO3F3
   SUBSTITUTION
   TEMPERATURE
   DIFFRACTION
Кл.слова (ненормированные):
Ferroelectrics -- Chemical synthesis -- Electronic structure -- Photoelectron spectroscopies
Аннотация: The low-temperature ferroelectric G2 polymorph of K3WO3F3 oxyfluoride is formed by chemical synthesis. The electronic parameters of G2-K3WO3F3 have been measured by X-ray photoelectron spectroscopy under excitation with Al K alpha radiation (1486.6 eV). Detailed spectra have been recorded for all element core levels and Auger lines. The chemical bonding effects in the WO3 F-3 and WO6 octahedrons are considered by using the binding energy difference Delta BE(O-W) = BE(O 1s) BE(W 4f(7/2)). (C) 2010 Elsevier Ltd. All rights reserved.

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Держатели документа:
[Atuchin, V. V.] SB RAS, Inst Semicond Phys, Lab Opt Mat & Struct, Novosibirsk 630090, Russia
[Gavrilova, T. A.] SB RAS, Inst Semicond Phys, Lab Nanolithog & Nanodiagnost, Novosibirsk 630090, Russia
[Kesler, V. G.] SB RAS, Inst Semicond Phys, Lab Phys Principles Integrated Microelect, Novosibirsk 630090, Russia
[Molokeev, M. S.
Aleksandrov, K. S.] SB RAS, Inst Phys, Lab Crystal Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН

Доп.точки доступа:
Atuchin, V. V.; Gavrilova, T. A.; Kesler, V. G.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Aleksandrov, K. S.; Александров, Кирилл Сергеевич
}
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