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Synthesis, crystal structure, and thermal properties of substituted titanates Bi2Pr2Ti3O12 and Bi2Nd2Ti3O12 / L. T. Denisova, M. S. Molokeev, N. A. Galiakhmetova [et al.] // Phys. Solid State. - 2021. - Vol. 63. Is. 8. - P. 1159-1164, DOI 10.1134/S1063783421080084. - Cited References: 39. - This study was carried out in part within the state assignment for the Siberian Federal University, project no. FSRZ-2020-0013 . - ISSN 1063-7834. - ISSN 1090-6460

РУБ Physics, Condensed Matter
Рубрики:
BI4-XRXTI3O12 R-X
   PHASE-EQUILIBRIA
   HEAT-CAPACITY
   ND
   BI4TI3O12
   PR
Кл.слова (ненормированные):
substituted bismuth titanate -- solid-state synthesis -- crystal structure -- high-temperature heat capacity -- thermodynamic functions
Аннотация: Titanates Bi2Pr2Ti3O12 and Bi2Nd2Ti3O12 have been obtained by the solid-phase synthesis using sequential annealing of the Bi2O3, Nd2O3, Pr6O11, and TiO2 stoichiometric mixtures in air at temperatures of 1003–1323 K. Their crystal structure has been established by X-ray diffractometry and the high-temperature heat capacity has been determined by differential scanning calorimetry. Based on the experimental Cp = f(T) data, the main thermodynamic functions have been calculated.

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Публикация на русском языке Синтез, кристаллическая структура и теплофизические свойства замещенных титанатов Bi2Pr2Ti3O12 и Bi2Nd2Ti3O12 [Текст] / Л. Т. Денисова, М. С. Молокеев, Н. А. Галиахметова [и др.] // Физ. тверд. тела. - 2021. - Т. 63 Вып. 8. - С. 1056-1061

Держатели документа:
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Denisova, L. T.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Galiakhmetova, N. A.; Denisov, V. M.; Vasil'ev, G. V.; [FSRZ-2020-0013]
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Synthesis, crystal structure, and physicochemical properties of Bi4-xPrxTi3O12 (x=0.4, 0.8, 1.2, 1.6) solid solutions / L. T. Denisova, M. S. Molokeev, Y. F. Kargin [et al.] // Inorg. Mater. - 2021. - Vol. 57, Is. 9. - P. 919-928, DOI 10.1134/S002016852109003X. - Cited References: 40 . - ISSN 0020-1685. - ISSN 1608-3172

РУБ Materials Science, Multidisciplinary
Рубрики:
BI4-XRXTI3O12 R-X
   HEAT-CAPACITY
   AURIVILLIUS PHASES
   PR
   ND
   BI4TI3O12
Кл.слова (ненормированные):
bismuth titanates -- solid-state synthesis -- crystal structure -- luminescence -- high-temperature heat capacity -- phase transition
Аннотация: Bi4–xPrxTi3O12 (x = 0.4, 0.8, 1.2, 1.6) solid solutions have been prepared by solid-state reactions, via multistep firing of stoichiometric mixtures of their constituent oxides in air at temperatures from 1003 to 1323 K. Their crystal structure has been determined using X-ray diffraction, and their luminescence spectra have been measured at room temperature. High-temperature heat capacity of polycrystalline substituted bismuth titanate samples has been determined by differential scanning calorimetry. The Cp(T) curves of the solid solutions with x = 0.4 and 0.8 have extrema related to phase transitions. Experimental data have been used to calculate the main thermodynamic functions of the solid solutions.

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Публикация на русском языке Синтез, кристаллическая структура и физико-химические свойства твердых растворов Bi4-xPrxTi3O12 (x = 0.4, 0.8, 1.2, 1.6) [Текст] / Л. Т. Денисова, М. С. Молокеев, Ю. Ф. Каргин [и др.] // Неорган. матер. - 2021. - Т. 57 № 9. - С. 968-977

Держатели документа:
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Fed Res Ctr, Siberian Branch, Kirensky Inst Phys,Krasnoyarsk Sci Ctr, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Baikov Inst Met & Mat Sci, Moscow 119991, Russia.

Доп.точки доступа:
Denisova, L. T.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Kargin, Yu F.; Gerasimov, V. P.; Герасимов, Виктор Петрович; Krylov, A. S.; Крылов, Александр Сергеевич; Aleksandrovskii, A. S.; Александровский, Александр Сергеевич; Chumilina, L. G.; Denisov, V. M.; Vasil'ev, G. V.; Васильев Г. В.
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Raman scattering from phonons and magnons in RFe3(BO3)(4) / D. . Fausti [et al.] // Phys. Rev. B. - 2006. - Vol. 74, Is. 2. - Ст. 24403, DOI 10.1103/PhysRevB.74.024403. - Cited References: 26 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
IRON BORATE GDFE3(BO3)(4)
   LIGHT-SCATTERING
   CRYSTALS
   ND
   CRYSTALLIZATION
   TRANSITIONS
   GENERATION
   LASER
Аннотация: Inelastic light scattering spectra of several members of the RFe3(BO3)(4) family reveal a cascade of phase transitions as a function of temperature, starting with a structural, weakly first-order, phase transition followed by two magnetic phase transitions. Those consist of the ordering of the Fe-spin sublattice, revealed by all the compounds, and a subsequent spin-reorientational transition for GdFe3(BO3)(4). The Raman data evidence a strong coupling between the lattice and magnetic degrees of freedom in these borates. The Fe-sublattice ordering leads to a strong suppression of the low-energy magnetic scattering, and a multiple peaked two-magnon scattering continuum is observed. Evidence for short-range correlations is found in the "paramagnetic" phase by the observation of a broad magnetic continuum in the Raman data, which persists up to surprisingly high temperatures.

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Держатели документа:
Univ Groningen, Ctr Mat Sci, NL-9747 AG Groningen, Netherlands
RAS, Inst Spect, Troitsk 142190, Moscow Region, Russia
RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Material Science Centre, University of Groningen, 9747 AG Groningen, Netherlands
Institute of Spectroscopy, RAS, 142190, Troitsk, Moscow Region, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch of RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Fausti, D.; Nugroho, A. A.; van Loosdrecht, PHM; Klimin, S. A.; Popova, M. N.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич
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Peschanskii, A. V.
Spectroscopic study of the TbAl3(BO3)4 single crystal: Raman and luminescence spectroscopy / A. V. Peschanskii, A. Y. Glamazda, I. A. Gudim // Физ. низких температур. - 2020. - Т. 46, Вып. 12. - С. 1437-1445. - Cited References: 20 . - ISSN 0132-6414. - ISSN 1816-0328

РУБ Physics, Applied
Рубрики:
SCATTERING
GENERATION
ND
Кл.слова (ненормированные):
TbAl3(BO3)4 -- vibrational spectrum -- electronic transitions -- Raman spectroscopy -- luminescence
Аннотация: The vibrational and luminescence properties of the TbAl3(BO3)4 single crystal were studied in the temperature range of 5–300 K. Raman spectra of the single crystal revealed 5 of 7 A1 and all E phonon modes predicted by the group-theory analysis. The splitting energy between the LO and TO components of polar E phonons is determined. A group of intense bands associated with the 5D4 → 7F0 electronic transition was observed in the energy range of 14520–14680 cm−1 of the luminescence spectra. The intensity of these bands decreases upon heating. At the same time, the bands which can be assigned with 5D4 → 7F6, 5D4 → 7F5, and 5D4 → 7F4 transitions were revealed in luminescence spectra at room temperature. The intensity of these bands is comparable to the intensity of the Raman spectrum of TbAl3(BO3)4. The observation of luminescence from the 5D4 multiplet (20600–20750 cm−1) upon excitation at λexc = 632.8 nm (15803 cm−1) and λexc = 532 nm (18797 cm−1) indicates strong nonlinear properties of the studied crystal. The structure of the main 7F6 multiplet of Tb+3 in the TbAl3(BO3)4 single crystal has been studied at 5 K by Raman spectroscopy. The energies of the electronic levels of 7F6 and 5D4 multiplets were determined from the luminescence spectra measured at 300 K.

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Переводная версия Peschanskii A. V. Spectroscopic study of the TbAl3(BO3)4 single crystal: Raman and luminescence spectroscopy [Текст] / A. V. Peschanskii, A. Y. Glamazda, I. A. Gudim // Low Temp. Phys. - 2020. - Vol. 46 Is. 12.- P.1223-1230

Держатели документа:
Natl Acad Sci Ukraine, B Verkin Inst Low Temp Phys & Engn, UA-61103 Kharkov, Ukraine.
RAS, Siberian Branch, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Glamazda, A. Yu.; Gudim, I. A.; Гудим, Ирина Анатольевна
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Peschanskii, A. V.
Spectroscopic study of the TbAl3(BO3)4 single crystal: Raman and luminescence spectroscopy / A. V. Peschanskii, A. Y. Glamazda, I. A. Gudim // Low Temp. Phys. - 2020. - Vol. 46, Is. 12. - P. 1223-1230, DOI 10.1063/10.0002478. - Cited References: 20 . - ISSN 1063-777X. - ISSN 1090-6517

Публикация в журнале "Физика низких температур" Peschanskii A. V. Spectroscopic study of the TbAl3(BO3)4 single crystal: Raman and luminescence spectroscopy [Текст] / A. V. Peschanskii, A. Y. Glamazda, I. A. Gudim // Физ. низких температур. - 2020. - Т. 46 Вып. 12.- С.1437-1445

Optical spectroscopy of PrFe3(BO3)(4): Crystal-field and anisotropic Pr-Fe exchange interactions / M. N. Popova [et al.] // Phys. Rev. B. - 2009. - Vol. 80, Is. 19. - Ст. 195101, DOI 10.1103/PhysRevB.80.195101. - Cited References: 36. - We thank S. Klimin for useful information concerning the structure of PrFeINF3/INF(BOINF3/INF)INF4/INF and E. Chukalina for participating in some measurements. This work was supported in part by the Russian Foundation for Basic Research (Grants No. 07-02-01185 and No. 09-02-00930) and by the Russian Academy of Sciences under the Programs for Basic Research. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
TRIGONAL GDFE3(BO3)(4)
   NDFE3(BO3)(4)
   DYFE3(BO3)(4)
   TRANSITIONS
   BORATE
   ION
   ND
Кл.слова (ненормированные):
antiferromagnetic materials -- crystal field interactions -- exchange interactions (electron) -- infrared spectra -- iron compounds -- magnetic susceptibility -- magneto-optical effects -- paramagnetic materials -- praseodymium compounds -- spin Hamiltonians -- visible spectra
Аннотация: High-resolution polarized optical absorption spectra of PrFe3(BO3)(4) in the paramagnetic and antiferromagnetic phases are reported. The measured energies of the crystal-field (CF) levels within the 4f(2) configuration of Pr3+ in the paramagnetic PrFe3(BO3)(4) are described by the CF model that involves the 4f(2)/4f5d and 4f(2)/4f6p configuration interactions. Ordering of Fe spins along the crystalline c axis below T-N=32 K is confirmed by the analysis of the spectra of Er3+ introduced as a probe into PrFe3(BO3)(4). To account for the observed changes in the optical spectra of Pr3+ at temperatures below T-N, in particular, for the shift of the CF levels, splitting of the CF doublets, and the appearance of forbidden lines, the Pr-Fe exchange Hamiltonian defined by seven parameters is considered. The theoretical approach has been tested by calculating the temperature dependence of the magnetic susceptibility. A good agreement between theory and optical and magnetic experimental data is found demonstrating the validity of the model used. The obtained results confirm that the model of the iron dimers inside the spiral chains of Fe3+(O2-)(6) octahedrons introduced by us earlier for NdFe3(BO3)(4) and modified in the present work may serve as a basis for analyzing the low-temperature properties of other rare-earth iron borates.

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Держатели документа:
[Popova, M. N.
Stanislavchuk, T. N.] Russian Acad Sci, Inst Spect, Troitsk 142190, Moscow Region, Russia
[Malkin, B. Z.] Kazan VI Lenin State Univ, Kazan 420008, Russia
[Bezmaternykh, L. N.] RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, 142190 Moscow Region, Russian Federation
Kazan State University, 420008 Kazan, Russian Federation
L.V. Kirensky Institute of Physics, Siberian Branch, RAS, 660036 Krasnoyarsk, Russian Federation

Доп.точки доступа:
Popova, M. N.; Stanislavchuk, T. N.; Malkin, B. Z.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Russian Foundation for Basic Research [07-02-01185, 09-02-00930]; Russian Academy of Sciences under the Programs for Basic Research
}
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Magnetoelastic effects in terbium ferroborate / G. A. Zvyagina [et al.] // Low Temp. Phys. - 2008. - Vol. 34, Is. 11. - P. 901-908 ; Физика низких температур, DOI 10.1063/1.3009584. - Cited References: 17 . - ISSN 1063-777X

РУБ Physics, Applied
Рубрики:
CRYSTAL-STRUCTURE
ND
Кл.слова (ненормированные):
acoustic wave velocity -- antiferromagnetic materials -- elastic moduli -- exchange interactions (electron) -- iron compounds -- magnetoelastic effects -- solid-state phase transformations -- terbium compounds
Аннотация: The behavior of the elastic moduli and sound absorption in a terbium orthoborate single crystal at low temperatures is studied. The components of the tensor of the elastic moduli of this system are determined. A structural phase transition and a transition of the magnetic subsystem into an antiferromagnetically ordered state appear in the temperature dependences of the sound velocities and absorption. The magnetic field dependences of the velocities of transverse sound exhibit singularities in the form of jumps at a magnetic field equal to the field of the spin-flop transition of the antiferromagnetic subsystem. Theoretical analysis shows that the observed behavior of the acoustic characteristics are associated not with the rare-earth subsystem of ferroborate but rather with the renormalization of the exchange interaction between iron ions as a result of the magnetoelastic coupling.

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Держатели документа:
[Zvyagina, G. A.
Zhekov, K. R.
Bilych, I. V.
Zvyagin, A. A.] Natl Acad Sci Ukraine, BI Verkin Inst Low Temp Phys & Engn, UA-61103 Kharkov, Ukraine
[Bezmaternykh, L. N.
Gudim, I. A.] Russian Acad Sci, LV Kirenskii Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
B. I. Verkin Institute for Low-Temperature Physics and Engineering, National Academy of Sciences of Ukraine, pr. Lenina 47, Kharkov 61103, Ukraine
L. V. Kirenskii Institute of Physics, Siberian Branch, Russian Adcademy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zvyagina, G. A.; Zhekov, K. R.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Bilych, I. V.; Zvyagin, A. A.

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    Magnetic and transport properties of Gd(0.9)A(0.1)CoO(3-delta) (A = Ba, Sr) / N. V. Kazak [et al.] // J. Magn. Magn. Mater. - 2009. - Vol. 321, Is. 9. - P. 1266-1271, DOI 10.1016/j.jmmm.2008.11.087. - Cited Reference Count: 31. - Гранты: This study was supported by the Rosnauka (Project no. MK-4278.2008.2), Russian Foundation for Basic Research (Project no. 08-02-90708 mob_st) and "Strongly correlated electrons'' program of the Department of Physical Sciences of RAS. - Финансирующая организация: Rosnauka [MK-4278.2008.2]; Russian Foundation for Basic Research [08-02-90708 mob_st]; "Strongly correlated electrons'' program of the Department of Physical Sciences of RAS . - ISSN 0304-8853
Рубрики:
PEROVSKITE
   PR
   LA
   EU
   ND
   LN
   TRANSITION
   SPIN
   GD
   SM
Кл.слова (ненормированные):
Perovskite structure -- Doped cobaltite -- Magnetic susceptibility -- Metal-insulator transition -- Doped cobaltite -- Magnetic susceptibility -- Metal-insulator transition -- Perovskite structure -- Antiferromagnetism -- Barium -- Cobalt compounds -- Electric conductivity -- Ferromagnetic materials -- Ferromagnetism -- Gadolinium -- Magnetic susceptibility -- Metal insulator boundaries -- Oxide minerals -- Paramagnetic materials -- Perovskite -- Phase separation -- Semiconductor insulator boundaries -- Transport properties -- Antiferromagnetic -- Doped cobaltite -- Doped samples -- Electrical conductivity measurements -- Ferromagnetic transitions -- Insulator-metal transitions -- Magnetic and transport properties -- Magnetic behaviors -- Perovskite structure -- Temperature ranges -- Transport datum -- X- ray diffractions -- Metal insulator transition
Аннотация: The X-ray diffraction, magnetization and electrical conductivity measurements for Gd(0.9)A(0.1)CoO(3-delta) (A = Ba, Sr) have been made. The complicated magnetic behavior, including the paramagnetic-ferromagnetic-antiferromagnetic and paramagnetic-ferromagnetic transitions, was found for Ba- and Sr-doped samples. The gradual insulator-metal transitions were observed in a wide temperature range T = 600-800 K. The complex magnetic and transport data could be explained on the basis of the structural phase separation. (C) 2009 Elsevier B.V. All rights reserved.

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Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Polytech Inst, Krasnoyarsk 660074, Russia
Univ Guadalajara, CUCEI, Dept Fis, Guadalajara 44430, Jalisco, Mexico
Siberian Fed Univ, Inst Nat & Humanitary Res, Krasnoyarsk 660041, Russia
AA Galkin Donetsk Phystech Natl Acad Sci Ukraine, UA-83114 Donetsk, Ukraine

Доп.точки доступа:
Kazak, N. V.; Казак, Наталья Валерьевна; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Balaev, A. D.; Балаев, Александр Дмитриевич; Ivanova, N.B.; Pashkevich, Yu. G.; Michel, C.R.; Bondarenko, G. V.; Бондаренко, Геннадий Васильевич
}
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Low-temperature magnetic behavior of the rare-earth cobaltites GdCoO3 and SmCoO3 / N. B. Ivanova [et al.] // Phys. Solid State. - 2007. - Vol. 49, Is. 11. - P. 2126-2131, DOI 10.1134/S1063783407110182. - Cited References: 32. - This study was supported by the Branch of General Physics and Astronomy of the Russian Academy of Sciences within the framework of the program “Strong Electron Correlations” and the Russian Science Support Foundation . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
METAL-INSULATOR-TRANSITION
   RCOO3 R
   SPIN-STATE
   OXIDE
   SM
   ND
   PEROVSKITE
   GLASSES
   PR
   EU
Аннотация: The temperature and magnetic field dependences of the static magnetization of the polycrystalline rare-earth cobaltites GdCoO3 and SmCoO3 have been measured. It is shown that, below room temperature, the magnetization of both compounds derives primarily from the rare-earth ion paramagnetism. The GdCoO3 and SmCoO3 compounds have been found to differ substantially in magnetic behavior, which can be traced to differences in their electronic shell structures. The magnetic behavior of GdCoO3 is close to that of an array of free Gd3+ ions, whereas in SmCoO3 the deviation from the free-ion properties is very large because of the Sm3+ ground state being crystal-field split. Van Vleck magnetic susceptibility measurements of SmCoO3 suggest that the splitting is similar to 10 K.

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Публикация на русском языке Сравнение одноэлектронного и многоэлектронного механизмов концентрационной зависимости зонной структуры ВТСП-купратов [Текст] / В. А. Гавричков [и др.] // Физ. тверд. тела. - 2007. - Т. 49 Вып. 11. - С. 1958-1963

Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
Univ Guadalajara, Dept Fis, CUCEI, Guadalajara 44430, Jalisco, Mexico
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation
Departamento de Fisica, C.U.C.E.I., Universidad de Guadalajara, Guadalajara, Jalisco 44430, Mexico

Доп.точки доступа:
Ivanova, N. B.; Иванова, Наталья Борисовна; Kazak, N. V.; Казак, Наталья Валерьевна; Michel, C. R.; Balaev, A. D.; Балаев, Александр Дмитриевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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10.

Low-temperature behavior of the magnetoelastic characteristics of praseodymium ferroborate / G. A. Zvyagina [et al.] // Low Temp. Phys. - 2010. - Vol. 36, Is. 4. - P. 296-302 ; Физика низких температур, DOI 10.1063/1.3420962. - Cited References: 16 . - ISSN 1063-777X

РУБ Physics, Applied
Рубрики:
CRYSTAL
STATE
ND
Аннотация: The behavior of the elastic moduli and sound absorption in a PrFe(3)(BO(3))(4) single crystal at low temperatures is studied. A transition of the magnetic subsystem into an antiferromagnetically ordered state is manifested in the temperature behavior of the sound velocities and absorption. The characteristic behavior of the elastic properties of PrFe(3)(BO(3))(4) in an external magnetic field is observed. A phenomenological theory that gives a qualitative description of the observed features is constructed. It is proposed that a weak magnetic moment exists in the crystal. (C) 2010 American Institute of Physics. [doi: 10.1063/1.3420962]

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Держатели документа:
[Zvyagina, G. A.
Zhekov, K. R.
Bilych, I. V.
Zvyagin, A. A.] Natl Acad Sci Ukraine, BI Verkin Inst Low Temp Phys & Engn, UA-61103 Kharkov, Ukraine
[Zvyagin, A. A.] Tech Univ Dresden, Inst Solid State Phys, D-01069 Dresden, Germany
[Bezmaternykh, L. N.
Gudim, I. A.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
B. I. Verkin Inst. for Low-Temperature Physics, Engineering, National Academy of Sciences of Ukraine, pr. Lenina 47, Kharkov 61103, Ukraine
B. I. Verkin Inst. for Low-Temperature Physics, Engineering, National Academy of Sciences of Ukraine, pr. Lenina 47, Kharkov 61103, Ukraine
Institute for Solid State Physics, Technical University Dresden, Dresden D-01069, Germany
L. V. Kirenskii Inst. of Physics of the Siberian Branch, The Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zvyagina, G. A.; Zhekov, K. R.; Bilych, I. V.; Zvyagin, A. A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна

}
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