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Вид документа : Статья из журнала
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Автор(ы) : Gavriliuk A. G., Trojan I. A., Lyubutin I. S., Ovchinnikov S. G., Sarkissian V. A.
Заглавие : High-pressure magnetic properties and P-T phase diagram of iron borate
Место публикации : J. Exp. Theor. Phys.: AMER INST PHYSICS, 2005. - Vol. 100, Is. 4. - P688-696. - ISSN 1063-7761, DOI 10.1134/1.1926429
Примечания : Cited References: 24
Предметные рубрики: FEBO3 SINGLE-CRYSTALS
NUCLEAR-RESONANCE
BAND-STRUCTURE
TRANSITION
TEMPERATURE
SCATTERING
Ключевые слова (''Своб.индексиров.''): antiferromagnetic materials--diamonds--ferromagnetic materials--high pressure effects--low temperature effects--magnetic moments--magnetic properties--magnetization--phase diagrams--powders--single crystals--synchrotron radiation--diamond anvil cells--electronic transition--iron borate--nuclear forward scattering (nfs)--iron compounds
Аннотация: The high-pressure magnetic states of iron borate (FeBO3)-Fe-57 single-crystal and powder samples have been investigated in diamond anvil cells by nuclear forward scattering (NFS) of synchrotron radiation at different temperatures. In the low-pressure (0 < P < 46 GPa) antiferromagnetic phase, an increase of the Neel temperature from 350 to 595 K induced by pressure was found. At pressures 46-49 GPa, a transition from the antiferromagnetic to a new magnetic state with a weak magnetic moment (magnetic collapse) was discovered. It is attributed to the electronic transition in Fe3+ ions from the high-spin 3d(5) (S = 5/2, (6)A(1g)) to the low-spin (S = 1/2, T-2(2g)) state (spin crossover) due to the insulator-semiconductor-type transition with extensive suppression of strong d-d electron correlations. At low temperatures, NFS spectra of the high-pressure phase indicate magnetic correlations in the low-spin system with a magnetic ordering temperature of about 50 K. A tentative magnetic P-T phase diagram of FeBO3 is proposed. An important feature of this diagram is the presence of two triple points where magnetic and paramagnetic phases of the high-spin and low-spin states coexist. © 2005 Pleiades Publishing, Inc.
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