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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Wu L. S., Nikitin S. E., Frontzek M., Kolesnikov A. I., Ehlers G., Lumsden M. D., Shaykhutdinov K. A., Guo, E. -J., Savici A. T., Gai Z., Sefat A. S., Podlesnyak A.
Заглавие : Magnetic ground state of the Ising-like antiferromagnet DyScO3
Коллективы : Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division
Место публикации : Phys. Rev. B: American Physical Society, 2017. - Vol. 96, Is. 14. - Ст.144407. - ISSN 2469-9950, DOI 10.1103/PhysRevB.96.144407. - ISSN 2469-9969(eISSN)
Примечания : Cited References:37. - We thank J. M. Sheng and Q. Zhang for the help with the neutron data refinement. We would like to thank A. Christianson, I. Zaliznyak, M. Mourigal, Z. T. Wang, and C. Batista for useful discussions. The research at the Spallation Neutron Source (ORNL) is supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). Research supported in part by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This work was partly supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division.
Предметные рубрики: THIN-FILMS
FERROELECTRICITY
VISUALIZATION
EXCITATIONS
Аннотация: We report on the low-temperature magnetic properties of the DyScO3 perovskite, which were characterized by means of single crystal and powder neutron scattering, and by magnetization measurements. Below TN = 3.15 K, Dy3+ moments form an antiferromagnetic structure with an easy axis of magnetization lying in the ab plane. The magnetic moments are inclined at an angle of ∼ +/- 28 degrees to the b axis. We show that the ground-state Kramers doublet of Dy3+ is made up of primarily |+/- 15/2 ⟩ eigenvectors and well separated by a crystal field from the first excited state at E1 = 24.9 meV. This leads to an extreme Ising single-ion anisotropy, M⊥/M∥∼ 0.05. The transverse magnetic fluctuations, which are proportional to M⊥2/M∥2, are suppressed, and only moment fluctuations along the local Ising direction are allowed. We also found that the Dy-Dy dipolar interactions along the crystallographic c axis are two to four times larger than in-plane interactions.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Skorobogatov S. A., Nikitin S. E., Shaykhutdinov K. A., Balaev A. D., Terentjev K. Yu., Ehlers G., Sala G., Pomjakushina, E., V, Conder K., Podlesnyak A.
Заглавие : Low-temperature spin dynamics in the TmFeO3 orthoferrite with a non-Kramers ion
Коллективы : International Max Planck Research School for Chemistry and Physics of Quantum Materials (IMPRS-CPQM)
Место публикации : Phys. Rev. B. - 2020. - Vol. 101, Is. 1. - Ст.014432. - ISSN 2469-9950, DOI 10.1103/PhysRevB.101.014432. - ISSN 2469-9969(eISSN)
Примечания : Cited References: 41. - We thank A. Sukhanov for stimulating discussions and D. Abernathy for support with data acquisition. This research used resources at the High Flux Isotope Reactor and Spallation Neutron Source, a DOE Office of Science User Facility operated by Oak Ridge National Laboratory. S.E.N. acknowledges support from the International Max Planck Research School for Chemistry and Physics of Quantum Materials (IMPRS-CPQM). Laue x-ray diffraction measurements were conducted at the Center for Nanophase Materials Sciences (CNMS) (CNMS2019-R18) at Oak Ridge National Laboratory (ORNL), which is a DOE Office of Science User Facility
Предметные рубрики: NEUTRON-SCATTERING
REORIENTATION
VISUALIZATION
EXCITATIONS
SOFTWARE
Аннотация: We investigate the magnetic dynamics of the orthorhombic perovskite TmFeO3 at low temperatures, below the spin reorientation transition at TSR≈80 K, by means of time-of-flight neutron spectroscopy. We find that the magnetic excitation spectrum combines two emergent collective modes associated with different magnetic sublattices. The Fe subsystem orders below TN∼632 K into a canted antiferromagnetic structure and exhibits sharp, high-energy magnon excitations. We describe them using linear spin-wave theory, and reveal a pronounced anisotropy between in- and out-of-plane exchange interactions, which was mainly neglected in previous reports on the spin dynamics in orthoferrites. At lower energies, we find two crystalline electrical field (CEF) excitations of Tm3+ ions at energies of ∼2 and 5 meV. In contrast to the sister compound YbFeO3, where the Yb3+ ions form quasi-one-dimensional chains along the c axis, the Tm excitations show dispersion along both directions in the (0KL) scattering plane. Analysis of the neutron scattering polarization factor reveals a longitudinal polarization of the 2 meV excitation. To evaluate the effect of the CEF on the Tm3+ ions, we perform point-charge model calculations, and their results quantitatively capture the main features of Tm single-ion physics, such as energies, intensities, and polarization of the CEF transitions, and the type of magnetic anisotropy.
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