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Low-temperature absorption spectra and electron structure of HoFe3(BO3)4 single crystal / A. V. Malakhovskii [et al.] // Физ. низких температур. - 2017. - Т. 43, Вып. 5. - С. 764-771. - Библиогр.: 33 . - ISSN 0132-6414
Кл.слова (ненормированные):
f-f transitions -- Ho3+ ion -- Excited states -- Local properties
Аннотация: Polarized absorption spectra of HoFe3(BO3)4 single crystal in the range of 8500-24500 cm-1 were studied as a function of temperature beginning from 2 K. The ground and excited electron states of Ho3+ were identified. The abrupt changes of the spectra at the reorientation phase transition at 4.7 K were observed. The exchange splitting of some excited states were revealed and measured. They changed at the reorientation phase transition. Several vibronic transitions were observed. The splitting of absorption lines corresponding to the C2 local symmetry of the Ho ion was not observed. Moreover, spectra of some absorption bands correspond to splitting in the cubic crystal field. There are some absorption lines, whose polarization can not be explained both in D3 and C2 local symmetries. Some lines appear or disappear as a result of the transition from the easy axis to the easy plane state of the crystal. All these observations testify to the substantial changes of the local magnetic and structural properties in the excited states of the Ho3+ ion and to the strong influence of the magnetic moments orientation on the polarization of the electron transitions.

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"Переводная" версия Low-temperature absorption spectra and electron structure of HoFe3(BO3)4 single crystal [Текст] / A. V. Malakhovskii [et al.] // Low Temp. Phys : American Institute of Physics, 2017. - Vol. 43 Is. 5.- P.610-616

Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk, Russian Federation
B. Verkin Institute for Low Temperature Physics and Engineering, National Academy of Sciences of Ukraine, Kharkov, Ukraine

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Gnatchenko, S. L.; Kachur, I. S.; Piryatinskaya, V. G.; Gudim, I. A.; Гудим, Ирина Анатольевна
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Magnetic field induced local structural transformations in the optically excited states 5F2 and 5F3 of HoFe3(BO3)4 single crystal / A. V. Malakhovskii [et al.] // J. Magn. Magn. Mater. - 2019. - Vol. 476. - P. 177-182, DOI 10.1016/j.jmmm.2018.12.078. - Cited References: 25. - A.V. Malakhovskii acknowledges the support from the Russian Foundation for Basic Researches grant 16-02-00273 and from the Project of Russian Academy of Science No. 0356-2017-0030. . - ISSN 0304-8853
Кл.слова (ненормированные):
f-f transitions -- Ho3+ ion -- Excited states -- Local properties
Аннотация: We measured absorption spectra of transitions 5I8 → 5F2, 5F3 in Ho3+ ion in the HoFe3(BO3)4 single crystal at temperature 2 K as a function of magnetic field 0–65 kOe directed along a and c axes. The spectra were decomposed to the Lorentz shape components and magnetic field dependences of their parameters: position, intensity and line width, were obtained. Substantial difference between dependences of the energy and intensity of the transitions on magnetic field was revealed. So, the abrupt changes of the electron transition energies were mainly observed at the reorientation magnetic phase transitions in the crystal. A number of singularities in the magnetic field dependences of the electron transition intensities were revealed both at the reorientation transitions and outside of them. The singularities in the average intensities of transitions into multiplets at the reorientation magnetic transitions are due to the changes of the odd part of the crystal field, responsible for the allowance of f-f transitions, and also are due to the changes of the magnetic state. The singularities in behavior of intensity of each separate transition are due to the local even distortions in the excited states, which mix the electron states.

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Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk, 660036, Russian Federation
B. Verkin Institute for Low Temperature Physics and Engineering, National Academy of Sciences of Ukraine, Kharkov, 61103, Ukraine

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Gnatchenko, S. L.; Kachur, I. S.; Piryatinskaya, V. G.; Gudim, I. A.; Гудим, Ирина Анатольевна
}
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Magnetic circular dichroism and absorption spectra of 5I8 → 5F5 transition in HoAl3(BO3)4 and HoFe3(BO3)4 single crystals / A. V. Malakhovskii [et al.] // Phys. Lett. A. - 2019. - Vol. 383, Is. 16. - P. 1960-1966, DOI 10.1016/j.physleta.2019.03.016. - Cited References: 34. - The work was supported by the Russian Foundation for Basic Researches grant 19-02-00034. . - ISSN 0375-9601
Кл.слова (ненормированные):
Ho3+ ion -- f-f transitions -- Magnetic circular dichroism -- Electron structure
Аннотация: Comparative study of magnetic circular dichroism (MCD) and absorption spectra of HoAl3(BO3)4 and HoFe3(BO3)4 single crystals in the region of 5I8 → 5F5 transition of the Ho3+ ion was carried out. Absorption spectra were decomposed into the Lorentz shape components and intensities of transitions were obtained. Unusually strong vibronic transitions were observed in HoAl3(BO3)4, but were not observed in HoFe3(BO3)4 that testified to the strong non diagonal vibronic interaction in HoAl3(BO3)4. The MCD spectra were analyzed in approximation of the ∣J,± MJ≻ of the wave functions of the free atom and using concept of the crystal quantum number. Peculiarity of application of this concept to ions with integer moments was revealed and modification of the concept was suggested. With the help of the MCD spectra, the Zeeman splitting of some transitions was found. In particular, the Landé factor gC ≈2 of the ground state of the Ho3+ ion in HoAl3(BO3)4 in the trigonal axis direction was determined. It appeared to be five times less than that in HoFe3(BO3)4 also found with the help of the MCD.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Rautskii, M. V.; Рауцкий, Михаил Владимирович
}
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