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    Eu2+ site preferences in the mixed cation K2BaCa(PO4)2 and thermally stable luminescence / J. W. Qiao [et al.] // J. Am. Chem. Soc. - 2018. - Vol. 140, Is. 30. - P. 9730-9736, DOI 10.1021/jacs.8b06021. - Cited References: 40. - This work is supported by the National Natural Science Foundation of China (No. 51722202, 91622125, 51572023, and 11574003), Natural Science Foundations of Beijing (2172036) and M.M. acknowledges support of the Russian Foundation for Basic Research (17-52-53031). . - ISSN 0002-7863
   Перевод заглавия: Предпочтительное положение ионов Eu2+ в смешанных катионах K2BaCa(PO4)2 и термически стабильная люминесценция

РУБ Chemistry, Multidisciplinary
Рубрики:
LIGHT-EMITTING-DIODES
   SOLID-SOLUTION
   PHOSPHORS
   GREEN
   BLUE
Аннотация: Site preferences of dopant Eu2+ on the locations of K+, Ba2+, and Ca2+ in the mixed cation phosphate K2BaCa(PO4)2 (KBCP) are quantitatively analyzed via a combined experimental and theoretical method to develop a blue-emitting phosphor with thermally stable luminescence. Eu2+ ions are located at K2 (M2) and K3 (M3) sites of KBCP, with the latter occupation relatively more stable than the former, corresponding to emissions at 438 and 465 nm, respectively. KBCP:Eu2+ phosphor exhibits highly thermal stable luminescence even up to 200 °C, which is interpreted as due to a balance between thermal ionization and recombination of Eu2+ 5d excited-state centers with the involvement of electrons trapped at crystal defect levels. Our results can initiate more exploration of activator site engineering in phosphors and therefore allow predictive control of photoluminescence tuning and thermally stable luminescence for emerging applications in white LEDs.

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Держатели документа:
Univ Sci & Technol Beijing, Beijing Municipal Key Lab New Energy Mat & Techno, Sch Mat Sci & Engn, Beijing 100083, Peoples R China.
Anhui Normal Univ, Dept Phys, Anhui Key Lab Optoelect Mat Sci & Technol, Wuhu 241000, Anhui, Peoples R China.
RAS, SB, KSC, Lab Crystal Phys,Kirensky Inst Phys,Fed Res Ctr, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Natl Synchrotron Radiat Res Ctr, Hsinchu 300, Taiwan.

Доп.точки доступа:
Qiao, Jianwei; Ning, Lixin; Molokeev, M. S.; Молокеев, Максим Сергеевич; Chuang, Yu-Chun; Liu, Quanlin; Xia, Zhiguo
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Synthesis and photophysical properties of copolyfluorenes for light-emitting applications: Spectroscopic experimental study and theoretical DFT consideration / R. Y. Smyslov [et al.] // Polymer. - 2019. - Vol. 168. - P. 185-198, DOI 10.1016/j.polymer.2019.02.015. - Cited References: 45. - The quantum yield measurements were performed at the Center for Optical and Laser Materials Research, St. Petersburg State University. P. Avramov gratefully acknowledges the financial support of National Research Foundation of Republic of Korea under Grant No. NRF-2017R1A2B4004440. This work has been carried out using computing resources of the federal collective usage center Complex for Simulation and Data Processing for Mega-science Facilities at NRC "Kurchatov Institute" . - ISSN 0032-3861. - ISSN 1873-2291

РУБ Polymer Science
Рубрики:
BETA-PHASE FORMATION
   SINGLE POLYMER
   POLYFLUORENE
   BLUE
   COPOLYMERS
Кл.слова (ненормированные):
Suzuki cross-coupling -- Yamamoto polycondensation -- Density functional theory
Аннотация: Using Suzuki and Yamamoto coupling reactions, copoly-(9,9-dioctylfluorenes) (CPF) were synthesized and compared regarding their photophysical properties using the spectroscopic and ab initio DFT approaches. The CPFs were functionalized by benzo [2,3,5] thiadiazole (BT) or carbazole-3,6-diyl (3,6-Cz). The latter was used to introduce different luminophore fragments, including Nile red and 4-pyrrolidinyl-1,8-naphthalimide derivatives. The effect of the two synthesis techniques on the polymer microstructure, the influence of embedding of 3,6-Cz moieties in the polymer backbone on polymer structuring, and the impact of the end groups like novel quinoxaline-containing compounds on the luminescent properties of CPFs were investigated. By comparing electron density distribution using the ab initio DFT approach with photoluminescence, it was shown that Suzuki reaction provides a chain microstructure with individual BT fragments separated by 9,9-dioctylfluorene monomeric units, while Yamamoto reaction leads to the blocks of BT units. This effect leads to different CPF photophysical properties (absorption and emission spectra).

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Держатели документа:
Russian Acad Sci, Inst Macromol Cpds, Bolshoy 31, St Petersburg 199004, Russia.
NRC Kurchatov Inst, Petersburg Nucl Phys Inst, Mkr Orlova Roscha 1, Gatchina 188300, Leningrad Regio, Russia.
Siberian Fed Univ, Svobodny 79, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Fed Res Ctr, Kirensky Inst Phys, Siberian Branch,Krasnoyarsk Sci Ctr, Akad Gorodok 50-38, Krasnoyarsk 660036, Russia.
St Petersburg State Univ, Unive Skaya Nab 7-9, St Petersburg 199034, Russia.
Yaroslavl State Tech Univ, Moskovskii 88, Yaroslavl 150023, Russia.
Kyungpook Natl Univ, Dept Chem & Greennano Mat Res Ctr, 80 Daehakro, Daegu 41556, South Korea.

Доп.точки доступа:
Smyslov, Ruslan Yu; Tomilin, F. N.; Томилин, Феликс Николаевич; Shchugoreva, I. A.; Nosova, G. I.; Zhukova, E. V.; Litvinova, L. S.; Yakimansky, A. V.; Kolesnikov, I.; Abramov, I. G.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Avramov, P. V.; Аврамов, Павел Вениаминович
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    Giant red-shifted emission in (Sr,Ba)Y2O4:Eu2+ phosphor toward broadband near-infrared luminescence / Z. Y. Yang, Y. F. Zhao, Y. Y. Zhou [et al.] // Adv. Funct. Mater. - 2022. - Vol. 32, Is. 1. - Ст. 2103927, DOI 10.1002/adfm.202103927. - Cited References: 60. - This research was supported by the International Cooperation Project of National Key Research and Development Program of China (2021YFE0105700), National Natural Science Foundations of China (Grant No. 51972118 and 51961145101), Guangzhou Science & Technology Project (202007020005), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137). This work is also funded by RFBR according to the research project No. 19-52-80003 . - ISSN 1616-301X. - ISSN 1616-3028
   Перевод заглавия: Излучение с гигантским красным смещением в люминофоре (Sr,Ba)Y2O4: Eu2 + для широкополосной люминесценции в ближней инфракрасной области

РУБ Chemistry, Multidisciplinary + Chemistry, Physical + Nanoscience & Nanotechnology + Materials Science, Multidisciplinary + Physics, Applied + Physics, Condensed Matter
Рубрики:
LIGHT-SOURCES
   PHOTOLUMINESCENCE
   TRANSITION
   CE3+
   BLUE
   SUBSTITUTION
Кл.слова (ненормированные):
near-infrared emission -- photoluminescence -- red emission
Аннотация: Near-infrared (NIR) light-emitting diodes (LEDs) light sources are desirable in photonic, optoelectronic, and biological applications. However, developing broadband red and NIR-emitting phosphors with good thermal stability is always a challenge. Herein, the synthesis of Eu2+-activated SrY2O4 red phosphor with high photoluminescence quantum efficiency and broad emission band ranging from 540 to 770 nm and peaking at 620 nm under 450 nm excitation is designed. Sr/Ba substitution in SrY2O4:Eu2+ has been further utilized to achieve tunable emission by modifying the local environment, which facilitates the giant red-shifted emission from 620 to 773 nm while maintaining the outstanding thermal stability of SrY2O4:Eu2+. The NIR emission is attributed to the enhanced Stokes shift and crystal field strength originated from the local structural distortions of [Y1/Eu1O6] and [Y2/Eu2O6]. The investigation in charge distribution around Y/Eu provides additional insight into increasing covalency to tune the emission toward the NIR region. As-fabricated NIR phosphor-converted LEDs demonstration shows its potential in night-vision technologies. This study reveals the NIR luminescence mechanism of Eu2+ in oxide-based hosts and provides a design principle for exploiting Eu2+-doped NIR phosphors with good thermal stability.

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Держатели документа:
South China Univ Technol, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, State Key Lab Luminescent Mat & Devices, Sch Mat Sci & Engn, Guangzhou 510641, Peoples R China.
Natl Synchrotron Radiat Res Ctr, Mat Sci Grp, Sci Res Div, Hsinchu 300, Taiwan.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Lab Crystal Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Dept Engn Phys & Radioelect, Krasnoyarsk 660041, Russia.
Kemerovo State Univ, Res & Dev Dept, Kemerovo 650000, Russia.

Доп.точки доступа:
Yang, Zhiyu; Zhao, Yifei; Zhou, Yayun; Qiao, Jianwei; Chuang, Yu-Chun; Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Zhiguo; International Cooperation Project of National Key Research and Development Program of China [2021YFE0105700]; National Natural Science Foundations of ChinaNational Natural Science Foundation of China (NSFC) [51972118, 51961145101]; Guangzhou Science & Technology Project [202007020005]; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01X137]; RFBRRussian Foundation for Basic Research (RFBR) [19-52-80003]
}
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    Competitive site occupation toward improved quantum efficiency of SrLaScO4:Eu red phosphors for warm white LEDs / Z. Y. Yang, G. C. Liu, Y. F. Zhao [et al.] // Adv. Opt. Mater. - 2022. - Vol. 10. Is. 6. - Ст. 2102373, DOI 10.1002/adom.202102373. - Cited References: 42. - This research was supported by the International Cooperation Project of National Key Research and Development Program of China (Program No. 2021YFE0105700), National Natural Science Foundation of China (Grant Nos. 51972118 and 51961145101), Guangzhou Science & Technology Project (Project No. 202007020005), the State Key Laboratory of Luminescent Materials and Devices (Grant No. Skllmd-2021-09), China Postdoctoral Science Foundation (Grant No. 2021M691053), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (Program No. 2017BT01X137). This work was also funded by RFBR according to the research Project No. 19-52-80003 and the NRF International: SA/China Joint Research Programme 2021 - CHIN2002265 06921 UID 132785 . - ISSN 2195-1071
   Перевод заглавия: Конкурентное заселение позиций для повышения квантовой эффективности красных люминофоров SrLaScO4:Eu для тепло-белых светодиодов

РУБ Materials Science, Multidisciplinary + Optics
Рубрики:
LUMINESCENCE
   EUROPIUM
   BLUE
   EU2+
   STABILIZATION
   EPR
Кл.слова (ненормированные):
light-emitting diodes -- photoluminescence -- red emission
Аннотация: The discovery of Eu2+-doped high-efficiency red phosphors remains a vital challenge for white light-emitting diode (WLED) applications. It is therefore urgent to find effective strategies managing the oxidation state to help reduce Eu3+ to Eu2+ and accordingly increase the photoluminescence quantum yield (PLQY). Herein, a new red-emitting SrLaScO4:Eu phosphor is designed, and the PLQY is enhanced from 13% to 67% under 450 nm excitation by employing (NH4)2SO4-assisted sintering. Combined structural analysis, optical spectroscopy, and theoretical calculation reveal that predominant Eu2+ prefers to occupy the Sr2+ sites in the SrLaScO4 enabling red emission, and a competitive site occupation of Eu3+ in La3+ can be restrained, and the reduction mechanism of Eu3+ to Eu2+ originating from the (NH4)2SO4 addition is analyzed. The fabricated WLED device using red-emitting SrLaScO4:Eu and yellow-emitting Y3(Al,Ga)5O12:Ce3+ exhibits a high color-rendering index of 86.7 at a low correlated color temperature of 4005 K. This work provides a feasible reduction strategy for guiding the development of high-efficiency Eu2+-doped red phosphor for WLED applications.

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Держатели документа:
South China Univ Technol, State Key Lab Luminescent Mat & Devices, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, Sch Mat Sci & Engn, Guangzhou 510641, Peoples R China.
City Univ Hong Kong, Dept Chem, Kowloon, Hong Kong 999077, Peoples R China.
KSC SB RAS, Lab Crystal Phys, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Dept Engn Phys & Radioelect, Krasnoyarsk 660041, Russia.
Kemerovo State Univ, Res & Dev Dept, Kemerovo 650000, Russia.
Univ Free State, Dept Phys, POB 339, ZA-9300 Bloemfontein, South Africa.
South China Univ Technol, Sch Phys & Optoelect, Guangzhou 510641, Peoples R China.

Доп.точки доступа:
Yang, Zhiyu; Liu, Gaochao; Zhao, Yifei; Zhou, Yayun; Qiao, Jianwei; Molokeev, M. S.; Молокеев, Максим Сергеевич; Swart, Hendrik C.; Xia, Zhiguo; International Cooperation Project of National Key Research and Development Program of China [2021YFE0105700]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51972118, 51961145101]; Guangzhou Science & Technology Project [202007020005]; State Key Laboratory of Luminescent Materials and Devices [Skllmd-2021-09]; China Postdoctoral Science FoundationChina Postdoctoral Science Foundation [2021M691053]; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01X137]; RFBRRussian Foundation for Basic Research (RFBR) [19-52-80003]; NRF International: SA/China Joint Research Programme 2021 [CHIN2002265 06921 UID 132785]
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