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Aver'yanov, E. M.
Structural and thermodynamic consequencies of the interaction of conformational degrees of freedom of azomethines in the nematic phase / E. M. Aver'yanov // J. Struct. Chem. - 2014. - Vol. 55, Is. 4. - P. 605-611, DOI 10.1134/S0022476614040039. - Cited References: 21 . - ISSN 0022-4766. - ISSN 1573-8779

РУБ Chemistry, Inorganic & Nuclear + Chemistry, Physical
Рубрики:
CONJUGATED POLY(AZOMETHINE)S
   TERMINAL SUBSTITUENTS
   ELECTRONIC-STRUCTURES
   FLUORINATED ANALOGS
   INTERNAL-ROTATION
   MOLECULES
   COMPOUND
   ANGLES
   STATE
   NMR
Кл.слова (ненормированные):
azomethines -- benzylideneaniline -- conformation -- steric effects of substituents -- nematic-isotropic liquid transition -- conformational polymorphism
Аннотация: The interaction of the conformational degrees of freedom of azomethines in the nematic phase, which is induced by electronic donor-acceptor properties of the terminal substituents of the benzylideneaniline core is studied. These degrees of freedom related to the rotation angles phi (k) around the bonds between the substituent and the aniline ring (phi(1)) and also between the CH=N bridge and the aniline ring (omega(2)) are characterized by the parameters Q (k) = aOE (c) cos(2)phi (k) >. It is found that the interaction of these degrees of freedom is manifested in the linear dependence Q (2)(Q (1)). Within the phenomenological theory the effect of this interaction on changes delta (k) in the Q (k) values during the nematic liquid crystal-isotropic liquid phase transition is revealed along with the temperature T (NI) and character of this transition. The derivation of previously established empirical dependences T (NI)(Q (k) ) is presented in the presence of direct and indirect steric effects of side substituents affecting the Q (k) values. A diverse combination of delta (k) signs in the nematic phase, which is a prerequisite for the conformational polymorphism of the nematic phases of azomethines, is shown.

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Публикация на русском языке Аверьянов, Евгений Михайлович. Структурные и термодинамические следствия взаимодействия конформационных степеней свободы азометинов [Текст] / Е. М. Аверьянов // Журн. структ. химии. - Новосибирск : Изд-во СО РАН, 2014. - Т. 55 № 4. - С. 641 - 647

Доп.точки доступа:
Аверьянов, Евгений Михайлович
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Structural and magnetic features of solid-phase transformations in Mn/Bi and Bi/Mn films / V. G. Myagkov [et al.] // JETP Letters. - 2016. - Vol. 103, Is. 4. - P. 254-259, DOI 10.1134/S0021364016040111. - Cited References: 47. - This work was supported by the Russian Foundation for Basic Research (project nos. 15-02-00948 and 16-03-00069), by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (project no. SP-317.2015.1), and by the Foundation for Promotion of the Development of Small Scientific and Engineering Enterprises (project nos. 0011727 and 6662GU2015, program Umnik). The electron microscopy studies were performed on the equipment of the Shared Usage Center, Krasnoyarsk Research Center, Siberian Branch, Russian Academy of Sciences. . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
High-temperature synthesis
   Epitaxial thin-films
   State synthesis
   Martensitic transformations
   Vacuum depositions
   MnBi filmsd
   Bi
   System
   Anisotropy
   Compound
Аннотация: Solid-phase transformations at different annealing temperatures in Mn/Bi (Mn on Bi) and Bi/Mn (Bi on Mn) films have been studied using X-ray diffraction, electron microscopy, and magnetic measurements. It has been shown that the synthesis of the α-MnBi phase in polycrystalline Mn/Bi films begins at a temperature of ~120°C and the Mn and Bi layers react completely at 300°C. The resulting α-MnBi(001) samples have a large perpendicular magnetic anisotropy (Ku ≃ 1.5 × 107 erg/cm3) and a coercive force H HC ~ 3 kOe. In contrast to Mn/Bi, the ferromagnetic α-MnBi phase in Bi/Mn films is not formed even at annealing processes up to 400°C and Mn clusters are formed in a Bi melt. This asymmetry in phase transformations occurs because chemosorbed oxygen existing on the surface of the Mn film in Bi/Mn films suppresses a solid-phase reaction between Mn and Bi. The analysis of the results obtained implies the existence of new low-temperature (~120°C) structural transformation in the Mn–Bi system. © 2016, Pleiades Publishing, Inc.

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Публикация на русском языке Структурные и магнитные особенности твердофазных превращений в Mn/Bi и Bi/Mn пленках [Текст] / В. Г. Мягков [и др.] // Письма в ЖЭТФ : Наука, 2016. - Т. 103 Вып. 4. - С. 280-285

Держатели документа:
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, Russian Federation
Siberian State Aerospace University, pr. Gazety Krasnoyarskii Rabochii, Krasnoyarsk, Russian Federation
Institute of Chemistry and Chemical Technology, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, Russian Federation
Siberian Federal University, Svobodnyi pr. 79, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Myagkov, V. G.; Мягков, Виктор Григорьевич; Bykova, L. E.; Быкова, Людмила Евгеньевна; Yakovchuk, V. Yu.; Яковчук, Виктор Юрьевич; Zhigalov, V. S.; Жигалов, Виктор Степанович; Volochaev, M. N.; Волочаев, Михаил Николаевич; Matsynin, A. A.; Мацынин, Алексей Александрович; Tambasov, I. A.; Тамбасов, Игорь Анатольевич; Seredkin, V. A.; Середкин, Виталий Александрович; Patrin, G. S.; Патрин, Геннадий Семёнович; Bondarenko, G. N.; Бондаренко, Галина Николаевна
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Role of Fe magnetic subsystems to form a magnetic spin glass state in RFeTi2O7 / T. V. Drokina [et al.] // J. Magn. Magn. Mater. - 2017. - Vol. 440. - P. 41-43, DOI 10.1016/j.jmmm.2016.12.088. - Cited References:6. - This work has been partially financed by projects MECOM (MAT2014-53921-R) and DGA (IMANA E34) . - ISSN 0304-8853. - ISSN 1873-4766

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
COMPOUND
Кл.слова (ненормированные):
Oxide materials -- Solid state reaction -- Cation substitution -- Spin glasses
Аннотация: The experimental studies on R3+Fe3+Ti2O7 (R=Sm, Gd, Tb, Tm, Dy) magnetic properties evidence the low temperature spin glass state in all compounds. The possibility of rare-earth cation substitution allows the investigation of the role of magnetic iron Fe3+ ions and rare earth R3+ ions subsystems in a ground state formation in these oxide compounds.

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Доп.точки доступа:
Drokina, T. V.; Дрокина, Тамара Васильевна; Petrakovskii, G. A.; Петраковский, Герман Антонович; Bayukov, O. A.; Баюков, Олег Артемьевич; Molokeev, M. S.; Молокеев, Максим Сергеевич; Bartolome, J.; Arauzo, A.; project MECOM [MAT2014-53921-R]; project DGA [IMANA E34]; Euro-Asian Symposium "Trends in MAGnetism"(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); "Trends in MAGnetism", Euro-Asian Symposium(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); Институт физики им. Л.В. Киренского Сибирского отделения РАН
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