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Magneto-optical properties of Dy3+ in oxide glasses: The origin of the magneto-optical activity of f-f transitions and its anomalous temperature dependence / A. V. Malakhovskii [et al.] // Phys. Solid State. - 2007. - Vol. 49, Is. 4. - P. 701-707, DOI 10.1134/S1063783407040178. - Cited References: 28 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
MAGNETIC CIRCULAR-DICHROISM
   FLUOROZIRCONATE ZBLAN GLASS
   OPTICAL-ABSORPTION SPECTRA
   DOPED SODA GLASS
   SPECTROSCOPIC PROPERTIES
   FLUOROBORATE GLASSES
   LITHIUM BORATE
   IONS
   PR3+
   GADOLINIUM
Аннотация: The temperature dependence of the absorption spectra and magnetic circular dichroism due to f-f transitions from the H-6(15/2) to F-6 (5/2) and (6)(F (7/2) + H (5/2)) states in the Dy3+ ion in (Dy2O3-P2O5-SiO2-GeO2) and (Dy2O3-La2O3-Al2O3-B2O3-SiO2-GeO2) glasses and the temperature dependence of the Faraday effect were studied. The temperature dependence of the Faraday effect caused by f-d transitions was found to differ from that of the magnetic circular dichroism due to f-f transitions. It was shown that f-f transitions occur preferentially in Dy3+ ions associated into clusters. The origin of the paramagnetic magneto-optical activity of f-f transitions was analyzed. It was shown that the contributions to this activity can differ in value and sign and that the ratio between these contributions depends on the transition type. In some cases, this difference results in an anomalous temperature dependence of the magneto-optical activity.

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
Krasnoyarsk State Univ, Krasnoyarsk 660041, Russia
SI Vavilov State Opt Inst, St Petersburg 192371, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation
Krasnoyarsk State University, Krasnoyarsk, 660041, Russian Federation
Vavilov State Optical Institute, Birzhevaya liniya 12, St. Petersburg, 192371, Russian Federation

Доп.точки доступа:
Malakhovskii, A. V.; Малаховский, Александр Валентинович; Isachenko, V. A.; Sukhachev, A. L.; Сухачев, Александр Леонидович; Potseluyko, A. M.; Zabluda, V. N.; Заблуда, Владимир Николаевич; Zarubina, T. V.; Edelman, I. S.; Эдельман, Ирина Самсоновна
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Unusual magnetic phase transitions in Gd3+ clusters in multicomponent oxide glasses / J. . Kliava [et al.] // J. Supercond. Nov. Magn. - 2007. - Vol. 20, Is. 2. - P. 149-153, DOI 10.1007/s10948-006-0116-4. - Cited References: 7 . - ISSN 1557-1939

РУБ Physics, Applied + Physics, Condensed Matter
Рубрики:
GADOLINIUM
RESONANCE
Кл.слова (ненормированные):
oxide glasses -- gadolinium -- magnetic clusters -- superparamagnetism -- Gadolinium -- Magnetic clusters -- Oxide glasses -- Superparamagnetism -- Magnetic clusters -- Magnetic phase transitions -- Oxide glasses -- Weiss constant -- Antiferromagnetic materials -- Ferromagnetic materials -- Gadolinium -- Magnetic anisotropy -- Magnetic susceptibility -- Paramagnetic resonance -- Phase transitions -- Positive ions -- Superparamagnetism -- Glass
Аннотация: Magnetic susceptibility, EPR and optical properties have been studied in a glass system {20La(2)O(3) - 22Al(2)O(3) - 23B(2)O(3) - 35(SiO2 + GeO2)} with a part of La2O3 substituted by Gd2O3 in different concentrations. Positive Weiss constants have been found in more heavily doped glasses; two magnetic transitions at 55 and 12 K have been detected and ascribed, respectively, to ferromagnetic and antiferromagnetic clusters of Gd3+ ions. The EPR spectra confirm the clustering at higher Gd contents. At low temperatures the cluster-related resonance indicates an onset of magnetic anisotropy. The clustering, depending on the Gd concentration, correlates with a shift to lower energies of the strong optical absorption band edge.

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Держатели документа:
Univ Bordeaux 1, Cours Liberat 351, CP MOH, UMR 5798, F-33405 Talence, France
RAS, SB, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia
Bar Ilan Univ, Dept Phys, IL-52900 Ramat Gan, Israel
SV Vavilov State Opt Inst, St Petersburg 199034, Russia
ИФ СО РАН
CPMOH, UMR 5798 CNRS-Universite Bordeaux-I, 33405 Talence Cedex, France
L.V. Kirensky Institute of Physics, SB, RAS, Krasnoyarsk 660036, Russian Federation
Bar-Ilan University, Department of Physics, Ramat-Gan 52900, Israel
S.V. Vavilov State Optical Institute, St.-Petersburg 199034, Russian Federation
CPMOH, Universite Bordeaux-I, 351 Cours de la Liberation, 33405 Talence Cedex, France

Доп.точки доступа:
Kliava, J.; Malakhovskii, A. V.; Малаховский, Александр Валентинович; Edelman, I. S.; Эдельман, Ирина Самсоновна; Potseluyko, A. M.; Petrakovskaja, E. A.; Петраковская, Элеонора Анатольевна; Bruckental, I.; Yeshurun, Y.; Zarubina, T.
}
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