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Theoretical study of the diffusion of lithium in crystalline and amorphous silicon / A. S. Fedorov [et al.] // JETP Letters. - 2012. - Vol. 95, Is. 3. - P. 143-147, DOI 10.1134/S0021364012030058. - Cited References: 28. - We are grateful to the Institute of Computational Modeling, Siberian Branch, Russian Academy of Sciences; the Interdepartmental Supercomputer Center, Russian Academy of Sciences; and the Computer Center, Siberian Federal University, for the use of their computer clusters for performing all calculations. This work was supported by the Ministry of Education and Science of the Russian Federation (federal program "Human Capital for Science and Education in Innovative Russia" for 2009-2013). . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
ACCELERATED MOLECULAR-DYNAMICS
   AB-INITIO
   INFREQUENT EVENTS
   SIMULATION
   RELAXATION
   HYDROGEN
   POINTS
   SI
Аннотация: The effect of the lattice deformation on potential barriers for the motion of a lithium atom in crystalline silicon has been studied through ab initio density functional calculations. A new universal method of calculating the diffusion coefficient of an admixture in amorphous solid media through the activation mechanism has been proposed on the basis of these data. The method is based on the calculation of the statistical distribution of potential barriers for the motion of an admixture atom between minima depending on the position of neighboring atoms. First, the amorphous structure, which is generated by annealing from the crystalline structure with vacancies, has been simulated. Then, the statistical distribution of the potential barriers in the amorphous structure for various local environments of the admixture atoms has been calculated by means of linear regression with the parameters determined for barriers in crystalline silicon subjected to different deformations. The diffusion coefficient of the admixture has been calculated from this distribution by using the Arrhenius formula. This method has been tested by the example of crystalline and amorphous silicon with admixture of lithium atoms. The method demonstrates that the diffusion of lithium in amorphous silicon is much faster than that in crystalline silicon; this relation is confirmed experimentally.

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Публикация на русском языке Теоретическое исследование диффузии лития в кристаллическом и аморфном кремнии [Текст] / А. С. Федоров [и др.] // Письма в Журн. эксперим. и теор. физ. : Наука, 2012. - Т. 95 Вып. 3-4. - С. 159-163

Держатели документа:
[Fedorov, A. S.
Popov, Z. I.
Ovchinnikov, S. G.] Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
[Kuzubov, A. A.] Siberian Fed Univ, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Fedorov, A. S.; Федоров, Александр Семенович; Popov, Z. I.; Попов, Захар Иванович; Kuzubov, A. A.; Кузубов, Александр Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
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    Effects of composition modulation on the luminescence properties of Eu3+ doped Li1-xAgxLu(MoO4)2 solid-solution phosphors / F. Cheng [et al.] // Dalton Trans. - 2015. - Vol. 44, Is. 41. - P. 18078-18089, DOI 10.1039/c5dt02760h. - Cited References: 42. - The present work was supported by the National Natural Science Foundations of China (Grant No. 51272242, 51572023, 51511130035), Natural Science Foundations of Beijing (2132050), the Program for New Century Excellent Talents in University of Ministry of Education of China (NCET-12-0950), Beijing Nova Program (Z131103000413047), Beijing Youth Excellent Talent Program (YETP0635), the Funds of the State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences (RERU2015022), and the excellent tutor section of the Fundamental Research Funds for the Central Universities of China University of Geosciences, Beijing (2-9-2015-028). This work was also partly supported by the Russian Foundation for Basic Research (Grant No. 15-52-53080 GFEN_a). . - ISSN 1477-9226
   Перевод заглавия: Влияние модуляции состава на люминесцентные свойства твердотельного люминофора Li1-xAgxLu(MoO4)2 допированного Eu3+

РУБ Chemistry, Inorganic & Nuclear
Рубрики:
RED PHOSPHORS
   PHOTOLUMINESCENCE PROPERTIES
   ENERGY-TRANSFER
   WHITE LEDS
   IONS
   NA
   POLYMORPHISM
   TUNGSTATES
   RELAXATION
   MOLYBDATES
Аннотация: Double molybdate scheelite-type solid-solution phosphors Li1−xAgxLu1−y(MoO4)2:yEu3+ were synthesized by the solid state reaction method, and their crystal structures and luminescence properties were investigated in detail. The composition modulation and structural evolution of this series of samples were studied and the selected AgEu(MoO4)2, AgLu(MoO4)2, LiLu(MoO4)2 and LiEu(MoO4)2 phases were analyzed based on the Rietveld refinement. Depending on the variation of the Li/Ag ratio in Li1−xAgxLu1−y(MoO4)2:yEu3+ phosphors, the difference in the luminescence properties of Li1−xAgxLu1−y(MoO4)2:yEu3+ phosphors was ascribed to two factors, one reason could be assigned to the coupling effect and the nonradiative transition between the energy levels of LixAg1−xLu(MoO4)2 matrices and the activator Eu3+, another could be due to the near ultraviolet energy absorption and transmission efficiency between the charge-transfer (CT) band of O2−–Mo6+ and the 4f → 4f emissive transitions of Eu3+. The ultraviolet-visible diffuse reflection spectra (UV-vis DRS) and Raman spectra analysis were also used to verify the above mechanism.

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Держатели документа:
School of Materials Sciences and Technology, China University of Geosciences, Beijing, China
School of Materials Sciences and Engineering, University of Science and Technology Beijing, Beijing, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, SB RAS, Krasnoyarsk, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, Russian Federation
Beijing National Laboratory for Molecular Sciences, State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing, China

Доп.точки доступа:
Cheng, F.; Xia, Zhiguo; Molokeev, M. S.; Молокеев, Максим Сергеевич; Jing, X.
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Morozov, E. V.
Probing flocculant-induced asphaltene precipitation via NMR imaging: from model toluene-asphaltene systems to natural crude oils / E. V. Morozov, O. N. Martyanov // Appl. Magn. Reson. - 2016. - Vol. 47, Is. 2. - P. 223-235, DOI 10.1007/s00723-015-0741-9. - Cited References:46. - This research was performed with the financial support of Russian Science Foundation (project no. 15-19-00119). . - ISSN 0937-9347. - ISSN 1613-7507

РУБ Physics, Atomic, Molecular & Chemical + Spectroscopy
Рубрики:
PETROLEUM ASPHALTENES
   MOLECULAR-DYNAMICS
   AGGREGATION
   MICROSCOPY
   SCATTERING
   RESONANCE
   SEDIMENTATION
   ASSOCIATION
   CALORIMETRY
   RELAXATION
Аннотация: An nuclear magnetic resonance (NMR) imaging approach for studying flocculant-induced asphaltene precipitation processes is introduced in this report. Unlike commonly accepted techniques, which primarily measure aggregation processes on the submicron scale (the level of asphaltene molecules and their aggregates), NMR imaging demonstrates the capability to obtain new useful information about bulk system behavior on the macro scale. To reveal the capabilities of the method, the model toluene-asphaltene system and two samples of natural crude oils with different chemical composition and physical properties (such as asphaltene content and density) were employed for experiments. The process of colloidal suspension formation and two different patterns of its evolution were observed depending on both the asphaltene content and the flocculant concentration. In the first pattern, the flocculant-induced precipitation leads to the slow uniform compacting of the suspension and descent of the sedimentation front, whereas the second pattern is characterized by sediment accumulation and the upwards drift of the front. It was found that the behavior of the precipitated asphaltenes in the model system correlates well with those observed in natural crude oils. The results achieved in this work are in agreement with the data obtained previously via other techniques. Thus, NMR imaging proved to be an efficient method for probing flocculant-induced precipitation in crude oils.

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Держатели документа:
Russian Acad Sci, Inst Chem & Chem Technol, Siberian Branch, Akademgorodok 50-24, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Akademgorodok 50-24, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Siberian Branch, Boreskov Inst Catalysis, Pr Ak Lavrentieva 5, Novosibirsk 630090, Russia.
Novosibirsk State Univ, Pirogova St 2, Novosibirsk 630090, Russia.

Доп.точки доступа:
Martyanov, O. N.; Морозов, Евгений Владимирович; Russian Science Foundation [15-19-00119]
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Quantum nonequilibrium approach for fast electron transport in open systems: Photosynthetic reaction centers / M. . Pudlak [et al.] // Phys. Rev. E. - 2011. - Vol. 84, Is. 5. - Ст. 51912, DOI 10.1103/PhysRevE.84.051912. - Cited References: 34. - This work is partly supported by the Slovak Academy of Sciences in the framework of Center of Excellence NANOFLUID, VEGA Grants No. 2/0069/10, No. FIS2008-00781/FIS (Spain), and RFBR No. 11-02-00086 (Russia). . - ISSN 1539-3755

РУБ Physics, Fluids & Plasmas + Physics, Mathematical
Рубрики:
BACTERIUM RHODOPSEUDOMONAS-VIRIDIS
   PRIMARY CHARGE SEPARATION
   AMINO-ACID-SEQUENCE
   BACTERIOPHEOPHYTIN
   RELAXATION
   SUBUNIT
   DONOR
   MODEL
Кл.слова (ненормированные):
Electron transfer -- External fields -- Fast electron transport -- Initial conditions -- Non equilibrium -- Path-integral -- Perturbation theory -- Photosynthetic reaction center -- Second orders -- Time convolution -- Vibrational modes -- Electron transitions -- Perturbation techniques -- Quantum chemistry -- Photosynthesis
Аннотация: Creation of electrons or excitons by external fields in a system with initially statistically independent unrelaxed vibrational modes leads to an initial condition term. The contribution of this term in the time convolution generalized master-equation approach is studied in the second order of the perturbation theory in path-integral formalism. The developed approach, applied for the analysis of dynamics in the photosynthetic reaction center, exhibits the key role of the initial condition terms at the primary stage of electron transfer.

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Держатели документа:
[Pudlak, M.
Pincak, R.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia
[Pichugin, K. N.] LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
[Nazmitdinov, R. G.] Univ Illes Balears, Dept Fis, ES-07122 Palma De Mallorca, Spain
[Nazmitdinov, R. G.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia
ИФ СО РАН
Institute of Experimental Physics, Slovak Academy of Sciences, 04353 Kosice, Slovakia
Kirensky Institute of Physics, Akademgorodok 50/38, 660036 Krasnoyarsk, Russian Federation
Departament de Fisica, Universitat de les Illes Balears, ES-07122 Palma de Mallorca, Spain
Bogoliubov Laboratory of Theoretical Physics, Joint Institute for Nuclear Research, 141980 Dubna, Russian Federation

Доп.точки доступа:
Pudlak, M.; Pichugin, K. N.; Пичугин, Константин Николаевич; Nazmitdinov, R. G.; Pincak, R.
}
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Short-range correlations and their thermal hysteresis in the paramagnetic phase of YFe3(BO3)(4) / L. . Rebbouh [et al.] // Phys. Rev. B. - 2011. - Vol. 83, Is. 14. - Ст. 140406, DOI 10.1103/PhysRevB.83.140406. - Cited References: 21. - This work was supported by grants from the Natural Sciences and Engineering Research Council of Canada and the Canada Foundation for Innovation. J.M.C. acknowledges support from the Canada Research Chairs program. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
MOSSBAUER-SPECTRA
GDFE3(BO3)(4)
RELAXATION
Аннотация: Neutron diffraction and Mossbauer spectroscopy have been used to examine the connections between long-and short-range magnetic order in the rare-earth iron ferroborate YFe3(BO3)(4). We establish the presence of short-range magnetic order in the pseudo-one-dimensional Fe-spin chains of the FeO6 octahedra while the ferroborates are in their (long-range) paramagnetic phase. The short-range order exists at temperatures several times the Neel temperature. In addition, we observe thermal hysteresis of the short-range ordered Fe spins. The observed Fe-spin dynamics are suggestive of the presence of solitons within the domains that form in the Fe-spin chains.

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Держатели документа:
[Rebbouh, L.
Desautels, R. D.
Cadogan, J. M.
van Lierop, J.] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada
[Ritter, C.] Inst Laue Langevin, F-38042 Grenoble, France
[Temerov, V.
Pankrats, A.] RAS, LV Kirenskii Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Department of Physics and Astronomy, University of Manitoba, Winnipeg, MB R3T 2N2, Canada
Institut Laue-Langevin, Boite Postale 156, F-38042 Grenoble, France
L. V. Kirenskii Institute of Physics, Siberian Branch of RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Rebbouh, L.; Desautels, R. D.; Ritter, C.; Cadogan, J. M.; Temerov, V.; Pankrats, A. I.; Панкрац, Анатолий Иванович; van Lierop, J.
}
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Unusual disorder effects in superconducting LaFeAs1-delta O0.9F0.1 as revealed by As-75 NMR spectroscopy / F. . Hammerath [et al.] // Phys. Rev. B. - 2010. - Vol. 81, Is. 14. - Ст. 140504, DOI 10.1103/PhysRevB.81.140504. - Cited References: 52. - This work has been supported by the DFG, through FOR 538, SPP 1458 and Contract No. Be1749/12. G. L. acknowledges support from the A. v. Humboldt-Stiftung. M. M. K. acknowledges support from RFBR under Grant No. 09-02-00127, RAS program on "Low temperature quantum phenomena" and President of Russia MK-1683.2010.2. S. L. D. thanks H. Kontani, K. Kuroki, K. Kikoin, and M. Kulic for useful discussions. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
GAPS
   BA0.6K0.4FE2AS2
   RELAXATION
   SCATTERING
Аннотация: We report As-75 nuclear magnetic resonance measurements of the spin-lattice relaxation in the superconducting (SC) state of LaFeAsO0.9F0.1 and As-deficient LaFeAs1-delta O0.9F0.1. The temperature behavior of 1/T-1 below T-c changes drastically from a T-3 dependence for LaFeAsO0.9F0.1 to a T-5 dependence for the As-deficient sample. These results, together with the previously reported unexpected increase in Tc and the slope of the upper critical field near Tc for the As-deficient sample, are discussed in terms of nonuniversal SC gaps in Fe pnictides and the effect of As deficiency as an exotic case where nonmagnetic "smart" impurities even stabilize an s(+/-)-wave superconductor or within a scenario of a disorder-driven change to s(++) superconductivity.

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Держатели документа:
Inst Solid State Res, D-01171 Dresden, Germany
Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Institute for Solid State Research, IFW Dresden, P.O. Box 270116, D-01171 Dresden, Germany
Max-Planck-Institut fur Physik Komplexer Systeme, D-01187 Dresden, Germany
L.V. Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, 660036 Krasnoyarsk, Russian Federation
Department of Physics, University of Florida, Gainesville, FL 32611, United States

Доп.точки доступа:
Hammerath, F.; Drechsler, S. L.; Grafe, H. J.; Lang, G.; Fuchs, G.; Behr, G.; Eremin, I.; Korshunov, M. M.; Коршунов, Максим Михайлович; Buchner, B.
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Zobov, V. E.
The coordinate of the singular point of generating functions of clusters in the high-temperature dynamics of spin lattice systems with axially symmetric interaction / V. E. Zobov, M. A. Popov // Theor. Math. Phys. - 2003. - Vol. 136, Is. 3. - P. 1297-1311, DOI 10.1023/A:1025603416535. - Cited References: 25 . - ISSN 0040-5779

РУБ Physics, Multidisciplinary + Physics, Mathematical
Рубрики:
CONSISTENT FLUCTUATING FIELD
   NUCLEAR-DOUBLE-RESONANCE
   HEISENBERG PARAMAGNET
   LINE SHAPE
   RELAXATION
   SPECTRUM
   APPROXIMATION
   CRYSTALS
   MOMENT
   CAF2
Кл.слова (ненормированные):
spin dynamics -- singular points -- expansion over the reciprocal space dimension -- Expansion over the reciprocal space dimension -- Singular points -- Spin dynamics
Аннотация: We investigate generating functions for equipped trees composed of double bonds of two sorts on a hypercubic lattice of dimension d with built-in fragments. Rules for constructing these clusters are chosen to ensure the estimate for coefficients of power series in time for the longitudinal and transverse autocorrelation functions of the spin system with axially symmetric interaction. We derive a system of two equations for the tree-generating functions and an equation for the generating functions of chains leading from the root to a fragment in a tree using the Bethe approximation and under the condition that mainly bonds of one sort are taken into account. For the face-centered hypercubic lattice, we find the First terms of the 1/d expansion for the coordinate of the singular point of the generating function in both the anisotropic and the isotropic cases taking fragments in the forms of a triangle from four bonds and a four-fold bound pair into account. The obtained result is written in terms of ratios of lattice sums and is generalized to nuclear spin systems with dipole-dipole interaction. The theoretical value of the singular-point coordinate agrees well with the experimental value calculated from the tail of the absorption spectrum of the nuclear magnetic resonance in a barium fluoride monocrystal.

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Держатели документа:
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Novosibirsk, Russia
Krasnoyarsk State Univ, Krasnoyarsk, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Branch, RAS, Russian Federation
Krasnoyarsk State University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Popov, M. A.; Зобов, Владимир Евгеньевич
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Specific features of the approximation of the dielectric spectra of alkylcyanobiphenyl liquid crystals / B. A. Belyaev [et al.] // Phys. Solid State. - 2003. - Vol. 45, Is. 3. - P. 598-602, DOI 10.1134/1.1562253. - Cited References: 16 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
DECIMETER WAVELENGTH RANGE
SERIES
RELAXATION
Аннотация: The frequency dependences of the longitudinal and transverse permittivities of oriented nematic liquid crystals belonging to the alkylcyanobiphenyl group nCB (n = 5-8) are measured in the relaxation region in the meter and decimeter wavelength ranges. It is established that the dispersion of the longitudinal permittivity is well approximated by the sum of two Debye processes with different relaxation times. The frequency dependence of the transverse permittivity is represented by the dispersion relation with a continuous distribution of relaxation times in a specified time range. It is demonstrated that, in the high-frequency range (f 200 MHz), in which the dielectric spectra exhibit a number of weakly pronounced dispersion features, the total dispersion of the permittivity is adequately described by the sum of relaxation and resonance processes. (C) 2003 MAIK "Nauka/Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Belyaev, B. A.; Беляев, Борис Афанасьевич; Drokin, N. A.; Дрокин, Николай Александрович; Shabanov, V. F.; Шабанов, Василий Филиппович; Shepov, V. N.; Шепов, Владимир Николаевич
}
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Observation of mixed two-phase state in Eu0.7Pb0.3MnO3 single crystal by magnetic resonance method / N. V. Volkov [et al.] // Physica B. - 2002. - Vol. 324, Is. 1-4. - P. 254-260, DOI 10.1016/S0921-4526(02)01397-2. - Cited References: 19 . - ISSN 0921-4526

РУБ Physics, Condensed Matter
Рубрики:
OPTIMALLY DOPED MANGANITES
   COLOSSAL MAGNETORESISTANCE
   PARAMAGNETIC ANOMALIES
   CURIE-TEMPERATURE
   LA1-XCAXMNO3
   RELAXATION
   SEPARATION
Кл.слова (ненормированные):
manganites -- CMR -- magnetic resonance -- phase separation -- CMR -- Magnetic resonance -- Manganites -- Phase separation -- Europium compounds -- Ferromagnetic materials -- Paramagnetic resonance -- Phase separation -- Phase transitions -- Manganites -- Single crystals
Аннотация: The magnetic resonance measurements show that the mixed two-phase state takes place in the Eu0.7Pb0.3MnO3 single crystal. The coexistence of the magnetic phases is observed in vicinity of the magnetic phase transition, where the sample exhibits the effect of the CMR. The frequency-field dependencies of the spectra allow to conclude that these phases are paramagnetic and ferromagnetic ones. Moreover, the study of the frequency dependencies shows the sensitivity of the mixed-phase state to the external magnetic field. This suggests that the scenario of the phase separation is realized in this case and the mixed two-phase state is not related to simple chemical inhomogeneity. (C) 2002 Elsevier Science B.V. All rights reserved.

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Держатели документа:
RAS, SB, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
L.V. Kirensky Institute of Physics SB RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Volkov, N. V.; Волков, Никита Валентинович; Petrakovskii, G. A.; Петраковский, Герман Антонович; Vasiliev, V. N.; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Sablina, K. A.; Саблина, Клара Александровна; Patrin, K. G.; Патрин, Константин Геннадьевич
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10.

Two-phase paramagnetic-ferromagnetic state of La0.7Pb0.3MnO3 single-crystal lanthanum manganite / N. V. Volkov [et al.] // Phys. Solid State. - 2002. - Vol. 44, Is. 7. - P. 1350-1354, DOI 10.1134/1.1494635. - Cited References: 17 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
COLOSSAL MAGNETORESISTANCE
   MAGNETIC-RESONANCE
   DOPED MANGANITES
   LA1-XCAXMNO3
   SEPARATION
   TRANSITION
   RELAXATION
   EPR
Аннотация: Two phases, paramagnetic and ferromagnetic, were shown by the magnetic resonance method to coexist below the temperature T-C in La0.7Pb0.3MnO3 single crystals exhibiting colossal magnetoresistance. The magnetic resonance spectra were studied in the frequency range 10-78 GHz. The specific features in the behavior of the spectral parameters were observed to be the strongest at the temperatures corresponding to the maximum magnetoresistance in the crystals. The concentration ratios of the paramagnetic and ferromagnetic phases in the samples were found to be sensitive to variations in temperature and external magnetic field. This behavior suggests realization of the electronic phase separation mechanism in the system under study. (C) 2002 MAIK "Nauka/Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Volkov, N. V.; Волков, Никита Валентинович; Petrakovskii, G. A.; Петраковский, Герман Антонович; Vasil'ev, V. N.; Sablina, K. A.; Саблина, Клара Александровна
}
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