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Zamkova, N. G.
Effect of Sr2+ Ion Substitution with Trivalent Ions (Sc3+, In3+, La3+, Bi3+) on Its Ferroelectric Instability in SrTiO3 / N. G. Zamkova, V. S. Zhandun, V. I. Zinenko // Phys. Solid State. - 2011. - Vol. 53, Is. 11. - P. 2290-2299, DOI 10.1134/S1063783411110345. - Cited References: 14. - This study was supported by the Russian Foundation for Basic Research (project no. 09-02-00067), the Federal Program of Support for Leading Scientific Schools (project no. NSh-4645.2010.2). . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
BEHAVIOR
RELAXOR
Аннотация: The vibration frequencies of unstable ferroelectric and antiferrodistortion modes and the dependences of the energy on the ion displacement amplitude have been calculated within the generalized Gordon-Kim model for distortions along eigenvectors of these modes in the mixed compounds Sr(1-x)A(x)Ti(1-x/4)square O-x/4(3) and Sr(1-y)A(2y/3)square y/3TiO3 (A = Sc3+, In3+, La3+, Bi3+; square is the vacancy). To compensate an excess positive charge, vacancies are introduced into the Ti4+ or Sr2+ site. Calculations have been performed in the "average" crystal approximation for impurity concentrations of 0.25 and 0.50. To this end, a set of 40 atomic superlattices with various orderings of heterovalent ions Sr2+ and impurity A(3+) has been considered. It has been found that each impurity type, independently of charge balance, induces ferroelectric instabilities in doped compounds. In the case of doping with In3+ and La3+ for concentration x = 0.25, the possibility of rotating the polarization vector has been shown.

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Держатели документа:
[Zamkova, N. G.
Zhandun, V. S.
Zinenko, V. I.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Science, Akademgorodok 50, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zhandun, V. S.; Жандун, Вячеслав Сергеевич; Zinenko, V. I.; Зиненко, Виктор Иванович; Замкова, Наталья Геннадьевна
}
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Zhandun, V. S.
Lattice dynamics and the ferroelectric phase transition in ordered Pb-2 B'BaEuro(3)O(6) (B' = Ga, In, Lu; BaEuro(3) = Nb, Ta) solid solutions / V. S. Zhandun, N. G. Zamkova, V. I. Zinenko // Phys. Solid State. - 2010. - Vol. 52, Is. 2. - P. 357-363, DOI 10.1134/S1063783410020228. - Cited References: 19. - This study is supported by the Russian Foundation for Basic Research (project no. 09-02-00067) and the Council on Grants from the President of the Russian Federation for Support of the Leading Scientific Schools (grant no. NSh-4137.2006.2). . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
PEROVSKITES
   CRYSTALS
   DISORDER
   RELAXOR
   BATIO3
   PBTIO3
Аннотация: The lattice vibration spectrum, rf permittivity, and dynamic Born charges have been calculated for ordered Pb-2 B'BaEuro(3)O(3) (B'=Ga, In, Lu; BaEuro(3)=Nb, Ta) solid solutions in terms of the generalized Gordon-Kim model. It has been shown that all compounds exhibit a ferroelectric instability and that the frequencies of "soft" ferroelectric modes are close in magnitude. The ferroelectric phase-transition temperatures and the spontaneous polarization in the ferroelectric phase of the solid solutions under consideration have been calculated by the Monte Carlo method using the model Hamiltonian in the local mode approximation. The transition temperature is found to increase with increasing atomic number of the B' ion.

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Держатели документа:
[Zhandun, V. S.
Zamkova, N. G.
Zinenko, V. I.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zamkova, N. G.; Замкова, Наталья Геннадьевна; Zinenko, V. I.; Зиненко, Виктор Иванович; Жандун, Вячеслав Сергеевич
}
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Zhandun, V. S.
Lattice dynamics, ferroelectric and antiferroeelctric instabilities, and the ferroelectric phase transition in disordered PbB(1/2)' B(1/2)'' O(3) (B ' = Ga, In, Lu; B '' = Nb, Ta) solid solutions / V. S. Zhandun, N. G. Zamkova, V. I. Zinenko // J. Exp. Theor. Phys. - 2008. - Vol. 106, Is. 6. - P. 1109-1117, DOI 10.1134/S1063776108060101. - Cited References: 29 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
STATISTICAL-MECHANICS
   PEROVSKITES
   CRYSTALS
   ORDER
   RELAXOR
   BATIO3
   PBTIO3
Кл.слова (ненормированные):
Crystal lattices -- Ferroelectricity -- Lattice vibrations -- Solids -- Ferroelectric (barium strontium titanate) -- Ferroelectric phase transitions -- Lattice (CO) -- Lattice dynamics -- Vibration spectrum -- Ferroelectric materials
Аннотация: The lattice vibration spectra, rf permittivity, and dynamic Born charges of disordered PbB(1/2)'B(1/2)'' O(3) (B' = Ga, In, Lu; B '' = Nb, Ta) solid solutions are calculated in terms of the generalized Gordon-Kim model. All the compounds are found to have soft modes related to the center (Gamma(15)) and boundary point R (R(15)) of the Brillouin zone; the frequencies of these modes are close. The ferroelectric phase transition temperatures and the spontaneous polarization in the ferroelectric phase are calculated for the solid solutions using a model Hamiltonian in the local mode approximation and the Monte Carlo method. These temperatures for the tantalum compounds are found to be higher than for the niobium compounds, and temperature t(s) increases with the atomic number of ion B'. A model where the antiferroelectric state is related to the condensation of modes Gamma(15) and R(15) is proposed. It is found that, for all compounds except for PbSc(1/2)Nb(1/2)O(3) and PbSc(1/2)Ta(1/2)O(3), the ferroelectric phase, which is only related to the condensation of mode R(15), and the antiferroelectric phase have similar energies. In PbIn(1/2)Ta(1/2)O(3), the antiferroelectric phase turns out to be energetically favorable.

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Держатели документа:
[Zhandun, V. S.
Zamkova, N. G.
Zinenko, V. I.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zamkova, N. G.; Замкова, Наталья Геннадьевна; Zinenko, V. I.; Зиненко, Виктор Иванович; Жандун, Вячеслав Сергеевич
}
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Temperature dependence of the spontaneous polarization, acoustic and strain anomalies in strontium barium niobate crystals of different chemical compositions probed by the second harmonic generation technique / A. M. Pugachev, I. V. Zaytseva, V. K. Malinovsky [et al.] // Ferroelectrics. - 2020. - Vol. 560, Is. 1. - P. 54-60, DOI 10.1080/00150193.2020.1722883. - Cited References: 19. - This work was supported by the Russian Foundation for Basic Research, projects no. 18-02-00399 and 19-42-543-016 and State assignment No AAAA-A17-117052410033-9. . - ISSN 0015-0193. - ISSN 1563-5112

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
SINGLE-CRYSTALS
RELAXOR
GROWTH
Кл.слова (ненормированные):
SBN-x crystals -- polar regions -- ferroelectric phase transition -- second harmonic generation -- Brillouin spectroscopy
Аннотация: In SrxBa1-xNb2O6 crystals (x = 0.33, 0.5, 0.61, and 0.75), temperature dependences of spontaneous polarization, strain, elastic modules, and second harmonic generation (SHG) signal are compared. It is revealed that SHG describes the temperature dependences of dipole moments in polar nanoregions in paraelectric phase. In the vicinity of the phase transition in paraelectric phase, SHG reflects the temperature behavior of relatively large and long-lived polar asymmetric regions as indicated by the presence of the intermediate temperature range on the temperature dependence of this nonlinear response.

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Держатели документа:
Russian Acad Sci, Inst Automat & Electrometry, Novosibirsk, Russia.
Kirensky Inst Phys Fed Res Ctr KSC SB RAS, Krasnoyarsk, Russia.
Siberian Fed Univ, Inst Engn Phys & Radioelect, Krasnoyarsk, Russia.
Russian Acad Sci, Prokhorov Gen Phys Inst, Moscow, Russia.

Доп.точки доступа:
Pugachev, A. M.; Zaytseva, I., V; Malinovsky, V. K.; Surovtsev, N., V; Gorev, M. V.; Горев, Михаил Васильевич; Ivleva, L. I.; Lykov, P. A.; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [18-02-00399, 19-42-543-016, AAAA-A17-117052410033-9]
}
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