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Local structure of disordered PbSc1/2Nb1/2O3 in the region of the diffuse tetragonal phase-rhombohedral phase transition / I. P. Aleksandrova [et al.] // Phys. Solid State. - 2012. - Vol. 54, Is. 2. - P. 316-323, DOI 10.1134/S1063783412020047. - Cited References: 16. - This study was supported by the Council on Grants from the President of the Russian Federation for Support of the Leading Scientific Schools of the Russian Federation (grant no. NSh-4645.2010.2). . - ISSN 1063-7834

РУБ Physics + Condensed Matter
Рубрики:
Neutron-diffraction
   Order
   BaTiO3
   PbNiO3
   NMR
Аннотация: The local structure of the ferroelectric-relaxor PbSc1/2Nb1/2O3 in the temperature range from 550 to 220 K has been investigated using 45Sc nuclear magnetic resonance. It has been found that, in the paraelectric phase at temperatures below 550 K, the crystal consists of regions of an ordered elpasolite structure and inclusions of the disordered tetragonal perovskite phase with displacements along directions of the [001] type. The relative weight of the tetragonal structure in the region of the paraelectric phase is approximately equal to 0.28. Below the temperature of the phase transition from the disordered modification to the polar phase, the relative weight of the tetragonal phase decreases with decreasing temperature. The tetragonal structure is replaced by the trigonal polar structure. In a wide temperature range (∼50 K), there exists a heterophase structure that is characteristic of relaxors. Note that the correlation length of displacements in the tetragonal phase should be very small to explain the absence of indications of the existence of this phase in the diffraction data.

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Публикация на русском языке Локальная структура разупорядоченного PbSc[1/2]Nb[1/2]O[3] в области размытого перехода тетрагональная фаза - тригональная фаза [Текст] / И. П. Александрова [и др.] // Физ. тверд. тела : Физико-технический институт им. А.Ф.Иоффе РАН, 2012. - Т. 54 Вып. 2. - С. 298-304

Доп.точки доступа:
Aleksandrova, I. P.; Александрова, Инга Петровна; Sukhovsky, A. A.; Суховский, Андрей Андреевич; Ivanov, Y. N.; Иванов, Юрий Николаевич; Raevsky, I. P.; Раевский И.П.
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Specific features of magnetic ordering in the SmFeGe2O7 compound / T. V. Drokina [et al.] // Phys. Solid State. - 2014. - Vol. 56, Is. 6. - P. 1131-1136, DOI 10.1134/S1063783414060122. - Cited References: 10 . - ISSN 1063-7834. - ISSN 1090-6460

РУБ Physics, Condensed Matter
Рубрики:
NEUTRON-DIFFRACTION
   PR
   FERGE2O7
   R=LA
Аннотация: The results of the experimental investigation of the magnetic properties of the SmFeGe2O7 compound have been presented. It has been found that the temperature dependence of the susceptibility exhibits two features that coincide with the anomalies in the temperature dependence of the specific heat and indicate magnetic phase transitions in SmFeGe2O7. The external magnetic field induces a magnetic transition, the critical field of which depends on the temperature.

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Публикация на русском языке Особенности магнитного упорядочения в соединении SmFeGe2O7 [Текст] / Т. В. Дрокина [и др.] // Физ. тверд. тела : ФТИ РАН, 2014. - Т. 56 Вып. 6. - С. 1088-1092

Держатели документа:
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Drokina, T. V.; Дрокина, Тамара Васильевна; Petrakovskii, G. A.; Петраковский, Герман Антонович; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Molokeev, M. S.; Молокеев, Максим Сергеевич
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    Reconstructive phase transition in (NH4)3TiF7 accompanied by the ordering of TiF6 octahedra / M. S. Molokeev [et al.] // Acta Crystallogr. B. - 2014. - Vol. 70. - P. 924-931, DOI 10.1107/S2052520614021192. - This study was supported by Russian Fund of Basic Research, project No. 12-02-00056 a . - ISSN 0108-7681. - ISSN 1600-5740
   Перевод заглавия: Реконструктивный фазовый переход в (NH4)3TiF7, сопровождающийся упорядочением октаэдров TiF6

РУБ Crystallography
Рубрики:
CRYSTAL-STRUCTURE
   NEUTRON-DIFFRACTION
   POWDER DIFFRACTION
   FLUORIDES
   DISORDER
   MECHANISM
   PATHWAYS
   COMPLEX
   LI3THF7
   ALPHA
Кл.слова (ненормированные):
reconstructive phase transition -- ammonium heptafluorotitanate -- order-disorder transition
Аннотация: An unusual phase transition P4/mnc →Pa3 has been detected after cooling the (NH4)3TiF7 compound. Some TiF6 octahedra, which are disordered in the room-temperature tetragonal structure, become ordered in the low-temperature cubic phase due to the disappearance of the fourfold axis. Other TiF6 octahedra undergo large rotations resulting in huge displacements of the F atoms by 1.5-1.8 Å that implies a reconstructive phase transition. It was supposed that phases P4/mbm and Pm3m could be a high-temperature phase and a parent phase, respectively, in (NH4)3TiF7. Therefore, the sequence of phase transitions can be written as Pm3m → P4/bm → P4/mnc → Pa3. The interrelation between (NH4)3TiF7, (NH4)3GeF7 and (NH4)3PbF7 is found, which allows us to suppose phase transitions in relative compounds.

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Держатели документа:
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
Siberian State Univ, Inst Engn Phys & Radioelect, Krasnoyarsk 660074, Russia
Inst Chem, Vladivostok 660022, Russia

Доп.точки доступа:
Molokeev, M. S.; Молокеев, Максим Сергеевич; Misjul, S. V.; Мисюль, Сергей Валентинович; Flerov, I. N.; Флёров, Игорь Николаевич; Laptash, N. M.
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    Ferroelastic phase transitions in fluorides with cryolite and elpasolite structures / I. N. Flerov [et al.] // Crystallogr. Rep. - 2004. - Vol. 49, Is. 1. - P. 100-107, DOI 10.1134/1.1643969. - Cited References: 43 . - ISSN 1063-7745
Рубрики:
NUCLEAR MAGNETIC-RESONANCE
   THERMODYNAMIC PROPERTIES
   RB2KMIIIF6 ELPASOLITES
   NEUTRON-DIFFRACTION
   CRYSTALS
   PEROVSKITES
   DIAGRAM
   SC
   RB2KGAXSC1-XF6
   SCATTERING
Аннотация: The ferroelastic phase transitions are investigated in several series of fluoride crystals belonging to the elpasolite and cryolite families (space group Fm (3) over barm) with the general formula A(2)BB'F-6. The influence of the size and shape of cations and anions on the entropy and the mechanism of structural distortions is discussed. (C) 2004 MAIK "Nauka/Interperiodica".

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Публикация на русском языке Сегнетоэластические фазовые переходы во фторидах со структурой криолита и эльпасолита [Текст] / И. Н. Флеров [и др.] // Кристаллография. - 2004. - Т. 49 Вып. 1. - С. 107-114

Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Siberian Div, Krasnoyarsk 660036, Russia
Inst Chim Mat Condensee Bordeaux, F-33608 Pessac, France
ИФ СО РАН

Доп.точки доступа:
Flerov, I. N.; Флёров, Игорь Николаевич; Gorev, M. V.; Горев, Михаил Васильевич; Aleksandrov, K. S.; Александров, Кирилл Сергеевич; Tressaud, A.; Fokina, V. D.; Фокина, Валентина Дмитриевна
}
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Makarova, I. P.
Structure and twinning of RbLiCrO4 crystals / I. P. Makarova, I. A. Verin, K. S. Aleksandrov // Acta Crystallogr. B. - 1993. - Vol. 49. - P. 19-28, DOI 10.1107/S0108768192006141. - Cited References: 14 . - ISSN 0108-7681

РУБ Crystallography
Рубрики:
LITHIUM POTASSIUM-SULFATE
   NEUTRON-DIFFRACTION
   THERMAL VIBRATIONS
   KLISO4
   PROGRAM
   LIKSO4
Аннотация: The crystal structures of the G3 (space group P31c) and G2 (space group P6(3)) phases of RbLiCrO4 have been determined from X-ray diffraction data (Mo Kalpha radiation) at 293, 428, 493 and 523 K (G3 phase) and 553 and 583 K (G2 phase). The RbLiCrO4 crystals exhibit twinning by merohedry with twin laws in the G3 phase: 2 parallel-to [001], m perpendicular-to [001], 1BAR; in the G2 phase: m parallel-to [001], 2 perpendicular-to [001], 1BAR. The analysis of diffraction intensities and influence of anomalous scattering on them provided the unambiguous determination of the twin laws for all the specimens investigated. The structure has been refined using the approximation of the anharmonic thermal vibrations of atoms.

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Держатели документа:
ACAD SCI,INST PHYS,SIBERIAN DIV,KRASNOYARSK 660036,RUSSIA
ИФ СО РАН

Доп.точки доступа:
Verin, I. A.; Aleksandrov, K. S.; Александров, Кирилл Сергеевич
}
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    Electronic structure of β-RbSm(MoO4)2 and chemical bonding in molybdates / V. V. Atuchin [et al.] // Dalton Trans. - 2015. - Vol. 44, Is. 4. - P. 1805-1815, DOI 10.1039/c4dt03203a. - Cited References: 121. - VVA and ASA gratefully acknowledge the Ministry of Education and Science of the Russian Federation for financial support. ZL acknowledges the support by National Natural Science Foundation of China (11174297 and 11474292), the National Basic Research Project of China (2011CB922204), and Foundation of the Director of Technical Institute of Physics and Chemistry, CAS. The work was partially supported by RAS Project 24-29 and RFBR Grant 13-02-00825. . - ISSN 1477-9226. - ISSN 1477-9234
   Перевод заглавия: Электронная структура бета-RbSm(MoO4)2 и химическая связь в молибдатах

РУБ Chemistry, Inorganic & Nuclear
Рубрики:
RAY PHOTOELECTRON-SPECTROSCOPY
   CRYSTAL-STRUCTURE
   X-RAY
   NEUTRON-DIFFRACTION
   MAGNETIC-PROPERTIES
   PHASE-FORMATION
   CORE LEVELS
   2ND-HARMONIC GENERATION
   LUMINESCENCE PROPERTIES
   VIBRATIONAL PROPERTIES
Аннотация: Microcrystals of orthorhombic rubidium samarium molybdate, beta-RbSm(MoO4)(2), have been fabricated by solid state synthesis at T = 450 degrees C, 70 h, and at T = 600 degrees C, 150 h. The crystal structure has been refined by the Rietveld method in space group Pbcn with cell parameters a = 5.0984(2), b = 18.9742(6) and c = 8.0449(3) angstrom (R-B = 1.72%). Thermal properties of beta-RbSm(MoO4)(2) were traced by DSC over the temperature range of T = 20-965 degrees C, and the earlier reported β ↔ α phase transition at T similar to 860-910 degrees C was not verified. The electronic structure of beta-RbSm(MoO4) 2 was studied by employing theoretical calculations and X-ray photoelectron spectroscopy. It has been established that the O 2p-like states contribute mainly to the upper part of the valence band and occupy the valence band maximum, whereas the Mo 4d-like states contribute mainly to the lower part of the valence band. Chemical bonding effects have been analysed from the element core level binding energy data. In addition, it was found that the luminescence spectrum of beta-RbSm(MoO4)(2) is rather peculiar among the Sm3+ containing materials. The optical refractive index dispersion in beta-RbSm(MoO4)(2) was also predicted by the first-principles calculations.

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Держатели документа:
RAS, Inst Semicond Phys, Lab Opt Mat & Struct, SB, Novosibirsk 630090, Russia
Tomsk State Univ, Funct Elect Lab, Tomsk 634050, Russia
Novosibirsk State Univ, Lab Semicond & Dielectr Mat, Novosibirsk 630090, Russia
RAS, Kirensky Inst Phys, Lab Coherent Opt, SB, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660041, Russia
RAS, Baikal Inst Nat Management, Lab Oxide Syst, SB, Ulan Ude 670047, Russia
Gen Res Inst Nonferrous Met, Beijing 100088, Peoples R China
RAS, Inst Semicond Phys, Lab Nanodiagnost & Nanolithog, SB, Novosibirsk 630090 90, Russia
RAS, Inst Semicond Phys, Lab Phys Bases Integrated Microelect, SB, Novosibirsk 630090 90, Russia
RAS, Kirensky Inst Phys, Lab Crystal Phys, SB, Krasnoyarsk 660036, Russia
RAS, Kirensky Inst Phys, Lab Mol Spect, SB, Krasnoyarsk 660036, Russia
Chinese Acad Sci, Tech Inst Phys & Chem, Beijing 100190, Peoples R China

Доп.точки доступа:
Atuchin, V. V.; Aleksandrovsky, A. S.; Александровский, Александр Сергеевич; Chimitova, O. D.; Diao, C. P.; Gavrilova, T. A.; Kesler, V. G.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Krylov, A. S.; Крылов, Александр Сергеевич; Bazarov, B. G.; Bazarova, J. G.; Lin, Z. S.; Ministry of Education and Science of the Russian Federation; National Natural Science Foundation of China [11174297, 11474292]; National Basic Research Project of China [2011CB922204]; Foundation of the Director of Technical Institute of Physics and Chemistry, CAS; RAS [24-29]; RFBR [13-02-00825]
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Single magnetic chirality in the magnetoelectric NdFe3((BO3)-B-11)(4) / M. . Janoschek [et al.] // Phys. Rev. B. - 2010. - Vol. 81, Is. 9. - Ст. 94429, DOI 10.1103/PhysRevB.81.094429. - Cited References: 55 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
NEUTRON-DIFFRACTION
   PHASE-TRANSITIONS
   SLOW-NEUTRONS
   CRYSTAL
   NDFE3(BO3)(4)
   EXTINCTION
   NUCLEAR
   ORDER
   MNSI
   ANTIFERROMAGNETS
Аннотация: We have performed an extensive study of single crystals of the magnetoelectric NdFe3 ((BO3)-B-11)(4) by means of a combination of single-crystal neutron diffraction and spherical neutron polarimetry. Our investigation did not detect significant deviations at low temperatures from space group R32 concerning the chemical structure. With respect to magnetic ordering our combined results demonstrate that in the commensurate magnetic phase below T-N approximate to 30 K all three magnetic Fe moments and the magnetic Nd moment are aligned ferromagnetically in the basal hexagonal plane but align antiferromagnetically between adjacent planes. The phase transition to the low-temperature incommensurate (IC) magnetic structure observed at T-IC approximate to 13.5 K appears to be continuous. By means of polarized neutron studies it could be shown that in the incommensurate magnetic phase the magnetic structure of NdFe3((BO3)-B-11)(4) is transformed into a long-period antiferromagnetic helix with single chirality. Close to the commensurate-incommensurate phase transition third-order harmonics were observed, which in addition indicate the formation of magnetic solitons.

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Держатели документа:
[Janoschek, M.
Fischer, P.
Schefer, J.
Roessli, B.
Pomjakushin, V.] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland
[Janoschek, M.
Fischer, P.
Schefer, J.
Roessli, B.
Pomjakushin, V.] ETH, CH-5232 Villigen, Switzerland
[Janoschek, M.] Tech Univ Munich, Phys Dept E21, D-85748 Garching, Germany
[Meven, M.] Tech Univ Munich, Forsch Neutronenquelle Heinz Maier Leibnitz FRM 2, D-85748 Garching, Germany
[Petricek, V.] ASCR, Vvi, Inst Phys, Prague 18221 8, Czech Republic
[Petrakovskii, G.
Bezmaternikh, L.] RAS, SB, Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
Laboratory for Neutron Scattering, Paul Scherrer Institut and ETH Zurich, CH-5232 Villigen PSI, Switzerland
Physik Department E21, Technische Universitat Munchen, D-85748 Garching, Germany
Department of Physics, University of California, San Diego, San Diego, CA 92093-0354, United States
Forschungsneutronenquelle Heinz Maier-Leibnitz (FRM II), Technische Universitat Munchen, D-85748 Garching, Germany
Institute of Physics, ASCR, V.v.i, Na Slovance 2, 182 21 Praha 8, Czech Republic
Institute of Physics, SB RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Janoschek, M.; Fischer, P.; Schefer, J.; Roessli, B.; Pomjakushin, V.; Meven, M.; Petricek, V.; Petrakovskii, G. A.; Петраковский, Герман Антонович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич
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Zinenko, V. I.
Lattice dynamics and the phase transition from the cubic phase to the tetragonal phase in the LaMnO3 crystal within the polarizable-ion model / V. I. Zinenko, M. S. Pavlovskii // Phys. Solid State. - 2007. - Vol. 49, Is. 9. - P. 1749-1758, DOI 10.1134/S1063783407090235. - Cited References: 23 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
NEUTRON-DIFFRACTION
   PEROVSKITES
   MANGANITES
   PHONONS
Аннотация: The paper reports on the results of ab initio calculations of the static and dynamic properties of the LaMnO3 crystal with a perovskite structure in the cubic, rhombohedral, and orthorhombic phases. The calculations are performed within the ionic crystal model, which takes into account the deformability and polarizability of the ions. It is revealed that the spectrum of lattice vibrations in the cubic phase contains unstable vibrational modes, which occupy the phase space in the entire Brillouin zone. The eigenvectors of the softest mode at the boundary point R of the Brillouin zone are associated with the displacements of the oxygen ions and correspond to the "rotation" of the MnO6 octahedron. The condensation of one, two, and three components of this mode leads to the tetragonal, orthorhombic, and rhombohedral distortions of the structure. The structural phase transition is described in terms of the local mode approximation with the use of the double perovskite unit cell, in which the MnO6 octahedron is explicitly separated. The parameters of the model Hamiltonian are determined. The static properties are investigated by the Monte Carlo method. The calculated temperature of the phase transition from the cubic phase (9800 K) is considerably higher than the melting temperature of the crystal under investigation. The calculated frequencies of long-wavelength lattice vibrations in the experimentally observed orthorhombic and rhombohedral phases are in reasonable agreement with experimental data.

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Держатели документа:
Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Pavlovskii, M. S.; Павловский, Максим Сергеевич; Зиненко, Виктор Иванович
}
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Aplesnin, S. S.
Effect of bond fluctuations on the transport properties of manganites and nickelates / S. S. Aplesnin // J. Exp. Theor. Phys. - 2007. - Vol. 104, Is. 5. - P. 766-774, DOI 10.1134/S1063776107050111. - Cited References: 26 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
NEUTRON-DIFFRACTION
   CHARGE DISPROPORTIONATION
   ELECTRONIC-STRUCTURE
   MAGNETIC ORDER
   TRANSITIONS
   PEROVSKITES
   PRNIO3
   GAP
Кл.слова (ненормированные):
Crystal structure -- Manganites -- Optimization -- Thermal conductivity -- Thermal effects -- Bond fluctuations -- Nickelates -- Orthorhombic crystal structure -- Nickel compounds
Аннотация: For the manganites RMnO(3) (R = La, Pr, Nd), a mechanism is proposed to explain the anomalous temperature dependences of the kinetic coefficients, resistivity, and thermoelectric power during the transition from the pseudocubic O to the orthorhombic O' crystal structure. The contributions of the bending and stretching modes of the octahedron to the formation of thermal-conductivity maxima and to the deviation from the linear dependence of ln(rho/T) on 1/T at low temperatures have been estimated. In nickelates, the metal-insulator transition is caused by lattice-polaron pinning by the stretching mode of the octahedron, and the low-temperature anomaly of the thermal conductivity is related to electron scattering by the bending mode of the octahedron.

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Reshetnev Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russian Federation
Reshetnev Siberian State Aerospace University, Krasnoyarsk, 660014, Russian Federation

Доп.точки доступа:
Аплеснин, Сергей Степанович
}
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10.

Structural, electronic and vibrational properties of LaF3 according to density functional theory and Raman spectroscopy / A. S. Oreshonkov [et al.] // J. Phys.: Condens. Matter. - 2018. - Vol. 30, Is. 25. - Ст. 255901, DOI 10.1088/1361-648X/aac452. - Cited References: 39. - The reported study was funded by RFBR according to the research project No. 17-52-53031 and 16-02-00102. It was partially supported by the Ministry of Education and Science of the Russian Federation and the 'Krasnoyarsky regional fund of scientific support and scientific-technical activity'. The computations were performed using facilities of the Computational Centre of the Research Park of St. Petersburg State University. . - ISSN 0953-8984. - ISSN 1361-648X

РУБ Physics, Condensed Matter
Рубрики:
CRYSTAL-STRUCTURE
   NEUTRON-DIFFRACTION
   NANOPARTICLES
   CONDUCTIVITY
Кл.слова (ненормированные):
LaF3 -- tysonite structure -- DFT -- electronic structure -- lattice vibrations -- Raman spectroscopy
Аннотация: Crystal structure of LaF3 single crystal is refined in tysonite-type trigonal unit cell P c1 using density functional theory calculations and Raman spectroscopy. It is shown that trigonal structure with P c1 space group is more energy-efficient than hexagonal structure with space group P63 cm. Simulated Raman spectra obtained using LDA approximation is in much better agreement with experimental data than that obtained with PBE and PBEsol functionals of GGA. The calculated frequency value of silent mode B 2 in case of hexagonal structure P63 cm was found to be imaginary (unstable mode), thus the energy surface obtains negative curvature with respect to the corresponding normal coordinates of the mode which leads to instability of the hexagonal structure in harmonic approximation. The A 1g line at 214 cm−1 in Raman spectra of LaF3 related to the translation of F2 ions along c axis can be connected with F2 ionic conductivity.

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Держатели документа:
RAS, SB, KSC, Fed Res Ctr,Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660079, Russia.
Ioffe Inst, St Petersburg 194021, Russia.

Доп.точки доступа:
Oreshonkov, A. S.; Орешонков, Александр Сергеевич; Roginskii, E. M.; Krylov, A. S.; Крылов, Александр Сергеевич; Ershov, A. A.; Ершов, Александр Андреевич; Voronov, V. N.; Воронов, Владимир Николаевич; RFBR [17-52-53031, 16-02-00102]; Ministry of Education and Science of the Russian Federation; Krasnoyarsky regional fund of scientific support and scientific-technical activity
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11.

Dipole glass in chromium-substituted bismuth pyrostannate / S. S. Aplesnin [et al.] // Mater. Res. Express. - 2018. - Vol. 5, Is. 11. - Ст. 115202, DOI 10.1088/2053-1591/aaddd9. - Cited References: 33. - This study was supported by the Russian Foundation for Basic Research project N 18-52-00009 Bel_a, No 18-32-00079 mol_a, the state order No 3.5743.2017/6.7. . - ISSN 2053-1591

РУБ Materials Science, Multidisciplinary
Рубрики:
BI4TI3O12 THIN-FILMS
   NEUTRON-DIFFRACTION
   RAMAN-SPECTROSCOPY
   BI2SN2O7
Кл.слова (ненормированные):
dipole glass -- permittivity -- polarization -- Raman scattering spectra -- structural transition
Аннотация: To establish the existence of dipole glass in the chromium-substituted bismuth pyrostannate solid solutions, the frequency and temperature dependences of the permittivity have been measured in the temperature range of 300–750 K. The field and dynamic dependences of polarization in the temperature range of 80–550 K have been determined. Using the Raman scattering spectra, the absence of inversion center has been established. The maximum of electrical resistance has been found in the vicinity of the dipole moment freezing point. The carrier type has been determined from the thermopower data. The polarization relaxation is shown to be nonexponential. The experimental data are explained within the model of dipole glass in the α- phase and the model of charged crystalline domain walls with the electron-polarization relaxation mechanism above the α–β structural transition.

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Держатели документа:
SB RAS, Kirensky Inst Phys, Fed Res Ctr KSC, Krasnoyarsk 660036, Russia.
Reshetnev Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Inst Solid State Phys, LV-1063 Riga, Latvia.

Доп.точки доступа:
Aplesnin, S. S.; Аплеснин, Сергей Степанович; Udod, L. V.; Удод, Любовь Викторовна; Sitnikov, M. N.; Kretinin, V. V.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Mironova-Ulmane, N.; Russian Foundation for Basic Research [N 18-52-00009 Bel_a, 18-32-00079 mol_a, 3.5743.2017/6.7]
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