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1.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Kolkov M. I., Balaev A. D., Freydman A. L., Vasiliev A. D., Balaev D. A.
Заглавие : Comparative study of the magnetic phase diagrams and spin-flop-driven magnetodielectric responses of the pure and Mn3+-doped Pb2Fe2Ge2O9 single crystals
Место публикации : J. Magn. Magn. Mater. - 2021. - Vol. 534. - Ст.168023. - ISSN 03048853 (ISSN), DOI 10.1016/j.jmmm.2021.168023
Примечания : Cited References: 21. - This study was supported by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory, and the Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project no. 18-42-240008 “Effect of the Magnetic Structure on the Magnetodielectric Properties of Oxide Crystals Containing Stereoactive Pb 2+ and Bi 3+ Ions”
Аннотация: The Pb2Fe2-xMnxGe2O9 (x = 0.43) orthorhombic antiferromagnet single crystals have been synthesized by a modified pseudo-flux technique and their magnetic and magnetodielectric properties have been investigated. It has been established that partial substitution of highly anisotropic Mn3+ ions for iron ones significantly affects the magnetic structure of the crystal. Under magnetization of the crystal along the rhombic b and c axes, magnetization jumps have been detected, which are indicative of the occurrence of orientational transitions identified as first-order ones. No weak ferromagnetism characteristic of the pure crystal in the rhombic a axis direction has been detected. The field dependences of the magnetization for the pure and Mn-doped crystals have been analyzed using the thermodynamic potential that takes into account the crystal symmetry. It has been shown that, in the Mn-substituted crystal, the antiferromagnetic vector in the ground state is parallel to the rhombic b axis; in this state, weak ferromagnetism has not been observed. Under magnetization along the b axis, a conventional spin-flop transition occurs. The orientational transition under magnetization along the c axis has been attributed to the reorientation of the antiferromagnetic vector relative to the a axis with the simultaneous occurrence of a weak ferromagnetic moment along the c axis. Magnetic phase diagrams of the Mn-doped crystal for the magnetic fields H||b and H||c have been built. In the Mn-doped crystal, at E||c and H||c, the orientational transition-induced magnetodielectric response jump has been detected, which is higher than the jumps observed for the undoped crystal by a factor of 3. The magnetodielectric properties of the pure and Mn-doped crystals have been analyzed using their magnetic phase diagrams.
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2.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Matveeva A. N., Zobkalo I. A., Meven M., Freidman A. L., Semenov S. V., Terentjev K. Yu., Pavlovskiy N. S., Kolkov M. I., Shaykhutdinov K. A., Hutanu V.
Заглавие : Complex interplay between 3d and 4f magnetic systems in multiferroic DyMnO3
Место публикации : J. Magn. Magn. Mater. - 2023. - Vol. 569. - Ст.170415. - ISSN 03048853 (ISSN), DOI 10.1016/j.jmmm.2023.170415
Примечания : Cited References: 28. - The authors are grateful to S.V. Gavrilov for the technical assistance. This work was supported by the Russian Foundation for Basic Research grant # 19-52-12047, and DFG grant # SA 3688/1-1, also by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science to the research projects number 18-42-243024 and 20-42-243008. The neutron data were obtained at the instrument HEiDi operated jointly by RWTH Aachen University and Jülich Centre for Neutron Science within JARA cooperation
Аннотация: Structural and magnetic properties of single crystals of DyMnO3 were investigated by neutron diffraction in order to study the peculiarities of 3d-4f interactions in this compound. Precise magnetic order and its detailed temperature evolution were determined using single crystal neutron diffraction. Elliptical cycloid on manganese subsystem below TCh = 19 K was confirmed, with temperature decrease the elipticity of the Mn magnetic structure reduces significantly, creating almost circular cycloid. Temperature evolution of the magnetic structure demonstrate specific hysteretic behavior. The results show a complex interplay between transition metal and rare earth magnetic sublattices leading to so-called “Mn- controlled” and “Dy- controlled” magnetic states. The strong and complicate 3d-4f interaction leads to the unusual very slow magnetic structure relaxation.
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3.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Freydman A. L., Horoshiy I. N., Kolkov M. I., Terent'ev K. Yu.
Заглавие : Direct and inverse magnetoelectric effect in orthorhombic single crystals of Dy1−xHoxMnO3
Место публикации : Phys. Solid State. - 2022. - Vol. 64, Is. 14. - P.2347-2352. - ISSN 10637834 (ISSN), DOI 10.21883/PSS.2022.14.54338.185. - ISSN 10906460 (eISSN)
Примечания : Cited References: 17. - The study was done with financial support from the Russian Foundation for Basic Research, Government of Krasnoyarsk Territory and the Krasnoyarsk Regional Fund of Science within the scientific project No. 20-42-243008
Аннотация: In this work, the magnetoelectric response in a series of Dy1−xHoxMnO3 crystals with substitution x from 0 to 0.4 was investigated. The measurement results showed that, as x increases, a decrease in both the polarization Pa and the magnitude of the susceptibility of the inverse magnetoelectric effect αba is observed. In addition, the field Hb increases, at which the Pc → Pa transition is observed, and the temperature range of the existence of the magnetoelectric response decreases. Thus, an increase in the substitution x suppresses the magnetoelectric effect in this series of compounds. The measurement results also indirectly indicate the prolongation of the Pa state and, consequently, of the magnetic state with a cycloid lying in the ab-plane by an external electric field Ea.
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4.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Pankrats A. I., Sablina K. A., Balaev A. D., Eremin M., Kolkov M. I., Tugarinov V. I., Bovina A. F.
Заглавие : Ferromagnetism and strong magnetic anisotropy of the orthoborate PbMnBO4 single crystals
Коллективы : Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium, Институт физики им. Л.В. Киренского Сибирского отделения РАН
Место публикации : VI Euro-Asian Symposium "Trends in MAGnetism" (EASTMAG-2016): abstracts/ ed.: O. A. Maksimova, R. D. Ivantsov. - Krasnoyarsk: KIP RAS SB, 2016. - Ст.P1.25. - P.85. - ISBN 978-5-904603-06-9 (Шифр -478014040)
Примечания : References: 3. - This work is supported by the RFBR grant No. 16-02-00563
Ключевые слова (''Своб.индексиров.''): ferromagnet--resonance--single crystal
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5.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Sablina K. A., Eremin M., Balaev A. D., Kolkov M., Tugarinov V. I., Bovina A. F.
Заглавие : Ferromagnetism and strong magnetic anisotropy of the PbMnBO4 orthoborate single crystals
Место публикации : J. Magn. Magn. Mater.: Elsevier, 2016. - Vol. 414. - P.82-89. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2016.04.042
Примечания : Cited References: 20. - We acknowledge the assistance of A. Dubrovsky in magnetic measurements.This work was supported by the Russian Foundation for Basic Research, Projects nos. 13-02-00897 and 16-02-00563. MVE thanks for support the Russian Government Program of Competitive Growth of the Kazan Federal University, decision no. 930_p, May 22, 2015.
Предметные рубрики: PbMBO4 M
Resonance
Symmetry
Mn
Fe
Cr
Ключевые слова (''Своб.индексиров.''): strong ferromagnetic anisotropy--ferromagnetic resonance--exchange interactions
Аннотация: The PbMnBO4 orthoborate single crystals were first grown and their magnetic properties and ferromagnetic resonance were studied. It was found that the ferromagnetic state below the Curie temperature TC=31 K is characterized by the strong magnetic anisotropy. The significant effective anisotropy fields of PbMnBO4 determine the energy gap in the FMR spectrum, which is extraordinary large for ferromagnets (112 GHz at T=4.2 K). It was shown that the static Jahn-Teller effect characteristic of the Mn3+ ion leads to both the ferromagnetic ordering and the strong magnetic anisotropy in the crystal. In the strong external magnetic field the induced ferromagnetic ordering is retained in the crystal above the Curie temperature up to the temperatures multiply higher than TC. A weak anomaly of the dielectric permittivity was observed in PbMnBO4 at the Curie temperature at which the long-range ferromagnetic order is established. © 2016 Elsevier B.V. All rights reserved.
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6.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Pankrats A. I., Kolkov M. I., Shabanov A. V., Vasiliev A. D.
Заглавие : Formation the ferrimagnetic-like structure under partial subtitution in the crystal PbMn1?xFexBO4 (x?0.1)
Коллективы : Российская академия наук, Уральское отделение РАН, Институт физики металлов им. М. Н. Михеева Уральского отделения РАН, Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Российский фонд фундаментальных исследований, Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium
Место публикации : Euro-asian symposium "Trends in magnetism" (EASTMAG-2019): Book of abstracts/ чл. конс. ком.: S. G. Ovchinnikov, N. V. Volkov [et al.] ; чл. прогр. ком. D. M. Dzebisashvili [et al.]. - 2019. - Vol. 1. - Ст.B.P2. - P.167. - ISBN 978-5-9500855-7-4 (Шифр В33/E12-125657784)
Примечания : Cited References: 2. - The reported study was funded by RFBR and the Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project no. 18-42-240008 ”Effect of magnetic structure on the magnetodielectric properties of oxide crystals containing stereoactive ions Pb2+ and Bi3+”
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7.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Kolkov M. I., Balaev A. D., Shabanov A. V., Vasiliev A. D.
Заглавие : Forming a ferrimagnetic-like structure in the PbMn1−xFexBO4 (x ≈ 0.1) single crystal upon partial substitution
Место публикации : J. Magn. Magn. Mater. - 2020. - Vol. 497. - Ст.165997. - ISSN 03048853 (ISSN), DOI 10.1016/j.jmmm.2019.165997
Примечания : Cited References: 25. - The authors are grateful to S. Nikitin for help in the specific heat measurements in a magnetic field and S. Martynov for fruitful discussions. This study was funded by RFBR and the Government of Krasnoyarsk Territory , Krasnoyarsk Regional Fund of Science , to the research project no. 18-42-240008 “Effect of Magnetic Structure on the Magnetodielectric Properties of Oxide Crystals Containing Stereoactive Ions Pb 2+ and Bi 3+”.
Аннотация: The PbMn1−xFexBO4 (x ≈ 0.1) orthoborate single crystals have been grown for the first time by spontaneous crystallization and their magnetic and resonance properties and specific heat have been examined. It has been established that partial substitution of iron ions for manganese ones leads to an increase in the Curie temperature to 34.2 K from its value of 30.3 K in the unsubstituted crystal, enhances the magnetic anisotropy, and reduces the saturation magnetization. The magnetization drop is explained in the framework of the model of a ferrimagnetic-like structure, in which the magnetic moments of iron and manganese ions form ferromagnetic subsystems coupled by the antiferromagnetic exchange. It has been found that under magnetization along the rhombic b axis the magnetic moments switch stepwise to the magnetic field direction in a certain critical field. The spin-reorientation transition is the first-order one. This feature of the crystal magnetization does not allow the experimental ferromagnetic resonance frequency-field dependence for the rhombic b axis to be described using the calculation for a simple rhombic ferromagnet. It has been established that the increase in the magnetic anisotropy of the crystal upon substitution leads to an increase in the energy gap in the ferromagnetic resonance spectrum to 121.5 GHz at T = 4.2 K.
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8.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Balaev A. D., Skorobogatov S. A., Krasikov A. A., Kolkov M. I., Zharkov S. M., Zeer G. M., Pavlovskii M. S., Balaev D. A.
Заглавие : Inclined magnetic structures and magnetic phase diagrams for the Pb2Fe2−xMnxGe2O9 (x = 0.16) single crystal
Место публикации : J. Magn. Magn. Mater. - 2022. - Vol. 563. - Ст.170021. - ISSN 03048853 (ISSN), DOI 10.1016/j.jmmm.2022.170021
Примечания : Cited References: 24. - This study was supported by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory, and the Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project no. 20-42-2 40006 “Synthesis and Study of Pb 2+ and Bi 3+ -Containing Oxide Single Crystals with Partial Substitution in One of the Subsystems: Magnetic Structures and Magnetodielectric Effect”. The SEM and EDS studies were carried out at the Joint Scientific Center of the Siberian Federal University within the state assignment (#FSRZ-2020-0011) of the Ministry of Science and Higher Education of the Russian Federation
Аннотация: Single crystals of the Pb2Fe2?xMnxGe2O9 (x = 0.16) antiferromagnet have been grown. Using the specific heat measurements, a Neel temperature of TN = (42.0 ± 0.5) K for the synthesized crystals has been found. It has been shown using the magnetic measurements that, due to the competition between the magnetoanisotropic contributions of the iron and manganese subsystems in the crystals, near a temperature of Tc = 22 K, a spontaneous spin-reorientation transition occurs, the temperature of which in an applied magnetic field changes with the field value and orientation relative to the rhombic axes of the crystal. Based on the analysis of the temperature and field dependences of the magnetization obtained at different orientations of the magnetic field, it has been established that, below Tc, an inclined magnetic structure is formed in the crystal. The antiferromagnetic vector of the inclined structure rotates smoothly in the rhombic bc plane with increasing temperature from a direction close to the b axis at T = 4.2 K and tends to the rhombic c axis at T = Tc. The rotation of the antiferromagnetic vector occurs also at fixed temperatures T < Tc with increasing magnetic field. In the temperature range of Tc < T < TN, the antiferromagnetic vector is oriented along the rhombic c axis. Magnetic phase diagrams of states have been built for different magnetic field orientations relative to the rhombic axes of the crystal. The richest phase diagram is shown to correspond to the orientation H||c and contains, along with the above-listed states, one more inclined phase, in which the antiferromagnetic vector rotates toward the rhombic a axis direction with a change in temperature or magnetic field.
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9.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Freidman A. L., Semenov S. V., Kolkov M. I., Terent'ev K. Yu., Pavlovskiy N. S., Gokhfeld D. M., Shaykhutdinov K. A., Balaev D. A.
Заглавие : Inverse and direct magnetoelectric effects in orthorhombic DyMnO3 manganite single crystals
Коллективы : Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science [18-42-243024]
Место публикации : J. Appl. Phys. - 2020. - Vol. 128, Is. 9. - Ст.094102. - ISSN 0021-8979, DOI 10.1063/5.0006595. - ISSN 1089-7550(eISSN)
Примечания : Cited References: 27. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science to the research project "Research, synthesis and investigation of new oxide single crystals showing the interrelation of magnetic, magnetoelastic and magnetoelectric properties" (Project No. 18-42-243024). The measurements were performed in part on the equipment at the Krasnoyarsk Territorial Center for Collective Use, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences
Аннотация: Correlations between the direct and inverse magnetoelectric effects in orthorhombic DyMnO3 single crystals have been investigated. In the inverse magnetoelectric effect, the magnetic moment of the crystal appears to have a contribution that is sinusoidal oscillating in ac electric fields below the temperature TFE of ferroelectric phase transition. The first and the second harmonics of the inverse magnetoelectric effect are clearly detected. The magnetoelectric susceptibilities α and β, corresponding to first and second harmonics, are found to correlate with the derivative of polarization with respect to the magnetic field. The influence of the magnetic and electric regimes during cooling on magnetoelectric effects has also been studied. The maximum change in the magnetic moment of a sample under the action of electric fields is observed under the same (T, H) conditions as the rotation of the spontaneous polarization vector from the crystallographic c direction to the a axis in the magnetic field H || b.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Sablina K. A., Velikanov D. A., Bayukov O. A., Vorotynov A. M., Balaev A. D., Molokeev M. S., Kolkov M. I.
Заглавие : Magnetic and dielectric properties of PbFeBO4 and PbMnBO4 single crystals
Коллективы : Euro-Asian Symposium "Trends in MAGnetism": Nanomagnetism
Место публикации : Solid State Phenom.: Selected, peer reviewed papers/ ed.: S. G. Ovchinnikov, A. Samardak: Trans Tech Publications, 2014. - Vol. 215: Trends in Magnetism: Nanomagnetism (EASTMAG-2013). - P.372-377. - ISSN 978-303835054-5, DOI 10.4028/www.scientific.net/SSP.215.372. - ISSN 1662-9779
Примечания : Cited References: 3. - This investigation was supported by the Russian Foundation for Basic Research (RFBR) (Grant No.13-02-00897).
Ключевые слова (''Своб.индексиров.''): borate oxide--dielectric permittivity--magnetic susceptibility--single crystal--strong anisotropy
Аннотация: PbFeBO4 and PbMnBO4 single crystals were synthesized. The X-ray, magnetic, dielectric, Mossbauer, and resonance investigations of the crystals were fulfilled. It is established that single-crystal PbFeBO4 is an antiferromagnet with a Neel temperature TN =114 K, while PbMnBO4 is a ferromagnet with a Curie temperature TC = 31 K. Both single-crystal compounds have a strong anisotropy of the magnetic and dielectric properties. © (2014) Trans Tech Publications, Switzerland.
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11.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Pankrats A. I., Balaev D. A., Nikitin S. E., Freydman A. L., Krasikov A. A., Balaev A. D., Popkov S. I., Kolkov M. I.
Заглавие : Magnetic and thermodynamic properties and spin-flop-driven magnetodielectric response of the antiferromagnetic Pb2Fe2Ge2O9 single crystals
Коллективы : Российская академия наук, Уральское отделение РАН, Институт физики металлов им. М. Н. Михеева Уральского отделения РАН, Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Российский фонд фундаментальных исследований, Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium
Место публикации : Euro-asian symposium "Trends in magnetism" (EASTMAG-2019): Book of abstracts/ чл. конс. ком.: S. G. Ovchinnikov, N. V. Volkov [et al.] ; чл. прогр. ком. D. M. Dzebisashvili [et al.]. - 2019. - Vol. 2. - Ст.K.O3. - P.301-302. - ISBN 978-5-9500855-7-4 (Шифр В33/E12-125657784)
Примечания : Cited References: 4. - The study was funded by RFBR and the Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project no. 18-42-240008 ”Effect of magnetic structure on the magnetodielectric properties of oxide crystals containing stereoactive ions Pb2+ and Bi3+”
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Balaev D. A., Nikitin S. E., Freydman A. L., Krasikov A. A., Balaev A. D., Popkov S. I., Kolkov M. I.
Заглавие : Magnetic and thermodynamic properties and spin-flop-driven magnetodielectric response of the antiferromagnetic Pb2Fe2Ge2O9 single crystals
Коллективы : Russian Foundation for Basic Research [16-02-00563]; RFBR; Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science [18-42-240008]; International Max Planck Research School for Chemistry and Physics of Quantum Materials (IMPRS-CPQM)
Место публикации : J. Magn. Magn. Mater. - 2019. - Vol. 479. - P.114-120. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2019.02.026. - ISSN 1873-4766(eISSN)
Примечания : Cited References: 23. - This study was supported by the Russian Foundation for Basic Research, project no. 16-02-00563; the reported study was also funded by RFBR and the Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, to the research project no. 18-42-240008 "Effect of magnetic structure on the magnetodielectric properties of oxide crystals containing stereoactive ions Pb2+ and Bi3+". S.E.N. acknowledges the support of the International Max Planck Research School for Chemistry and Physics of Quantum Materials (IMPRS-CPQM).
Предметные рубрики: FERROMAGNETISM
TRANSITION
Аннотация: Orthorhombic Pb2Fe2Ge2O9 antiferromagnetic single crystals have been synthesized by a modified pseudo-flux technique and their magnetic, thermodynamic, and magnetodielectric properties have been investigated. It has been found that, below the Ned temperature (45.2 K), iron moments are arranged in a canted antiferromagnetic structure with a weak ferromagnetic moment parallel to the a axis. According to the specific heat measurement data, the T-N value remains invariable in applied magnetic fields of up to 50 kOe within the experimental accuracy. The magnetic entropy in the investigated crystals attains 2Rln(2S + 1) right above T-N, which is indicative of a purely magnetic nature of the transition. It has been shown that the weak ferromagnetic moment is induced by the interplay between the single-ion anisotropy and antisymmetric Dzyaloshinskii-Moriya exchange interaction, with the latter contribution being dominant. It has been established from the angular dependences of the magnetization in three orthorhombic planes that the symmetries of the magnetic and crystal structure are identical. The magnetodielectric properties of the Pb2Fe2Ge2O9 single crystals have been studied at different mutual orientations of the electric and magnetic fields. The most prominent anomalies have been observed in the vicinity of the spin-flop transition in a magnetic field applied along the c axis.
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13.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Pankrats A. I., Kolkov M. I., Popkov S. I., Sablina K. A., Balaev A. D., Miskiv A.
Заглавие : Magnetic order-disorder transition in the ferromagnet PbMnBO4 under the external magnetic field
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow International Symposium on Magnetism (MISM-2017): 1-7 July 2017 : book of abstracts. - 2017. - Ст.4PO-I1-45. - P.900 (Шифр 29916280)
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Matveeva A. N., Zobkalo I. A., Sazonov A., Freidman A. L., Semenov S. V., Kolkov M. I., Terentjev K. Yu., Pavlovskiy N. S., Shaykhutdinov K. A., Hutanu V.
Заглавие : Magnetic ordering and chirality in multiferroic Dy1-xHoxMnO3 (x = 0.2)
Место публикации : Phys. B: Condens. Matter. - 2023. - Vol. 658. - Ст.414821. - ISSN 09214526 (ISSN), DOI 10.1016/j.physb.2023.414821. - ISSN 18732135 (eISSN)
Примечания : Cited References: 41. - The authors are grateful to D.A. Balaev for fruitful discussions and crystal growth management. This work was supported by the Russian Foundation for Basic Research grant # 19-52-12047, and DFG grant # SA3688/1-1, also by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science to the research projects number 18-42-243024 and 20-42-243008. The neutron data were obtained at the instrument POLI operated jointly by RWTH Aachen University and Jülich Centre for Neutron Science within JARA cooperation
Аннотация: Effect of substitution Dy by Ho on the magneto-electric behavior of the compound Dy0.8Ho0.2MnO3 was investigated by the different methods of polarized and classical neutron diffraction and macroscopic methods. It is shown that substitution by Ho of 20% on the position of Dy do not change overall crystal symmetry of compound. It remains of Pbnm type down to the very low temperatures. Magnetic ordering, its temperature and field evolution was determined by the use of single crystal neutron diffraction and magnetization measurements. Chiral type of magnetic structure on Mn subsystem is confirmed below Tc ≈ 16 K. Using polarized neutron diffraction the 3-component character of rare earth magnetic ordering in Dy0.8Ho0.2MnO3 in contrast to DyMnO3 could be revealed. It was shown that doping by 20% Ho suppresses the spontaneous rare-earth ordering with its own propagation vector and provides the situation when two magnetic subsystems, manganese and rare earth ones have a coherent incommensurate spatial propagation. The influence of the external electric field on the magnetic chirality could be directly evidenced, proving strong magneto-electric coupling in multiferroic phase. The study of the electric polarization under similar temperatures and fields on the same samples provides the direct correlation between the results of the microscopic and macroscopic investigations.
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15.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Pankrats A. I., Sablina K. A., Tugarinov V. I., Balaev A. D., Kolkov M. I.
Заглавие : Magnetic resonance and dielectric properties of PbMnBO4 single crystal
Коллективы : "Spin Waves", International Simposium, Физико-технический институт им. А.Ф. Иоффе РАН
Место публикации : Spin Waves 2015, Int. Symp.: abstracts. - СПб., 2015. - P.49
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Freydman A. L., Pankrats A. I., Skorobogatov S. A., Horoshiy I. N., Kolkov M. I.
Заглавие : Magnetodielectric effect insingle crystals sequence of Pb2Fe2–xMnxGe2O9 (x=0–0.4)
Место публикации : Phys. Solid State. - 2022. - Vol. 64, Is. 12. - P.1912-1918. - ISSN 10637834 (ISSN), DOI 10.21883/PSS.2022.12.54385.455. - ISSN 10906460 (eISSN)
Примечания : Cited References: 30. - The research was funded by RFBR, Government of Krasnoyarsk Territory and Krasnoyarsk Territory Science Foundation under scientific projects No. 20-42-243008 and 20-42-240006
Аннотация: In this work, the magnetodielectric response have been studied in a series of single crystals of Pb2Fe2–xMnxGe2O9 with substitution x from 0 to 0.43. The research results showed that an increase in x leads to a change in the orientation of the antiferromagnetism vector in a zero magnetic field. The application of an external magnetic field leads to spin-flop and spin-reorientation magnetic transitions, which are accompanied by anomalies in the behavior of the permittivity. When Fe3+ ions are replaced by Mn3+ ions, the response of the magnetic subsystem to an external magnetic field changes, which is naturally reflected in the change in the magnetodielectric response. The permittivity changes stepwise when the magnetic subsystem passes into a state with a nonzero vector of the weakly ferromagnetic moment, or when its magnitude and orientation change due to a spin-flop transition. The latter indicates that a sharp change in polarizability is a consequence of a change in the contribution of the exchange energy, as well as the contribution of the Dzyaloshinskii–Moriya term, due to a change in the skew angle between two interacting magnetic moments.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankrats A. I., Kolkov M. I., Martynov S. N., Popkov S. I., Krasikov A. A., Balaev A. D., Gorev M. V.
Заглавие : Peculiarities of a magnetic transition in a quasi-one-dimensional ferromagnet PbMnBO4
Место публикации : J. Magn. Magn. Mater. - 2019. - Vol. 471. - P.416-422. - ISSN 03048853 (ISSN) , DOI 10.1016/j.jmmm.2018.09.098
Примечания : Cited References: 22. - This work was supported by the Russian Foundation for Basic Research, Project no. 16-02-00563. The authors thank V. Zinenko and V. Sosnin for the fruitful and useful discussions.
Аннотация: Near the Curie temperature TC = 30.3 K, the temperature dependences of the magnetization and heat capacity of a single-crystal ferromagnet PbMnBO4 in the magnetic fields of 1, 3, 10 and 30 kOe are studied. In the strong magnetic fields, both the magnetic contribution to the specific heat and the nonlinearity of the field dependences of the magnetization are maintained up to the temperatures exceeding TC more than twice. It is assumed that in PbMnBO4 the difference between TC, the paramagnetic Curie temperature θ = 49 K and the broad temperature region above TC where the magnetic contribution to the specific heat is significant is due to the quasi-one-dimensional character of the magnetic structure of this ferromagnet. Using both the estimation of TC from the Ginzburg-Landau field theory and the θ value, the total exchange interaction parameters 2J ≈ 40.4 K (intrachain) and z′J′ ≈ 8.8 K (interchain) are determined, with z′ = 4 being the number of neighboring chains. The estimation shows that the Ginzburg-Landau field theory describing the quasi-one-dimensional behavior of PbMnBO4 is well applicable in the temperature range from to T = S2J ≈ 80 K. Above this temperature, the mean field approximation with the exchange parameter λθ based on the paramagnetic Curie temperature θ describes well the experimental temperature dependences of the magnetization in the strong magnetic field and the specific heat is determined by the lattice contribution.
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18.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Balaev D. A., Freydman A. L., Krasikov A. A., Balaev A. D., Pankrats A. I., Popkov S. I., Kolkov M. I., Sablina K. A., Bovina A. F.
Заглавие : Spin-flop driven magneto-dielectric effect in single crystals Cu3B2O6 and Pb2Fe2Ge2O9
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow International Symposium on Magnetism (MISM-2017): 1-7 July 2017 : book of abstracts. - 2017. - Ст.5PO-I2-4. - P.1049 (Шифр 29916280)
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Prosnikov M. A., Bal M. E., Kolkov M. I., Pankrats A. I., Pisarev, R., V, Christianen, P. C. M.
Заглавие : Subterahertz and terahertz spin and lattice dynamics of the insulating ferromagnet PbMnBO4
Коллективы : RFBRRussian Foundation for Basic Research (RFBR); Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science [20-42-240006]; BASIS Foundation [21-1-4-33-1]; HFML-RU/NWO-I, a member of the European Magnetic Field Laboratory (EMFL)
Место публикации : Phys. Rev. Res. - 2022. - Vol. 4, Is. 1. - Ст.013004. - ISSN 2643-1564(eISSN), DOI 10.1103/PhysRevResearch.4.013004
Примечания : Cited References: 62. - M.A.P. greatly acknowledges D. A. Andronikova for aid, B. T. Crow for fruitful discussions, and P. Albers for technicalassistance. Crystal growth was supported by RFBR and the Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, through Research Project No. 20-42-240006. The theoretical part of the spin dynamics calculations was supported by BASIS Foundation Grant No. 21-1-4-33-1. The support of HFML-RU/NWO-I, a member of the European Magnetic Field Laboratory (EMFL) , is acknowledged
Предметные рубрики: LIGHT-SCATTERING
ANTI-STOKES
BRILLOUIN-SCATTERING
Аннотация: Orthorhombic PbMnBO4 is a rare example of an insulating ferromagnet in which the magnetic properties, in particular the strong magnetic anisotropy, are determined by the Mn3+ Jahn-Teller ion. Here, we report on the detailed investigation of magnetic excitations in the subterahertz and terahertz frequency ranges, as well as lattice excitations in the terahertz range. Using polarized azimuthally resolved Raman spectroscopy, four branches of magnetic excitations were observed and assigned to one acoustic and three optical one-magnon modes. The coupling between ferromagnetic ordering at TC=31K and the Jahn-Teller distortions of [MnO6] octahedra due to the spin-phonon interaction was directly observed for some specific phonon modes involved in these distortions. A spin-wave Hamiltonian was developed that allowed us to determine a unique set of exchange and effective anisotropy parameters. The intensity ratio of the anti-Stokes to Stokes acoustic magnon peaks is found to be anomalous and directly indicates the involvement of the magneto-optical parameters in the magnetic Raman scattering process.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Semenov S. V., Kolkov M. I., Terent'ev K. Yu., Pavlovskiy N. S., Pavlovskiy M. S., Vasiliev A. D., Shabanov A. V., Shaykhutdinov K. A., Balaev D. A.
Заглавие : Synthesis of the Orthorhombic Dy1−xHoxMnO3 Single Crystals and Study of Their Magnetic Properties
Место публикации : J. Supercond. Novel Magn. - 2019. - Vol. 32, Is. 10. - P.3315–3320. - ISSN 15571939 (ISSN) , DOI 10.1007/s10948-019-5090-8
Примечания : Cited References: 20. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science to the research project: “Research, synthesis and investigation of new oxide single crystals showing the interrelation of magnetic, magnetoelastic and magnetoelectric properties” (project № 18-42-243024).
Аннотация: In this report, we prepared for the first time the orthorhombic Dy1−xHoxMnO3 single crystals with x = 0, 0.1, 0.2, 0.3, and 0.4 using the flux technique. The post-growth processing and chemical and structural characterization of the synthesized samples were performed. Also, we examined the samples obtained by their magnetic properties and the magnetic anisotropy in wide ranges of temperatures and magnetic fields.
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