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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Boldyrev K. N., Stanislavchuk T. N., Sirenko A. A., Kamenskyi D., Bezmaternykh L. N., Popova M. N.
Заглавие : Bifurcations of coupled electron-phonon modes in an antiferromagnet subjected to a magnetic field
Место публикации : Phys. Rev. Lett.: American Physical Society, 2017. - Vol. 118, Is. 16. - Ст.167203. - ISSN 00319007 (ISSN), DOI 10.1103/PhysRevLett.118.167203
Примечания : Cited References: 26. - This research was supported by the Russian Scientific Foundation under Grant No. 14-12-01033, the President of Russian Federation (MK-3577.2017.2, K. N. B.), and the U.S. Department of Energy under Grant No. DE-FG02-07ER46382 (experiments at U4-IR beam line NSLS-BNL, T. N. S. and A. A. S.). The National Synchrotron Light Source is operated as a user facility for the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. Part of this work was supported by EMFL (Contract No. 26211). M. N. P. thanks B. Z. Malkin and A. V. Popov for helpful discussions.
Ключевые слова (''Своб.индексиров.''): antiferromagnetic materials--bifurcation (mathematics)--electron-phonon interactions--electrons--magnetic fields--magnetism--temperature--antiferromagnetic crystals--bifurcation points--electron phonon couplings--electronic excitation--external magnetic field--field independents--low temperatures--reflection spectra--phonons
Аннотация: We report on a new effect caused by the electron-phonon coupling in a stoichiometric rare-earth antiferromagnetic crystal subjected to an external magnetic field, namely, the appearance of a nonzero gap in the spectrum of electronic excitations in an arbitrarily small field. The effect was registered in the low-temperature far-infrared (terahertz) reflection spectra of an easy-axis antiferromagnet PrFe3(BO3)4 in magnetic fields Bext-c. Both paramagnetic and magnetically ordered phases (including a spin-flop one) were studied in magnetic fields up to 30 T, and two bifurcation points were observed. We show that the field behavior of the coupled modes can be successfully explained and modeled on the basis of the equation derived in the framework of the theory of coupled electron-phonon modes, with the same field-independent electron-phonon interaction constant |W|=14.8 cm-1. © 2017 American Physical Society.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Chukalina E. P., Boldyrev K. N., Stanislavchuk T. N., Malkin B. Z., Gudim I. A.
Заглавие : Spectroscopy of f-f transitions, crystal-field calculations, and magnetic and quadrupole helix chirality in DyFe3(BO3)4
Место публикации : Phys. Rev. B: American Physical Society, 2017. - Vol. 95, Is. 12. - Ст.125131. - ISSN 10980121 (ISSN), DOI 10.1103/PhysRevB.95.125131
Примечания : Cited References: 49. - This paper was supported by the Russian Scientific Foundation (Grant No. 14-12-01033). I.A.G. thanks L. N. Bezmaternykh for useful comments concerning the crystal growth and the Russian Foundation for Basic Research for financial support under Grant No. 14-02-00307a.
Аннотация: We present the results of temperature- and polarization-dependent high-resolution optical spectroscopy studies of DyFe3(BO3)4 performed in spectral ranges 40-300cm-1 and 3000-23000cm-1. The crystal-field (CF) parameters for the Dy3+ ions in the P3121 (P3221) phase of DyFe3(BO3)4 are obtained from calculations based on the analysis of the measured f-f transitions. Recently, quadrupole helix chirality and its domain structure was observed in resonant x-ray diffraction experiments on DyFe3(BO3)4 using circularly polarized x rays [T. Usui, Y. Tanaka, H. Nakajima, M. Taguchi, A. Chainani, M. Oura, S. Shin, N. Katayama, H. Sawa, Y. Wakabayashi, and T. Kimura, Nat. Mater. 13, 611 (2014)10.1038/nmat3942]. Using the obtained set of the CF parameters, we calculate temperature dependencies of the electronic quadrupole moments of the Dy3+ ions induced by the low-symmetry (C2) CF component and show that the quadrupole helix chirality can be explained quantitatively. We also consider the temperature dependencies of the bulk magnetic dc-susceptibility and the helix chirality of the single-site magnetic susceptibility tensors of the Dy3+ ions in the paramagnetic P3121 (P3221) phase and suggest the neutron and resonant x-ray diffraction experiments in a magnetic field to reveal the helix chirality of field-induced magnetic moments. © 2017 American Physical Society.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Kuzmenko A. M., Mukhin A. A., Ivanov V. Yu., Shuvaev A., Dziom V., Pimenov A., Boldyrev K. N., Bezmaternykh L. N., Gudim, I. A.
Заглавие : Terahertz optical activity at crystal field transitions in Tm3+ Ions in magnetoelectric alumoborates
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow International Symposium on Magnetism (MISM-2017): 1-7 July 2017 : book of abstracts. - 2017. - Ст.4PO-J-33. - P.912 (Шифр 29916280)
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Boldyrev K. N., Molchanova A. D., Moshkina E. M.
Заглавие : The electronic and magnetic structures of manganese doped copper metaborate Cu0.98Mn0.02B2O4
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow International Symposium on Magnetism (MISM-2017): 1-7 July 2017 : book of abstracts. - 2017. - Ст.4OR-O-11. - P.752 (Шифр 29916280)
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Malkin B. Z., Stanislavchuk T. N., Chukalina E. P., Boldyrev K. N., Gudim, I. A.
Заглавие : High-resolution spectroscopy, crystal-field calculations, and quadrupole helix chirality of DyFe3(BO3)(4)
Коллективы : Congress on Spectroscopy
Место публикации : XXV Congress on Spectroscopy: E D P Sciences, 2017. - Vol. 132. - Ст.03041. - (EPJ Web of Conferences). - ISSN 2100-014X, DOI 10.1051/epjconf/201713203041
Примечания : Cited References:2
Аннотация: High-resolution polarized transmission spectra of DyFe3(BO3)(4) single crystals were investigated in broad spectral (10-23000 cm(-1)) and temperature (3.5-300 K) ranges. Energies of the dysprosium levels in the paramagnetic and antiferromagnetic phases were determined. On the basis of these data and preliminary calculations in the frameworks of the exchange-charge model, we determined the crystal-field and Dy-Fe exchange interaction parameters of the Dy3+ ions at sites with the point C-2 symmetry corresponding to the enantiomorphic P3(1)21 and P3(2)21 space groups. The values of electronic quadrupole moments of the Dy3+ ions were calculated, which enabled us to interpret results of the work [Usui et al., Nature Mater. 13, 611 (2014)] on the observation of domains of different quadrupole chirality in DyFe3(BO3)(4).
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Malkin B. Z., Boldyrev K. N., Stanislavchuk T. N., Erofeev D. A., Temerov V. L., Gudim, I. A.
Заглавие : Evidence for a collinear easy-plane magnetic structure of multiferroic EuFe3(BO3)4: Spectroscopic and theoretical studies
Место публикации : Phys. Rev. B: American Physical Society, 2016. - Vol. 94, Is. 18. - Ст.184418. - ISSN 10980121 (ISSN), DOI 10.1103/PhysRevB.94.184418
Примечания : Cited References: 49. - This work was supported by the Russian Science Foundation under Grant No. 14-12-01033. I.A.G. and V.L.T. are grateful to L. N. Bezmaternykh for useful comments concerning the crystal growth, to M. S. Molokeev for the XRD characterization of the samples, and to the Russian Foundation for Basic Research for a financial support (Grants No. 13-02-12442 and No. 14-02-00307a).
Аннотация: We performed high-resolution polarized optical transmission spectroscopy and theoretical studies of multiferroic EuFe3(BO3)4 single crystals in the three phases: paramagnetic R32(T˃Ts=84K) and P3121(Ts˃T˃TN=34K), and antiferromagnetic (T˂TN) ones. The analysis of the spectra reveals interesting details of the magnetic structure, namely, a collinear arrangement of the iron magnetic moments along the C2 symmetry axis in the ab crystallographic plane of EuFe3(BO3)4 below TN. Spectral signatures of the phase transitions and the spin-phonon interaction are observed and discussed. Reliable crystal-field and exchange-interaction parameters are obtained and used to model the magnetic susceptibility of the compound. The results of detailed calculations of the electric polarization of EuFe3(BO3)4 in the R32 phase are presented, and mechanisms of the magnetoelectric response are discussed. We detect a strong effect of impurities (that enter the crystal from a flux in the course of the crystal growth) on the structural phase-transition temperature and demonstrate a coexistence of both R32 and P3121 phases down to the lowest temperatures in a EuFe3(BO3)4 crystal grown with the Bi2Mo3O12 based flux, due to inhomogeneous distribution of impurity Bi3+ ions. Our study can be considered as a demonstration of the abilities of optical spectroscopy in delivering new information on a magnetic compound, even in the case when other methods fail. © 2016 American Physical Society.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Chukalina E. P., Boldyrev K. N., Stanislavchuk T. N., Malkin B. Z., Gudim I. A.
Заглавие : Spectroscopy of f-f transitions, crystal-field calculations, and magnetic and quadrupole helix chirality in DyFe3(BO3)4 [Electronic resource]
Место публикации : ArXiv. - 2016. - Ст.1611.07092
Вид и объем ресурса: Electronic text data
Примечания : Cited References: 47. - This work was supported by the Russian Science Foundation (Grant No14-12-01033). I. A. G. thanks L. N. Bezmaternykh for useful comments concerning the crystal growth and the Russian Foundation for Basic Research for a financial support under Grant No 14-02-00307a.
Аннотация: Recently, quadrupole helix chirality and its domain structure was observed in resonant x-ray diffraction experiments on DyFe3(BO3)4 using circularly polarized x rays [T. Usui et al., Nature Materials 13, 611 (2014)]. We show that this effect can be explained quantitatively by calculating the quadrupole moments of the Dy3+ ions induced by the low-symmetry (C2) crystal-field (CF) component. In this work, the CF parameters for the Dy3+ ions in the P3121 (P3221) phase of DyFe3(BO3)4 are obtained from CF calculations based on the analysis of high-resolution temperature-dependent optical spectroscopy data. We also consider the helix chirality of the single-site magnetic susceptibility tensors of the Dy3+ ions in the paramagnetic P3121 (P3221) phase and suggest a neutron diffraction experiment to reveal it.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Boldyrev K. N., Stanislavchuk T. N., Sirenko A. A., Kamenskyi D., Bezmaternykh L. N., Popova M. N.
Заглавие : Bifurcations observed in the spectra of coupled electron-phonon modes in multiferroic PrFe3(BO3)4 subjected to a magnetic field [Electronic resource]
Место публикации : ArXiv. - 2016. - Ст.1609.02125
Вид и объем ресурса: Electronic text data
Примечания : Cited References: 19. - This research was supported by the Russian Scientific Foundation under Grant No 14-12-01033, the President of Russian Federation (MK-3521-2015.2, K.N.B.), and the U.S. Department of Energy under Grant No DE-FG02-07ER46382 (experiments at U4-IR beamline NSLS-BNL, T.N.S. and A.A.S.). The National Synchrotron Light Source is operated as a User Facility for he U.S. Department of Energy under Contract No. DE-AC02-98CH10886. Part of this work was supported by EMFL (contract No. 26211). M.N.P. thanks B.Z. Malkin helpful discussions.
Аннотация: We report on bifurcations effect mediated by the electron-phonon coupling in a concentrated rare-earth-containing antiferromagnet, observed in the spectra of coupled 4f-electron-phonon modes under the influence of an external magnetic field. The effect was observed in the low-temperature far-infrared (terahertz) reflection spectra of a multiferroic easy-axis antiferromagnet PrFe3(BO3)4 in magnetic fields Bext||c. Both paramagnetic and magnetically ordered phases (including a spin-flop one) were studied in magnetic fields up to 30 T. We show that the field behavior of the coupled modes can be successfully explained and modeled on the base of the equation derived in the frame of the theory of coupled electron-phonon modes, with the same field-independent electron-phonon interaction constant |W|=14.8cm−1.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Molchanova A. D., Moshkina E. M., Molokeev M. S., Tropina E. V., Bovina A. F., Boldyrev K. N.
Заглавие : Synthesis and optical properties of nickel-doped copper metaborate crystals
Место публикации : Opt. Spectrosc. - 2022. - Vol. 130, Is. 1. - P.105-109. - ISSN 0030400X (ISSN), DOI 10.21883/EOS.2022.01.52994.41-21. - ISSN 15626911 (eISSN)
Примечания : Cited References: 18. - The study was performed with the support of Russian Science Foundation, RSF grant № 19-12-00413
Аннотация: This work presents information on the growth and spectroscopic study of single crystals of copper metaborate doped with nickel Cu1–xNixB2O4 (x = 0.05, 0.1). In the absorption spectra of both crystals, satellites related to Cu centers distorted by impurity Ni atoms were observed near the lines of zero phonon transitions. Polarization studies in the isotropic ab-plane of the tetragonal crystal Cu1–xNixB2O4 show the presence of linear magnetic dichroism in the magnetically ordered state, which was previously observed both in manganese-doped and undoped copper metaborates CuB2O4. The temperature of magnetic phase transitions into the collinear antiferromagnetic and into helicoidal structures, TN = 19.1 K and T* = 8.6 K, respectively, were determined from the temperature dependence of the dichroic signal.
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10.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Boldyrev K.N., Popova M. N., Bezmaternykh L. N., Bettinelli M., Loiseau P., Leonyuk N. I.
Заглавие : Higt-resolution spectroscopy of Yb3+ centers in RAl3(BO3)4:Yb single crystals
Коллективы : Excited States of Transition Elements and Workshop on Luminescence
Место публикации : Excit. St. of Trans. Elem. and Worksh. on Luminesc.: ESTE2010: book of abstracts. - Wrocław: Wydział Chemii Uniwersytetu Wrocławskiego, 2010. - Ст.Tu-7
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