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Dynamics of asphaltene aggregates under high-pressure CO2 revealed by pulsed-field gradient NMR / E. V. Morozov, S. N. Trukhan, I. V. Kozhevnikov [et al.] // Energy & Fuels. - 2023. - Vol. 37, Is. 22. - P. 17215-17226, DOI 10.1021/acs.energyfuels.3c02862. - Cited References: 90. - The present research was performed with the financial support of the Russian Science Foundation (project no. 21-13-00171, http://rscf.ru/project/21-13-00171/) using the equipment of the Krasnoyarsk Regional Center of Research Equipment of the Federal Research Center “Krasnoyarsk Science Center SB RAS” . - ISSN 0887-0624. - ISSN 1520-5029
Аннотация: The work demonstrates the results of the first experimental PFG NMR study in situ of the complex phase behavior of asphaltenes in the presence of high-pressure CO2. To perform the experiments, a series of sealed, thick-walled quartz capillaries were prepared with a mixture of CO2 and asphaltenes dissolved either in chloroform or benzene at different initial concentrations. Then, the temperature dependence of the diffusion coefficients of the asphaltene aggregates was measured for each sample after the mixture reached its equilibrium state, at which, in accordance with the solubility limit, only part of the initial asphaltenes remained dissolved. Despite quite low residual asphaltene concentrations in solution, experimental data clearly demonstrated the presence of aggregated structures (up to 70–80 wt %) attributed solely to nanoaggregates, with no signs of the presence of macroaggregates in the samples. Temperature dependencies of aggregate diffusivity clearly showed that the scenario, according to which the evolution of the asphaltene aggregates will develop, strongly depends on the initial asphaltene concentration, mass fraction of CO2 loaded into the system, and chemical nature of the solvent used. In particular, the most diluted asphaltene solution, expected to be the most resistive to the aggregation processes in a high-pressure CO2 environment, revealed the most pronounced aggregation-dependent translational dynamics as compared to those with a moderate initial asphaltene concentration. Contrarily, the concentrated asphaltene solution may not show drastic aggregation processes if the mass fraction of the CO2 loaded will not appear to be so high. Finally, the experimental results provide evidence that the temperature-triggered structural transformation of asphaltene aggregates due to the noncovalent bond breakup is not hindered under high-pressure CO2, but instead becomes more emphasized. The results obtained shed new light on asphaltene aggregate dynamics and brought new knowledge about the fundamental behavior of asphaltene in high-pressure CO2 conditions.

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Держатели документа:
Institute of Chemistry and Chemical Technology, Federal Research Center “Krasnoyarsk Science Center of Siberian Branch of the Russian Academy of Sciences”, Akademgorodok 50/24, Krasnoyarsk 660036, Russia
Kirensky Institute of Physics, Federal Research Center “Krasnoyarsk Science Center of Siberian Branch of the Russian Academy of Sciences”, Akademgorodok 50/38, Krasnoyarsk 660036, Russia
Federal Research Center “Krasnoyarsk Science Center of Siberian Branch of the Russian Academy of Sciences”, Akademgorodok 50, Krasnoyarsk 660036, Russia
Boreskov Institute of Catalysis, Siberian Branch of the Russian Academy of Sciences, Ak. Lavrentieva 5, Novosibirsk 630090, Russia

Доп.точки доступа:
Morozov, E. V.; Морозов, Евгений Владимирович; Trukhan, Sergey N.; Kozhevnikov, Ivan V.; Peterson, Ivan V.; Martyanov, Oleg N.
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    Processes underlying the laser photochromic effect in colloidal plasmonic nanoparticle aggregates* / A. E. Ershov, V. S. Gerasimov, I. L. Isaev [et al.] // Chin. Phys. B. - 2020. - Vol. 29, Is. 3. - Ст. 037802, DOI 10.1088/1674-1056/ab6551. - Cited References: 38. - Project funded by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science (Grant 18-42-243023), the RF Ministry of Science and Higher Education, and the State Contract with Siberian Federal University for Scientific Research. A.E. thanks the grant of the President of Russian Federation (agreement 075-15-2019-676). . - ISSN 1674-1056. - ISSN 1741-4199
Рубрики:
SELECTIVE PHOTOMODIFICATION
   LIGHT
   FORCES
   OPTICS
Кл.слова (ненормированные):
nanoparticle -- surface plasmon resonance -- photochromic process -- pulsed laser radiation
Аннотация: We have studied the dynamic and static processes occurring in disordered multiparticle colloidal Ag aggregates with natural structure and affecting their plasmonic absorption spectra under pico- and nanosecond pulsed laser radiations, as well as the physical origin responsible for these processes. We have shown that depending on the duration of the laser pulse, the mechanisms of laser modification of such aggregates can be associated both with changes in the resonant properties of the particles due to their heating and melting (picosecond irradiation mode) and with the particle shifts in the resonant domains of the aggregates (nanosecond pulses) which depend on the wavelength, intensity, and polarization of the radiation. These mechanisms result in formation of a narrow dip in the plasmonic absorption spectrum of the aggregates near the laser radiation wavelength and affect the shape and position of the dip. The effect of polydispersity of nanoparticle aggregates on laser photochromic reaction has been studied.

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Держатели документа:
RAS, SB, Inst Computat Modeling, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
RAS, SB, KSC, Kirensky Inst Phys,Fed Res Ctr, Krasnoyarsk 660036, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660014, Russia.

Доп.точки доступа:
Ershov, A. E.; Gerasimov, V. S.; Isaev, I. L.; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Government of the Krasnoyarsk Territory [18-42-243023]; Krasnoyarsk Regional Fund of Science [18-42-243023]; RF Ministry of Science and Higher Education; Siberian Federal University for Scientific Research; Russian FederationRussian Federation [075-15-2019-676]
}
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Morozov, E. V.
Temperature-Triggered Rearrangement of Asphaltene Aggregates as Revealed by Pulsed-Field Gradient NMR / E. V. Morozov, P. V. Yushmanov, O. N. Martyanov // Energy Fuels. - 2019. - Vol. 33, Is. 8. - P. 6934-6945, DOI 10.1021/acs.energyfuels.9b00600. - Cited References: 119. - This research was performed using the equipment of Krasnoyarsk Regional Research Equipment Centre of Siberian Branch of Russian Academy of Sciences with the financial support of Russian Science Foundation (Project No. 15-19-00119). . - ISSN 0887-0624. - ISSN 1520-5029

РУБ Energy & Fuels + Engineering, Chemical
Рубрики:
CRITICAL NANOAGGREGATE CONCENTRATION
ELECTRON-SPIN-RESONANCE
Аннотация: The tendency of asphaltenes for aggregation followed by precipitation and deposition plays a crucial role in the petroleum industry since these processes present severe problems during the production, recovery, and processing of crude oils and fossil hydrocarbon feedstocks. The dynamics of oil asphaltene aggregates dissolved in chloroform at different concentrations varied in a wide range that was investigated at temperatures from 0 to 55 °C using the Pulsed-Field Gradient NMR technique. The components attributed to nanoaggregates and macroaggregates were successfully resolved, which allowed us to measure their diffusion coefficients. The diffusion coefficients for all types of aggregates grow as the asphaltene concentration decreases, whereas the partial weight of the aggregates increases with the increase of asphaltene concentration. The difference in diffusion behavior of the aggregates of different types was registered when passing the critical concentration range 10–20 g/L. The nano- and macroaggregates behave independently when the asphaltene concentration is higher than 20 g/L (concentrated regime), while below 20 g/L (semidiluted regime) the components related to the different types of aggregates cannot be properly resolved. It was found that regardless of the asphaltene concentration, the diffusion coefficients for nano- and macroaggregates demonstrate similar temperature behavior giving the straight lines in the Arrhenius coordinates which change their slopes when passing the temperature range 20–30 °C. The phenomenon evidences the thermally induced cleavage of noncovalent bonds with subsequent rearrangement of asphaltene aggregates that is observed for all concentration regimes covering the existence of asphaltene aggregates of all types. The data obtained are well consistent with the modern concept of asphaltene aggregate structure and fairly agree with the data obtained earlier. We believe these results will contribute essentially to a better understanding of the fundamental behavior of asphaltenes and their aggregates, providing a deep insight into aggregate transformation triggered by the temperature.

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Держатели документа:
SB RAS, Inst Chem & Chem Technol, Fed Res Ctr, Krasnoyarsk Sci Ctr, Akademgorodok 50-24, Krasnoyarsk 660036, Russia.
SB RAS, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk Sci Ctr, Akademgorodok 50-38, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Siberian Branch, Boreskov Inst Catalysis, Ak Lavrentieva 5, Novosibirsk 630090, Russia.
P&L Sci Instrument Serv, Box 1241, S-18124 Lidingo, Sweden.
Novosibirsk State Univ, Pirogova Str 2, Novosibirsk 630090, Russia.

Доп.точки доступа:
Yushmanov, Pavel, V; Martyanov, Oleg N.; Морозов, Евгений Владимирович; Russian Science FoundationRussian Science Foundation (RSF) [15-19-00119]
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Surface plasmon resonances in liquid metal nanoparticles / A. E. Ershov [et al.] // Appl. Phys. B. - 2017. - Vol. 123, Is. 6. - Ст. 182, DOI 10.1007/s00340-017-6755-2. - This work was performed within the State contract of the RF Ministry of Education and Science for Siberian Federal University for scientifc research in 2017–2019. The numerical calculations were performed using the MVS-1000 M cluster at the Institute of Computational Modeling, Siberian Branch, Russian Academy of Sciences. . - ISSN 0946-2171
Кл.слова (ненормированные):
Aggregates -- Dimers -- Gold -- Liquids -- Metal nanoparticles -- Nanoparticles -- Nonlinear optics -- Silver -- Surface plasmon resonance -- Au nanoparticle -- Colloidal aggregates -- Experimental values -- Experimental verification -- Metallic nanoparticles -- Nonlinear optical response -- Plasmonic nanoparticle -- Surface plasmon frequency -- Plasmons
Аннотация: We have shown significant suppression of resonant properties of metallic nanoparticles at the surface plasmon frequency during the phase transition “solid–liquid” in the basic materials of nanoplasmonics (Ag, Au). Using experimental values of the optical constants of liquid and solid metals, we have calculated nanoparticle plasmonic absorption spectra. The effect was demonstrated for single particles, dimers and trimers, as well as for the large multiparticle colloidal aggregates. Experimental verification was performed for single Au nanoparticles heated to the melting temperature and above up to full suppression of the surface plasmon resonance. It is emphasized that this effect may underlie the nonlinear optical response of composite materials containing plasmonic nanoparticles and their aggregates. © 2017, Springer-Verlag Berlin Heidelberg.

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Держатели документа:
Institute of Computational Modeling, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Institute of Nanotechnology, Spectroscopy and Quantum Chemistry, Siberian Federal University, Krasnoyarsk, Russian Federation
Siberian State University of Science and Technologies, Krasnoyarsk, Russian Federation
L.V. Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Евгеньевич; Gerasimov, V. S.; Герасимов, Валерий Сергеевич; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич
}
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Thermal effects in systems of colloidal plasmonic nanoparticles in high-intensity pulsed laser fields [Invited] / V. S. Gerasimov [et al.] // Opt. Mater. Express. - 2017. - Vol. 7, Is. 2. - P. 555-568, DOI 10.1364/OME.7.000555. - Cited References: 68. - This work was performed within the State contract of the RF Ministry of Education and Science for Siberian Federal University for scientific research in 2017-2019 and SB RAS Program No II.2P (0358-2015-0010). The calculations were performed using the MVS-1000 M cluster at the Institute of Computational Modeling, Federal Research Center KSC SB RAS. . - ISSN 2159-3930
Кл.слова (ненормированные):
Aggregates -- Gold -- Nanoparticles -- Plasmons -- Silver -- Ag nanoparticle -- High intensity -- Light-induced process -- Nanoparticle aggregate -- Physical model -- Plasmonic nanoparticle -- Pulsed-laser field -- Thermal interaction -- Pulsed lasers
Аннотация: We have studied light induced processes in nanocolloids and composite materials containing ordered and disordered aggregates of plasmonic nanoparticles accompanied by their strong heating. A universal comprehensive physical model that combines mechanical, electrodynamical, and thermal interactions at nanoscale has been developed as a tool for investigations. This model was used to gain deep insight on phenomena that take place in nanoparticle aggregates under high-intensity pulsed laser radiation resulting in the suppression of nanoparticle resonant properties. Verification of the model was carried out with single colloidal Au and Ag nanoparticles and their aggregates. © 2017 Optical Society of America.

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Держатели документа:
Siberian Federal University, Krasnoyarsk, Russian Federation
Institute of Computational Modeling, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Siberian State Aerospace University, Krasnoyarsk, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Royal Institute of Technology, Stockholm, Sweden
The Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, IL, United States

Доп.точки доступа:
Gerasimov, V. S.; Герасимов, Валерий Сергеевич; Ershov, A. E.; Karpov, S. V.; Карпов, Сергей Васильевич; Gavrilyuk, A. P.; Zakomirnyi, V. I.; Rasskazov, I. L.; Agren, H.; Polyutov, S. P.
}
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Magnetic parameters of separation products and impurity aggregates in concentrates / E. K. Yakubailik [et al.] // J. Min. Sci. - 2017. - Vol. 53, Is. 6. - P. 1133-1140, DOI 10.1134/S1062739117063233. - Cited References: 14 . - ISSN 1062-7391. - ISSN 1573-8736

РУБ Mining & Mineral Processing

Кл.слова (ненормированные):
Processing circuit -- wet laboratory separation -- concentrate impurity -- magnetic characteristics
Аннотация: The changes in separation performance and magnetic characteristics of separation products is traced along the processing circuit of Abagur concentrator at a laboratory scale in order to determine the limit content of magnetite iron in impurity aggregates in the concentrate. The wet magnetic analysis is carried out in the field of H = 175 kA/m, and the magnetic characteristics are determined in the vibration magnetic detector in the field up to 800 kA/m. The concentrate impurity content is governed by the relative content of barren rock and ore aggregates removable in concentration at the given level of the technology.

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Публикация на русском языке Определение магнитных параметров продуктов сепарации и засоряющих концентрат рудных сростков [Текст] / Э. К. Якубайлик [и др.] // Физ.-техн. проблемы разраб. полез. ископаемых. - 2017. - № 6. - С. 182-190

Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.
EVRAZRUDA, Novokuznetsk 654018, Russia.

Доп.точки доступа:
Yakubailik, E. K.; Якубайлик, Эдуард Константинович; Ganzhenko, I. M.; Balaev, A. D.; Балаев, Александр Дмитриевич; Butov, P. Yu.
}
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Morozov, E. V.
Reversibility of asphaltene aggregation as revealed by magnetic resonance imaging in situ / E. V. Morozov, O. N. Martyanov // Energy Fuels. - 2017. - Vol. 31, Is. 10. - P. 10639-10647, DOI 10.1021/acs.energyfuels.7b01755. - Cited References: 56. - This research was performed on the equipment of Krasnoyarsk Regional Research Equipment Centre of Siberian Branch of Russian Academy of Sciences with the financial support of Russian Science Foundation (Project No. 15-19-00119). . - ISSN 0887-0624
Кл.слова (ненормированные):
Aggregates -- Crude oil -- Flocculation -- Heavy oil production -- Magnetic resonance imaging -- Asphaltene aggregates -- Asphaltene aggregation -- Asphaltene precipitation -- Equilibrium compositions -- Flocculant concentrations -- Inhomogeneous distribution -- Mechanical stirring -- Multi-component systems -- Asphaltenes
Аннотация: Aggregation of asphaltenes followed by precipitation presents severe problems for existing technologies in the production, recovery, and processing of heavy oils. Better understanding of asphaltene behavior behind the processes of their precipitation and dissolution is vital to address this issue. While investigating the inhomogeneity of different oil systems, the reversibility of the asphaltene aggregation process initiated by flocculant in either asphaltene solution in toluene or crude heavy oil was revealed and investigated using magnetic resonance imaging methods. It was found that the inhomogeneous distribution of the flocculant initiates local spatial-selective asphaltene aggregation registered in a thin layer around the flocculant/oil sample interface. The local excess of flocculant concentration over the threshold of asphaltene precipitation onset is a driving force of this process. As the flocculant diffuses into the volume of the sample, a decrease of the asphaltene flocculated area is observed until it disappears when the equilibrium composition throughout the whole volume of the system is achieved. Depending on the overall flocculant concentration, the asphaltene aggregation may not be reversible and could be followed by subsequent precipitation of the asphaltene aggregates. The similarity of the phenomena observed for the model asphaltene solutions and crude heavy oil samples was established. Partial mechanical stirring of the multicomponent system comprising flocculant and oil or asphaltene solution does not prevent the formation of the local zones with increased concentration of asphaltene aggregates; those sizes evolve depending on the flocculant concentration. The results obtained in this work are consistent with the generally accepted concept of asphaltene precipitation reversibility depending on the system composition and are compatible with the observations obtained by other methods. The approach presented can provide deeper insight into the asphaltene precipitation reversibility issue and can facilitate the understanding of asphaltene behavior in heavy oils.

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Держатели документа:
Institute of Chemistry and Chemical Technology, Siberian Branch of the Russian Academy of Sciences, Akademgorodok 50/24, Krasnoyarsk, Russian Federation
Kirensky Institute of Physics, Siberian Branch of the Russian Academy of Sciences, Akademgorodok 50/38, Krasnoyarsk, Russian Federation
Boreskov Institute of Catalysis, Siberian Branch of the Russian Academy of Sciences, Pr. Ak. Lavrentieva 5, Novosibirsk, Russian Federation
Novosibirsk State University, Pirogova str. 2, Novosibirsk, Russian Federation

Доп.точки доступа:
Martyanov, O. N.; Морозов, Евгений Владимирович
}
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Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields / A. E. Ershov [et al.] // Chin. Phys. B. - 2016. - Vol. 25, Is. 11. - Ст. 117806, DOI 10.1088/1674-1056/25/11/117806. - Cited References: 47. - This work was performed within the state contract of the RF Ministry of Education and Science for Siberian Federal University for scientific research in 2016 (Reference number 1792) and SB RAS Program No II.2P (0358-2015-0010). Numerical computations were performed on the cluster MVS-1000 M of the Institute of computational modeling SB RAS. . - ISSN 1674-1056
Кл.слова (ненормированные):
optodynamics -- nanoparticle -- surface plasmon -- laser radiation
Аннотация: We have studied processes of interaction of pulsed laser radiation with resonant groups of plasmonic nanoparticles (resonant domains) in large colloidal nanoparticle aggregates having different interparticle gaps and particle size distributions. These processes are responsible for the origin of nonlinear optical effects and photochromic reactions in multiparticle aggregates. To describe photo-induced transformations in resonant domains and alterations in their absorption spectra remaining after the pulse action, we introduce the factor of spectral photomodification. Based on calculation of changes in thermodynamic, mechanical, and optical characteristics of the domains, the histograms of the spectrum photomodification factor have been obtained for various interparticle gaps, an average particle size, and the degree of polydispersity. Variations in spectra have been analyzed depending on the intensity of laser radiation and various combinations of size characteristics of domains. The obtained results can be used to predict manifestation of photochromic effects in composite materials containing different plasmonic nanoparticle aggregates in pulsed laser fields. © 2016 Chinese Physical Society and IOP Publishing Ltd.

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Держатели документа:
Institute of Computational Modeling, Russian Academy of Sciences, Krasnoyarsk, Russian Federation
L. V. Kirensky Institute of Physics of the Russian Academy of Sciences, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation
Siberian State Aerospace University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Ershov, A. E.; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Polyutov, S. P.
}
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Ershov, A. E.
Plasmonic nanoparticle aggregates in high-intensity laser fields: effect of pulse duration / A. E. Ershov, A. P. Gavrilyuk, S. V. Karpov // Plasmonics. - 2016. - Vol. 11, No. 2. - P. 403-410, DOI 10.1007/s11468-015-0054-8. - Cited References: 20. - Authors are thankful to Prof. V.A. Markel (University of Pennsylvania) for supplying program codes with realization of coupled dipole method for polydisperse nanoparticle aggregates. This work was performed within the state contract of the RF Ministry of Education and Science for Siberian Federal University for scientific research in 2014 (Reference number 1792) . - ISSN 1557-1955

РУБ Chemistry, Physical + Nanoscience & Nanotechnology + Materials Science, Multidisciplinary
Рубрики:
METAL NANOPARTICLES
Кл.слова (ненормированные):
Nanoparticle -- Surface plasmon -- Colloidal aggregate -- Optodynamics
Аннотация: We use an optodynamic model to study the interaction of pulsed laser radiation of different duration with mono- and polydisperse dimers and trimers of plasmonic nanoparticles as resonant domains of colloid Ag multiparticle aggregates. A comparative analysis of the influence of pulse duration on the kinetic characteristics of domains accompanied by the change in their local structure was carried out taking into account the intensity of incident radiation. The obtained results explain the reasons for laser photochromic reactions in materials containing colloidal aggregates of plasmonic nanoparticles.

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Доп.точки доступа:
Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Ершов, Александр Андреевич
}
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10.

Gerasimov, V. S.
Variations in extinction spectra of plasmonic nanoparticle aggregates upon deformation during deposition on planar dielectric substrate / V. S. Gerasimov, I. L. Rasskazov, S. V. Karpov // Annual Int. Conf. "Days on Diffraction". - 2015. - P. 141-142

Материалы конференции

Доп.точки доступа:
Rasskazov, I. L.; Рассказов, Илья Леонидович; Karpov, S. V.; Карпов, Сергей Васильевич; Герасимов, Валерий Сергеевич; "Days on diffraction", International conference(2015 ; may ; 25-29 ; St. Petersburg); Санкт-Петербургское отделение Института математики им. В. А. Стеклова; Санкт-Петербургский государственный университет; Euler International Mathematical Institute; Российский фонд фундаментальных исследований
}
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11.

Effect of local environment in resonant domains of polydisperse plasmonic nanoparticle aggregates on optodynamic processes in pulsed laser fields / A. E. Ershov [et al.] // Chin. Phys. B. - 2015. - Vol. 24, Is. 4. - Ст. 047804, DOI 10.1088/1674-1056/24/4/047804. - Cited References:25. - Project supported by the Russian Academy of Sciences (Grant Nos. 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101), and 3-9-5). . - ISSN 1674. - ISSN 1741-4199. -

РУБ Physics, Multidisciplinary
Рубрики:
METAL NANOPARTICLES
GOLD NANOPARTICLES
OPTICAL-PROPERTIES
Кл.слова (ненормированные):
nanoparticle -- surface plasmon -- colloid aggregate -- optodynamics
Аннотация: Interactions of pulsed laser radiation with resonance domains of multiparticle colloidal aggregates having an increasingly complex local environment are studied via an optodynamic model. The model is applied to the simplest configurations, such as single particles, dimers, and trimers consisting of mono- and polydisperse Ag nanoparticles. We analyze how the local environment and the associated local field enhancement by surrounding particles affect the optodynamic processes in domains, including their photomodification and optical properties.

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Держатели документа:
Russian Acad Sci, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia
Russian Acad Sci, Inst Computat Modeling, Krasnoyarsk 660036, Russia
Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia
Siberian Fed Univ, Krasnoyarsk 660028, Russia

Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Евгеньевич; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Semina, P. N.; Семина, Полина Николаевна; Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101), 3-9-5]
}
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12.

Optodynamic phenomena in aggregates of polydisperse plasmonic nanoparticles / A. E. Ershov [et al.] // Appl. Phys. B. - 2014. - Vol. 115, Is. 4. - P. 547-560, DOI 10.1007/s00340-013-5636-6. - Cited References: 48. - Authors are thankful to Prof. V. A. Markel (University of Pennsylvania) for supplying program codes for realization of the coupled dipole method for polydisperse metal nanoparticle aggregates. This research was supported by the Russian Academy of Sciences under the Grants 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101); Ministry of Education and Science of Russian Federation under Contract 14.B37.21.0457. . - ISSN 0946-2171. - ISSN 1432-0649

РУБ Optics + Physics, Applied
Рубрики:
SMALL-PARTICLE COMPOSITES
   OPTICAL-PROPERTIES
   NOBLE-METALS
   SILVER
   ELECTRON
   LIQUID
   GENERATION
   DYNAMICS
   FORCES
   GOLD
Аннотация: We propose an optodynamical model of interaction of pulsed laser radiation with aggregates of spherical metallic nanoparticles embedded into host media. The model takes into account polydispersity of particles, pair interactions between the particles, dissipation of absorbed energy, heating and melting of the metallic core of particles and of their polymer adsorption layers, and heat exchange between electron and ion components of the particle material as well as heat exchange with the interparticle medium. Temperature dependence of the electron relaxation constant of the particle material and the effect of this dependence on interaction of nanoparticles with laser radiation are first taken into consideration. We study in detail light-induced processes in the simplest resonant domains of multiparticle aggregates consisting of two particles of an arbitrary size in aqueous medium. Optical interparticle forces are realized due to the light-induced dipole interaction. The dipole moment of each particle is calculated by the coupled dipole method (with correction for the effect of higher multipoles). We determined the role of various interrelated factors leading to photomodification of resonant domains and found an essential difference in the photomodification mechanisms between polydisperse and monodisperse nanostructures.

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Russian Acad Sci, LV Kirenski Inst Phys, Krasnoyarsk 660036, Russia
Russian Acad Sci, Inst Computat Modeling, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660028, Russia

Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Евгеньевич; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Semina, P. N.; Семина, Полина Николаевна; Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101)]; Ministry of Education and Science of Russian Federation [14.B37.21.0457]
}
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13.

Optodynamic and photochrome effects in composite media with aggregates of plasmonic nanoparticles in pulsed laser fields / A. E. Ershov [et al.] // ICONO/LAT 2013 : Advance conference program. - 2013. - P.

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Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Евгеньевич; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Semina, P. N.; Семина, Полина Николаевна; International Conference on Lasers, Applications, and Technologies (LAT 2013) (2013 ; June ; 18-22 ; Moscow)
}
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14.

    Карпов, Сергей Васильевич.
    Оптическая память агрегатов металлических наночастиц / С. В. Карпов // Фотоника. - 2012. - Т. 33, № 2. - С. 52-61 . - ISSN 1993-7296
   Перевод заглавия: Metallic Nanoparticles Aggregates Optical Memory
Аннотация: Исследование наноколлоидов представ- ляет практический интерес. Их можно использовать для повышения чувстви- тельности спектральных методов ана- лиза состава веществ, в устройствах оптической записи информации, для создания новых типов метаматериалов и синтеза самоорганизующихся сверх- решеток различной размерности, вклю- чая фотонные кристаллы, которые могут найти применение в наносенсорике и в задачах управления электромагнит- ным излучением на наномасштабах. В статье показано, что ключевую роль в оптических эффектах играет локаль- ная анизотропия окружения частиц в агрегате другими его частицами.
Nanocolloids investigation has practical interest. Nanocolloids can be used for sensitivity enhancement of spectral compositional analysis methods sensitivity, in optical information recording systems, for creation of new mathamaterials types and for synthesis of self-organizing different dimension superlattices, including photon crystals that can be used in nanosensory and for solution problems of nanoscale controlling electromagnetic emission. The key role of local anisotropy of particles surrounding the aggregate particles in optical effects is discussed.

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Институт физики им. Л.В. Киренского СО РАН

Доп.точки доступа:
Karpov, S. V.
}
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15.

Effects of size polydispersity on the extinction spectra of colloidal nanoparticle aggregates / A. E. Ershov [et al.] // Phys. Rev. B. - 2012. - Vol. 85, Is. 4. - Ст. 045421. - P. , DOI 10.1103/PhysRevB.85.045421. - Cited References: 41. - This work was supported by grants from the following foundations of the Russian Federation: Presidium of RAS, OFN RAS, and SB RAS. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
METAL FRACTAL CLUSTERS
   OPTICAL-PROPERTIES
   ABSORPTION
   NONLINEARITIES
   COMPOSITES
   SCATTERING
   PARTICLES
   SPHERES
   GRAINS
Аннотация: We investigate the effect of particle polydispersity on the optical extinction spectra of colloidal aggregates of spherical metallic (silver) nanoparticles, taking into account the realistic interparticle gaps caused by layers of stabilizing polymer adsorbed on the metal surface (adlayers). The spectra of computer-generated aggregates are computed using two different methods. The coupled-multipole method is used in the quasistatic approximation and the coupled-dipole method beyond the quasistatics. The latter approach is applicable if the interparticle gaps are sufficiently wide relative to the particle radii. Simulations are performed for two different particle size distribution functions (bimodal and Gaussian), varying the number of particles per aggregate, and different distribution functions of the interparticle gap width. The strong influence of the latter factor on the spectra is demonstrated and investigated in detail.

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Держатели документа:
[Ershov, Alexander E.
Isaev, Ivan L.
Semina, Polina N.
Karpov, Sergei V.] Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[Ershov, Alexander E.
Karpov, Sergei V.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
[Markel, Vadim A.] Univ Penn, Dept Bioengn, Dept Radiol, Philadelphia, PA 19104 USA
[Markel, Vadim A.] Univ Penn, Grad Grp Appl Math & Computat Sci, Philadelphia, PA 19104 USA

Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Евгеньевич; Isaev, I. L.; Исаев, Иван Леонидович; Semina, P. N.; Семина, Полина Николаевна; Markel, V. A.; Karpov, S. V.; Карпов, Сергей Васильевич
}
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16.

Dynamic Changes of Optical Characteristics of Resonant Domains in Metal Nanoparticle Aggregates under Pulsed Laser Fields [Text] / Gavrilyuk A.P., Karpov S.V. // Applied Physics B: Lasers and Optics. - 2010. - Vol. 101. - P512

Доп.точки доступа:
Gavrilyuk, A.P.; Karpov, S.V.
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17.

Transformation of the local structure of photomodified disordered aggregates of silver nanoparticles and its manifestations in the spectra of plasmon absorption [Text] / S. V. Karpov, I. L. Isaev [et al.] // Technical digest International conference ICONO/LAT 2010. - Казань, 2010. - Ст. IThO32

Доп.точки доступа:
Karpov, S.V.; Isaev, I.L.; Gavrilyuk, A.P.; Gerasimov, V.S.; Grachev, A.S.; International Conference on Coherent and Nonlinear Optics(2010 ; Aug. ; 23-26 ; Казань); International Conference on Lasers, Applications, and Technologies(2010 ; Aug. ; 23-26 ; Казань)
}
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18.

Dynamic changes of optical characteristics of resonant domains in metal nanoparticle aggregates under pulsed laser fields [Text] / A. P. Gavrilyuk, S. V. Karpov. // Technical digest International conference ICONO/LAT 2010. - Казань, 2010. - Ст. ITuQ39

Доп.точки доступа:
Gavrilyuk, A.P.; Karpov., S.V.; International Conference on Coherent and Nonlinear Optics(2010 ; Aug. ; 23-26 ; Казань); International Conference on Lasers, Applications, and Technologies(2010 ; Aug. ; 23-26 ; Казань)
}
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19.

    Processes in resonant domains of metal nanoparticle aggregates and optical nonlinearity of aggregates in pulsed laser fields / A. P. Gavrilyuk, S. V. Karpov // Appl. Phys. B-Lasers Opt. - 2009. - Vol. 97, Is. 1. - P163-173, DOI 10.1007/s00340-009-3592-y. - Cited Reference Count: 43. - Гранты: Authors are thankful to Prof. V. A. Markel ( University of Pennsylvania) for computation of multipole polarizability of silver nanoparticle bispheres, for the attention to this paper, fruitful discussions and great support. This research was supported by grants: 27.1 of the Presidium of RAS, 9.1 DPS RAS, 5 SB RAS, 3818.2008.3 and 6612.2006.3 of the President of RF ( SS RAS), DSP 2.1.1.1814, 05- 03- 32642 RFBR. - Финансирующая организация: [27.1 of the Presidium of RAS]; [9.1 DPS RAS]; [5 SB RAS]; [3818.2008.3]; [6612.2006.3] . - SEP. - ISSN 0946-2171
Рубрики:
SMALL-PARTICLE COMPOSITES
   FRACTAL CLUSTERS
   SELECTIVE PHOTOMODIFICATION
   ABSORPTION-COEFFICIENTS
   REFRACTIVE-INDEXES
   SILVER
   ENHANCEMENT
   RESPONSES
   GOLD
Кл.слова (ненормированные):
Metal nanoparticles -- Nanosecond pulsed laser -- Nonlinear refractive index -- Optical nonlinearity -- Physical effects -- Pulsed-laser field -- Resonant domain -- Silver nanoparticles -- Simple Physical Models -- Aggregates -- Laser excitation -- Nanoparticles -- Nonlinear optics -- Organic polymers -- Pulsed laser applications -- Refractive index -- Silver
Аннотация: Optical nonlinearities in aggregates of nanoparticles formed in silver hydrosols (SHs) are studied under pico- and nanosecond pulsed laser excitation. The dependence of the nonlinear refractive index n (2) on the degree of hydrosol aggregation is studied experimentally at the wavelength lambda=1.064 mu m. It is found that n (2) changes sign when the degree of hydrosol aggregation is increased. Various physical effects occurring in resonant domains of the aggregates are analyzed using a simple physical model of two bound silver nanoparticles. The theory takes into account thermal, elastic, electrostatic, and light-induced effects. Experimental results are discussed in the context of this theory.

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Russian Acad Sci, Inst Computat Modeling, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660028, Russia

Доп.точки доступа:
Gavrilyuk, A. P.; Гаврилюк, Анатолий Петрович; Karpov, S. V.; Карпов, Сергей Васильевич
}
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20.

Описание изобретения к патенту 2351064


    Способ рекуперации электрической энергии в импульсных установках и устройство для его осуществления / Д. А. Великанов ; патентообладатель Институт физики им. Л.В. Киренского Сибирского отделения РАН. - № 2007126455/09 ; Заявл. 11.07.2007 // Изобретения. Полезные модели : офиц. бюл. Фед. службы по интеллектуал. собственности (Роспатент). - 2009. - № 9
   Перевод заглавия: Method of electric energy recuperation in impulse aggregates, and device for method implementation
Аннотация: Изобретение относится к электротехнике и может быть использовано для генерации импульсов в активно-индуктивных нагрузках. Технический результат состоит в снижении тепловых потерь при перезарядке, в получении однополярных импульсов тока, в отсутствии необходимости коммутации полярности тока дозарядки, в упрощении конструкции и схемы управления ключом. Способ рекуперации электрической энергии заключается в преобразовании магнитной энергии электрического тока, полученной в результате преобразования энергии заряженного емкостного накопителя в магнитную энергию электрического тока, в энергию емкостного накопителя. В течение одного цикла работы импульсной установки преобразование энергии емкостного накопителя в магнитную энергию электрического тока и наоборот производится дважды. На первом этапе энергия емкостного накопителя преобразуется в магнитную энергию тока в активно-индуктивной нагрузке с последующей рекуперацией энергии в емкостный накопитель. На втором этапе энергия емкостного накопителя преобразуется в магнитную энергию тока в катушке индуктивности с последующей рекуперацией энергии в емкостный накопитель. Устройство содержит подключаемый к зарядному устройству емкостный накопитель энергии, параллельно которому подключены последовательно соединенные активно-индуктивная нагрузка и первый ключ. В него введена цепь из последовательно соединенных катушки индуктивности и второго ключа, которая подключена параллельно емкостному накопителю энергии. Первый вывод емкостного накопителя, первый вывод активно-индуктивной нагрузки и первый вывод катушки индуктивности соединены между собой и подключаются к положительному выводу зарядного устройства. Второй вывод активно-индуктивной нагрузки подключен к аноду первого ключа, второй вывод катушки индуктивности подключен к катоду второго ключа. Второй вывод емкостного накопителя, катод первого ключа и анод второго ключа соединены между собой и подключаются к отрицательному выводу зарядного устройства. 2 н. и 5 з.п. ф-лы, 3 ил.
Invention concerns electric equipment and can be applied for impulse generation in active inductance loads. Method of electric power recuperation involves transformation of magnetic energy of electric current, obtained by transformation of charged capacitive storage energy into magnetic energy of electric current, into capacitive storage energy. During one cycle of impulse aggregate operation capacitive storage energy to magnetic energy of electric current and back is performed twice. At the first stage, capacitive storage energy is transformed into magnetic current energy in active inductance load with further energy recuperation to capacitive storage. At the second stage, capacitive storage energy is transformed into magnetic current energy in inductance coil with further energy recuperation to capacitive storage. Device includes capacitive storage connected to charging device and parallel to sequence of active inductance load and first key. Additionally device includes a circuit of sequential inductance coil and second key, circuit connected parallel to capacitive storage. First output of capacitive storage, first output of active inductance load and first output of inductance coil are interconnected and connected to positive output of charging device. Second output of active inductance load is connected to anode of first key, second output of inductance coil is connected to cathode of second key. Second output of capacitive storage, cathode of first key and anode of second key are interconnected and connected to negative output of charging device./p p num="34"EFFECT: reduced heat loss during recharge, obtaining monopolar current impulses, eliminated necessity of charge current polarity commutation, simplified construction and key control scheme./p p num="35"7 cl, 3 dwg, 2 ex/p

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Институт физики им. Л.В. Киренского Сибирского отделения РАН

Доп.точки доступа:
Великанов, Дмитрий Анатольевич; Институт физики им. Л.В. Киренского Сибирского отделения РАНФедеральная служба по интеллектуальной собственности (Роспатент); Федеральный институт промышленной собственности
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