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An update on inert anodes for aluminium electrolysis / A. S. Yasinskiy, S. K. Padamata, P. V. Polyakov, A. V. Shabanov // Non-Ferrous Met. - 2020. - Vol. 48, Is. 1. - P. 15-23, DOI 10.17580/nfm.2020.01.03. - Cited References: 62. - The work is performed as a part of the state assignment for the science of Siberian Federal University, project number FSRZ-2020-0013. Use of equipment of Krasnoyarsk Regional Center of Research Equipment of Federal Research Center “Krasnoyarsk Science Center SB RAS” is acknowledged . - ISSN 2072-0807
Кл.слова (ненормированные):
Inert anodes -- aluminium electrolysis -- CO2 emission -- metallic anode -- cermet anode -- ceramic anode -- oxygenevolving electrode -- fluoride melt -- corrosion -- oxidation -- low-temperature electrolyte -- Hall-Heroult cell
Аннотация: This update includes the literature related to the inert anodes which were published in the past decade. The metallic anodes are widely regarded as promising candidates to replace the carbon anodes due to its attractive properties like good electrical conductivity, easy to manufacture and high resistance to high thermal shocks. The metals have been tested in pure state and alloy (binary, ternary) form. The oxide scale formed on the anode surface acts as a barrier between the electrolyte and the anode, which protects the anode from being dissolved. The layer of molten fluorides is formed between the scale and the metal anode after a certain time of polarization, and the oxide scale acts as a bipolar electrode. Metal like Cu is reduced at the internal side of the scale. This paper elaborates the effects of various parameters on the performance of the anode. Cu-based alloys (Cu – Ni – Fe and Cu – Al) have shown promising results and could perform well in low-temperature electrolytes. It has been well established that the Cu content in Cu – Ni – Fe and Cu – Al alloys plays a major role in the metal dissolution as the CuO/Cu2O scales formed on the outer layer act as a sacrificial one. The corrosion rate of an anode can be reduced by decreasing the operating temperature, which is possible by using the KF – AlF3 melts. The use of suspensions can increase the purity of the produced metal by stop-ping the anode products to come in contact with cathode metal. Many industries including RUSAL and ELYSIS are still conducting a considerable amount of research to develop an inert anode and are expecting to have a carbon-free cell in the nearest future.

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Держатели документа:
Laboratory of Physics and Chemistry of Metallurgical Processes and Materials, Siberian Federal University, Krasnoyarsk, Russian Federation
Laboratory of Molecular Spectroscopy, Krasnoyarsk Science Center SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Yasinskiy, A. S.; Padamata, S. K.; Polyakov, P. V.; Shabanov, A. V.; Шабанов, Александр Васильевич
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Bi2(Sn0.95Cr0.05)2O7: Structure, IR spectra, and dielectric properties / S. S. Aplesnin [et al.] // Ceram. Int. - 2016. - Vol. 42, Is. 4. - P. 5177-5183, DOI 10.1016/j.ceramint.2015.12.040. - Cited References: 45. - This work was supported by the Russian Foundation for Basic Research Projects no. 15-42-04099 r_siberia_a, Siberian Branch of Science and NAS of Belarus “Electronic and magnetic phase transitions in materials with magnetoelectric affect” and government work no. 114090470016. . - ISSN 0272-8842

РУБ Materials Science, Ceramics
Рубрики:
BISMUTH PYROSTANNATE
   PYROCHLORE STRUCTURE
   MAGNETIC-PROPERTIES
   PARTIAL OXIDATION
   HIGH-TEMPERATURE
   X-RAY
   Bi2Sn2O7
   SUBSTITUTION
   CATALYSTS
   DIFFRACTION
Кл.слова (ненормированные):
Bismuth pyrostannate -- Infrared absorption spectra -- Structural transition -- Permittivity -- Debye model
Аннотация: Infrared absorption spectra of the bismuth pyrostannate Bi2(Sn0.95Cr0.05)2O7 were investigated in the frequency range 350-1100 cm-1 at temperatures of 110-525 K. Four frequency regions with split absorption lines are distinguished. Softening of frequencies at the structural transitions was observed. The maxima of permittivity measured in the frequency range 1-200 kHz at temperatures 100-400 K were determined. It was found that the magnetic susceptibility changes its sign in the low-temperature region. The correlation between anomalies in the magnetic susceptibility, permittivity, and absorption line intensity was established. Softening of frequencies is explained by the variation in the coefficient of thermal expansion of the lattice. The temperature behavior of permittivity is described using the Debye model. © 2015 Elsevier Ltd and Techna Group S.r.l.

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Держатели документа:
Kirensky Institute of Physics, Russian Academy of Sciences, Siberian Branch, Akademgorodok 50, Krasnoyarsk, Russian Federation
Siberian State Aerospace University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Aplesnin, S. S.; Аплеснин, Сергей Степанович; Udod, L. V.; Удод, Любовь Викторовна; Sitnikov, M. N.; Shestakov, N. P.; Шестаков, Николай Петрович
}
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Chemistry of vinylidene complexes—XXVII—new µ-vinylidene MnPt complexes with platinum-coordinated 1-adamantyl isocyanide ligand: spectroscopic, structural and electrochemical study / V. V. Verpekin, O. S. Chudin, A. A. Kondrasenko [et al.] // Transition Met. Chem. - 2022. - Vol. 47. Is. 7-8. - P. 283-292, DOI 10.1007/s11243-022-00511-w. - Cited References: 46. - This work was conducted within the framework of the budget project 0287–2021-0012 for Institute of Chemistry and Chemical Technology SB RAS . - ISSN 0340-4285
Кл.слова (ненормированные):
Binary alloys -- Cyanides -- Ligands -- Manganese alloys -- Nuclear magnetic resonance spectroscopy -- Platinum compounds -- Redox reactions -- Chemical oxidation -- Electrochemical studies -- Isocyanide ligands -- Redox property -- Spectroscopic studies -- Structural studies -- Vinylidene complexes -- X-ray diffraction studies -- Platinum alloys
Аннотация: New binuclear MnPt µ-vinylidene complexes Cp(CO)2Mn(µ-C=CHPh)Pt(CN–Ad)(L) [L=PPh3 (1a), P(OPri)3 (2a)] bearing a terminal platinum-coordinated 1-adamantyl isocyanide ligand were prepared by the treatment of Cp(CO)2Mn(µ-C=CHPh)Pt(CO)(L) [L=PPh3 (1b), P(OPri)3 (2b)] with CN-Ad. At the same time the reaction between Cp(CO)2Mn(µ-C=CHPh)Pt(L)2 [L=PPh3 (1c), P(OPri)3 (2c)] and CN-Ad did not proceed. The new complexes were characterized by IR and 1H, 13C, 31P NMR spectroscopy. The molecular structure of Cp(CO)2Mn(µ-C=CHPh)Pt(CN–Ad)[P(OPri)3] (2a) was determined by an X-ray diffraction study. The redox properties of the new complexes and their reactions of chemical oxidation were studied. An influence of the platinum-coordinated 1-adamantyl isocyanide ligand on the properties of the synthesized µ-vinylidene compounds 1a and 2a was revealed.

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Держатели документа:
Institute of Chemistry and Chemical Technology SB RAS, Federal Research Center “Krasnoyarsk Science Center SB RAS”, Akademgorodok, 50-24, Krasnoyarsk, 660036, Russian Federation
Institute of Physics SB RAS, Federal Research Center “Krasnoyarsk Science Center SB RAS”, Akademgorodok, 50-38, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Svobodny Prospect, 79, Krasnoyarsk, 660041, Russian Federation

Доп.точки доступа:
Verpekin, V. V.; Chudin, O. S.; Kondrasenko, A. A.; Burmakina, G. V.; Vasiliev, A. D.; Васильев, Александр Дмитриевич; Zimonin, D. V.; Rubaylo, A. I.
}
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Chiganov, A. S.
Selective inhibition of the oxidation of nanodiamonds for their cleaning / A. S. Chiganov // Phys. Solid State. - 2004. - Vol. 46, Is. 4. - P. 620-621, DOI 10.1134/1.1711436. - Cited References: 6 . - ISSN 1063-7834

РУБ Physics, Condensed Matter

Аннотация: The effect of selective inhibition of nanodiamond oxidation upon heating of detonation carbon in air is used to extract nanodiamonds from the detonation products. The methods for cleaning nanodiamonds from nondiamond carbon modifications are described depending on the synthesis conditions. (C) 2004 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, Siberian Div, Krasnoyarsk Sci Ctr, Dept Phys Nanophase Mat, Krasnoyarsk 660036, Russia
КНЦ СО РАН, ОФНМ
Dept. of the Phys. of Nanophase Mat., Krasnoyarsk Scientific Center, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
}
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    Crystal structure and magnetic properties of Mn substituted ludwigite Co3O2BO3 / Yu. V. Knyazev [et al.] // J. Magn. Magn. Mater. - 2012. - Vol. 324, Is. 6. - P. 923-927, DOI 10.1016/j.jmmm.2011.07.044. - Cited References: 15. - The study was supported by the Russian Foundation for Basic Research (Project no. 09-02-00171-a), the Federal Agency for Science and Innovation (Rosnauka) (Project no. MK-5632.2010.2), the Physical Division of the Russian Academy of Science, the program "Strongly Correlated Electrons", Project 2.3.1. . - ISSN 0304-8853
   Перевод заглавия: Кристаллическая структура и магнитные свойства Mn-замещенного людвигита Co3O2BO3

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
BOND VALENT SUMS
   COORDINATION CHEMISTRY
   OXIDATION -STATE
   O BONDS
   COMPLEXES
   MANGANESE
   COBALT
Кл.слова (ненормированные):
Transition metal oxyborate -- Distinct crystallographic position -- Spin glass magnetic ordering
Аннотация: The needle shape single crystals Co3−x MnxO2BO3 with ludwigite structure have been prepared. According to the X-ray diffraction data the preferable character of distinct crystallographic positions occupation by Mn ions is established. Magnetization field and temperature dependencies are measured. Paramagnetic Curie temperature value Θ=−100 K points out the predominance of antiferromagnetic interactions. Spin-glass magnetic ordering takes the onset at TN=41 K. The crystallographic and magnetic properties of Co3O2BO3:Mn are compared with the same for the isostructural analogs Co3O2BO3 and CoO2BO3:Fe.

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Доп.точки доступа:
Knyazev, Yu.V.; Князев, Юрий Владимирович; Ivanova, N. B.; Иванова, Наталья Борисовна; Kazak, N. V.; Казак, Наталья Валерьевна; Platunov, M. S.; Платунов, Михаил Сергеевич; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Vasiliev, A. D.; Васильев, Александр Дмитриевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Yurkin, G. Yu.; Юркин, Глеб Юрьевич
}
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Decoration of carbon nanomaterial powders with dispersed platinum metal particles / V. G. Isakova [et al.] // Russ. J. Appl. Chem. - 2018. - Vol. 91, Is. 7. - P. 1209-1216, DOI 10.1134/S1070427218070212. - Cited References: 22. - The study was performed with the support and equipment of the Center for Shared Use of the Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences. . - ISSN 1070-4272. - ISSN 1608-3296

РУБ Chemistry, Applied
Рубрики:
NANOPARTICLES
   PALLADIUM
   FULLERENE
   ELECTRODE
   NANOTUBES
   OXIDATION
Кл.слова (ненормированные):
carbon nanomaterials -- platinum metal nanoparticles -- in situ one-step method
Аннотация: Carbon nanomaterials (fullerite, detonation nanodiamonds, Taunit, fullerenol, fullerene-containing black) were decorated with platinum group metal nanoparticles in situ in one step by low-temperature combustion (~250–270°С) of a powdered mixture of platinum metal acetylacetonate [Pt-M(асас)n, Pt-М = Pt(II), Pd(II), Rh(III), Ir(III), acac = CH3COCHCOCH3, n is the oxidation state of Pt-М] with carbon nanomaterials in air. As shown by thermal analysis, the process is based on thermal oxidative degradation of the organometallic complex, catalyzed by carbon nanomaterials, with oxidation (combustion) of the organic moiety and release of the metal into the condensed phase. The thermal process in an open system occurs in the glowing mode (210–250°С); the size of the nanoparticles formed is 7–30 nm. Under the conditions restricting the air access to the reaction mixture and free outflow of gaseous products formed by oxidation of acac ligands, the nanoparticle size decreases to 3–10 nm. The particle size depends on the metal amount in the initial powder mixture and on the support morphology.

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Публикация на русском языке Декорирование порошков углеродных наноматериалов дисперсными частицами платиновых металлов [Текст] : статья / В. Г. Исакова [и др.] // Журн. прикл. химии. - 2018. - Т. 91 № 7. - С. 1040-1048

Держатели документа:
Russian Acad Sci, Kirenksy Inst Phys, Separate Dept, Fed Res Ctr,Krasnoyarsk Sci Ctr,Siberian Branch, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Fed Res Ctr, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Isakova, V. G.; Исакова, Виктория Гавриловна; Osipova, I. V.; Осипова, Ирина Владимировна; Dudnik, A. I.; Дудник, Александр Иванович; Cherepakhin, A. V.; Черепахин, Александр Владимирович; Zharikova, N. V.; Nemtsev, I. V.; Volochaev, M. N.; Center for Shared Use of the Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences
}
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Effect of calcination temperature on activity of Fe2O3-Al2O3 nanocomposite catalysts in CO oxidation / A. M. Kremneva, A. V. Fedorov, O. A. Bulavchenko [et al.] // Catal. Lett. - 2020. - Vol. 150. - P. 3377-3385, DOI 10.1007/s10562-020-03250-8. - Cited References: 31. - This work was supported by the Russian Science Foundation (Grant No. 17-73-20157). The experiments were performed using facilities of the shared research center "National center of investigation of catalysts" at Boreskov Institute of Catalysis. The authors thank A.Yu. Gladky for the TPR measurements and Z.S. Vinokurov for the XRD measurements. . - ISSN 1011-372X. - ISSN 1572-879X

РУБ Chemistry, Physical
Рубрики:
MOSSBAUER
   SPECTROSCOPY
   CHEMISTRY
   IRON
   XPS
   ADSORPTION
   OXYGEN
   FE
Кл.слова (ненормированные):
Environmental catalysis -- Nanostructure -- Gasification -- Oxidation -- Mossbauer spectroscopy
Аннотация: Nanocomposite Fe–Al oxide catalysts were prepared by the melting of iron and aluminum nitrates with the subsequent calcination in air at different temperatures. It was found that the catalysts calcined at 450 °C are more active in the oxidation of CO than the catalysts calcined at 700 °C. X-ray diffraction and X-ray photoelectron spectroscopy showed that all the catalysts consist of hematite, α-Fe2O3 nanoparticles, and Al2O3 in an amorphous state. Iron oxide is the active component, which provides the oxidation of CO, while alumina is a texture promoter. The increase in the calcination temperature leads to a minor increase in the average size of hematite nanoparticles and an insignificant decrease in the specific surface area. Kinetic measurements showed that the oxidation of CO over the Fe–Al catalysts calcined at 450 and 700 °C proceeds with the activation energy of 61–69 and 91 kJ/mol, respectively. This means that the low-temperature and high-temperature catalysts contain different active species. Temperature-programmed reduction with CO indicated that the decrease in the calcination temperature improves the reducibility of the Fe-Al nanocomposites. According to 57Fe Mössbauer spectroscopy, the low-temperature catalysts contain hydrated iron oxides (acagenite and ferrihydrite) and a significant amount of highly defective hematite, which is absent in the high-temperature catalyst. These species can provide the enhanced activity of the low-temperature catalysts in the oxidation of CO.

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Держатели документа:
Boreskov Inst Catalysis, Novosibirsk 630090, Russia.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kremneva, A. M.; Fedorov, A. V.; Bulavchenko, O. A.; Knyazev, Yu. V.; Князев, Юрий Владимирович; Saraev, A. A.; Yakovlev, V. A.; Kaichev, V. V.; Russian Science FoundationRussian Science Foundation (RSF) [17-73-20157]; National center of investigation of catalysts" at Boreskov Institute of Catalysis
}
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Effect of exposure to optical radiation and temperature on the electrical and optical properties of In2O3 films produced by autowave oxidation / I. A. Tambasov [et al.] // Semiconductors. - 2014. - Vol. 48, Is. 2. - P. 207-211, DOI 10.1134/S1063782614020286. - Cited References: 42. - This study was supported by the Ministry of Education and Science of the Russian Federation, Federal Targeted Program "Research and Development in Priority Fields of Development of the Science and Technology Complex of Russia for 2007-2013", state contract no. 14.513.11.0023. . - ISSN 1063-7826. - ISSN 1090-6479

РУБ Physics, Condensed Matter
Рубрики:
GAS SENSOR RESPONSE
   INDIUM OXIDE-FILMS
   THIN-FILMS
   HIGH-PERFORMANCE
   TIN OXIDE
   TRANSPARENT CONDUCTORS
   SUBSTRATE-TEMPERATURE
   ROOM-TEMPERATURE
   TRANSISTORS
   PHOTOREDUCTION
Аннотация: Indium-oxide films are synthesized by the autowave-oxidation reaction. It is shown that, upon exposure to optical radiation, the resistance of the films sharply decreases and the maximal relative change in the resistance is 52% at room temperature. Two resistance relaxation rates after termination of the irradiation, 15 Omega s(-1) during the first 30 s and 7 Omega s(-1) over the remaining time, are determined. The data of infrared spectroscopy of the films show that exposure to optical radiation induces a 2.4% decrease in the transmittance at a wavelength of 6.3 mu m. It is found that, after termination of the irradiation, the transmittance gradually increases with a rate of 0.006% s(-1). It is suggested that photoreduction is the dominant mechanism responsible for changes in the electrical and optical properties of the In2O3 films.

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Публикация на русском языке Влияние фотооблучения и температуры на электрические и оптические свойства пленок In2O3, полученных автоволновым окислением [Текст] / И. А. Тамбасов [и др.] // Физ. и техника полупроводников : Санкт-Петербургская издательская фирма "Наука" РАН, 2014. - Т. 48 Вып. 2. - С. 220-224

Держатели документа:
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Siberian State Aerosp Univ, Krasnoyarsk 660037, Russia
Joint Stock Co Academician MF Reshetnev Informat, Zheleznogorsk 662972, Russia

Доп.точки доступа:
Tambasov, I. A.; Тамбасов, Игорь Анатольевич; Myagkov, V. G.; Мягков, Виктор Григорьевич; Ivanenko, A. A.; Иваненко, Александр Анатольевич; Bykova, L. E.; Быкова, Людмила Евгеньевна; Yozhikova, E. V.; Maksimov, I. A.; Ivanov, V. V.; Ministry of Education and Science of the Russian Federation [14.513.11.0023]
}
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    Features of phase equilibria and properties of phases in the Sb-Sm-Se system / M. A. Shtykova, V. P. Vorob'eva, P. P. Fedorov [et al.] // J. Solid State Chem. - 2022. - Vol. 316. - Ст. 123573, DOI 10.1016/j.jssc.2022.123573. - Cited References: 101. - This research was funded by the Tyumen Oblast Government, as part of the West-Siberian Interregional Science and Education Center's project No. 89-DON (3) . - ISSN 0022-4596
   Перевод заглавия: Особенности фазовых равновесий и свойства фаз в системе Sb-Sm-Se
Кл.слова (ненормированные):
Continuous solid solutions -- Electronic structure -- Multi band -- Optical spectroscopy -- Oxidation state -- Peritectic points -- Phase equilibriums -- Phase properties -- Sb components -- Tie-line -- Energy gap
Аннотация: The purpose of the paper is to establish the position of the tie-lines in the Sb-Sm-Se system at 450 °C and 620 °C, to determine the optical band gap of the phases. The Sb component is in equilibrium with the γ-Sm2Se3-X-Sm3Se4 (ST Th3P4) solid solution region with α-Sm2Se3. A continuous solid solution forms between the SmSb and SmSe (ST NaCl) phases, with which the Sm3Se4 and Sm4Sb3 phases are in equilibrium. The SmSb-Sm3Se4, Sm3Se4-SmSb2, SmSe-Sm3Sb2 phases are also in equilibrium. In the Sb–Sm2Se3–Se system at 450°С, the tie-line passes between the Sb2Se3–Sm2Se3, Sb2Se3-SmSe1.9 phases. In the Sb–Se system based on Sb2Se3, a solid solution of the subtraction type Sb2-X□XSe3 (X = 0–0.04) is formed. In the Sb-Sm-Se system, there is a solid solution of the substitution type along the cuts from Sb2Se3 to the Sm2Se3 (7 mol. % Sm2Se3), SmSe1.9 (4 mol. % SmSe1.9) phases. The extreme compositions of solid solutions have a peritectic point. Due to the change in the position of the tie-lines in the Sb–Sm2Se3–Se system at 620 °C, additional phases appear in the equilibrium samples from the Sb2Se3–Sm2Se3 section (annealing at 450 °C) when heated above 620 °C: Sb, SmSe1.9. The optical band gap of the phases is: Sb2-xSmxSe3 solid solution 1.17–1.19 eV, α-Sm2Se3 1.62 eV. Optical properties of incommensurate SmSe1.9 crystal that were investigated for the first time for this class of crystals indicate complex electronic structure that can be characterized as a multi band gap one, with at least two values of the band gap, 1.08 and 1.68 eV. Using optical spectroscopy, Sm ions in SmSe1.9 are proved to be predominantly in 3+ oxidation state. Previously, the formation of ternary compounds in the system was reported in the literature. Carefully conducted research allows us to assert their absence.

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Держатели документа:
Tyumen State University, Volodarsky Str. 6, Tyumen, 625003, Russian Federation
Institute of Physical Materials Science SB RAS, Sakhyanova Str. 6, Ulan-Ude, 670047, Russian Federation
Prokhorov General Physics Institute of the Russian Academy of Sciences, Vavilov Str. 38, Moscow, 119991, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Akademgorodok Str. 50, Building 38660036, Russian Federation
Siberian Federal University, Krasnoyarsk, Svobodnyj Av. 79660079, Russian Federation
Department of Physical and Applied Chemistry, Kurgan State University, Sovetskaya Str. 63/4, Kurgan640020, Russian Federation
Urals Scientific-Research Institute of Chemicals with Experimental Plant, Montazhnikov Str. 9, Yekaterinburg, 620050, Russian Federation
Institute of Solid State Chemistry, Ural Branch, Russian Academy of Sciences, Pervomaiskaya Str. 91, Yekaterinburg, 620990, Russian Federation

Доп.точки доступа:
Shtykova, M. A.; Vorob'eva, V. P.; Fedorov, P. P.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Aleksandrovsky, A. S.; Александровский, Александр Сергеевич; Elyshev, A. V.; Palamarchuk, I. V.; Yurev, I. O.; Ivanov, A. V.; Habibullayev, N. N.; Abulkhaev, M. U.; Andreev, O. V.
}
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10.

Fransson, J.
Effects of non-orthogonality and electron correlations on the time-dependent current through quantum dots / J. . Fransson, O. . Eriksson, I. . Sandalov // Phys. Rev. B. - 2002. - Vol. 66, Is. 19. - Ст. 195319, DOI 10.1103/PhysRevB.66.195319. - Cited References: 46 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
GREENS-FUNCTION APPROACH
   TUNNEL-JUNCTIONS
   LOCAL OXIDATION
   ANDERSON MODEL
   TRANSPORT
   NONORTHOGONALITY
   CONDUCTANCE
   EQUILIBRIUM
   TRANSISTOR
   IMPURITY
Аннотация: Three issues are analyzed in the physics of time-dependent tunneling current through a quantum dot with strongly correlated electrons coupled to two external contact leads: (i) nonorthogonality of the states of electrons in the leads and in the quantum dot, (ii) non-Fermi statistics of the excitations in the quantum dot, and iii) kinematic shift of the quantum dot levels. The contributions from nonorthogonality effectively decrease the mixing interaction between the leads and the quantum dot and the width of the quantum dot level whereas the Gibbs statistics slightly changes the spectral weights of quantum dot levels, and decreases the widths, but does not introduce drastical changes to the current. The kinematic interactions are taken into account within the loop correction. For the case of block signal, the time-dependent current shows oscillations starting at the onset and termination of the bias voltage pulse.

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Держатели документа:
Univ Uppsala, Condensed Matter Theory Grp, S-75121 Uppsala, Sweden
RAS, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН

Доп.точки доступа:
Eriksson, O.; Sandalov, I.
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