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Разделение локальных магнитных вкладов в монокристалле Co[2]FeBO[5] посредством XMCD-спектроскопии / М. С. Платунов [и др.] // Письма в "Журн. эксперим. и теор. физ.". - 2012. - Т. 96, Вып. 9-10. - С. 723-727. - 16 . - ISSN 0370-274X

ГРНТИ

29.19.41

Аннотация: Проведены температурные измерения спектров рентгеновского поглощения (XAS) и рентгеновского магнитного кругового дихроизма (XMCD) вблизи L[3,2]-краев поглощения Co и Fe на монокристалле людвигита Co[2]FeBO[5]. Обнаружена антипарал. ориентация магн. моментов кобальта и железа. Определены величины коэрц. полей, обусловленных ионами кобальта и железа. Разделены орбитальный (m[l]) и спиновый (m[s]) вклады в полные магн. моменты ионов кобальта и железа. Определены соотношение и направление m[l] и m[s]

Держатели документа:
Институт физики им. Л.В. Киренского СО РАН

Доп.точки доступа:
Платунов, Михаил Сергеевич; Platunov, M. S.; Овчинников, Сергей Геннадьевич; Ovchinnikov, S. G.; Казак, Наталья Валерьевна; Kazak, N. V.; Иванова, Наталья Борисовна; Ivanova, N. B.; Заблуда, Владимир Николаевич; Zabluda, V. N.; Весчке, И.; Счайле, И.; Ламонова, К. В.
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Samoshkina, Yu. E.
Electronic and magnetic states of Pr and Mn in the Pr1–xSrxMnO3 films studied by XANES and XMCD spectroscopy / Y. E. Samoshkina, A. Rogalev // J. Exp. Theor. Phys. - 2018. - Vol. 126, Is. 5. - P. 660-665, DOI 10.1134/S1063776118040131. - Cited References: 35. - We thank V.I. Chichkov and N.V. Andreev (National University of Science and Technology MISiS) for the preparation of the manganite films. - This work was supported by the Russian Foundation for Basic Research (project no. 16-32-00209 mol_a) and a grant of the President of the Russian Federation (NSh-7559.2016.2). . - ISSN 1063-7761
Кл.слова (ненормированные):
Circular dichroism spectroscopy -- Dichroism -- Film growth -- Magnetic moments -- Manganese -- Praseodymium -- Strontium compounds -- X ray absorption
Аннотация: The spectral dependences of X-ray absorption near-edge spectroscopy (XANES) and X-ray magnetic circular dichroism (XMCD) and the field dependences of XMCD near the K edge of Mn and the L2,3 edges of Pr in the Pr0.8Sr0.2MnO3 and Pr0.6Sr0.4MnO3 films at T = 90 K are studied. The spectral dependences point to a mixed valence state of Mn and Pr in the films. It is found that, as compared to XANES, XMCD is more sensitive to the valence state of Pr4+. The field dependences of XMCD point to ferromagnetic behavior of Mn ions and the Van Vleck paramagnetism of Pr ions, which makes a significant contribution to the total magnetization of the films. It is shown that as the Sr concentration increases, the XMCD intensity at the K edge of Mn increases, which indicates a growth of the total magnetic moment of the film due to an increase in the 4p–3d hybridization.

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Публикация на русском языке Самошкина, Юлия Эрнестовна. Электронные и магнитные состояния Pr и Mn в пленках Pr1-xSrxMnO3 по данным спектроскопии XANES и XMCD [Текст] / Ю. Э. Самошкина, А. Л. Рогалев // Журн. эксперим. и теор. физ. - 2018. - Т. 153 Вып. 5. - С. 794-799

Держатели документа:
Kirensky Institute of Physics, Federal Research Center “Krasnoyarsk Scientific Center,” Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, Russian Federation
European Synchrotron Radiation Facility, Grenoble, CS, France

Доп.точки доступа:
Rogalev, A.; Самошкина, Юлия Эрнестовна
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    Magnetic and XMCD studies of Pr1-xSrxMnO3 manganite films / Y. E. Samoshkina [et al.] // J. Magn. Magn. Mater. - 2017. - Vol. 428. - P. 43-49, DOI 10.1016/j.jmmm.2016.12.014. - Cited References: 52. - The work was supported by the Russian Foundation for Basic Research, Project no's. 14-02-01211, 16-32-00209 mol_a, and also the Grant of the President of the Russian Federation no. NSh- 7559.2016.2, and the Ministry of Education and Science of the Russian Federation, Project no. 1362. . - ISSN 0304-8853
   Перевод заглавия: Магнитное и XMCD изучение пленок манганита Pr1−xSrxMnO3
Кл.слова (ненормированные):
Hole-doped manganites -- Thin films -- Magnetic measurements -- Spin-glass behavior -- X-ray magnetic circular dichroism
Аннотация: Magnetic properties of the Pr0.8Sr0.2MnO3 and Pr0.6Sr0.4MnO3 polycrystalline films have been studied using temperature and magnetic field dependences of the static magnetization and X-ray magnetic circular dichroism (XMCD) spectroscopy. For the both compositions, the difference between the temperature dependences of magnetization obtained in the zero fields cooling (ZFC) and field cooling (FC) modes has been revealed. The ZFC curves demonstrate a pronounced maximum at temperature Tm. It is shown that the Tm value dependence on the magnetic field follows the Almeida-Thouless line typical for the classic spin glass, what allows us to assume the possible spin-glass behavior of the films. Effect of the disorder in a direction of the crystallites easy-axis on the difference between FC and ZFC curves has been discussed also. Magnetic field dependences of the sample magnetization are presented by the hysteresis loops with the shape changing upon temperature variation. This behavior has been attributed to the effect of crystallographic anisotropy and Pr ions. The spectra and magnetic field dependences of XMCD at the Pr L2- and Mn K-edges have been studied at 90 K. The magnetic field dependences of the XMCD at the Pr L2-edge had shown Van Vleck paramagnetism from Pr3+ ions. © 2016 Elsevier B.V.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Ural Federal University, Yekaterinburg, Russian Federation
European Synchrotron Radiation Facility (ESRF), BP 220, Grenoble, France
National University of Science and Technology “MISiS”, Moscow, Russian Federation

Доп.точки доступа:
Samoshkina, Yu. E.; Самошкина, Юлия Эрнестовна; Edelman, I. S.; Эдельман, Ирина Самсоновна; Stepanova, E. A.; Neznakhin, D. S.; Ollefs, K.; Andreev, N. V.; Chichkov, V. I.
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Crystal growth, structure, magnetic properties and theoretical exchange interaction calculations of Cu2MnBO5 / S. Sofronova [et al.] // J. Magn. Magn. Mater. - 2016. - Vol. 420. - P. 309-316, DOI 10.1016/j.jmmm.2016.07.019. - Cited References: 35. - X-ray diffraction experiment was carried out at the Centre on Molecular Design and Ecologically Safe Technologies at the Novosibirsk State University. The reported study was funded by Russian Foundation for Basic Research (RFBR) and Government of Krasnoyarsk Territory according to the research project No. 16-42-243028. . - ISSN 0304-8853

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
SPIN-GLASS BEHAVIOR
   SINGLE-CRYSTALS
   SUPEREXCHANGE INTERACTIONS
   LUDWIGITE
   DIELECTRICS
   CO3B2O6NI3B2O6
   WARWICKITES
   FE3O2BO3
   IFEFFIT
   NI3B2O6
Кл.слова (ненормированные):
Oxyborates -- Ludwigites -- XMCD -- EXAFS -- Magnetism
Аннотация: Single crystals of ludwigite Cu2MnBO5 were synthesized by flux growth technique. The detailed structural and magnetic characterizations of the synthesized samples have been carried out. The cations composition of the studied crystal was determined using X-ray diffraction and EXAFS technique, the resulting composition differ from the content of the initial Mn2O3–CuO components of the flux. Magnetic susceptibility measurements and the calculations of the exchange integrals in frameworks of indirect coupling model revealed that monoclinic distortions strongly affect exchange interactions and appearance of magnetic ordering phase at the temperature T=93 K. The hypothesis of the existence of several magnetic subsystems was supposed. © 2016 Elsevier B.V.

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Держатели документа:
L.V. Kirensky Institute of Physics, Siberian Branch of Russian Academy of Science, Krasnoyarsk, Russian Federation
M V Reshetnev Siberian State Aerospace University, Krasnoyarsk, Russian Federation
V.S. Sobolev Institute of Geology and Mineralogy, SB RAS, Novosibirsk, Russian Federation
Novosibirsk State University, Novosibirsk, Russian Federation
Institute of Physics, University of Mainz, Mainz, Germany
Institute of Inorganic and Analytical Chemistry, University of Mainz, Mainz, Germany
Lund University, MAX IV Laboratory, Lund, Sweden
National Research Centre “Kurchatov Institute”, Moscow, Russian Federation

Доп.точки доступа:
Sofronova, S. N.; Софронова, Светлана Николаевна; Moshkina, E. M.; Мошкина, Евгения Михайловна; Nazarenko, I. I.; Назаренко, Илья Иванович; Seryotkin, Yu. V.; Nepijko, S. A.; Ksenofontov, V.; Medjanik, K.; Veligzhanin, A. A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич
}
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Evidence of Co-Fe antiferromagnetic coupling in Co2FeO2BO3 through XMCD study / M. S. Platunov [et al.] // VI Euro-Asian Symposium "Trends in MAGnetism" (EASTMAG-2016) : abstracts / ed.: O. A. Maksimova, R. D. Ivantsov. - Krasnoyarsk : KIP RAS SB, 2016. - Ст. P3.1. - P. 183. - References: 3. - This work has been partially financed by the Council for Grants of the President of the Russian Federation (SP-938.2015.5), the Russian Foundation for Basic Research (project nos. 16-32-60049 mol_a_dk, 16-32-00206 mol_a), SB RAS program № II.2P contract 0358-2015-0005, and UMNIK program . - ISBN 978-5-904603-06-9
Кл.слова (ненормированные):
oxides -- magnetization -- XANES -- XMCD

Доп.точки доступа:
Platunov, M. S.; Платунов, Михаил Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Knyazev, Yu. V.; Князев, Юрий Владимирович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Rogalev, A.; Рогалев А.; Wilhelm, Fabrice; Eugen Weschke, Eugen; Schierle, Enrico; Счайле И.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Euro-Asian Symposium "Trends in MAGnetism"(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); "Trends in MAGnetism", Euro-Asian Symposium(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); Институт физики им. Л.В. Киренского Сибирского отделения РАН

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XMCD and ab initio study of interface-engineered ultrathin Ru/Co/W/Ru films with perpendicular magnetic anisotropy and strong Dzyaloshinskii-Moriya interaction / A. S. Samardak, A. V. Ognev, A. G. Kolesnikov [et al.] // Phys. Chem. Chem. Phys. - 2022. - Vol. 24, Is. 14. - P. 8225-8232, DOI 10.1039/d1cp05456b. - Cited References: 47. - A. V. O., I. G. I. and T. O. thank the Russian Ministry of Science and Higher Education for state support of scientific research conducted under the supervision of leading scientists in Russian institutions of higher education, scientific foundations and state research centers (Project No. 075-15-2021-607) in parts of sample preparation and its magnetic characterization. The micromagnetic simulations performed by M. E. S. were supported by the Russian Ministry of Science and Higher Education under the state task (0657-2020-0013). A. A. P. (ab initio calculations) acknowledges the support from the Russian Foundation for Basic Research (Project No. 19-32-60020) and the Russian Federation President Scholarship for Young Scientists (SP-1640.2021.5). The work of A. S. S. related to the experimental and analytical study of DMI and skyrmion bubbles was supported by the Russian Science Foundation (Project No. 21-42-00041). The authors acknowledge the use of computational resources of the Skoltech supercomputer Zhores47 to obtain the theoretical results presented in this paper. The authors thank ID12 beamline staff for their help during the XMCD experiment and gratefully acknowledge the provision of beamtime (Proposal MA-3661) by the ESRF. The research contribution of M. P. (XMCD anaysis) was partially funded by the Russian Ministry of Science and Higher Education via the budget project of SRF SKIF, Boreskov Institute of Catalysis . - ISSN 1463-9076. - ISSN 1463-9084

РУБ Chemistry, Physical + Physics, Atomic, Molecular & Chemical
Рубрики:
TOTAL-ENERGY CALCULATIONS
CIRCULAR-DICHROISM
MOLECULAR-DYNAMICS
Аннотация: Understanding the nature of recently discovered spin–orbital induced phenomena and a definition of a general approach for “ferromagnet/heavy-metal” layered systems to enhance and manipulate spin–orbit coupling, spin–orbit torque, and the Dzyaloshinskii–Moriya interaction (DMI) assisted by atomic-scale interface engineering are essential for developing spintronics and spin-orbitronics. Here, we exploit X-ray magnetic circular dichroism (XMCD) spectroscopy at the L2,3-edges of 5d and 4d non-magnetic heavy metals (W and Ru, respectively) in ultrathin Ru/Co/W/Ru films to determine their induced magnetic moments due to the proximity to the ferromagnetic layer of Co. The deduced orbital and spin magnetic moments agree well with the theoretically predicted values, highlighting the drastic effect of constituting layers on the system's magnetic properties and the strong interfacial DMI in Ru/Co/W/Ru films. As a result, we demonstrate the ability to simultaneously control the strength of magnetic anisotropy and intermixing-enhanced DMI through the interface engineered inversion asymmetry in thin-film chiral ferromagnets, which are a potential host for stable magnetic skyrmions.

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Держатели документа:
Far Eastern Fed Univ, Inst High Technol & Adv Mat, Vladivostok 690922, Russia.
Skolkovo Inst Sci & Technol, Moscow 121205, Russia.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Boreskov Inst Catalysis SB RAS, Synchrotron Radiat Facil SKIF, Koltsov 630559, Russia.
Kyoto Univ, Inst Chem Res, Uji, Kyoto, Japan.
ESRF European Synchrotron, F-38043 Grenoble 9, France.

Доп.точки доступа:
Samardak, Alexander S.; Ognev, Alexey, V; Kolesnikov, Alexander G.; Stebliy, Maksim E.; Samardak, Vadim Yu; Iliushin, Ilia G.; Pervishko, Anastasiia A.; Yudin, Dmitry; Platunov, M. S.; Платунов, Михаил Сергеевич; Ono, Teruo; Wilhelm, Fabrice; Rogalev, Andrey; Russian Ministry of Science and Higher Education [075-15-2021-607, 0657-2020-0013]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [19-32-60020]; Russian Federation President Scholarship for Young Scientists [SP-1640.2021.5]; Russian Science FoundationRussian Science Foundation (RSF) [21-42-00041]; Russian Ministry of Science and Higher Education
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Unraveling dynamic Jahn-Teller effect and magnetism in FeTiF6×6H2O single crystal / M. S. Platunov, N. A. Fedorova, Yu. V. Pyastolova [et al.] // J. Alloys Compd. - 2024. - Vol. 999. - Ст. 175104, DOI 10.1016/j.jallcom.2024.175104. - Cited References: 51. - The authors thank the Joint Supercomputer Center (JSCC) of the Russian Academy of Sciences. The authors would like to express their sincere gratitude to the ID12 beamline staff their exceptional dedication and professionalism in performing the synchrotron experiment during the challenging circumstances of the COVID-pandemic. We are particularly grateful to the postdocs, scientists, and technicians who took part in the experiment, ensuring its successful completion. We also gratefully acknowledge the provision of beamtime (Proposal HC-4375) by the European Synchrotron Radiation Facility (ESRF). The access to this world-class facility was instrumental in obtaining the high-quality data that formed the basis of our research. We are deeply appreciative of the contributions of all involved, and we extend our heartfelt thanks to each and every one of them . - ISSN 0925-8388. - ISSN 1873-4669
Кл.слова (ненормированные):
Dynamic Jahn-Teller effect -- Density functional theory -- B3LYP -- Magnetic and electronic properties -- Mossbauer spectroscopy -- XMCD -- XANES
Аннотация: Hydrated iron fluoridotitanate (FeTiF6 × 6 H2O) single crystals are fascinating magnetic materials with unique properties. To understand the underlying mechanisms, this study combines X-ray absorption near-edge structure (XANES) and X-ray magnetic circular dichroism (XMCD) techniques, complemented by density functional theory (DFT) calculations. Polarization-dependent X-ray absorption spectroscopy, encompassing XANES and XMCD, is a powerful technique for probing the local structures and magnetic properties of materials. It is element-selective, bulk-sensitive, and compatible with a wide range of experimental conditions. In this study, we used XANES and XMCD spectroscopies to investigate the local structures and magnetic properties of Fe and Ti in FeTiF6 × 6 H2O single crystals. XANES analysis revealed distinct local environments around Fe and Ti, providing insights into their coordination environments. Element-selective magnetization measurement at the Fe K-edge demonstrated that iron sites in the oxidation state Fe2+ have an unambiguous paramagnetic contribution to the magnetization along the b-axis. Notably, the absence of an XMCD signal at the Ti K-edge confirmed the absence of a magnetic moment in Ti atoms within the crystal. DFT calculations corroborate the experimental findings and provide insights into the electronic structure and magnetic interactions. The combined results provide a comprehensive understanding of the dynamic Jahn-Teller effect in FeTiF6 × 6 H2O single crystals, highlighting the significance of polarization-dependent X-ray absorption spectroscopy in unraveling the intricate magnetic behavior of such materials. This study contributes to the fundamental understanding of magnetism in these materials and paves the way for the development of novel magnetic materials with tailored properties.

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Держатели документа:
Synchrotron Radiation Facility SKIF, Boreskov Institute of Catalysis SB RAS, Kol’tsovo 630559 , Russia
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk 660036, Russia
Institute of Chemistry, Far Eastern Branch of RAS, Vladivostok 690022, Russia

Доп.точки доступа:
Platunov, M. S.; Платунов, Михаил Сергеевич; Fedorova, N. A.; Федорова, Наталья А.; Pyastolova, Yu. V.; Пястолова, Юлия Валентиновна; Laptash, N. M.; Knyazev, Yu. V.; Князев, Юрий Владимирович; Tomilin, F. N.; Томилин, Феликс Николаевич; Dubrovskiy, A. A.; Дубровский, Андрей Александрович
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Competing magnetic states in silicene and germanene 2D ferromagnets / D. V. Averyanov, I. S. Sokolov, M. S. Platunov [et al.] // Nano Res. - 2020. - Vol. 13, Is. 12. - P. 3396-3402, DOI 10.1007/s12274-020-3027-y. - Cited References: 58. - This work was supported by National Research Center (NRC) "Kurchatov Institute" (No. 1359, characterization) and the Russian Science Foundation (No. 19-19-00009 (synthesis) and No. 20-79-10028 (magnetization measurements)). D. V. A. also acknowledges support from the President's scholarship (SP 1398.2019.5). The measurements have been carried out using equipment of the resource centers of electrophysical and electron microscopy techniques in NRC "Kurchatov Institute" . - ISSN 1998-0124. - ISSN 1998-0000

РУБ Chemistry, Physical + Nanoscience & Nanotechnology + Materials Science,
Рубрики:
RAY CIRCULAR-DICHROISM
ABSORPTION
Кл.слова (ненормированные):
silicene -- germanene -- 2D ferromagnetism -- X-ray magnetic circular dichroism (XMCD) -- monolayer
Аннотация: Two-dimension (2D) magnets have recently developed into a class of stoichiometric materials with prospective applications in ultra-compact spintronics and quantum computing. Their functionality is particularly rich when different magnetic orders are competing in the same material. Metalloxenes REX2 (RE = Eu, Gd; X = Si, Ge), silicene or germanene — heavy counterparts of graphene — coupled with a layer of rare-earth metals, evolve from three-dimension (3D) antiferromagnets in multilayer structures to 2D ferromagnets in a few monolayers. This evolution, however, does not lead to fully saturated 2D ferromagnetism, pointing at a possibility of coexisting/competing magnetic states. Here, REX2 magnetism is explored with element-selective X-ray magnetic circular dichroism (XMCD). The measurements are carried out for GdSi2, EuSi2, GdGe2, and EuGe2 of different thicknesses down to 1 monolayer employing K absorption edges of Si and Ge as well as M and L edges of the rare-earths. They access the magnetic state in REX2 and determine the seat of magnetism, orbital, and spin contributions to the magnetic moment. High-field measurements probe remnants of the bulk antiferromagnetism in 2D REX2. The results provide a new platform for studies of complex magnetic structures in 2D materials.

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Держатели документа:
Natl Res Ctr Kurchatov Inst, Kurchatov Sq 1, Moscow 123182, Russia.
ESRF European Synchrotron, CS 40220, F-38043 Grenoble 9, France.
ALBA Synchrotron Light Source, Barcelona 08290, Spain.
LOrme Merisiers, Synchrotron SOLEIL, F-91192 Gyf Sur Yvette, France.
RAS, Kirensky Inst Phys, Fed Res Ctr KSC SB, Akad Gorodok 50,Bld 38, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Averyanov, D. V.; Sokolov, Ivan S.; Platunov, M. S.; Платунов, Михаил Сергеевич; Wilhelm, Fabrice; Rogalev, Andrei; Gargiani, Pierluigi; Valvidares, Manuel; Jaouen, Nicolas; Parfenov, Oleg E.; Taldenkov, Alexander N.; Karateev, Igor A.; Tokmachev, Andrey M.; Storchak, V. G.
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Самошкина, Юлия Эрнестовна.
Электронные и магнитные состояния Pr и Mn в пленках Pr1-xSrxMnO3 по данным спектроскопии XANES и XMCD / Ю. Э. Самошкина, А. Л. Рогалев // Журн. эксперим. и теор. физ. - 2018. - Т. 153, Вып. 5. - С. 794-799, DOI 10.7868/S0044451018050115. - Библиогр.: 35. - Работа выполнена при финансовой поддержке РФФИ (грант №16-32-00209 «мол_а»), а также гранта Президента РФ (НШ-7559.2016.2). . - ISSN 0044-4510
Аннотация: Исследованы спектральные зависимости рентгеновского поглощения (XANES) и магнитного кругового дихроизма (XMCD), а также полевые зависимости XMCD вблизи K-края Mn и L2,3-краев Pr в пленках Pr0.8Sr0.2MnO3 и Pr0.6Sr0.4MnO3 при T=90 K. Спектральные зависимости указывают на смешанное валентное состояние Mn и Pr в образцах. При этом установлено, что XMCD-метод по сравнению с XANES является наиболее чувствительным к валентному состоянию Pr4+. Полевые зависимости XMCD-сигнала свидетельствуют о ферромагнитном поведении ионов Mn и ван-флековском парамагнетизме ионов Pr, который вносит существенный вклад в суммарную намагниченность образцов. Показано, что с увеличением концентрации Sr в пленке происходит рост интенсивности XMCD-сигнала на K-крае Mn, что указывает на рост суммарного магнитного момента образца вследствие увеличения 4p-3d-гибридизации.

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Переводная версия Samoshkina Yu. E. Electronic and magnetic states of Pr and Mn in the Pr1–xSrxMnO3 films studied by XANES and XMCD spectroscopy [Текст] / Y. E. Samoshkina, A. Rogalev // J. Exp. Theor. Phys. - 2018. - Vol. 126 Is. 5.- P.660-665

Держатели документа:
European Synchrotron Radiation Facility
Институт физики им. Л. В. Киренского, ФИЦ КНЦ Сибирского отделения Российской академии наук

Доп.точки доступа:
Рогалев, А.Л.; Samoshkina, Yu. E.
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10.

XMCD study of Ru/Co/W/Ru films with strong Dzyaloshinskii-Moriya interaction / A. S. Samardaki [et al.] // IEEE International Magnetics Conference (INTERMAG). - 2018. - Ст. UNSP 1800GW01, DOI 10.1109/INTMAG.2018.8508080. - Cited References: 5 . - ISBN 978-1-5386-6425-4
Аннотация: An enhancement of the spin-orbit effects arising on an interface between a ferromagnet (FM) and a heavy metal (HM) is possible through the strong breaking of the structural inversion symmetry in the layered films. We have found that the introduction of an ultrathin W interlayer between Co and Ru in Ru/Co/Ru films enables to preserve perpendicular magnetic anisotropy (PMA) and simultaneously induce a large interfacial Dzyaloshinskii-Moriya interaction (iDMI). We find that the Ru/Co/W/Ru films have PMA up to 0.35 nm of the nominal thickness of W(tW). The study of the spin-wave propagation in the Damon-Eshbach geometry by Brillouin light scattering (BLS) spectroscopy reveals the drastic increase of the iDMI value with the rising tW. The maximum iDMI of -3.1 erg/cm 2 is observed for tW=0.24 nm, which is 10 times larger than the latter for the quasi-symmetrical Ru/Co/Ru films [1]. Our polycrystalline Ru/Co/W/Ru films were prepared by magnetron sputtering on the SiO 2 substrates at room temperature. The base pressure in the chamber was 10−8 Torr. The working pressure of Ar+ was 10−4 Torr. In order to precise control the thickness of layers, we used low sputtering rates: V(Ru)=0.011 nm/s, V(Co)=0.018 nm/s, V(W)=0.02 nm/s. The Co thickness (tCo) was varied from 0.7 to 1.5 nm. The thickness of the buffer and capping Ru layers (tRu) was 10 and 2 nm, correspondingly. The W thickness (tW) was taken in the range from 0 to 0.4 nm. Polarization dependent X-ray spectroscopy measurements at the Co K− (7709 eV), WL3− (10207 eV) and WL2− (11544 eV) edges on the Ru(10nm)/Co(1nm)/W(x)/Ru(2nm) structures were performed at the ESRF ID12 beamline. Four different samples have been measured with x=0, 0.21, 0.25 and 0.29, where x is the thickness of the layer in nm. The APPLE-II undulator and a Si(111) double crystal monochromator were used to collect the spectra.

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Держатели документа:
Far Eastern Fed Univ, Sch Nat Sci, Vladivostok, Russia.
ESRF, Grenoble, France.
Kirensky Inst Phys, Krasnoyarsk, Russia.

Доп.точки доступа:
Samardaki, A. S.; Kolesnikovi, A.; Ognev, A.; Platunov, M. S.; Платунов, Михаил Сергеевич; Rogalev, A.; IEEE International Magnetics Conference(2018 ; Apr. ; 23-27 ; Singapore)
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