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Belyaev, B. A.
Impedance spectroscopy study of the electrical properties of cation-substituted barium hexaaluminate ceramics / B. A. Belyaev, N. A. Drokin, V. A. Poluboyarov // Phys. Solid State. - 2018. - Vol. 60, Is. 2. - P. 274-280, DOI 10.1134/S1063783418020063. - Cited References:18 . - ISSN 1063-7834. - ISSN 1090-6460

РУБ Physics, Condensed Matter
Рубрики:
DIELECTRIC-RELAXATION
LIQUID-CRYSTALS
SPECTRA
Аннотация: We report on the behavior of frequency and temperature dependences of the impedance of a measuring cell in the form of a parallel-plate capacitor filled with barium hexaaluminate ceramics with four aluminum cations replaced by iron (BaO · 2Fe2O3 · 4Al2O3). The measurements have been performed in the frequency range of 0.5–108 Hz at temperatures of 20-375°C. A technique for determining the electrical properties of the investigated ceramics is proposed, which is based on an equivalent electric circuit allowing the recorded impedance spectra to be approximated with sufficiently high accuracy. The established spectral features are indicative of the presence of two electric relaxation times different from each other by three orders of magnitude. This fact is explained by the difference between the charge transport processes in the bulk of crystallites and thin intercrystallite spacers, for which the charge activation energies have been determined.

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Публикация на русском языке Беляев, Борис Афанасьевич. Исследование электрофизических характеристик катион-замещенной керамики гексаалюмината бария методом импедансной спектроскопии [Текст] / Б. А. Беляев, Н. А. Дрокин, В. А. Полубояров // Физ. тверд. тела. - 2018. - Т. 60 Вып. 2. - С. 269–275

Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Fed Res Ctr KSC SB RAS, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia.
Russian Acad Sci, Inst Solid State Chem & Mechanochem, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Drokin, N. A.; Дрокин, Николай Александрович; Poluboyarov, V. A.; Беляев, Борис Афанасьевич
}
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Korshunov, A. V.
Raman spectra of 1,3,5-trichlorobenzene and 1,3,5-tribromobenzene / A. V. Korshunov, V. E. Volkov // J. Struct. Chem. - 1961. - Vol. 2, Is. 2. - P. 142-147, DOI 10.1007/BF00750990 . - ISSN 0022-4766
Аннотация: 1. Low-frequency Raman spectra of 1,3,5-trichlorobenzene and 1,3,5-tribromobenzene were studied; the results suggest that the compounds are isomorphous. 2. A method for interpreting the lines in low-frequency Raman spectra is described. 3. Certain differences between the spectral characteristics of 1,3,5-trichlorobenzene and 1,3,5-tribromobenzene are attributed to steric factors.

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Публикация на русском языке Коршунов, Анатолий Васильевич. Спектры комбинационного рассеяния света кристаллов 1,3,5-трихлорбензола и 1,3,5-трибромбензола [Текст] / В. Е. Волков, А. В. Коршунов // Журн. структ. химии. - 1961. - Т. 2 № 2. - С. 151-157

Держатели документа:
Institute of Physics, Siberian Division, Academy of Sciences USSR, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Volkov, V. E.; Волков, Валентин Ефремович; Коршунов, Анатолий Васильевич
}
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Tetragonal-tetragonal phase transition in CsScF4 crystal. Study of lattice dynamics and ramsn scattering spectra / A. S. Krylov [et al.] // Фаз. переходы и критич. явл. в конденс. средах : программа межд. конф. / предс. орг. ком. К. С. Александров. - Махачкала, 1998. - Ст. Б2-7. - P. 12

Доп.точки доступа:
Александров, Кирилл Сергеевич \предс. орг. ком.\; Aleksandrov, K. S.; Krylov, A. S.; Крылов, Александр Сергеевич; Vtyurin, A. N.; Втюрин, Александр Николаевич; Shmygol, I. V.; Ageev, A. G.; Институт физики им. Х. И. Амирханова Дагестанского научного центра РАН; Дагестанский государственный университет; "Фазовые переходы и критические явления в конденсированных средах", международная конференция(1998 ; сент. ; 8-11 ; Махачкала)
}
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Effects of orientational disorder in lattice dynamics and raman spectra of Rb2ZnCl4 and CsLiSO4 crystals / A. N. Vtyurin [et al.] // Фаз. переходы и критич. явл. в конденс. средах : программа межд. конф. / предс. орг. ком. К. С. Александров. - Махачкала, 1998. - Ст. Б2-8. - P. 13

Доп.точки доступа:
Александров, Кирилл Сергеевич \предс. орг. ком.\; Aleksandrov, K. S.; Vtyurin, A. N.; Втюрин, Александр Николаевич; Ageev, A. G.; Krylov, A. S.; Крылов, Александр Сергеевич; Shmygol, I. V.; Институт физики им. Х. И. Амирханова Дагестанского научного центра РАН; Дагестанский государственный университет; "Фазовые переходы и критические явления в конденсированных средах", международная конференция(1998 ; сент. ; 8-11 ; Махачкала)
}
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    Manifestation of magnetoelastic interactions in Raman spectra of HoxNd1-хFe3(BO3)4 crystals / A. S. Krylov [et al.] // J. Adv. Dielectr. - 2018. - Vol. 08, Is. 02. - Ст. 1850011, DOI 10.1142/S2010135X1850011X. - Cited References: 32 . - ISSN 2010-135X
   Перевод заглавия: Проявление магнитоупругих взаимодействий в спектрах комбинационного рассеяния кристаллов HoxNd1-xFe3(BO3)4
Кл.слова (ненормированные):
Multiferroic -- magnetoelastic interaction -- Raman spectra -- phase transition -- magnetic ordering
Аннотация: Raman spectra of Ho1-xNdxFe(BO3)4 (x=1, 0.75, 0.5, 0.25) have been studied in temperature range 10-400K. Two compositions (x=1, x=0.75) demonstrate structural phase transition with soft mode restoration. The addition of Nd atoms increases interatomic spacing and decreases the temperature of structural phase transition. The solid solutions (x=0.75, 0.5, 0.25) demonstrate the emergence of the peaks corresponding to magnetoelastic interaction below Neel temperature. The order parameter of the magnetic phase transition has been determined. The equal concentrations of holmium and neodymium atoms prevent magnon soft modes condensation caused by exchange interactions in Fe-O-Fe chains are observed. Calculations confirm the data obtained in the experiment.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Material Research Laboratory, Discipline of Physics and MEMS, Indian Institute of Technology Indore, Simrol, India

Доп.точки доступа:
Krylov, A. S.; Крылов, Александр Сергеевич; Sofronova, S. N.; Софронова, Светлана Николаевна; Gudim, I. A.; Гудим, Ирина Анатольевна; Krylova, S. N.; Крылова, Светлана Николаевна; Kumar, R.; Vtyurin, A. N.; Втюрин, Александр Николаевич; International Workshop on Advanced Dielectric Materials and Their Applications(Oct. 8-11, 2017 ; Xi'an, China)
}
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    Zobov, V. E.
    On the effect of an inhomogeneous magnetic field on high-frequency asymptotic behaviors of correlation functions of spin lattices / V. E. Zobov, M. M. Kucherov // JETP Letters. - 2018. - Vol. 107, Is. 9. - P. 553-557, DOI 10.1134/S002136401809014X. - Cited References: 39 . - ISSN 0021-3640. - ISSN 1090-6487
Рубрики:
HEISENBERG PARAMAGNET
   SYSTEMS
   TIME
   RELAXATION
   DYNAMICS
   SPECTRA
Аннотация: Singular points of spin autocorrelation functions on the imaginary time axis, which determine the arguments of exponential high-frequency asymptotic behaviors, have been analyzed. It has been shown that randomly distributed inhomogeneous magnetic fields expand the wings of spectra of autocorrelation functions and, thereby, intensify the heating of a system subjected to variable magnetic fields, which are used to create effective Hamiltonians or at the saturation of inhomogeneously broadened EPR lines.

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Публикация на русском языке Зобов, Владимир Евгеньевич. О влиянии неоднородного магнитного поля на высокочастотные асимптотики корреляционных функций спиновых решеток [Текст] / В. Е. Зобов, М. М. Кучеров // Письма в Журн. эксперим. и теор. физ. - 2018. - Т. 107 Вып. 9-10. - С. 578-582

Держатели документа:
Russian Acad Sci, Siberian Branch, Fed Res Ctr KSC, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Inst Space & Informat Technol, Krasnoyarsk 660074, Russia.

Доп.точки доступа:
Kucherov, M. M.; Зобов, Владимир Евгеньевич
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Identification of anhydrous CaCl2 and KCaCl3 in natural inclusions by Raman spectroscopy / S. Grishina [et al.] // Chem. Geol. - 2018. - Vol. 493. - P. 532-543, DOI 10.1016/j.chemgeo.2018.07.017. - Cited References: 52. - The manuscript was greatly benefited from revisions of Dr. Matthew Steele-MacInnis and anonymous Reviewer. The authors are grateful to Dr. Sharigin V. for providing the sample and photograph of the chloride segregation from Udachnaya-East pipe, Dr. Mazurov M.P. for providing apatite and forsterite samples and Dr. Polozov A. for drawing the map. The computations were performed using facilities of the Computational Centre of the Research Park of St. Petersburg State University. This work is financially supported by the Russian Foundation for Basic Research (grants 15-05-09345 , 18-05-00682 ) and VEGA grant 1/0560/15. . - ISSN 0009-2541
Кл.слова (ненормированные):
Polymorphs CaCl2 -- Raman spectra -- Magma-salt interaction -- Chlorocalcite -- Daughter mineral -- Ab initio calculations
Аннотация: Anhydrous chlorides - CaCl2, and KCaCl3 (chlorocalcite) were identified as mineral inclusions in halite from the Siberian Large Igneous Province at the contact of magmatic intrusions and evaporates. Chlorocalcite was also found as daughter mineral in polyphase hypersaline inclusions. While Raman spectra of KCaCl3 (chlorocalcite) in natural inclusions are similar to spectra of synthetic analogue, the Raman spectra of natural CaCl2 do not correspond to the published Raman spectra of synthetic CaCl2. Simulations of Raman spectra using ab initio density-functional theory (DFT) allowed us to calculate the spectra of individual polymorphs of CaCl2 and to discriminate anhydrous CaCl2 phases in natural inclusions and synthetic CaCl2. In the spectrum of the Pbcn polymorph of CaCl2 twelve different peaks could be identified at 74, 95, 99, 107, 124, 158, 164, 179, 212, 236, 244, 256 cm−1 in contrast to five peaks in the spectrum of the Pnnm polymorph of CaCl2 at 115, 157, 160, 211 and 252 cm−1. Naturally occurring CaCl2 in inclusions in halite consist of Pbcn polymorph only, which probably results from a mechanical stress on cooling from magmatic to ambient temperatures. However, the Raman spectra of the synthetic CaCl2 corresponds to the Pnnm phase with small contributions of the Pbcn phase. Raman spectra of synthetic KCaCl3 with main peaks at 58, 67, 90, 97, 133, 139, 147, 193 cm−1 agrees well with the spectra of chlorocalcite in the natural inclusions. Positions of each atom in the KCaCl3 structure were refined using the density-functional theory. There are no imaginary phonon modes for the optimized structure, indicating that the structure of KCaCl3 is stable. Calculated Raman spectrum is in a good agreement with the Raman spectrum of synthetic and natural KCaCl3 samples.

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Держатели документа:
Sobolev Institute of Geology and Mineralogy, Siberian Branch of the Russian Academy of Sciences, Koptuyg Avenue 3, Novosibirsk, Russian Federation
Department of Economic Geology, Comenius University, Faculty of Natural Sciences, Ilkovicova 6, Bratislava, Slovakia
Universite de Lille, CNRS, UMR 8516, LASIR, Laboratoire de Spectrochimie Infrarouge et Raman, Lille, France
Universite de Lorraine, CNRS, CREGU, GeoRessources laboratory (UMR 7359), Vandoeuvre-les-Nancy, BP-70239, France
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Akademgorodok 50/38, Krasnoyarsk, Russian Federation
Siberian Federal University, Svobodniy 79, Krasnoyarsk, Russian Federation
Institute of Inorganic Chemistry, Slovak Academy of Sciences, Dubravska cesta 9, Bratislava, Slovakia
Ioffe Institute, St. Petersburg, Russian Federation

Доп.точки доступа:
Grishina, S.; Kodera, P.; Uriarte, L. M.; Dubessy, J.; Oreshonkov, A. S.; Орешонков, Александр Сергеевич; Goryainov, S.; Simko, F.; Yakovlev, I.; Roginskii, E. M.
}
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Restoration of soft modes in Raman spectra of antiferroeelectric (Pb-La)(Zr-Sn-Ti)O3 ceramics / A. N. Vtyurin [et al.] // Joint 14th Rus./CIS/Baltic/Japan Symp. on Ferroelectricity (RCBJSF)/ Young sci. school on the spect. studies of critical dynamics at struct. phase trans. : Abstract book / org. comm. A. N. Vtyurin ; progr. comm. I. N. Flerov. - 2018. - P. 26. - Cited References: . - ISBN 978-5-9651-1144-2

Материалы конференции

Доп.точки доступа:
Vtyurin, A. N. \org. comm.\; Втюрин, Александр Николаевич; Flerov, I. N. \progr. comm.\; Флёров, Игорь Николаевич; Vtyurin, A. N.; Krylov, A. S.; Крылов, Александр Сергеевич; Krylova, S. N.; Крылова, Светлана Николаевна; Oreshonkov, A. S.; Орешонков, Александр Сергеевич; Wei, Xiaoyong; Feng, Yujun; Xu, Ran; Zhao, Tian; Joint Russia/CIS/Baltic/Japan Symposium on Ferroelectricity(14 ; May 14-18, 2018 ; St. Perersburg); Young scientists school on the spectroscopic(May 14-18, 2018 ; St. Perersburg); Физико-технический институт им. А.Ф. Иоффе РАН; Санкт-Петербургский политехнический университет им. Петра Великого
}
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Malakhovskii, A. V.
Influence of the low local symmetry of Er3+ ions on magnetic circular dichroism and absorption spectra of f-f transitions in ErFe3(BO3)4 single crystal / A. V. Malakhovskii, V. V. Sokolov, I. A. Gudim // J. Magn. Magn. Mater. - 2018. - Vol. 465. - P. 700-708, DOI 10.1016/j.jmmm.2018.06.057. - Cited References: 29. - The work was supported by the Russian Foundation for Basic Researches grant 16-02-00273 and by the Project of Russian Academy of Science No. 0356-2017-0030. . - ISSN 0304-8853
Кл.слова (ненормированные):
Er3+ ion -- f-f transitions -- Magnetic circular dichroism -- Rare earth ferroborates
Аннотация: Linearly polarized absorption spectra and magnetic circular dichroism (MCD) spectra of ErFe3(BO3)4 single crystal were measured in the range of 9000–23000 cm−1 at 90 K. The absorption spectra of f-f transitions were decomposed into the Lorentz shape components and intensities of the components were found. MCD spectra permitted us to measure the Zeeman splitting of some transitions and so to determine changes of the Landé factor along the C3 axis of the crystal during these transitions. Optical and magneto-optical properties of f-f transitions in the ErFe3(BO3)4 crystal were compared with those in the ErAl3(BO3)4 crystal. Substantial difference of the properties connected with the difference of the Er3+ ions local symmetry in two crystals was revealed. Large splitting of one of the f-f transitions without magnetic field, which is not possible for the Kramers doublets, was observed. It was explained by appearance of two absorbing centers due to the local decrease of symmetry in the excited state. Appreciable difference of the local vibrations energy in some excited states was revealed.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Малаховский, Александр Валентинович
}
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10.

Magnetic resonance studies of mixed chalcospinel CuCr2SxSe4−x (x = 0; 2) and CoxCu1−xCr2S4 (x = 0.1; 0.2) nanocrystals with strong interparticle interactions / A. I. Pankrats [et al.] // J. Magn. Magn. Mater. - 2018. - Vol. 452. - P. 297-305, DOI 10.1016/j.jmmm.2017.12.092. - Cited References: 31. - The authors thank D.A. Balaev for fruitful and useful discussions. The work at the University of Alabama was supported by the National Science Foundation, United States under Grant No. CHE-1508259. . - ISSN 0304-8853
Кл.слова (ненормированные):
Freezing temperatures -- Individual nanoparticles -- Inhomogeneous broadening -- Inter-particle interaction -- Magnetic dipolar field -- Magnetic resonance spectra -- Nano-sized crystallites -- Resonance characteristic
Аннотация: Magnetic resonance characteristics of mixed chalcospinel nanocrystals CuCr2SxSe4−x (x = 0 and 2) and CoxCu1−xCr2S4 (x = 0.1 and 0.2) have been investigated. It has been established based on TEM, SEM and resonance data that all the samples contain both blocks with sizes from 1 to 50 m of compacted nanosized crystallites and individual nanoparticles with sizes from 10 to 30 nm. The studies provide evidence of strong interparticle interaction in all the samples leading to high values of the blocking temperature. Magnetic dipolar field arise in the boundary regions of interacting adjacent nanocrystals below the blocking temperature. This results in inhomogeneous broadening of the magnetic resonance spectrum along with appearance of additional absorption lines. With increase in magnetic anisotropy at low temperatures, a shift of the resonance field along with line broadening are observed for all the studied compounds due to freezing of the moments in the nanoparticles, both in the individual and compacted ones. A gapped characteristic of the resonance spectrum is established below the freezing temperature Tfr, with the energy gap defined by the averaged magnetic anisotropy . Anionic substitution of sulfur by selenium results in a decrease in the magnetic anisotropy. In contrast, cationic substitution of copper by cobalt increases the magnetic anisotropy due to a strong contribution from the latter ion.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation
UbiQD, LLC, 134 Eastgate Dr, Los Alamos, NM, United States
MINT Center, The University of Alabama, Tuscaloosa, AL, United States

Доп.точки доступа:
Pankrats, A. I.; Панкрац, Анатолий Иванович; Vorotynov, A. M.; Воротынов, Александр Михайлович; Tugarinov, V. I.; Тугаринов, Василий Иванович; Zharkov, S. M.; Жарков, Сергей Михайлович; Zeer, G. M.; Ramasamy, K.; Gupta, A.
}
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