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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Wu L. S., Nikitin S. E., Frontzek M., Kolesnikov A. I., Ehlers G., Lumsden M. D., Shaykhutdinov K. A., Guo, E. -J., Savici A. T., Gai Z., Sefat A. S., Podlesnyak A.
Заглавие : Magnetic ground state of the Ising-like antiferromagnet DyScO3
Коллективы : Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division
Место публикации : Phys. Rev. B: American Physical Society, 2017. - Vol. 96, Is. 14. - Ст.144407. - ISSN 2469-9950, DOI 10.1103/PhysRevB.96.144407. - ISSN 2469-9969(eISSN)
Примечания : Cited References:37. - We thank J. M. Sheng and Q. Zhang for the help with the neutron data refinement. We would like to thank A. Christianson, I. Zaliznyak, M. Mourigal, Z. T. Wang, and C. Batista for useful discussions. The research at the Spallation Neutron Source (ORNL) is supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). Research supported in part by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This work was partly supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division.
Предметные рубрики: THIN-FILMS
FERROELECTRICITY
VISUALIZATION
EXCITATIONS
Аннотация: We report on the low-temperature magnetic properties of the DyScO3 perovskite, which were characterized by means of single crystal and powder neutron scattering, and by magnetization measurements. Below TN = 3.15 K, Dy3+ moments form an antiferromagnetic structure with an easy axis of magnetization lying in the ab plane. The magnetic moments are inclined at an angle of ∼ +/- 28 degrees to the b axis. We show that the ground-state Kramers doublet of Dy3+ is made up of primarily |+/- 15/2 ⟩ eigenvectors and well separated by a crystal field from the first excited state at E1 = 24.9 meV. This leads to an extreme Ising single-ion anisotropy, M⊥/M∥∼ 0.05. The transverse magnetic fluctuations, which are proportional to M⊥2/M∥2, are suppressed, and only moment fluctuations along the local Ising direction are allowed. We also found that the Dy-Dy dipolar interactions along the crystallographic c axis are two to four times larger than in-plane interactions.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Sitnikov M. N.
Заглавие : Magnetocapacitance effect in GdxMn1–xS
Место публикации : Phys. Solid State: MAIK Nauka-Interperiodica / Springer, 2016. - Vol. 58, Is. 6. - P.1148-1153. - ISSN 10637834 (ISSN), DOI 10.1134/S1063783416060032
Примечания : Cited References: 15. - This study was supported by the Russian Foundation for Basic Research (project no. 15-42-04099 r_si-bir_a) and the Ministry of Education and Science of the Russian Federation (state contract no. 114090470016).
Предметные рубрики: Ferroelectricity
Аннотация: The capacitance and dielectric loss tangent of GdxMn1–xS (x ≤ 0.2) solid solutions have been measured at a frequency of 10 kHz without magnetic field and in a magnetic field of 8 kOe in the temperature range of 90–450 K. An increase in the permittivity and a dielectric loss maximum have been detected in the low-temperature region. It has been found that the temperature of the maximum of the imaginary part of the permittivity shifts to higher temperatures with increasing concentration. The magnetocapacitance effect has been revealed for two compositions. The dielectric loss has been described in the Debye model with “freezing” dipole moments and in the orbital-charge ordering model.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mukhin A. A., Vorob'ev G. P., Ivanov V. Y., Kadomtseva A. M., Narizhnaya A. S., Kuz'menko A. M., Popov Y. F., Bezmaternykh L. N., Gudim I. A.
Заглавие : Colossal magnetodielectric effect in SmFe3(BO3)(4) multiferroic
Разночтения заглавия :авие SCOPUS: Colossal magnetodielectric effect in SmFe 3(BO 3) 4 multiferroic
Место публикации : JETP Letters. - 2011. - Vol. 93, Is. 5. - P.275-281. - ISSN 0021-3640, DOI 10.1134/S0021364011050079
Примечания : Cited References: 17. - We are grateful to A.K. Zvezdin and A.P. Pyatakov for the discussion of this work and valuable comments. This work was supported by the Russian Foundation for Basic Research, project nos. 10-02-00846 and 09-02-01355.
Предметные рубрики: FERROELECTRICITY
MAGNETOSTRICTION
GARNETS
Аннотация: The colossal (more than threefold) decrease in the dielectric constant E in the easy-plane SmFe3(BO3)(4) ferroborate in a magnetic field of similar to 5 kOe applied in the basal ab plane of the crystal has been found. A close relation of this effect to anomalies in the field dependence of the electric polarization has been established. It has been shown that this magnetodielectric effect is due to the contribution to E from the electric susceptibility, which is related to the rotation of spins in the ab plane, arises in the region of the antiferromagnetic ordering T T (N) and electric polarization in the magnetic field has been proposed, taking into account the additional anisotropy in the basal plane induced by the magnetoelastic stresses.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kuz'menko A. M., Mukhin A. A., Ivanov V. Y., Kadomtseva A. M., Bezmaternykh L. N.
Заглавие : Effects of the Interaction between R and Fe Modes of the Magnetic Resonance in RFe3(BO3)(4) Rare-Earth Iron Borates
Разночтения заглавия :авие SCOPUS: Effects of the interaction between R and Fe modes of the magnetic resonance in RFe 3(BO 3) 4 rare-earth iron borates
Место публикации : JETP Letters. - 2011. - Vol. 94, Is. 4. - P.294-300. - ISSN 0021-3640, DOI 10.1134/S0021364011160119
Примечания : Cited References: 27. - We are grateful to A. S. Prokhorov for discussion of this work and valuable comments. This work was supported by the Russian Foundation for Basic Research, project nos. 10-02-00846 and 09-02-01355, and the Ministry of Education and Science of the Russian Federation, project no. 16.518.11.7034.
Предметные рубрики: MULTIFERROICS
GDFE3(BO3)(4)
FERROELECTRICITY
Аннотация: Resonance modes that are due to magnetic excitations in the exchange-coupled subsystems of rare-earth ions (R = Nd3+, Sm3+, and Gd3+) and Fe3+ ions have been detected in submillimeter transmission spectra (0.1-0.6 THz) of RFe3(BO3)(4) iron borate-multiferroic single crystals. The strong interaction between spin oscillations of the Fe and R subsystems has been revealed, which determines the behavior of the modes depending on the anisotropy of the exchange splitting of the ground doublet of the R ion. It has been shown that the intensities of coupled modes (contributions to the magnetic permeability) depend strongly on the difference between the g factors of Fe and R ions. This dependence makes it possible to determine the sign of the latter g factor. In particular, a noticeable intensity of exchange Nd modes in NdFe3(BO3)(4) is due to an increase in their contribution at g(perpendicular to,parallel to)(Nd) 0, while in GdFe3(BO3)(4) with g(Gd) approximate to g(Fe) approximate to 2, the Fe and Gd contributions compensate each other and the exchange (Gd) mode is not observed. In spite of the weak interaction of Sm ions with the magnetic field, SmFe3(BO3)(4) exhibits resonance modes, which are attributed to the excitation of Sm ions through the Fe subsystem. DOI: 10.1134/S0021364011160119
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liang K. C., Chaudhury R. P., Lorenz B., Sun Y. Y., Bezmaternykh L. N., Temerov V. L., Chu C. W.
Заглавие : Giant magnetoelectric effect in HoAl3(BO3)(4)
Разночтения заглавия :авие SCOPUS: Giant magnetoelectric effect in HoAl 3(BO 3) 4
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2011. - Vol. 83, Is. 18. - Ст.180417. - ISSN 1098-0121, DOI 10.1103/PhysRevB.83.180417
Примечания : Cited References: 29. - This work was supported by the DOE, the AFOSR, the T.L.L. Temple Foundation, the J.J. and R. Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston.
Предметные рубрики: ELECTRIC POLARIZATION
SINGLE-CRYSTALS
MULTIFERROICS
FERROELECTRICITY
GDFE3(BO3)(4)
TEMPERATURE
TBPO4
Аннотация: A giant magnetoelectric polarization is found in HoAl3(BO3)(4). The polarization in transverse field geometry at 70 kOe reaches 3600 mu C/m(2), which is significantly higher than reported values of linear magnetoelectric or even multiferroic compounds. The magnetostrictive effect is also measured and compared with the magnetoelectricity. The results show that spin-lattice coupling in HoAl3(BO3)(4) is extremely strong and that the magnetic field causes a large polar distortion of the ionic positions in the unit cell.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mo H. D., Nelson C. S., Bezmaternykh L. N., Temerov V. T.
Заглавие : Magnetic structure of the field-induced multiferroic GdFe3(BO3)(4)
Коллективы :
Разночтения заглавия :авие SCOPUS: Magnetic structure of the field-induced multiferroic GdFe 3(BO3)4
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2008. - Vol. 78, Is. 21. - Ст.214407. - ISSN 1098-0121, DOI 10.1103/PhysRevB.78.214407
Примечания : Cited References: 35. - We thank W. Schoenig, D. Coburn, S. Wilkins, and J. Hill for their support at X22C, S. LaMarra for his support at X21, and D. Connor for a critical reading of the manuscript. Use of the National Synchrotron Light Source, Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886.
Предметные рубрики: IRON BORATE GDFE3(BO3)(4)
X-RAY-SCATTERING
POLARIZATION DEPENDENCE
EXCHANGE SCATTERING
RESONANCE
FERROELECTRICITY
Ключевые слова (''Своб.индексиров.''): ferromagnetic materials--gadolinium compounds--iron compounds--magnetic structure--multiferroics--neel temperature--spin dynamics--x-ray scattering
Аннотация: We report a magnetic x-ray scattering study of the field-induced multiferroic GdFe3(BO3)(4). Resonant x-ray magnetic scattering at the Gd L-II,L-III edges indicates that the Gd moments order at T-N approximate to 37 K. The magnetic structure is incommensurate below T-N, with the incommensurability decreasing monotonically with decreasing temperature until a transition to a commensurate magnetic phase is observed at T approximate to 10 K. Both the Gd and Fe moments undergo a spin reorientation transition at T-SR approximate to 9 K such that the moments are oriented along the crystallographic c axis at low temperatures. With magnetic field applied along the a axis, our measurements suggest that the field-induced polarization phase has a commensurate magnetic structure with Gd moments rotated similar to 45 degrees toward the basal plane, which is similar to the magnetic structure of the Gd subsystem observed in zero field between 9 and 10 K, and the Fe subsystem has a ferromagnetic component in the basal plane.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zinenko V. I., Zamkova N. G.
Заглавие : Lattice dynamics of MF3 crystals (M = Al, Ga, and In)
Место публикации : Phys. Solid State: AMER INST PHYSICS, 2000. - Vol. 42, Is. 7. - P1348-1353. - ISSN 1063-7834, DOI 10.1134/1.1131391
Примечания : Cited References: 11
Предметные рубрики: RAMAN-SCATTERING
FERROELECTRICITY
BATIO3
PBTIO3
Аннотация: The phonon spectra, Born effective charges, and dielectric constants epsilon(infinity) for the square AlF3, square GaF3, and square InF3 crystals (where is a vacancy) have been calculated in terms of the generalized Gordon-Kim method. The calculated spectra of lattice vibrations contain no imaginary vibrational frequencies. This suggests the stability of the cubic phase of these compounds but contradicts the observable structural transition from cubic to rhombohedral phase. It is assumed that such a transition in the square AlF3, square GaF3, and square InF3 crystals is brought about by structural defects. The calculated spectrum of lattice vibrations of the "completely defective" crystal M square F-3 (M = Al, Ga, and In) indicates a strong instability of the cubic phase. Within the mean crystal approximation, the cubic phase of M-x M1 - xF3 crystals appears to be unstable at small x less than or equal to 0.05. (C) 2000 MAIK "Nauka/Interperiodica".
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