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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavriliuk A. G., Struzhkin V. V., Lyubutin I. S., Ovchinnikov S. G., Hu M. Y., Chow P.
Заглавие : Another mechanism for the insulator-metal transition observed in Mott insulators
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2008. - Vol. 77, Is. 15. - Ст.155112. - ISSN 1098-0121, DOI 10.1103/PhysRevB.77.155112
Примечания : Cited References: 26
Предметные рубрики: ELECTRONIC-STRUCTURE
SPIN TRANSITION
HIGH-PRESSURES
GDFE3(BO3)(4)
Аннотация: The two widely accepted mechanisms of the insulator-metal Mott-Hubbard transitions which have been considered up until now are driven by the band-filling or bandwidth effects. We found a different mechanism of the Mott-Hubbard insulator-metal transition, which is controlled instead by the changes in the Mott-Hubbard energy U. In contrast to the changes in the bandwidth W in the "bandwidth control" scenario or to the variations of the band-filling n parameter in the "band-filling" scenario, a dramatic decrease in the Mott-Hubbard energy U plays the key role in this mechanism. We have experimentally observed this type of the insulator metal transition in the transition metal oxide BiFeO(3). The decrease in the Mott-Hubbard energy is caused by the high-spin-low-spin crossover in the electronic d shell of 3d transition metal ion Fe(3+) with d(5) configuration under high pressure. The pressure-induced spin crossover in BiFeO(3) was investigated and confirmed by synchrotron x-ray diffraction, nuclear forward scattering, and x-ray emission methods. The insulator-metal transition at the same pressures was found by the optical absorption and dc resistivity measurements.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kuz'menko A. M., Mukhin A. A., Ivanov V. Y., Kadomtseva A. M., Lebedev S. P., Bezmaternykh L. N.
Заглавие : Antiferromagnetic Resonance and Dielectric Properties of Rare-earth Ferroborates in the Submillimeter Frequency Range
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2011. - Vol. 113, Is. 1. - P113-120. - ISSN 1063-7761, DOI 10.1134/S106377611105013X
Примечания : Cited References: 27. - This work was supported by the Russian Foundation for Basic Research, project no. 10-02-00846.
Предметные рубрики: GDFE3(BO3)(4)
SPECTROSCOPY
CRYSTAL
Ключевые слова (''Своб.индексиров.''): antiferromagnetic resonance--basic parameters--effective anisotropy constant--ferroborates--ferroics--ferromagnetic orderings--frequency ranges--magnetic interactions--magnetoresonance--millimeter frequency range--rare earth ions--submillimeters--antiferromagnetic materials--crystallography--erbium--europium--ferromagnetic resonance--ion exchange--magnetic anisotropy--magnetic devices--magnetic structure--permittivity--resonance--antiferromagnetism
Аннотация: The magnetoresonance and dielectric properties of a number of crystals of a new family of multiferroics, namely, rare-earth ferroborates RFe(3)(BO(3))(4) (R = Y, Eu, Pr, Tb, Tb(0.25)Er(0.75)), are studied in the submillimeter frequency range (nu = 3-20 cm(-1)). Ferroborates with R = Y, Tb, and Eu exhibit permittivity jumps at temperatures of 375, 198, and 58 K, respectively, which are caused by the R32 - P3(1)2(1) phase transition. Antiferromagnetic resonance (AFMR) modes in the subsystem of Fe(3+) ions are detected in the range of antiferromagnetic ordering (T T(N)
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Stanislavchuk T. N., Malkin B. Z., Bezmaternykh L. N.
Заглавие : Breaking of the Selection Rules for Optical Transitions in the Dielectric PrFe3(BO3)(4) Crystal by a Praseodymium-Iron Exchange Interaction
Коллективы : RFBR [07-02-01185, 07-02-00704]; Russian Academy of Sciences
Разночтения заглавия :авие SCOPUS: Breaking of the selection rules for optical transitions in the dielectric PrFe3(BO3)4 crystal by a praseodymium-iron exchange interaction
Место публикации : Phys. Rev. Lett.: AMER PHYSICAL SOC, 2009. - Vol. 102, Is. 18. - Ст.187403. - ISSN 0031-9007, DOI 10.1103/PhysRevLett.102.187403
Примечания : Cited References: 26. - This work was supported in part by the RFBR under Grants No. 07-02-01185 and No. 07-02-00704 and by the Russian Academy of Sciences under the Programs for Basic Research.
Предметные рубрики: SINGLE-CRYSTAL
GDFE3(BO3)(4)
PHASE
DYFE3(BO3)(4)
SPECTRUM
LINES
Ключевые слова (''Своб.индексиров.''): magnetic ordering temperatures--optical spectrum--order parameters--point symmetries--selection rules--exchange interactions--neon--praseodymium--single crystals--crystal symmetry
Аннотация: We report on the emergence of new lines in the optical spectrum of the PrFe3(BO3)(4) single crystal at the magnetic ordering temperature. The transitions between singlet crystal-field sublevels of Pr3+ ion with the same transformational properties, strictly forbidden for the trigonal D-3 point symmetry of this ion in PrFe3(BO3)(4), appear below the Neel temperature and grow in intensity as a square of the order parameter. We show that the phenomenon originates from the mixing of wave functions of different Pr3+ sublevels by the Pr-Fe exchange interaction.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kazak N. V., Platunov M. S., Ivanova N. B., Knyazev Yu. V., Bezmaternykh L. N., Eremin E. V., Vasil'ev A. D., Bayukov O. A., Ovchinnikov S. G., Velikanov D. A., Zubavichus Y. V.
Заглавие : Crystal structure and magnetization of a Co3B2O6 single crystal
Место публикации : J. Exp. Theor. Phys.: MAIK Nauka-Interperiodica / Springer, 2013. - Vol. 117, Is. 1. - P.94-107. - ISSN 1063-7761, DOI 10.1134/S1063776113060186
Примечания : Cited References: 43. - The synchrotron measurements were performed at the Kurchatov Center of Synchrotron Radiation and Nanotechnologies (state contract no. 16.552.11.7055).This work was supported by the Russian Foundation for Basic Research (project nos. 12-02-00175-a, 12-02-90410-Ukr_a, 12-02-31543mol_a, 13-02-00958-a), the President of the Russian Federation (grant no. NSh-1044.2012.2), the Siberian Branch of the Russian Academy of Sciences (project no. 38), the Ministry of Education and Science of the Russian Federation (project no. 8365), and an integration project of SO RAN-NAN of Belarus (project no. 29).
Предметные рубрики: ABSORPTION FINE-STRUCTURE
NICKEL ORTHOBORATE
RAY
GDFE3(BO3)(4)
LUDWIGITE
NI3(BO3)2
NI3B2O6
SPECTRA
Аннотация: The crystal structure and magnetic properties of Co3B2O6 single crystals are studied. Orthorhombic symmetry with space group Pnnm is detected at room temperature. The measurements of static magnetization and dynamic magnetic susceptibility reveal two magnetic anomalies at T (1) = 33 K and T (2) = 10 K and an easy-axis magnetic anisotropy. The effective magnetic moment indicates a high-spin state of the Co2+ ion. A spin-flop transition is found at low temperatures and H (sf) = 23 kOe. EXAFS spectra of the K-edge absorption of Co are recorded at various temperatures, the temperature-induced changes in the parameters of the local environment of cobalt are analyzed, and the effective Co-Co and Co-O distances are determined. The magnetic interactions in the crystal are analyzed in terms of an indirect coupling model.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kuz'menko A. M., Mukhin A. A., Ivanov V. Y., Kadomtseva A. M., Bezmaternykh L. N.
Заглавие : Effects of the Interaction between R and Fe Modes of the Magnetic Resonance in RFe3(BO3)(4) Rare-Earth Iron Borates
Разночтения заглавия :авие SCOPUS: Effects of the interaction between R and Fe modes of the magnetic resonance in RFe 3(BO 3) 4 rare-earth iron borates
Место публикации : JETP Letters. - 2011. - Vol. 94, Is. 4. - P.294-300. - ISSN 0021-3640, DOI 10.1134/S0021364011160119
Примечания : Cited References: 27. - We are grateful to A. S. Prokhorov for discussion of this work and valuable comments. This work was supported by the Russian Foundation for Basic Research, project nos. 10-02-00846 and 09-02-01355, and the Ministry of Education and Science of the Russian Federation, project no. 16.518.11.7034.
Предметные рубрики: MULTIFERROICS
GDFE3(BO3)(4)
FERROELECTRICITY
Аннотация: Resonance modes that are due to magnetic excitations in the exchange-coupled subsystems of rare-earth ions (R = Nd3+, Sm3+, and Gd3+) and Fe3+ ions have been detected in submillimeter transmission spectra (0.1-0.6 THz) of RFe3(BO3)(4) iron borate-multiferroic single crystals. The strong interaction between spin oscillations of the Fe and R subsystems has been revealed, which determines the behavior of the modes depending on the anisotropy of the exchange splitting of the ground doublet of the R ion. It has been shown that the intensities of coupled modes (contributions to the magnetic permeability) depend strongly on the difference between the g factors of Fe and R ions. This dependence makes it possible to determine the sign of the latter g factor. In particular, a noticeable intensity of exchange Nd modes in NdFe3(BO3)(4) is due to an increase in their contribution at g(perpendicular to,parallel to)(Nd) 0, while in GdFe3(BO3)(4) with g(Gd) approximate to g(Fe) approximate to 2, the Fe and Gd contributions compensate each other and the exchange (Gd) mode is not observed. In spite of the weak interaction of Sm ions with the magnetic field, SmFe3(BO3)(4) exhibits resonance modes, which are attributed to the excitation of Sm ions through the Fe subsystem. DOI: 10.1134/S0021364011160119
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liang K. C., Chaudhury R. P., Lorenz B., Sun Y. Y., Bezmaternykh L. N., Temerov V. L., Chu C. W.
Заглавие : Giant magnetoelectric effect in HoAl3(BO3)(4)
Разночтения заглавия :авие SCOPUS: Giant magnetoelectric effect in HoAl 3(BO 3) 4
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2011. - Vol. 83, Is. 18. - Ст.180417. - ISSN 1098-0121, DOI 10.1103/PhysRevB.83.180417
Примечания : Cited References: 29. - This work was supported by the DOE, the AFOSR, the T.L.L. Temple Foundation, the J.J. and R. Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston.
Предметные рубрики: ELECTRIC POLARIZATION
SINGLE-CRYSTALS
MULTIFERROICS
FERROELECTRICITY
GDFE3(BO3)(4)
TEMPERATURE
TBPO4
Аннотация: A giant magnetoelectric polarization is found in HoAl3(BO3)(4). The polarization in transverse field geometry at 70 kOe reaches 3600 mu C/m(2), which is significantly higher than reported values of linear magnetoelectric or even multiferroic compounds. The magnetostrictive effect is also measured and compared with the magnetoelectricity. The results show that spin-lattice coupling in HoAl3(BO3)(4) is extremely strong and that the magnetic field causes a large polar distortion of the ionic positions in the unit cell.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Stanislavchuk T. N., Chukalina E. P., Popova M. N., Bezmaternykh L. N., Gudim I. A.
Заглавие : Investigation of the iron borates DyFe3(BO3)(4) and HoFe3(BO3)(4) by the method of Er3+ spectroscopic probe
Разночтения заглавия :авие SCOPUS: Investigation of the iron borates DyFe3(BO3)4 and HoFe3(BO3)4 by the method of Er3+ spectroscopic probe
Место публикации : Phys. Lett. A: ELSEVIER SCIENCE BV, 2007. - Vol. 368, Is. 5. - P408-411. - ISSN 0375-9601, DOI 10.1016/j.physleta.2007.04.044
Примечания : Cited References: 16
Предметные рубрики: GDFE3(BO3)(4)
CRYSTALS
Ключевые слова (''Своб.индексиров.''): rare-earth iron borates--magnetic ordering--optical spectroscopy--magnetic ordering--optical spectroscopy--rare-earth iron borates
Аннотация: Temperature-dependent high-resolution optical spectra of the Er3+ probe ion in DyFe3(BO3)(4) and HoFe3(BO3)(4) are reported. The data provide the temperature of magnetic ordering and direction of the Fe3+ magnetic moments. Both compounds order magnetically at T-N = 39 +/- 1K. The magnetic structure of DyFe3(BO3)(4) is of the easy-axis type, while that of HoFe3(BO3)(4) is of the easy-plane type. The role of anisotropic interactions between the iron and the rare-earth subsystems is discussed. (c) 2007 Elsevier B.V. All rights reserved.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pashchenko M. I., Bedarev V. A., Kut'ko V. I., Besmaternykh L. N., Temerov V. L.
Заглавие : IR active vibrations of a TbFe3(BO3)(4) crystal
Разночтения заглавия :авие SCOPUS: IR active vibrations of a TbFe3(BO3)4 crystal
Место публикации : Low Temp. Phys. - 2010. - Vol. 36, Is. 7. - P.638-641. - ISSN 1063-777X, DOI 10.1063/1.3479413; \b Физика низких температур
Примечания : Cited References: 12
Предметные рубрики: GDFE3(BO3)(4)
Аннотация: The IR reflection spectra of a TbFe3(BO3)(4) crystal are measured in the spectral range 200-2000 cm(-1) in E perpendicular to c polarization at temperatures 10 and 300 K. The reflection spectrum so obtained is analyzed and its interpretation is given on the basis of the internal vibrations of the ionic complexes BO33-, FeO69-, and TbO69- of the TbFe3(BO3)(4) crystal. Davydov splitting on the internal vibrational modes at a structural phase transition, which is accompanied by multiplication of the unit cell, was not observed in the experimental spectral range. This is due to the localization of the vibrations of the ionic complexes BO33-, FeO69-, and TbO69- of the TbFe3(BO3)(4) crystal. (c) 2010 American Institute of Physics. [doi:10.1063/1.3479413]
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Dyakonov V. P., Szymczak R., Prokhorov A. D., Zubov E., Prokhorov A. A., Petrakovskii G. A., Bezmaternykh L. N., Berkowski M., Varyukhin V., Szymczak H.
Заглавие : Magnetic and EPR studies of the EuFe3(BO3)(4) single crystal
Коллективы :
Разночтения заглавия :авие SCOPUS: Magnetic and EPR studies of the EuFe 3(BO 3) 4 single crystal
Место публикации : Eur. Phys. J. B: SPRINGER, 2010. - Vol. 78, Is. 3. - P291-298. - ISSN 1434-6028, DOI 10.1140/epjb/e2010-10059-3
Примечания : Cited References: 23. - A.A. Prokhorov is grateful to Mianowski Fund for financial support.
Предметные рубрики: EARTH
GDFE3(BO3)(4)
MULTIFERROICS
Ключевые слова (''Своб.индексиров.''): absorption lines--antiferromagnetic orderings--applied magnetic fields--basal planes--easy direction of magnetizations--electron paramagnetic resonance--epr measurements--epr spectra--epr studies--europium ions--exchange fields--g factors--lorentz--magnetic measurements--magnetic subsystems--orientation dependence--sub-lattices--temperature dependence--temperature range--trigonal symmetry--zeeman effect--antiferromagnetism--crystal orientation--europium--magnetic fields--magnetic moments--magnetic variables measurement--magnetization--paramagnetic resonance--paramagnetism--single crystals--spectroscopy--electron spin resonance spectroscopy
Аннотация: Magnetic and electron paramagnetic resonance (EPR) properties of EuFe3(BO3)(4) single crystals have been studied over the temperature range of 300-4.2 K and in a magnetic field up to 5 T. The temperature, field and orientation dependences of susceptibility, magnetization and EPR spectra are presented. An antiferromagnetic ordering of the Fe subsystem occurs at about 37 K. The easy direction of magnetization perpendicular to the c axis is determined by magnetic measurements. Below 10 K, we observe an increase of susceptibility connected with the polarization of the Eu sublattice by an effective exchange field of the ordered Fe magnetic subsystem. In a magnetic field perpendicular to the c axis, we have observed an increase of magnetization at T 10 K in the applied magnetic field, which can be attributed to the appearance of the magnetic moment induced by the magnetic field applied in the basal plane. According to EPR measurements, the distance between the maximum and minimum of derivative of absorption line of the Lorentz type is equal to 319 Gs. The anisotropy of g-factor and linewidth is due to the influence of crystalline field of trigonal symmetry. The peculiarities of temperature dependence of both intensity and linewidth are caused by the influence of excited states of europium ion (Eu3+). It is supposed that the difference between the g-factors from EPR and the magnetic measurements is caused by exchange interaction between rare earth and Fe subsystems via anomalous Zeeman effect.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova E. A., Vasiliev A. N., Temerov V. L., Bezmaternykh L. N., Tristan N., Klingeler R., Buchner B.
Заглавие : Magnetic and specific heat properties of YFe3(BO3)(4) and ErFe3(BO3)(4)
Коллективы :
Разночтения заглавия :авие SCOPUS: Magnetic and specific heat properties of YFe3(BO3) 4 and ErFe3(BO3)4
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2010. - Vol. 22, Is. 11. - Ст.116006. - ISSN 0953-8984, DOI 10.1088/0953-8984/22/11/116006
Примечания : Cited References: 26. - This work was supported by DFG grants 436 RUS and HE 3439/6 (FOR 520). The authors are indebted to M N Popova and B Z Malkin for valuable discussions.
Предметные рубрики: LINEAR-CHAIN ANTIFERROMAGNETISM
CRYSTAL-STRUCTURE
GDFE3(BO3)(4)
MULTIFERROICS
BA2COS3
ORDER
Ключевые слова (''Своб.индексиров.''): antiferromagnetic orders--basal planes--experimental data--magnetically ordered state--antiferromagnetism--calorimetry--erbium--magnetic moments--single crystals--specific heat--magnetic domains
Аннотация: The present paper reports on the specific heat and magnetization of the YFe3(BO3)(4) and ErFe3(BO3)(4) single crystals. In both compounds, antiferromagnetic order of the iron spins evolves at T-N = 38 K. The experimental data suggest that the magnetic moments are in the basal plane of the trigonal crystal for both compounds. In the magnetically ordered state the crystal is subdivided into three types of domains, the magnetic moments of the Fe3+ ions being aligned along the a axis within each domain. For ErFe3(BO3)(4), two non-equivalent magnetic positions of the Er3+ ions in each domain are observed.
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