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Application of Raman spectroscopy for identification of rinneite (K3NaFeCl6) in inclusions in minerals / S. Grishina, P. Kodera, S. Goryainov [et al.] // J. Raman Spectrosc. - 2020. - Vol. 51, Is. 12. - P. 2505-2516, DOI 10.1002/jrs.6005. - Cited References: 55. - Russian Foundation for Basic Research, Grant/Award Numbers: 18-05-00682, 18-05-00682; European Regional Development Fund, Grant/Award Number: ITMS 26240220086; Vedecka Grantova Agentura MSVVaS SR a SAV, Grant/Award Number: 1/0313/20 . - ISSN 0377-0486. - ISSN 1097-4555

РУБ Spectroscopy
Рубрики:
SALT MELT
   IRON
   DEPOSIT
   FLUIDS
   TRANSFORMATIONS
   FERRIHYDRITE
Кл.слова (ненормированные):
daughter mineral -- Fe-oxyhydroxides -- fluid inclusion -- rinneite -- weathering
Аннотация: Solid daughter phases in fluid and salt melt inclusions in minerals provide important clues to characterization of mineral‐forming processes. The analysis of the fluid inclusions often requires the exposure of the daughter minerals. Rinneite (K3NaFeCl6), which is a hygroscopic mineral, decomposes in air and cannot thus be identified by conventional methods. A combined approach has been applied for investigation of synthetic and natural rinneite to acquire its diagnostic Raman spectrum for a nondestructive identification. We used natural rinneite inclusions in halite, suitable for applying a complex of methods, to clear up the reference spectrum. Improved high‐resolution X‐ray diffraction (XRD) data obtained from natural rinneite inclusion are comparable with that of previously published, with similar unit cell dimensions. Polarized Raman spectra of natural inclusions were obtained using different geometries and polarization of the incident and scattered light. Interpretation of experimental Raman spectra was performed within the framework of lattice dynamics simulations and group analysis. Individual spectral bands are interpreted in terms of Raman‐active vibrational modes of K3NaFeCl6 structural units. Raman spectrum of synthetic rinneite with main peaks at 75, 91, 103, 143, 167, 171, 187, and 239 cm−1 agrees well with the spectra of rinneite inclusions in halite from the Nepa potash deposit and rinneite daughter minerals in salt melt inclusions hosted by quartz veinlets from the porphyry gold systems in the Central Slovakia Volcanic Field. This provides a firm basis for any future identification of this mineral worldwide, using nondestructive Raman spectroscopy.

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Держатели документа:
Russian Acad Sci, Sobolev Inst Geol & Mineral, Dept Mineral, Siberian Branch, Novosibirsk, Russia.
Comenius Univ, Dept Econ Geol, Fac Nat Sci, Bratislava, Slovakia.
Kirensky Inst Phys, Mol Spect Lab, Krasnoyarsk, Russia.
Siberian Fed Univ, Inst Engn Phys & Radio Elect, Krasnoyarsk, Russia.
Novosibirsk State Univ, Dept Geol, Novosibirsk, Russia.
Slovak Acad Sci, Inst Inorgan Chem, Bratislava, Slovakia.
Russian Acad Sci, Inst Geol Ore Deposits Petrog Mineral & Geochem, Moscow, Russia.

Доп.точки доступа:
Grishina, Svetlana; Kodera, Peter; Goryainov, Sergey; Oreshonkov, A. S.; Орешонков, Александр Сергеевич; Seryotkin, Yurii; Simko, Frantisek; Polozov, Alexander G.; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [18-05-00682]; European Regional Development FundEuropean Union (EU) [ITMS 26240220086]; Vedecka Grantova Agentura MSVVaS SR a SAV [1/0313/20]
}
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Comparative analysis of characteristic electron energy loss spectra and inelastic scattering cross-section spectra of Fe / A. S. Parshin [et al.] // Phys. Solid State. - 2016. - Vol. 58, Is. 5. - P. 908-914, DOI 10.1134/S106378341605019X. - Cited References: 29 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
Loss-spectroscopy
   Quantitative-analysis
   Iron
   Si
   Ge
Аннотация: The inelastic electron scattering cross section spectra of Fe have been calculated based on experimental spectra of characteristic reflection electron energy loss as dependences of the product of the inelastic mean free path by the differential inelastic electron scattering cross section on the electron energy loss. It has been shown that the inelastic electron scattering cross-section spectra have certain advantages over the electron energy loss spectra in the analysis of the interaction of electrons with substance. The peaks of energy loss in the spectra of characteristic electron energy loss and inelastic electron scattering cross sections have been determined from the integral and differential spectra. It has been shown that the energy of the bulk plasmon is practically independent of the energy of primary electrons in the characteristic electron energy loss spectra and monotonically increases with increasing energy of primary electrons in the inelastic electron scattering cross-section spectra. The variation in the maximum energy of the inelastic electron scattering cross-section spectra is caused by the redistribution of intensities over the peaks of losses due to various excitations. The inelastic electron scattering cross-section spectra have been analyzed using the decomposition of the spectra into peaks of the energy loss. This method has been used for the quantitative estimation of the contributions from different energy loss processes to the inelastic electron scattering cross-section spectra of Fe and for the determination of the nature of the energy loss peaks. © 2016, Pleiades Publishing, Ltd.

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Публикация на русском языке Сравнительный анализ спектров характеристических потерь энергии электронов и спектров сечения неупругого рассеяния в Fe [Текст] / А. С. Паршин [и др.] // Физ. тверд. тела : Физико-технический институт им. А. Ф. Иоффе РАН, 2016. - Т. 58 Вып. 5. - С. 881–887

Держатели документа:
Siberian State Aerospace University, ul. Gazety Krasnoyarskii Rabochii 31, Krasnoyarsk, Russian Federation
Institute of Chemistry and Chemical Technology, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50/24, Krasnoyarsk, Russian Federation
Rzhanov Institute of Semiconductor Physics, Siberian Branch, Russian Academy of Sciences, pr. Akademika Lavrent’eva 13, Novosibirsk, Russian Federation
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50/38, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Parshin, A. S.; Igumenov, A. Y.; Mikhlin, Y. L.; Pchelyakov, O. P.; Zhigalov, V. S.; Жигалов, Виктор Степанович
}
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Dimensionality of a system of exchange-coupled grains and magnetic properties of nanocrystalline and amorphous ferromagnets / R. S. Iskhakov [et al.] // JETP Letters. - 2000. - Vol. 72, Is. 6. - P. 304-307, DOI 10.1134/1.1328443. - Cited References: 15 . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
RANDOM ANISOTROPY
   FILMS
   IRON
   SIZE
Аннотация: Characteristics of random magnetic anisotropy in ferromagnetic films of amorphous Co90P10 and nanocrystalline Ni75C25 , Fe80B4C16 , and Co80C20 alloys and also in multilayer films [Co93P7(x)/Pd(14 Angstrom)](20) and [Co90P10(x)/Pd(14 Angstrom)](20) obtained by various technological procedures were studied experimentally. It was found that the spatial dimensionality (d) of the system of ferromagnetically coupled grains (2R(c)) in the materials under study determined the exponent in the power dependence of the approach of magnetization to saturation in the region of fields H 2A / MRc2. The dependence DeltaM similar to H-1/2 was observed for nanocrystalline and amorphous films with a three-dimensional grain arrangement. The approach to saturation in multilayer films with a two-dimensional grain arrangement in an individual magnetic layer follows the law DeltaM similar to H-1. The main micromagnetic characteristics of random anisotropy, such as the ferromagnetic correlation radius R-f and the average anisotropy [K] of a ferromagnetic domain with a size of 2R(f) , were determined for multilayer Co/Pd films. Correlation was found between the coercive field and these characteristics of random anisotropy. (C) 2000 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН

Доп.точки доступа:
Iskhakov, R. S.; Исхаков, Рауф Садыкович; Komogortsev, S. V.; Комогорцев, Сергей Викторович; Balaev, A. D.; Балаев, Александр Дмитриевич; Chekanova, L. A.; Чеканова, Лидия Александровна
}
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Effect of calcination temperature on activity of Fe2O3-Al2O3 nanocomposite catalysts in CO oxidation / A. M. Kremneva, A. V. Fedorov, O. A. Bulavchenko [et al.] // Catal. Lett. - 2020. - Vol. 150. - P. 3377-3385, DOI 10.1007/s10562-020-03250-8. - Cited References: 31. - This work was supported by the Russian Science Foundation (Grant No. 17-73-20157). The experiments were performed using facilities of the shared research center "National center of investigation of catalysts" at Boreskov Institute of Catalysis. The authors thank A.Yu. Gladky for the TPR measurements and Z.S. Vinokurov for the XRD measurements. . - ISSN 1011-372X. - ISSN 1572-879X

РУБ Chemistry, Physical
Рубрики:
MOSSBAUER
   SPECTROSCOPY
   CHEMISTRY
   IRON
   XPS
   ADSORPTION
   OXYGEN
   FE
Кл.слова (ненормированные):
Environmental catalysis -- Nanostructure -- Gasification -- Oxidation -- Mossbauer spectroscopy
Аннотация: Nanocomposite Fe–Al oxide catalysts were prepared by the melting of iron and aluminum nitrates with the subsequent calcination in air at different temperatures. It was found that the catalysts calcined at 450 °C are more active in the oxidation of CO than the catalysts calcined at 700 °C. X-ray diffraction and X-ray photoelectron spectroscopy showed that all the catalysts consist of hematite, α-Fe2O3 nanoparticles, and Al2O3 in an amorphous state. Iron oxide is the active component, which provides the oxidation of CO, while alumina is a texture promoter. The increase in the calcination temperature leads to a minor increase in the average size of hematite nanoparticles and an insignificant decrease in the specific surface area. Kinetic measurements showed that the oxidation of CO over the Fe–Al catalysts calcined at 450 and 700 °C proceeds with the activation energy of 61–69 and 91 kJ/mol, respectively. This means that the low-temperature and high-temperature catalysts contain different active species. Temperature-programmed reduction with CO indicated that the decrease in the calcination temperature improves the reducibility of the Fe-Al nanocomposites. According to 57Fe Mössbauer spectroscopy, the low-temperature catalysts contain hydrated iron oxides (acagenite and ferrihydrite) and a significant amount of highly defective hematite, which is absent in the high-temperature catalyst. These species can provide the enhanced activity of the low-temperature catalysts in the oxidation of CO.

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Держатели документа:
Boreskov Inst Catalysis, Novosibirsk 630090, Russia.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kremneva, A. M.; Fedorov, A. V.; Bulavchenko, O. A.; Knyazev, Yu. V.; Князев, Юрий Владимирович; Saraev, A. A.; Yakovlev, V. A.; Kaichev, V. V.; Russian Science FoundationRussian Science Foundation (RSF) [17-73-20157]; National center of investigation of catalysts" at Boreskov Institute of Catalysis
}
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    Factor analysis of inelastic electron scattering cross section spectra of FeSi2 / A. Y. Igumenov [et al.] // IOP Conf. Ser.: Mater. Sci. Eng. - 2019. - Vol. 467: 21st International Scientific Conference Reshetnev Readings-2017. - Ст. 012010, DOI 10.1088/1757-899X/467/1/012010. - Cited References: 21
Рубрики:
ENERGY-LOSS SPECTROSCOPY
   IRON
Аннотация: Iron disilicide is widely used in creation of such nanotechnology devices as photoelectric converters. The investigation of iron silicide FeSi2 with the method of inelastic electron scattering cross-section spectroscopy was carried out. The decomposition of inelastic electron scattering cross-section spectra of FeSi2 to bulk and surface energy loss components using factor analysis was carried out. The amplitude of energy loss components can be used for identification of their origin.

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Держатели документа:
Reshetnev Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.
Emperor Alexander I St Petersburg State Transport, St Petersburg 190031, Russia.
Russian Acad Sci, Inst Chem & Chem Technol, Siberian Branch, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Rzhanov Inst Semicond Phys, Siberian Branch, Novosibirsk 630090, Russia.
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Igumenov, A. Yu; Parshin, A. S.; Kanzychakova, V. O.; Demin, A. M.; Andryushchenko, T. A.; Mikhlin, Yu L.; Pehelyakov, O. P.; Zhigalov, V. S.; Жигалов, Виктор Степанович; International Scientific Conference Reshetnev Readings(21st ; Nov 08-11, 2017 ; Krasnoyarsk, Russia)
}
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Frequency-dependent magnetotransport phenomena in a hybrid Fe/SiO2/p-Si structure / N. V. Volkov [et al.] // J. Appl. Phys. - 2012. - Vol. 112, Is. 12. - Ст. 123906, DOI 10.1063/1.4769788. - Cited References: 31. - This study was supported by the Russian Foundation for Basic Research, Project No. 11-02-00367-a; the Presidium of the Russian Academy of Sciences, program Quantum Mesoscopic and Disordered Structures, Project No. 20.8; the Division of Physical Sciences of the Russian Academy of Sciences, program Spin Phenomena in Solids Nanostructures and Spintronics, Project No. II.4.3; the Siberian Branch of the Russian Academy of Sciences, Integration Projects Nos. 85 and 102, and the Federal target program Scientific and Pedagogical Personnel of Innovative Russia (State Contract No. NK-556P_15). . - ISSN 0021-8979

РУБ Physics, Applied
Рубрики:
SILICON
   IRON
   SPINTRONICS
   PAIRS
Аннотация: We report the large magnetoimpedance effect in a hybrid Fe/SiO2/p-Si structure with the Schottky barrier. The pronounced effect of magnetic field on the real and imaginary parts of the impedance has been found at temperatures 25-100K in two relatively narrow frequency ranges around 1 kHz and 100MHz. The observed frequency-dependent magnetotransport effect is related to the presence of localized "magnetic" states near the SiO2/p-Si interface. In these states, two different recharging processes with different relaxation times are implemented. One process is capture-emission of carriers that involves the interface levels and the valence band; the other is the electron tunneling between the ferromagnetic electrode and the interface states through SiO2 potential barrier. In the first case, the applied magnetic field shifts energy levels of the surface states relative to the valence band, which changes recharging characteristic times. In the second case, the magnetic field governs the spin-dependent tunneling of carriers through the potential barrier. The "magnetic" interface states originate, most likely, from the formation of the centers that contain Fe ions, which can easily diffuse through the SiO2 layer. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4769788]

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Держатели документа:
[Volkov, N. V.
Tarasov, A. S.
Eremin, E. V.
Eremin, A. V.
Varnakov, S. N.
Ovchinnikov, S. G.] Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
[Volkov, N. V.
Eremin, E. V.
Varnakov, S. N.] Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia

Доп.точки доступа:
Volkov, N. V.; Волков, Никита Валентинович; Tarasov, A. S.; Тарасов, Антон Сергеевич; Eremin, E. V.; Еремин, Евгений Владимирович; Eremin, A. V.; Ерёмин, Александр Владимирович; Varnakov, S. N.; Варнаков, Сергей Николаевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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Gavrichkov, V. A.
Cation spin and superexchange interaction in oxide materials below and above spin crossover under high pressure / V. A. Gavrichkov, S. I. Polukeev, S. G. Ovchinnikov // Phys. Rev. B. - 2020. - Vol. 101, Is. 9. - Ст. 094409, DOI 10.1103/PhysRevB.101.094409. - Cited References: 65. - We acknowledge the support of the Russian Science Foundation through Grant No. 18-12-00022 . - ISSN 2469-9950. - ISSN 2469-9969

РУБ Materials Science, Multidisciplinary + Physics, Applied + Physics, Condensed Matter
Рубрики:
EXCHANGE INTERACTION
   PHASE-TRANSITIONS
   STATE
   ELECTRON
   IRON
Аннотация: We derived simple rules for the sign of 180° superexchange interaction based on the multielectron calculations of the superexchange interaction in the transition metal oxides that are valid both below and above spin crossover under high pressure. The superexchange interaction between two cations in dn configurations is given by a sum of partial contributions related to the electron-hole virtual excitations to the different states of the dn+1 and dn−1 configurations. Using these rules, we have analyzed the sign of the 180° superexchange interaction of a number of oxides with magnetic cations in electron configurations from d2 until d8: the iron, cobalt, chromium, nickel, copper, and manganese oxides with increasing pressure. The most interesting result concerns the magnetic state of cobalt and nickel oxides CoO, Ni2O3 and also La2CoO4, LaNiO3 isostructural to well-known high-TC and colossal magnetoresistance materials. These oxides have a spin 12 at the high pressure. Change of the interaction from antiferromagnetic below spin crossover to ferromagnetic above spin crossover is predicted for oxide materials with cations in d5(FeBO3) and d7(CoO) configurations, while for materials with the other dn configurations spin crossover under high pressure does not change the sign of the 180∘ superexchange interaction.

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Держатели документа:
Kirensky Inst Phys, Akadeingorodok 50,Bld 38, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Polukeev, S. I.; Полукеев, Семен Игоревич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Гавричков, Владимир Александрович; Russian Science FoundationRussian Science Foundation (RSF) [18-12-00022]
}
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Ho and Fe magnetic ordering in multiferroic HoFe3(BO3)4 / D. K. Shukla [et al.] // Phys. Rev. B. - 2012. - Vol. 86, Is. 22. - Ст. 224421, DOI 10.1103/PhysRevB.86.224421. - Cited References: 32 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
X-RAY SCATTERING
POLARIZATION DEPENDENCE
IRON
Аннотация: Resonant and nonresonant x-ray scattering studies on HoFe3(BO3)4 reveal competing magnetic ordering of Ho and Fe moments. Temperature and x-ray polarization dependent measurements employed at the Ho L3 edge directly reveal a spiral spin order of the induced Ho moments in the ab plane propagating along the c axis, a screw-type magnetic structure. At about 22.5 K the Fe spins are observed to rotate within the basal plane inducing spontaneous electric polarization, P. Components of P in the basal plane and along the c axis can be scaled with the separated magnetic x-ray scattering intensities of the Fe and Ho magnetic sublattices, respectively.

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Держатели документа:
[Shukla, D. K.
Francoual, S.
Skaugen, A.
von Zimmermann, M.
Walker, H. C.
Strempfer, J.] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany
[Bezmaternykh, L. N.
Gudim, I. A.
Temerov, V. L.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Shukla, D. K.; Francoual, S.; Skaugen, A.; von Zimmermann, M.; Walker, H. C.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Temerov, V. L.; Темеров, Владислав Леонидович; Strempfer, J.
}
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Infrared absorption spectrum of HoFe3(BO3)4 crystal / S. N. Sofronova [et al.] // Vib. Spectrosc. - 2014. - Vol. 72. - P. 20-25, DOI 10.1016/j.vibspec.2014.02.005. - Cited References: 18. - The work was partially supported by the RFBR through Grants No. 13-02-00825 and 13-02-98041, SS-4828.2012.2. . - ISSN 0924-2031. - ISSN 1873-3697

РУБ Chemistry, Analytical + Chemistry, Physical + Spectroscopy
Рубрики:
MAGNETOELASTIC INTERACTIONS
IRON
GDFE3(BO3)4
Кл.слова (ненормированные):
Holmium ferroborate -- Infrared absorption
Аннотация: Infrared (IR) absorption spectra of HoFe3(BO3)4 crystal have been obtained in spectral range 30–7000 cm−1 at temperatures from 4 to 423 K. Vibrational frequencies have been simulated with ‘Lady’ software package both for high-temperature and low-temperature phases. The experimental spectra have been analyzed on the basis of calculated data, and interpreted within the framework of internal vibrations of ionic complexes of HoFe3(BO3)4 crystal lattice. The spectral range under study was observed to have no Davydov splitting of internal vibrational modes due to unit cell multiplication. No effects of magnetic ordering on the IR spectra of the crystal under study were observed in the low-temperature range.

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Держатели документа:
Kirensky Inst Phys SB RAS, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660079, Russia

Доп.точки доступа:
Sofronova, S. N.; Софронова, Светлана Николаевна; Gerasimova, Y. V.; Герасимова, Юлия Валентиновна; Vtyurin, A. N.; Втюрин, Александр Николаевич; Gudim, I. A.; Гудим, Ирина Анатольевна; Shestakov, N. P.; Шестаков, Николай Петрович; Ivanenko, A. A.; Иваненко, Александр Анатольевич; RFBR [13-02-00825, 13-02-98041, SS-4828.2012.2]
}
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10.

    Korshunov, M. M.
    Uniform impurity scattering in two-band s ± and s ++ superconductors / M. M. Korshunov, Y. N. Togushova, O. V. Dolgov // J. Supercond. Nov. Magn. - 2016. - Vol. 29, Is. 4. - P1089-1095, DOI 10.1007/s10948-016-3385-6. - Cited References:28. - We are grateful to D.V. Efremov and A. A. Golubov for useful discussions. We acknowledge the partial support by RFBR (Grant 16-02-00098) and President Grant for Government Support of the Leading Scientific Schools of the Russian Federation (NSh-2886.2014.2). . - ISSN 1557-1939. - ISSN 1557-1947
   Перевод заглавия: Однородное примесное рассеяние в двухзонных s± и s++ сверхпроводниках

РУБ Physics, Applied + Physics, Condensed Matter
Рубрики:
High-temperature superconductivity
Iron
Кл.слова (ненормированные):
Multiband superconductivity -- Impurity scattering -- Fe-based -- superconductors
Аннотация: The s ± and s ++ models for the superconducting state are subject of intense studies regarding Fe-based superconductors. Depending on the parameters, disorder may leave intact or suppress T c in these models. Here, we study the special case of disorder with equal values of intra- and interband impurity potentials in the two-band s ± and s ++ models. We show that this case can be considered as an isolated point and T c there has maximal damping for a wide range of parameters.

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Держатели документа:
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Svobodny Prospect 79, Krasnoyarsk 660041, Russia.
Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany.
RAS, PN Lebedev Phys Inst, Moscow 117901, Russia.

Доп.точки доступа:
Togushova, Yu. N.; Dolgov, O. V.; Коршунов, Максим Михайлович; RFBR [16-02-00098]; Leading Scientific Schools of the Russian Federation [NSh-2886.2014.2]
}
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11.

Magnetic properties of biomineral particles produced by bacteria Klebsiella oxytoca / Y. L. Raikher [et al.] // Phys. Solid State. - 2010. - Vol. 52, Is. 2. - P. 298-305, DOI 10.1134/S1063783410020125. - Cited References: 29. - This study was supported by the Russian Foundation for Basic Research (project nos. 07-02-96026, 07- 02-96017, and 08-02-00802) and performed within the framework of the Federal Target Program "Research and Research-Pedagogical Personnel of Innovation Russia for 2009-2013." . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
FERRITIN
   NANOPARTICLES
   IRON
   SUSCEPTIBILITY
   FERRIHYDRITE
   BEHAVIOR
   FINS
Аннотация: Ferrihydrite nanoparticles (2-5 nm in size) produced by bacteria Klebsiella oxytoca in the course of biomineralization of iron salt solutions from a natural medium exhibit unique magnetic properties: they are characterized by both the antiferromagnetic order inherent in a bulk ferrihydrite and the spontaneous magnetic moment due to the decompensation of spins in sublattices of a nanoparticle. The magnetic susceptibility enhanced by the superantiferromagnetism effect and the magnetic moment independent of the magnetic field provide the possibility of magnetically controlling these natural objects. This has opened up the possibilities for their use in nanomedicine and bioengineering. The results obtained from measurements of the magnetic properties of the ferrihydrite produced by Klebsiella oxytoca in its two main crystalline modifications are reported, and the data obtained are analyzed theoretically. This has made it possible to determine numerical values of the magnetic parameters of real biomineral nanoparticles.

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Держатели документа:
[Raikher, Yu. L.
Stepanov, V. I.] Russian Acad Sci, Ural Div, Inst Continuum Media Mech, Perm 614013, Russia
[Stolyar, S. V.
Balaev, D. A.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
[Stolyar, S. V.
Balaev, D. A.
Ishchenko, L. A.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
[Ladygina, V. P.] Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Int Sci Ctr Res Organism Extreme Condit, Krasnoyarsk 660036, Russia
[Balasoiu, M.] Joint Inst Nucl Res, Dubna 141980, Moscow Oblast, Russia
ИФ СО РАН
Institute of Continuum Media Mechanics, Ural Division, Russian Academy of Sciences, ul. Akademika Koroleva 1, Perm 614013, Russian Federation
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50, Krasnoyarsk 660036, Russian Federation
Siberian Federal University, pr. Svobody 79, Krasnoyarsk 660041, Russian Federation
International Scientific Center for Research of Organism under Extreme Conditions, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation
Joint Institute for Nuclear Research, ul. Joliot-Curie 6, Dubna, Moscow oblast 141980, Russian Federation

Доп.точки доступа:
Raikher, Y. L.; Stepanov, V. I.; Stolyar, S. V.; Столяр, Сергей Викторович; Ladygina, V. P.; Balaev, D. A.; Балаев, Дмитрий Александрович; Ishchenko, L. A.; Balasoiu, M.
}
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12.

    Magnetic properties of few nanometers ɛ-Fe2O3 nanoparticles supported on the silica / S. S. Yakushkin [et al.] // J. Appl. Phys. - 2012. - Vol. 111, Is. 4. - Ст. 44312, DOI 10.1063/1.3686647. - Cited References: 27. - authors thank A. D. Balaev and N. V. Volkov for fruitful discussions and comments. This work was supported by Program of RAS No. 27.46. . - ISSN 0021-8979
Рубрики:
HIGH-TEMPERATURE
   IRON
   STABILIZATION
   OXIDE
   GEL
Аннотация: Magnetic properties of ɛ-Fe2O3nanoparticles supported on silica with the average size of few nanometers, narrow size distribution and no admixture of any other iron oxide polymorphs are investigated. The investigation of the temperature behavior of magnetization within the temperature range from 4.2 to 1000 K revealed the presence of several magnetic subsystems in the species under study. The temperatures’ behavior of the magnetic moment value indicates ferrimagnetic ordering in the ɛ-Fe2O3nanoparticles with a Curie temperature of about 800 K and points to the existence of a significant paramagnetic contribution becoming apparent at low temperatures. According to the electron spin resonance data, the particles possess superparamagnetic behavior at temperature higher ∼120 K. The model of the magnetic structure of monophase system of few nanometers ɛ-Fe2O3nanoparticles supported on silica is proposed.

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Держатели документа:
[Yakushkin, S. S.
Bukhtiyarova, G. A.
Martyanov, O. N.] Russian Acad Sci, Boreskov Inst Catalysis, Siberian Branch, Novosibirsk 630090, Russia
[Dubrovskiy, A. A.
Balaev, D. A.
Shaykhutdinov, K. A.] Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Yakushkin, S. S.; Dubrovskiy, A. A.; Дубровский, Андрей Александрович; Balaev, A. D.; Балаев, Александр Дмитриевич; Shaykhutdinov, K. A.; Шайхутдинов, Кирилл Александрович; Bukhtiyarova, G. A.; Martyanov, O. N.
}
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13.

Magnetic properties of nanoparticles of 3d metals / G. I. Frolov [et al.] // Tech. Phys. - 2008. - Vol. 53, Is. 8. - P. 1059-1064, DOI 10.1134/S1063784208080136. - Cited References: 19. - This study was supported by the targeted program "Development of the Research Potential of Higher Education Institutions," grant no. RNP.2.1.1.7376. . - ISSN 1063-7842

РУБ Physics, Applied
Рубрики:
CLUSTERS
IRON
PARTICLES
Аннотация: The influence of size effects on the coercive force, magnetization, and Curie temperature in nanoparticles of 3d metals is considered. It is shown that experimental results obtained during the last two decades provide new information on peculiar magnetic properties of these particles.

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Держатели документа:
[Frolov, G. I.
Bachina, O. I.
Zav'yalova, M. M.
Ravochkin, S. I.] Russian Acad Sci, Siberian Branch, Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Frolov, G. I.; Фролов, Георгий Иванович; Bachina, O. I.; Zav'yalova, M. M.; Ravochkin, S. I.
}
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14.

Magnetic properties, morphology and interfaces of (Fe/Si)n nanostructures / Bartolome J. [et al.] // J. Magn. Magn. Mater. - 2016. - Vol. 400. - P. 271-275, DOI 10.1016/j.jmmm.2015.07.046. - Cited References: 43. - The financial support of the Spanish MINECOMAT2011-23791 and MAT2015-53921-R, Aragonese DGA-IMANAE34 (cofounded by Fondo Social Europeo) and European FEDER funds is acknowledged. Program of the President of the Russian Federation for the support of leading scientific schools (Scientific School 2886.2014.2), RFBR (Grant no. 13-02-01265), the Ministry of Education and Science of the Russian Federation (State contract no. 02.G25.31.0043 and State task no. 16.663.2014К) . - ISSN 0304-8853

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
INTERLAYER EXCHANGE
   Fe/Si(100) INTERFACE
   SILICIDE FORMATION
   ULTRAHIGH-VACUUM
   FILMS
   IRON
   MAGNETORESISTANCE
   SUPERLATTICES
   SPECTROSCOPY
   DEPOSITION
Аннотация: A systematic study of the iron–silicon interfaces formed upon preparation of (Fe/Si) multilayers has been performed by the combination of modern and powerful techniques. Samples were prepared by molecular beam epitaxy under ultrahigh vacuum onto Si wafers or single crystalline Ag(100) buffer layers grown on GaAs(100). The morphology of these films and their interfaces was studied by a combination of scanning transmission electron microscopy, X-ray reflectivity, angle resolved X-ray photoelectron spectroscopy and hard X-ray photoelectron spectroscopy. The Si-on-Fe interface thickness and roughness were determined to be 1.4(1) nm and 0.6(1) nm, respectively. Moreover, determination of the stable phases formed at both Fe-on-Si and Si-on-Fe interfaces was performed using conversion electron Mössbauer spectroscopy on multilayers with well separated Si-on-Fe and Fe-on-Si interfaces. It is shown that while a fraction of Fe remains as α-Fe, the rest has reacted with Si, forming the paramagnetic FeSi phase and a ferromagnetic Fe rich silicide. We conclude that there is an identical paramagnetic c-Fe1−xSi silicide sublayer in both Si-on-Fe and Fe-on-Si interfaces, whereas an asymmetry is revealed in the composition of the ferromagnetic silicide sublayer.

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Доп.точки доступа:
Bartolome, J.; Badía-Romano, L.; Rubin J.; Bartolome F.; Varnakov, S. N.; Варнаков, Сергей Николаевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Burgler D.E.; International Conference on Magnetism(20 ; 2015 ; Jul ; 5-10 ; Barselona, Spain)
Свободных экз. нет}
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15.

    Magnetism in spin crossover systems: Short-range order and effects beyond the Heisenberg model / V. I. Kuz'min [et al.] // Phys. Rev. B. - 2019. - Vol. 100, Is. 14. - Ст. 144429, DOI 10.1103/PhysRevB.100.144429. - Cited References: 72. - The authors thank the Russian Scientific Foundation for the financial support under Grant No. 18-12-00022. . - ISSN 2469-9950. - ISSN 2469-9969
   Перевод заглавия: Магнетизм в системах со спиновыми кроссоверами: ближний порядок и эффекты за пределами модели Гейзенберга

РУБ Materials Science, Multidisciplinary + Physics, Applied + Physics, Condensed Matter
Рубрики:
LOWER-MANTLE
   STATE
   TRANSITION
   PRESSURE
   IRON
   SUSCEPTIBILITY
Аннотация: To study non-Heisenberg effects in the vicinity of spin crossover in strongly correlated electron systems we derive an effective low-energy Hamiltonian for the two-band Kanamori model. It contains a Heisenberg high-spin term proportional to exchange constant as well as a low-spin term proportional to spin gap parameter ɛs. Using cluster mean field theory we obtain several non-Heisenberg effects. Near the critical value of spin gap ɛcs there is a magnetic phase transition of first order. In the vicinity of ɛcs in the paramagnetic phase we observe nontrivial behavior of the Curie constant in the paramagnetic susceptibility in the wide range of temperature. Reentrant temperature behavior of nearest-neighbor spin-spin correlations is observed at ɛsɛcs. Finally, the pressure-temperature magnetic phase diagram for ferroperriclase is obtained using the effective Hamiltonian.

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Держатели документа:
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Inst Engn Phys & Radio Elect, Krasnoyarsk 660041, Russia.
Fed Res Ctr KSC SB RAS, Sukhachov Inst Forest, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kuz'min, V. I.; Кузьмин, Валерий Ипполитович; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Zarubin, A. E.; Ovchinnikova, T. M.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Russian Scientific FoundationRussian Science Foundation (RSF) [18-12-00022]
}
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16.

Magnetization and specific heat of DyFe3(BO3)(4) single crystal / E. A. Popova [et al.] // Eur. Phys. J. B. - 2008. - Vol. 62, Is. 2. - P. 123-128, DOI 10.1140/epjb/e2008-00146-5. - Cited References: 18 . - ISSN 1434-6028

РУБ Physics, Condensed Matter
Рубрики:
IRON
NDFE3(BO3)(4)
GDFE3(BO3)(4)
Кл.слова (ненормированные):
Antiferromagnetic orders -- Iron subsystems -- Antiferromagnetic materials -- Dysprosium compounds -- Magnetic field effects -- Magnetization -- Specific heat -- Thermodynamics -- Single crystals
Аннотация: We present thermodynamic and magnetic studies of single crystalline DyFe3(BO3)(4). The data indicate an easy axis antiferromagnetic order below T-N similar to 38 K which we attribute to the Fe subsystem. The Dy subsystem remains paramagnetic down to the lowest investigated temperatures of 2 K, but it is polarized by the Fe spins due to a f-d interaction. External magnetic field leads to a spin-flop transition in the iron subsystem as well as to superposed magnetization in the Dy subsystem. The repopulation of two low-lying Kramers doublets in Dy3+ ions results in well defined Schottky anomalies in specific heat and magnetization.

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Держатели документа:
Vasiliev, A. N.] Moscow MV Lomonosov State Univ, Low Temp Phys Dept, Moscow 119991, Russia
Klingeler, R.] IFW Dresden, Leibniz Inst Soild State & Mat Res, D-01171 Dresden, Germany
Bezmaternykh, L. N.] RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Low Temperature Physics Department, Moscow State University, Moscow 119991, Russian Federation
Leibniz Institute for Solid State and Materials Research, IFW Dresden, Dresden 01171, Germany
L.V. Kirensky Institute of Physics, Siberian Branch, RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Popova, E. A.; Tristan, N.; Vasiliev, A. N.; Temerov, V. L.; Темеров, Владислав Леонидович; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Leps, N.; Buechner, B.; Klingeler, R.
}
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17.

Magnetodielectric and magnetoelastic coupling in TbFe3(BO3)(4) / U. . Adem [et al.] // Phys. Rev. B. - 2010. - Vol. 82, Is. 6. - Ст. 64406, DOI 10.1103/PhysRevB.82.064406. - Cited References: 23. - We thank K. L. and S. G. for technical support. Work was supported by the DFG through Grants No. HE 3439/6 and No. 486 RUS 113/982/0-1. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
DIELECTRIC-CONSTANTS
   IRON
   GDFE3(BO3)(4)
   MULTIFERROICS
   TEMPERATURE
Аннотация: We have studied the magnetodielectric and magnetoelastic coupling in TbFe3(BO3)(4) single crystals by means of capacitance, magnetostriction, and Raman spectroscopy measurements. The data reveal strong magnetic field effects on the dielectric constant and on the macroscopic sample length which are associated to long-range magnetic ordering and a field-driven metamagnetic transition. We discuss the coupling of the dielectric, structural, and magnetic order parameters and attribute the origin of the magnetodielectric coupling to phonon mode shifts according to the Lyddane-Sachs-Teller relation.

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Держатели документа:
[Adem, U.
Wang, L.
Schottenhamel, W.
Buechner, B.
Hess, C.
Klingeler, R.] IFW Dresden, Leibniz Inst Solid State & Mat Res, Dresden, Germany
[Fausti, D.] Univ Hamburg, CFEL, Max Planck Grp Struct Dynam, Hamburg, Germany
[van Loosdrecht, P. H. M.] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands
[Vasiliev, A.] Moscow MV Lomonosov State Univ, Moscow 119992, Russia
[Bezmaternykh, L. N.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
[Klingeler, R.] Univ Heidelberg, Kirchhoff Inst Phys, Heidelberg, Germany
ИФ СО РАН
Leibniz Institute for Solid State and Materials Research, IFW Dresden, Dresden, Germany
Max Planck Group for Structural Dynamics, University of Hamburg-CFEL, Hamburg, Germany
Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen, Netherlands
Moscow State University, Moscow 119992, Russian Federation
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation
Kirchhoff Institute for Physics, University of Heidelberg, Heidelberg, Germany

Доп.точки доступа:
Adem, U.; Wang, L.; Fausti, D.; Schottenhamel, W.; van Loosdrecht, PHM; Vasiliev, A.; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Buchner, B.; Hess, C.; Klingeler, R.
}
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18.

Maiti, S.
Gap symmetry in KFe2As2 and the cos 4θ gap component in LiFeAs / S. Maiti, M. M. Korshunov, A. V. Chubukov // Phys. Rev. B. - 2012. - Vol. 85, Is. 1. - Ст. 14511, DOI 10.1103/PhysRevB.85.014511. - Cited References: 49. - We are thankful to S. Borisenko, S. Davis, R. Fernandes, P. Hirschfeld, I. Eremin, D. Evtushinsky, A. Kordyuk, K. Kuroki, Y. Matsuda, A. Rost, M. Vavilov, and V. Zabolotnyy for useful discussions. This work was supported by NSF-DMR-0906953 (SM and AVC) and by the Humboldt Foundation (AVC). MMK is grateful for support from RFBR (Grant No. 09-02-00127), the Presidium of RAS program N5.7, the FCP Scientific and Research and Educational Personnel of Innovative Russia for 2009-2013 (GK P891 and GK16.740.12.0731), and the President of Russia (Grant No. MK-1683.2010.2). . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
SUPERCONDUCTING GAPS
IRON
Аннотация: We revisit the issue of the gap symmetry in KFe2As2, which is an Fe pnictide superconductor with only hole pockets. Previous theoretical studies mostly argued for a d−wave gap in KFe2As2 since transport and thermodynamic measurements point to the presence of the gap nodes. However, a d-wave gap is inconsistent with recent laser-based angle-resolved photoemission measurements. We propose a scenario for a nodal s−wave superconductivity induced by a nonmagnetic intraband and interband interactions between fermions near hole pockets. The superconducting gap changes sign between the hole pockets and has cos4θ angular dependence and accidental nodes on one or several hole pockets. We argue that strong angle dependence is the consequence of near-degeneracy between interpocket and intrapocket interaction on the hole pockets. We also analyze the cos4θ angular dependence of the gap in other Fe pnictides and compare theoretical results with the photoemission experiments of LiFeAs.

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Держатели документа:
[Maiti, S.
Chubukov, A. V.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA
[Korshunov, M. M.] Russian Acad Sci, Siberian Branch, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia
[Korshunov, M. M.] Siberian Fed Univ, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Korshunov, M. M.; Коршунов, Максим Михайлович; Chubukov, A.V.
}
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19.

Nature of the active sites of ferrospheres in the oxidative condensation of methane / A. G. Anshits [et al.] // Kinet. Catal. - 2015. - Vol. 56, Is. 4. - P. 523-531, DOI 10.1134/S0023158415040023. - Cited References:37. - This work was supported by the Russian Science Foundation (grant no. 14-13-00289). . - ISSN 0023. - ISSN 1608-3210. -

РУБ Chemistry, Physical
Рубрики:
GLASS CRYSTAL CATALYSTS
   HIGH-TEMPERATURE
   MOSSBAUER
   MAGNETITES
   MICROSPHERES
   SELECTIVITY
   CONVERSION
   FERRITES
   ASHES
   IRON
Кл.слова (ненормированные):
oxidative condensation of methane -- ferrospheres -- iron spinel -- Mossbauer spectroscopy -- structural defects
Аннотация: The catalytic properties of ferrospheres containing 76–97 wt % Fe2O3 in the oxidative condensation of methane were compared with their phase composition and the distribution of iron cations over the crystallographic positions of iron-containing phases in a steady state. It was established that the reaction route of methane oxidation changed at a Fe2O3 content of 89 wt %. Deep oxidation was the main reaction route on ferrospheres with a Fe2O3 content of <88.8 wt %. At a Fe2O3 content of ≥89 wt %, the yield of C2 hydrocarbons sharply increased and the contribution of deep oxidation decreased. The yield of C2 hydrocarbons correlated with the amount of defects in the structure of iron spinel, which are iron ions with the tetrahedral cation of Ca2+ and the octahedral cation vacancy among the nearest neighbors.

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Публикация на русском языке Природа активных центров ферросфер в процессе окислительной конденсации метана [Текст] / А. Г. Аншиц [и др.] // Кинетика и катализ : Наука, 2015. - Т. 56 № 4. - С. 529-538

Доп.точки доступа:
Anshits, A. G.; Аншиц, Александр Георгиевич; Bayukov, O. A.; Баюков, Олег Артемьевич; Anshits, N. N.; Pletnev, O. N.; Плетнев, Олег Николаевич; Rabchevskii, E. V.; Vereshchagin, S. N.; Kondratenko, E. V.; Russian Science Foundation [4-13-00289]; Russian Congress on Catalysis (2 ; 2014 ; Oct. ; 2–5 ; Samara)
}
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20.

Novel pressure-induced magnetic transition in magnetite (Fe(3)O(4)) / Y. . Ding [et al.] // Phys. Rev. Lett. - 2008. - Vol. 100, Is. 4. - Ст. 45508, DOI 10.1103/PhysRevLett.100.045508. - Cited References: 39 . - ISSN 0031-9007

РУБ Physics, Multidisciplinary
Рубрики:
MULTIPLE-SCATTERING THEORY
   X-RAY DICHROISM
   LOWER MANTLE
   VERWEY TRANSITION
   K-EDGE
   CIRCULAR-DICHROISM
   SPIN TRANSITION
   BAND-STRUCTURE
   IRON
   FE
Кл.слова (ненормированные):
Emission spectroscopy -- Magnetoelectronics -- Pressure effects -- Synchrotron radiation -- Diamond anvil cell -- Magnetic transition -- X-ray magnetic circular dichroism -- Magnetite
Аннотация: Fe K-edge x-ray magnetic circular dichroism of magnetite (Fe(3)O(4)) powders was measured with synchrotron radiation under variable pressure and temperature conditions in diamond anvil cell. The magnetic dichroism was observed to decrease discontinuously by similar to 50% between 12 and 16 GPa, independent of temperature. The magnetic transition is attributed to a high-spin to intermediate-spin transition of Fe(2+) ions in the octahedral sites and could account for previously observed structural and electrical anomalies in magnetite at this pressure range. The interpretation of x-ray magnetic circular dichroism data is supported by x-ray emission spectroscopy and theoretical cluster calculations.

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Держатели документа:
Mao, Ho-kwang] Carnegie Inst Washington, HPSynC, Argonne, IL 60439 USA
Lang, Jonathan C.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[Ovchinnikov, Sergei G.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Orlov, Yuri S.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
[Mao, Ho-kwang] Carnegie Inst Washington, Geophys Lab, Washington, DC 20015 USA
[Mao, Ho-kwang] Carnegie Inst Washington, HPCAT, Argonne, IL 60439 USA
HPSynC, Carnegie Institution of Washington, 9700 South Cass Avenue, Argonne, IL 60439, United States
Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439, United States
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Science, 660036 Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Geophysical Laboratory, Carnegie Institution of Washington, 5251 Broad Branch Road NW, Washington, DC 20015, United States
HPCAT, Carnegie Institution of Washington, Building 434E, 9700 South Cass Avenue, Argonne, IL 60439, United States

Доп.точки доступа:
Ding, Y.; Haskel, D.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Tseng, Y. C.; Orlov, Y. S.; Lang, J. C.; Mao, H. K.
}
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