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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Isaev I. L., Semina P. N., Markel V. A., Karpov S. V.
Заглавие : Effects of size polydispersity on the extinction spectra of colloidal nanoparticle aggregates
Место публикации : Phys. Rev. B: American Physical Society, 2012. - Vol. 85, Is. 4. - Ст.045421. - P. - ISSN 1098-0121, DOI 10.1103/PhysRevB.85.045421
Примечания : Cited References: 41. - This work was supported by grants from the following foundations of the Russian Federation: Presidium of RAS, OFN RAS, and SB RAS.
Предметные рубрики: METAL FRACTAL CLUSTERS
OPTICAL-PROPERTIES
ABSORPTION
NONLINEARITIES
COMPOSITES
SCATTERING
PARTICLES
SPHERES
GRAINS
Аннотация: We investigate the effect of particle polydispersity on the optical extinction spectra of colloidal aggregates of spherical metallic (silver) nanoparticles, taking into account the realistic interparticle gaps caused by layers of stabilizing polymer adsorbed on the metal surface (adlayers). The spectra of computer-generated aggregates are computed using two different methods. The coupled-multipole method is used in the quasistatic approximation and the coupled-dipole method beyond the quasistatics. The latter approach is applicable if the interparticle gaps are sufficiently wide relative to the particle radii. Simulations are performed for two different particle size distribution functions (bimodal and Gaussian), varying the number of particles per aggregate, and different distribution functions of the interparticle gap width. The strong influence of the latter factor on the spectra is demonstrated and investigated in detail.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Alekseev K. N., Alekseeva N. V., Perina J.
Заглавие : Quantum-classical correspondence and nonclassical state generation in dissipative quantum optical systems
Место публикации : J. Exp. Theor. Phys.: AMER INST PHYSICS, 2000. - Vol. 90, Is. 4. - P592-599. - ISSN 1063-7761, DOI 10.1134/1.559142
Примечания : Cited References: 32
Предметные рубрики: 2ND-HARMONIC GENERATION
STATISTICAL PROPERTIES
HARMONIC-GENERATION
SQUEEZED STATES
CHAOS
LIGHT
NONLINEARITIES
INSTABILITIES
DYNAMICS
ATOMS
Аннотация: We develop a semiclassical method to determine the nonlinear dynamics of dissipative quantum optical systems in the limit of large number of photons N; it is based on the 1/N-expansion and the quantum-classical correspondence. The method is used to tackle two problems: the study of the dynamics of nonclassical state generation in higher order anharmonic dissipative oscillators and the establishment of the difference between the quantum and classical dynamics of the second-harmonic generation in a self-pulsing regime. In addressing the first problem, we obtain an explicit time dependence of the squeezing and the Fano factor for an arbitrary degree of anharmonism in the short-time approximation. For the second problem, we analytically find a characteristic time scale at which the quantum dynamics differs insignificantly from the classical one. (C) 2000 MAIK "Nauka/Interperiodica".
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