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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Stanislavchuk T. N., Malkin B. Z., Bezmaternykh L. N.
Заглавие : Phase transitions and crystal-field and exchange interactions in TbFe3(BO3)4 as seen via optical spectroscopy
Место публикации : J. Phys.: Condens. Matter: IOP Publishing Ltd, 2012. - Vol. 24, Is. 19. - Ст.196002. - ISSN 0953-8984, DOI 10.1088/0953-8984/24/19/196002
Примечания : Cited References: 45. - The assistance of E P Chukalina is acknowledged. This work was supported in part by the Russian Foundation for Basic Research (grants No 10-02-01071-a and No 09-02-00171-a), by the Ministry of Education and Science (grant HIII-4828.2012.2), and by the Russian Academy of Sciences under the Programs for Basic Research.
Предметные рубрики: IRON BORATE GDFE3(BO3)4
PROBE
ION
Аннотация: High-resolution polarized broadband (1800–23 000 cm−1) optical absorption spectra of Tb3+ in TbFe3(BO3)4 single crystals are studied between room temperature and 4.2 K. The spectral signatures of the structural (R32–P3121, TS = 192 K) and magnetic (TN = 41 K) phase transitions are found and analyzed. Energies and symmetries of the Tb3+ crystal-field (CF) levels were determined for both the high-temperature R32 and the low-temperature P3121 structures of TbFe3(BO3)4 and compared with the calculated ones. It follows unambiguously from the spectral data that the ground state is the Γ1 + Γ2 quasi-doublet of the local D3 point symmetry group for Tb3+ in the R32 high-temperature structure. The CF calculations revealed the CF parameters and wavefunctions for Tb3+ in TbFe3(BO3)4. The value of the Tb–Fe exchange integral and of the effective magnetic field created by the ordered Fe subsystem were estimated as Jfd = 0.26 K and Beff = 3.92 T, using the observed splitting Δ = 32 cm−1 of the Tb3+ ground quasi-doublet at the temperature 5 K. The reliability of the obtained parameters was proven by modeling the literature data on the magnetic susceptibility of TbFe3(BO3)4. Lattice distortions below TS were evidenced by the observed changes of probabilities of the forced electric dipole transitions of Tb3+.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Malakhovskii A. V., Sokolov V. V., Sukhachev A. L., Aleksandrovsky A. S., Gudim, I. A., Molokeev M. S.
Заглавие : Spectroscopic properties and structure of the ErFe3(BO3)4 single crystal
Коллективы : Russian Foundation for Basic Research [12-02-00026]; Council on Grants from the Russian Federation for Support of Leading Scientific Schools [NSh-2886.2014.2]; Department of Physical Sciences of the Russian Academy of Sciences [3.9.5]
Место публикации : Phys. Solid State: Pleiades Publishing, 2014. - Vol. 56, Is. 10. - P.2056-2063. - ISSN 1063-7834, DOI 10.1134/S1063783414100199. - ISSN 1090-6460
Примечания : Cited References: 28. - This study was supported by the Russian Foundation for Basic Research (project no. 12-02-00026), the Council on Grants from the President of the Russian Federation for Support of Leading Scientific Schools (grant no. NSh-2886.2014.2), and the Department of Physical Sciences of the Russian Academy of Sciences (program no. 3.9.5).
Предметные рубрики: RARE-EARTH IONS
ABSORPTION INTENSITIES
Er3+ IONS
SPECTRA
PROBE
Аннотация: Single crystals of the ErFe3(BO3)4 borate were synthesized and their structure was studied. Absorption spectra of the Er3+ ion in σ- and π-polarizations of f-f transitions 4 I 15/2 → 4 I 13/2, 4 I 11/2, 4 I 9/2, 4 F 9/2, 4 S 3/2, 2 H 11/2, and 4 F 7/2 were measured. The refractive index and birefringence were measured as a function of the wavelength. The transition intensities were analyzed within the Judd-Ofelt theory, and the following parameters of the theory were obtained: Ω2 = 7.056 × 10−20 cm2, Ω4 = 1.886 × 10−20 cm2, and Ω6 = 2.238 × 10−20 cm2. Using these parameters, the radiative transition probabilities, luminescence branching ratios, and radiative lifetimes of multiplets were calculated.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bulgakov E. N., Rotter I., Sadreev A. F.
Заглавие : Phase rigidity and avoided level crossings in the complex energy plane
Место публикации : Phys. Rev. E: AMERICAN PHYSICAL SOC, 2006. - Vol. 74, Is. 5. - Ст.56204. - ISSN 1539-3755, DOI 10.1103/PhysRevE.74.056204
Примечания : Cited References: 40
Предметные рубрики: OPEN QUANTUM-SYSTEMS
FANO RESONANCES
S-MATRIX
DOT
CONTINUUM
TRANSMISSION
COHERENCE
TRANSPORT
BILLIARDS
PROBE
Ключевые слова (''Своб.индексиров.''): eigenvalues and eigenfunctions--hamiltonians--resonance--rigidity--semiconductor quantum dots--biorthogonal eigenfunctions--open quantum system--phase rigidity--quantum theory
Аннотация: We consider the effective Hamiltonian of an open quantum system, its biorthogonal eigenfunctions phi(lambda), and define the value r(lambda)=(phi(lambda)parallel to phi(lambda))/phi(lambda)parallel to phi(lambda) that characterizes the phase rigidity of the eigenfunctions phi(lambda). In the scenario with avoided level crossings, r(lambda) varies between 1 and 0 due to the mutual influence of neighboring resonances. The variation of r(lambda) is an internal property of an open quantum system. In the literature, the phase rigidity rho of the scattering wave function Psi(E)(C) is considered. Since Psi(E)(C) can be represented in the interior of the system by the phi(lambda), the phase rigidity rho of the Psi(E)(C) is related to the r(lambda) and therefore also to the mutual influence of neighboring resonances. As a consequence, the reduction of the phase rigidity rho to values smaller than 1 should be considered, at least partly, as an internal property of an open quantum system in the overlapping regime. The relation to measurable values such as the transmission through a quantum dot, follows from the fact that the transmission is, in any case, resonant at energies that are determined by the real part of the eigenvalues of the effective Hamiltonian. We illustrate the relation between phase rigidity rho and transmission numerically for small open cavities.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liu, Ji-Cai, Savchenko, Viktoriia, Kimberg V., Gel'mukhanov F., Odelius, Michael
Заглавие : High-resolution x-ray spectra of carbon monoxide reveal ultrafast dynamics induced by long UV pulse
Коллективы : RFBRRussian Foundation for Basic Research (RFBR) [19-29-12015]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [11974108, 11574082]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [2021MS046]; European UnionEuropean Commission [860553]; Carl Tryggers Foundation [CTS18:285]; Helmholtz Virtual Institute [VI419]; Swedish Research CouncilSwedish Research CouncilEuropean Commission [VR 2019-03470, 2018-05973]
Место публикации : New J. Phys. - 2021. - Vol. 23, Is. 6. - Ст.063030. - ISSN 1367-2630, DOI 10.1088/1367-2630/ac0198
Примечания : Cited References: 47. - The reported study was funded by RFBR, project number 19-29-12015. J-CL thanks the support by the National Science Foundation of China under Grant Nos. 11974108, 11574082, and the Fundamental Research Funds for the Central Universities (No. 2021MS046). MO acknowledges funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skodowska-Curie Grant Agreement No. 860553 and the Carl Tryggers Foundation (contract CTS18:285). FG acknowledges also the support from the Helmholtz Virtual Institute VI419 'Dynamic Pathways in Multidimensional Landscapes'. VK acknowledges the Swedish Research Council (VR 2019-03470). The calculations were partially enabled by resources provided by the Swedish National Infrastructure for Computing (SNIC) partially funded by the Swedish Research Council through Grant Agreement No. 2018-05973
Предметные рубрики: VIBRATIONAL STRUCTURE
SCATTERING
RAMAN
CO
COLLAPSE
PROBE
Аннотация: In theoretical simulations of a UV + x-ray pump-probe (UVX-PP) setup, we show that frequency detuning of the pump UV pulse acts as a camera shutter by regulating the duration of the UVX-PP process. This two-photon absorption with long overlapping UV and x-ray pulses, allowing for high spectral resolution, thereby provides information about ultrafast dynamics of the nuclear wave packet without the requirement of ultrashort pulses and controlled delay times. In a case study of carbon monoxide, the calculated UVX-PP spectra of the O1s−12π1 and C1s−12π1 core-excited states show different vibrational profiles. The interference of intermediate vibrational states reveals details of nuclear dynamics in the UVX-PP process related to a variable duration time controlled by the UV detuning. Both O1s−12π1 and C1s−12π1 pump-probe channels display a splitting of the spectral profile, which however is associated with different physical mechanisms. At the O1s−12π1 resonance, the observed dispersive and non-dispersive spectral bands intersect and result in destructive interference.
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