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Malakhovskii, A. V.
Optical and magneto-optical spectra and electron structure of ErAl3(BO3)4 single crystal / A. V. Malakhovskii, V. V. Sokolov, I. A. Gudim // J. Alloys Compd. - 2017. - Vol. 698. - P. 364-374, DOI 10.1016/j.jallcom.2016.12.200. - Cited References: 32. - The work was supported by the Russian Foundation for Basic Researches grant 16-02-00273 and by the President of Russia grant No Nsh-7559.2016.2. . - ISSN 0925-8388
Кл.слова (ненормированные):
Electron structure -- Er3+ ion -- f-f transitions -- Magnetic circular dichroism
Аннотация: Linearly polarized absorption spectra and magnetic circular dichroism (MCD) spectra of ErAl3(BO3)4 single crystal were measured in the range of 10000–27000 cm−1 at 90 K. The Stark components of the ground and excited multiplets of Er3+ ion were identified in terms of the irreducible representations, basing on the linearly polarized absorption spectra. MCD spectra permitted us to measure the Zeeman splitting of some transitions and so to determine changes of the Landé factors along the C3 axis during these transitions. Additionally, the MCD spectra permitted us to identify some states in the |J,±MJ〉function approximation. In particular, it was shown that the ground state of the Er3+ ion in this approximation has MJ = ± 13/2 that corresponds to magnetic moment m = ±7.8 μB. Very intensive f-f vibronic transitions, corresponding to electron transitions from the upper components of the ground multiplet, were revealed. Energies of the local vibrations in a number of the excited states were found.

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Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Малаховский, Александр Валентинович
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Malakhovskii, A. V.
Natural optical activity of f-f transitions in ErAl3(BO3)4 single crystal / A. V. Malakhovskii, V. V. Sokolov, I. A. Gudim // Chem. Phys. - 2017. - Vol. 493. - P. 102-110, DOI 10.1016/j.chemphys.2017.06.011. - Cited References: 50. - The work was supported by the Russian Foundation for Basic Researches grant 16-02-00273 and by the President of Russia grant No Nsh-7559.2016.2. . - ISSN 0301-0104
Кл.слова (ненормированные):
f-f transitions -- Natural circular dichroism -- Er3+ ion
Аннотация: Absorption and natural circular dichroism (NCD) spectra of ErAl3(BO3)4 single crystal were measured at 90 K in the range of 10,000–28,200 cm−1. The spectra were decomposed on the Lorentz shape components and the natural optical activities (NOA) of f-f transitions between Stark components of the ground and excited multiplets were found. The NCD spectra permitted us to find out existence of two non equivalent positions of Er3+ ion in one of its excited states, which are due to the local decrease of the crystal symmetry in this state. Very large NOA of a vibronic line was revealed. This phenomenon was accounted for basing on the new quantum mechanical formula for the NOA of electron transitions. The principle difference of the NOA properties of electric dipole allowed and parity forbidden transitions is discussed.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Малаховский, Александр Валентинович
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Malakhovskii, A. V.
Influence of the low local symmetry of Er3+ ions on magnetic circular dichroism and absorption spectra of f-f transitions in ErFe3(BO3)4 single crystal / A. V. Malakhovskii, V. V. Sokolov, I. A. Gudim // J. Magn. Magn. Mater. - 2018. - Vol. 465. - P. 700-708, DOI 10.1016/j.jmmm.2018.06.057. - Cited References: 29. - The work was supported by the Russian Foundation for Basic Researches grant 16-02-00273 and by the Project of Russian Academy of Science No. 0356-2017-0030. . - ISSN 0304-8853
Кл.слова (ненормированные):
Er3+ ion -- f-f transitions -- Magnetic circular dichroism -- Rare earth ferroborates
Аннотация: Linearly polarized absorption spectra and magnetic circular dichroism (MCD) spectra of ErFe3(BO3)4 single crystal were measured in the range of 9000–23000 cm−1 at 90 K. The absorption spectra of f-f transitions were decomposed into the Lorentz shape components and intensities of the components were found. MCD spectra permitted us to measure the Zeeman splitting of some transitions and so to determine changes of the Landé factor along the C3 axis of the crystal during these transitions. Optical and magneto-optical properties of f-f transitions in the ErFe3(BO3)4 crystal were compared with those in the ErAl3(BO3)4 crystal. Substantial difference of the properties connected with the difference of the Er3+ ions local symmetry in two crystals was revealed. Large splitting of one of the f-f transitions without magnetic field, which is not possible for the Kramers doublets, was observed. It was explained by appearance of two absorbing centers due to the local decrease of symmetry in the excited state. Appreciable difference of the local vibrations energy in some excited states was revealed.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Sokolov, V. V.; Соколов, Валерий Владимирович; Gudim, I. A.; Гудим, Ирина Анатольевна; Малаховский, Александр Валентинович
}
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