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Bulgakov, E. N.
Correlated behavior of conductance and phase rigidity in the transition from the weak-coupling to the strong-coupling regime / E. N. Bulgakov, I. . Rotter, A. F. Sadreev // Phys. Rev. B. - 2007. - Vol. 76, Is. 21. - Ст. 214302, DOI 10.1103/PhysRevB.76.214302. - Cited References: 42 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
OPEN QUANTUM-SYSTEMS
   NUCLEAR CROSS-SECTIONS
   UNIFIED THEORY
   FLUCTUATIONS
   CONTINUUM
   BILLIARD
   STATES
Аннотация: We study the transmission through different small systems as a function of the coupling strength v to the two attached leads. The leads are identical with only one propagating mode xi(E)(C) in each of them. In addition to the conductance G, we calculate the phase rigidity rho of the scattering wave function Psi(E)(C) in the interior of the system. Most interesting results are obtained in the regime of strongly overlapping resonance states where the crossover from staying to traveling modes takes place. The crossover is characterized by collective effects. Here, the conductance is plateaulike enhanced in some energy regions of finite length while corridors with zero transmission (total reflection) appear in other energy regions. This transmission picture depends only weakly on the spectrum of the closed system. It is caused by the alignment of some resonance states of the system with the propagating modes xi(E)(C) in the leads. The alignment of resonance states takes place stepwise by resonance trapping, i.e., it is accompanied by the decoupling of other resonance states from the continuum of propagating modes. This process is quantitatively described by the phase rigidity rho of the scattering wave function. Averaged over energy in the considered energy window, G is correlated with 1-rho . In the regime of strong coupling, only two short-lived resonance states survive each aligned with one of the channel wave functions xi(E)(C). They may be identified with traveling modes through the system. The remaining M-2 trapped narrow resonance states are well separated from one another.

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Держатели документа:
[Bulgakov, E. N.
Rotter, I.
Sadreev, A. F.] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
[Bulgakov, E. N.
Sadreev, A. F.] LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
Max Planck Institute for the Physics of Complex Systems, D-01187 Dresden, Germany
Kirensky Institute of Physics, 660036, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Rotter, I.; Sadreev, A. F.; Садреев, Алмаз Фаттахович; Булгаков, Евгений Николаевич
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Bulgakov, E. N.
Phase rigidity and avoided level crossings in the complex energy plane / E. N. Bulgakov, I. . Rotter, A. F. Sadreev // Phys. Rev. E. - 2006. - Vol. 74, Is. 5. - Ст. 56204, DOI 10.1103/PhysRevE.74.056204. - Cited References: 40 . - ISSN 1539-3755

РУБ Physics, Fluids & Plasmas + Physics, Mathematical
Рубрики:
OPEN QUANTUM-SYSTEMS
   FANO RESONANCES
   S-MATRIX
   DOT
   CONTINUUM
   TRANSMISSION
   COHERENCE
   TRANSPORT
   BILLIARDS
   PROBE
Кл.слова (ненормированные):
Eigenvalues and eigenfunctions -- Hamiltonians -- Resonance -- Rigidity -- Semiconductor quantum dots -- Biorthogonal eigenfunctions -- Open quantum system -- Phase rigidity -- Quantum theory
Аннотация: We consider the effective Hamiltonian of an open quantum system, its biorthogonal eigenfunctions phi(lambda), and define the value r(lambda)=(phi(lambda)parallel to phi(lambda))/ that characterizes the phase rigidity of the eigenfunctions phi(lambda). In the scenario with avoided level crossings, r(lambda) varies between 1 and 0 due to the mutual influence of neighboring resonances. The variation of r(lambda) is an internal property of an open quantum system. In the literature, the phase rigidity rho of the scattering wave function Psi(E)(C) is considered. Since Psi(E)(C) can be represented in the interior of the system by the phi(lambda), the phase rigidity rho of the Psi(E)(C) is related to the r(lambda) and therefore also to the mutual influence of neighboring resonances. As a consequence, the reduction of the phase rigidity rho to values smaller than 1 should be considered, at least partly, as an internal property of an open quantum system in the overlapping regime. The relation to measurable values such as the transmission through a quantum dot, follows from the fact that the transmission is, in any case, resonant at energies that are determined by the real part of the eigenvalues of the effective Hamiltonian. We illustrate the relation between phase rigidity rho and transmission numerically for small open cavities.

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Держатели документа:
Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
Linkoping Univ, Dept Phys & Measurement Technol, S-58183 Linkoping, Sweden
ИФ СО РАН
Max-Planck-Institut fur Physik Komplexer Systeme, D-01187 Dresden, Germany
Kirensky Institute of Physics, 660036 Krasnoyarsk, Russian Federation
Department of Physics and Measurement, Technology Linkoping University, S-581 83 Linkoping, Sweden

Доп.точки доступа:
Rotter, I.; Sadreev, A. F.; Садреев, Алмаз Фаттахович; Булгаков, Евгений Николаевич
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Bulgakov, E. N.
Spectroscopic properties of large open quantum-chaotic cavities with and without separated time scales / E. N. Bulgakov, I. . Rotter // Phys. Rev. E. - 2006. - Vol. 73, Is. 6. - Ст. 66222, DOI 10.1103/PhysRevE.73.066222. - Cited References: 24 . - ISSN 1539-3755

РУБ Physics, Fluids & Plasmas + Physics, Mathematical
Рубрики:
HELMHOLTZ EQUATION
   SYSTEMS
   DYNAMICS
   STATES
   TRANSMISSION
   BILLIARDS
Кл.слова (ненормированные):
Hamiltonians -- Numerical analysis -- Phase control -- Quantum theory -- Spectroscopic analysis -- Wave transmission -- Bunimovich cavity -- Hamiltonian formalism -- Phase rigidity -- Quantum-chaotic cavities -- Cavity resonators
Аннотация: The spectroscopic properties of an open large Bunimovich cavity are studied numerically in the framework of the effective Hamiltonian formalism. The cavity is opened by attaching two leads to it in four different ways. In some cases, the transmission takes place via standing waves with an intensity that closely follows the profile of the resonances. In other cases, short-lived and long-lived resonance states coexist. The short-lived states cause traveling waves in the transmission while the long-lived ones generate superposed fluctuations. The traveling waves oscillate as a function of energy. They are not localized in the interior of the large chaotic cavity. In all considered cases, the phase rigidity fluctuates with energy. It is mostly near to its maximum value and agrees well with the theoretical value for the two-channel case.

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Держатели документа:
Kirensky Inst Phys, Krasnoyarsk 660036, Russia
Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
ИФ СО РАН
Kirensky Institute of Physics, 660036, Krasnoyarsk, Russian Federation
Max Planck Institute for the Physics of Complex Systems, D-01187 Dresden, Germany

Доп.точки доступа:
Rotter, I.; Булгаков, Евгений Николаевич
}
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    Aliovalent substitution toward reinforced structural rigidity in Ce3+-doped garnet phosphors featuring improved performance / T. Hu [et al.] // J. Mater. Chem. C. - 2019. - Vol. 7, Is. 46. - P. 14594-14600, DOI 10.1039/c9tc05354a. - Cited References: 38. - This work was supported by the National Natural Science Foundation of China (No. 51722202 and 51972118), the Guangdong Provincial Science & Technology Project (2018A050506004) and the Fundamental Research Funds for the Central Universities (D2190980). . - ISSN 2050-7534
   Перевод заглавия: Алиовалентное замещение с целью усиления структурной жесткости в люминофорных гранатах, легированных Ce3 + и имеющих улучшенные характеристики
Кл.слова (ненормированные):
Color -- Deterioration -- Efficiency -- Gallium alloys -- Garnets -- III-V semiconductors -- Indium alloys -- Photoluminescence -- Reinforcement -- Rigidity -- Semiconductor alloys -- Thermal Engineering -- Thermodynamic stability
Аннотация: Highly efficient phosphors with thermal stability and color-tunable emission are required for the fabrication of phosphor-converted white light-emitting diodes (pc-WLEDs). Currently developed engineering strategies are generally successful in photoluminescence tuning but, unfortunately, suffer severe deterioration in emission intensity/efficiency and/or thermal stability. Herein, an efficient aliovalent substitution strategy toward reinforced structural rigidity is proposed and demonstrated experimentally. By incorporating Be2+ ion into the garnet-type Lu2SrAl4SiO12:Ce3+ phosphor, the phosphor shows enhanced internal/external quantum efficiency, from 79.2%/26.7% to 84.5%/32.9%, photoluminescence tuning from green (peaking at ∼512 nm) to yellow (peaking at ∼552 nm), and zero thermal quenching, even up to 200 °C. The Be2+ substitution at the Al2/Si2 site enables stable and rigid local surroundings around the Ce3+ activator, which is responsible for the unprecedented performance. In addition, high-quality warm WLED devices with a luminous efficiency of 158.1 lm W-1, correlated color temperature of 3858 K and high color rendering index of 81.7, are obtained by combining Lu2SrAl4SiO12:Ce3+,Be2+ as the yellow emitter, CaAlSiN3:Eu2+ as the red emitter and a blue-emitting InGaN chip. These findings highlight a new strategy for performance optimization of LED phosphors by selecting rigid covalent compounds with further reinforced structural rigidity via aliovalent substitution.

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Держатели документа:
State Key Laboratory of Luminescent Materials and Devices, Institute of Optical Communication Materials, South China University of Technology, Guangzhou, 510641, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, 680021, Russian Federation

Доп.точки доступа:
Hu, T.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Z.; Zhang, Q.
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    Liu, Gaochao.
    Structural rigidity control toward Cr3+-based broadband near-infrared luminescence with enhanced thermal stability / G. C. Liu, M. S. Molokeev, Z. G. Xia // Chem. Mat. - 2022. - Vol. 34, Is. 3. - P. 1376-1384, DOI 10.1021/acs.chemmater.1c04131. - Cited References: 59. - This work was supported by the International Cooperation Project of the National Key Research and Development Program of China (2021YFE0105700) , National Natural Science Foundation of China (Nos.: 51972118 and 51961145101) , Guangzhou Science & Technology Project (202007020005) , and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137) . This work was also funded by RFBR according to the research Project No. 19-52-80003 . - ISSN 0897-4756. - ISSN 1520-5002
   Перевод заглавия: Контроль структурной жесткости для получения широкополосной люминесценции в ближней инфракрасной области на основе Cr3+ с повышенной термической стабильностью

РУБ Chemistry, Physical + Materials Science, Multidisciplinary
Рубрики:
PHOSPHOR
   PHOTOLUMINESCENCE
   EFFICIENT
   EMISSION
   CR3+
Аннотация: Broadband near-infrared (NIR) light sources based on phosphor-converted light-emitting diodes (pc-LEDs) are desirable for biochemical analysis and medical diagnosis applications; however, the development of target NIR phosphor is still a challenge. Herein, broadband NIR phosphors, Cr3+-activated CaSc1–xAl1+xSiO6 (λem = 950 nm), are designed and optimized by chemical substitution toward enhanced quantum efficiency and thermal stability. Structural and spectral analyses along with density functional theory calculations reveal that Sc3+/Al3+ substitution contributes to enhancing the structural rigidity and the local symmetry of the [Sc/AlO6] octahedron so that the nonradiative relaxation of Cr3+ emission centers is suppressed significantly. The as-fabricated phosphor-in-glass-based NIR LED light source demonstrates great potential in the detection of alcohol concentration. This study provides a local structure design principle for exploring NIR phosphors with enhanced thermal stability and will also stimulate further studies on material discovery and quantitative analysis of NIR spectroscopy.

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Держатели документа:
South China Univ Technol, Sch Mat Sci & Engn, Guangdong Prov Key Lab Fiber Laser Mat & Appl Tec, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Peoples R China.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Lab Crystal Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Kemerovo State Univ, Res & Dev Dept, Kemerovo 650000, Russia.
South China Univ Technol, Sch Phys & Optoelect, Guangzhou 510641, Peoples R China.

Доп.точки доступа:
Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Zhiguo; International Cooperation Project of the National Key Research and Development Program of China [2021YFE0105700]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51972118, 51961145101]; Guangzhou Science & Technology Project [202007020005]; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01X137]; RFBRRussian Foundation for Basic Research (RFBR) [19-52-80003]
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