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Electric and magnetic field-assisted orientational transitions in the ensembles of domains in a nematic liquid crystal on the polymer surface / A. M. Parshin [et al.] // Int. J. Mol. Sci. - 2014. - Vol. 15, Is. 10. - P. 17838-17851, DOI 10.3390/ijms151017838. - Cited References: 21. - This work was partially supported by the Russian Foundation for Basic Research (project No. 12-03-00816), and by the Siberian Branch of the Russian Academy of Sciences (SB RAS) through Grants Nos. 30, 24.29, 24.32, and by SB RAS through a Taiwan-SB-RAS joint project. . - ISSN 1422-0067

РУБ Chemistry, Multidisciplinary
Рубрики:
FRANK CONSTANTS
   INTERFACE
   ALIGNMENT
   DISCLINATIONS
   STABILITY
   COATINGS
   DIRECTOR
Кл.слова (ненормированные):
liquid crystal -- polycarbonate -- domain structure -- electric field -- magnetic field
Аннотация: Using electro- and magneto-optical techniques, we investigated orientational transitions in the ensembles of domains in a nematic liquid crystal on the polycarbonate film surface under the conditions of competing surface forces that favor radial and uniform planar alignment of nematic molecules. Having analyzed field dependences of the intensity of light passed through a sample, we established the threshold character of the orientational effects, plotted the calculated intensity versus magnetic coherence length, and compared the latter with the equilibrium length that characterizes the balance of forces on the polymer surface.

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Dept Energy, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Parshin, A. M.; Паршин, Александр Михайлович; Gunyakov, V. A.; Гуняков, Владимир Алексеевич; Zyryanov, V. Ya.; Зырянов, Виктор Яковлевич; Shabanov, V. F.; Шабанов, Василий Филиппович; Russian Foundation for Basic Research [12-03-00816]; Siberian Branch of the Russian Academy of Sciences (SB RAS) [30, 24.29, 24.32]; SB RAS through a Taiwan-SB-RAS joint project
}
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    Electronic structure of β-RbSm(MoO4)2 and chemical bonding in molybdates / V. V. Atuchin [et al.] // Dalton Trans. - 2015. - Vol. 44, Is. 4. - P. 1805-1815, DOI 10.1039/c4dt03203a. - Cited References: 121. - VVA and ASA gratefully acknowledge the Ministry of Education and Science of the Russian Federation for financial support. ZL acknowledges the support by National Natural Science Foundation of China (11174297 and 11474292), the National Basic Research Project of China (2011CB922204), and Foundation of the Director of Technical Institute of Physics and Chemistry, CAS. The work was partially supported by RAS Project 24-29 and RFBR Grant 13-02-00825. . - ISSN 1477-9226. - ISSN 1477-9234
   Перевод заглавия: Электронная структура бета-RbSm(MoO4)2 и химическая связь в молибдатах

РУБ Chemistry, Inorganic & Nuclear
Рубрики:
RAY PHOTOELECTRON-SPECTROSCOPY
   CRYSTAL-STRUCTURE
   X-RAY
   NEUTRON-DIFFRACTION
   MAGNETIC-PROPERTIES
   PHASE-FORMATION
   CORE LEVELS
   2ND-HARMONIC GENERATION
   LUMINESCENCE PROPERTIES
   VIBRATIONAL PROPERTIES
Аннотация: Microcrystals of orthorhombic rubidium samarium molybdate, beta-RbSm(MoO4)(2), have been fabricated by solid state synthesis at T = 450 degrees C, 70 h, and at T = 600 degrees C, 150 h. The crystal structure has been refined by the Rietveld method in space group Pbcn with cell parameters a = 5.0984(2), b = 18.9742(6) and c = 8.0449(3) angstrom (R-B = 1.72%). Thermal properties of beta-RbSm(MoO4)(2) were traced by DSC over the temperature range of T = 20-965 degrees C, and the earlier reported β ↔ α phase transition at T similar to 860-910 degrees C was not verified. The electronic structure of beta-RbSm(MoO4) 2 was studied by employing theoretical calculations and X-ray photoelectron spectroscopy. It has been established that the O 2p-like states contribute mainly to the upper part of the valence band and occupy the valence band maximum, whereas the Mo 4d-like states contribute mainly to the lower part of the valence band. Chemical bonding effects have been analysed from the element core level binding energy data. In addition, it was found that the luminescence spectrum of beta-RbSm(MoO4)(2) is rather peculiar among the Sm3+ containing materials. The optical refractive index dispersion in beta-RbSm(MoO4)(2) was also predicted by the first-principles calculations.

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Держатели документа:
RAS, Inst Semicond Phys, Lab Opt Mat & Struct, SB, Novosibirsk 630090, Russia
Tomsk State Univ, Funct Elect Lab, Tomsk 634050, Russia
Novosibirsk State Univ, Lab Semicond & Dielectr Mat, Novosibirsk 630090, Russia
RAS, Kirensky Inst Phys, Lab Coherent Opt, SB, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660041, Russia
RAS, Baikal Inst Nat Management, Lab Oxide Syst, SB, Ulan Ude 670047, Russia
Gen Res Inst Nonferrous Met, Beijing 100088, Peoples R China
RAS, Inst Semicond Phys, Lab Nanodiagnost & Nanolithog, SB, Novosibirsk 630090 90, Russia
RAS, Inst Semicond Phys, Lab Phys Bases Integrated Microelect, SB, Novosibirsk 630090 90, Russia
RAS, Kirensky Inst Phys, Lab Crystal Phys, SB, Krasnoyarsk 660036, Russia
RAS, Kirensky Inst Phys, Lab Mol Spect, SB, Krasnoyarsk 660036, Russia
Chinese Acad Sci, Tech Inst Phys & Chem, Beijing 100190, Peoples R China

Доп.точки доступа:
Atuchin, V. V.; Aleksandrovsky, A. S.; Александровский, Александр Сергеевич; Chimitova, O. D.; Diao, C. P.; Gavrilova, T. A.; Kesler, V. G.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Krylov, A. S.; Крылов, Александр Сергеевич; Bazarov, B. G.; Bazarova, J. G.; Lin, Z. S.; Ministry of Education and Science of the Russian Federation; National Natural Science Foundation of China [11174297, 11474292]; National Basic Research Project of China [2011CB922204]; Foundation of the Director of Technical Institute of Physics and Chemistry, CAS; RAS [24-29]; RFBR [13-02-00825]
}
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    Parshin, A. M.
    The director field distribution with the strongly pinned alignment in nematic structures at the polymer surface / A. M. Parshin, V. Y. Zyryanov, V. F. Shabanov // Liq. Cryst. - 2015. - Vol. 42, Is. 1. - P. 57-64, DOI 10.1080/02678292.2014.960904. - Cited References:18. - This work was partially supported by the Russian Foundation for BasicResearch [project No. 12-03-00816] and by the Siberian Branch of theRussian Academy of Sciences (SB RAS) [grants nos. 30, 24.29, 24.32] andby SB RAS through a Taiwan-SB RAS joint project. . - ISSN 0267. - ISSN 1366-5855
   Перевод заглавия: Распределение поля директора с сильно фиксированным упорядочением в нематических структурах на поверхности полимера

РУБ Chemistry, Multidisciplinary + Crystallography + Materials Science,
Рубрики:
LIQUID-CRYSTALS
DISCLINATION LINES
DEFECTS
Кл.слова (ненормированные):
orientational order -- disclination -- adsorption -- nematic -- polymer surface -- director configuration
Аннотация: We investigate orientational nematic liquid crystal structures that form at the polymer surface due to adsorption, their stability against the schlieren texture and features of point and linear singularities in them. We demonstrate that surface disclination lines, which also occur due to molecular adsorption, can lead to azimuthal anchoring of a bulk layer and make the singularities with the charge m=+/- 1 stable. We consider the director field distribution in a nematic layer as a result of the combination of two aligning factors, which are the linear disclination that tend to impose uniform planar ordering and point defects that impart the radial configuration to the director. With the use of the calculation, we analyse the energies of elastic distortions of the director field for the radial-planar, radial-homeotropic and radial-radial configurations, depending on the nematic layer thickness.

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk, Russia.
Siberian Fed Univ, Dept Energy, Krasnoyarsk, Russia.

Доп.точки доступа:
Zyryanov, V. Ya.; Зырянов, Виктор Яковлевич; Shabanov, V. F.; Шабанов, Василий Филиппович; Паршин, Александр Михайлович; Russian Foundation for Basic Research [12-03-00816]; Siberian Branch ofthe Russian Academy of Sciences (SB RAS) [30, 24.29, 24.32]; SB RASthrough a Taiwan-SB RAS joint project
}
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    Паршин, Александр Михайлович.
    Конфигурации директора в структурах нематика, адсорбированного на поверхности полимера / А. М. Паршин, В. Я. Зырянов, В. Ф. Шабанов // Жидк. кристаллы и их практич. использ. - 2015. - Т. 15, Вып. 1. - С. 56-65 ; Liquid Crystals and their Application. - Библиогр.: 20. - Работа выполнена частично при финансовой поддержке программ Президиума РАН и РФФИ (грант № 15-02-06924). . - ISSN 1991-3966
   Перевод заглавия: Director configurations in the structures of the nematic adsorbed on a polymer surface
Кл.слова (ненормированные):
нематический жидкий кристалл -- полимер -- адсорбция -- дисклинация -- конфигурация директора -- nematic liquid crystal -- polymer -- adsorption -- disclination -- director configuration
Аннотация: Исследованы ориентационные структуры нематических жидких кристаллов, возникающие на поверхности полимера в результате адсорбции, и их устойчивость относительно шлирен-текстуры. Изучены особенности точечных и линейных сингулярностей в исследуемых структурах. Рассмотрены конфигурации директора в слое нематика, определяемые комбинацией двух ориентирующих факторов: воздействием линейной дисклинации, фактора, стремящегося задать однородное планарное упорядочение, а также влиянием точечного дефекта, задающего радиальную структуру директора. С использованием расчетного метода проведен сравнительный анализ энергии упругих искажений поля директора для различных видов конфигураций: радиально-планарной, радиально-гомеотропной и радиально-радиальной в зависимости от толщины слоя нематика.
The orientational structures of nematic liquid crystals that form at the polymer surface due to adsorption and their stability with respect to the schlieren texture are investigated. Features of point and linear singularities in these structures are studied. The director configurations in nematic layer as a result of the combination of two aligning factors, which are the linear disclination that tends to impose uniform planar ordering and point defect that imparts the radial structure to the director are considered. The analysis of the elastic distortions energies of the director configurations for the radial-planar, radial-homeotropic and radial-radial structures, depending on the nematic layer thickness was performed using the calculation method.

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Держатели документа:
Институт физики им. Л.В. Киренского СО РАН

Доп.точки доступа:
Зырянов, Виктор Яковлевич; Zyryanov, V. Ya.; Шабанов, Василий Филиппович; Shabanov, V. F.; Parshin, A. M.

}
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    Experimental results and theoretical model to describe angular dependence of light scattering by monolayer of nematic droplets / V. A. Loiko [et al.] // J. Quant. Spectrosc. Radiat. Transf. - 2016. - Vol. 178: Electromagnetic and light scattering by nonspherical particles XV: Celebrating 150 years of Maxwell's electromagnetics. - P. 263-268, DOI 10.1016/j.jqsrt.2015.10.024. - Cited References:25 . - ISSN 0022-4073. - ISSN 1879-1352
   Перевод заглавия: Экспериментальные результаты и теоретическая модель, описывающая угловую зависимость рассеяния света монослоем капель нематика

РУБ Optics + Spectroscopy
Рубрики:
Dispersed liquid-crystals
   Inhomogeneous boundary-conditions
   Films
   Transmittance
   Radiation
Кл.слова (ненормированные):
Polymer-dispersed liquid crystal film -- Liquid crystal droplet -- Director -- configuration -- Light scattering -- Monolayer of droplets
Аннотация: Light scattering by a monolayer of bipolar nematic droplets encapsulated in polymer film is examined both experimentally and theoretically. A method for the simulation of the angular distribution of scattered light is based on the anomalous diffraction and interference approximations taking into account the director configuration within liquid crystal droplets and their bipolar axes orientation. The director configuration in nematic droplets is calculated using the relaxation method of the free energy minimization. The characteristics of the sample, including distribution of droplet sizes and shape anisometry, are measured in details. The experimental results and theoretical data agree closely with each other. (C) 2015 Elsevier Ltd. All rights reserved.

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Доп.точки доступа:
Loiko, V. A.; Krakhalev, M. N.; Крахалев, Михаил Николаевич; Konkolovich, A. V.; Prishchepa, O. O.; Прищепа, Оксана Олеговна; Miskevich, A. A.; Zyryanov, V. Ya.; Зырянов, Виктор Яковлевич; Conference on Electromagnetic and Light Scattering(15 ; June 21-26, 2015 ; Leipzig, Germany)
}
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Prishchepa, O. O.
Director configurations in nematic droplets with inhomogeneous boundary conditions / O. O. Prishchepa, A. V. Shabanov, V. Y. Zyryanov // Phys. Rev. E. - 2005. - Vol. 72, Is. 3. - Ст. 31712, DOI 10.1103/PhysRevE.72.031712. - Cited References: 22 . - ISSN 1539-3755

РУБ Physics, Fluids & Plasmas + Physics, Mathematical
Рубрики:
DISPERSED LIQUID-CRYSTALS
TRANSITION
Кл.слова (ненормированные):
Lecithin contents -- Nematic droplets -- Polarizers -- Radial structures -- Approximation theory -- Boundary conditions -- Drop breakup -- Free energy -- Polarization -- Textures -- Nematic liquid crystals
Аннотация: The nematic droplets with director configurations intermediate between the bipolar and radial structures have been investigated experimentally and theoretically. The liquid crystal 4(')-n-pentyl-4-cyanobiphenyl (5CB) with a variable addition of the lecithin dispersed in polyvinylbutyral has been used. The characteristic textures of the droplets formed at various lecithin contents have been examined using polarizing microscope both in the crossed polarizers and without analyzer. The computer simulation has been performed for proper ordering of the director in spherical nematic droplets by minimizing the free energy in the one-constant approximation. The inhomogeneous boundary conditions with strong anchoring of the molecules at the interface have been used. The distribution of the anchoring angle at the droplet surface has been estimated based on analysis of observed patterns. The simulated textures of the droplets under crossed polarizers are shown to compare well with the experimental ones.

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Держатели документа:
LV Kirenskii Inst Phys, Akademgorodok, Krasnoyarsk 660036, Russia
ИФ СО РАН
L.V. Kirensky Institute of Physics, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Shabanov, A. V.; Шабанов, Александр Васильевич; Zyryanov, V. Y.; Зырянов, Виктор Яковлевич; Прищепа, Оксана Олеговна
}
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Prischepa, O. O.
Transformation of director configuration upon changing boundary conditions in droplets of nematic liquid crystal / O. O. Prischepa, A. V. Shabanov, V. Y. Zyryanov // JETP Letters. - 2004. - Vol. 79, Is. 6. - P. 257-261, DOI 10.1134/1.1759405. - Cited References: 12 . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
ISOTROPIC LIQUID
DROPS
Аннотация: The transformation of the director configuration upon changing boundary conditions from planar to homeotropic for bipolar nematic droplets dispersed in a polymeric matrix was studied. The characteristic textural patterns are presented for droplets with different concentrations of homeotropic surfactants, and their orientational structure is identified. The scenario predicted earlier by G.E. Volovik and O.D. Lavrentovich (ZhETF 85, 1997 (1983)) for the transformation of orientational structure of nematic droplets from bipolar to radial, without the formation of additional disclinations, is revealed. It is shown that, by using the computational method of minimization of the director elastic-strain energy in the droplet bulk and by introducing the inhomogeneous boundary conditions, one can obtain orientational structures that are analogous to the observed ones.(C) 2004 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Division, Russian Academy of Sciences, Krasnoyarsk, Akademgorodok, 660036, Russian Federation

Доп.точки доступа:
Shabanov, A. V.; Шабанов, Александр Васильевич; Zyryanov, V. Y.; Зырянов, Виктор Яковлевич; Prishchepa, O. O.
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    Near-zero thermal expansion and high ultraviolet transparency in a borate crystal of Zn4B6O13 / X. X. Jiang [et al.] // Adv. Mater. - 2016. - Vol. 28, Is. 36. - P. 7936-7940, DOI 10.1002/adma.201601816. - Cited References:38. - The authors acknowledge Zhuohong Yin for useful discussion and Dr. Siyang Luo for the help in crystal fabrication. This work was supported by the Special Foundation of the Director of Technical Institute of Physics and Chemistry (TIPC), the National Scientific Foundations of China (Grant 11474292 and 51401224), and China "863" project (No. 2015AA034203). . - ISSN 0935-9648. - ISSN 1521-4095
   Перевод заглавия: Нулевое тепловое расширение и высокая ультрафиолетовая прозрачность в борате Zn4B6O13

РУБ Chemistry, Multidisciplinary + Chemistry, Physical + Nanoscience
Рубрики:
ZN4O(BO2)6
   TETRAHEDRA
   BEHAVIOR
   RANGE
Аннотация: Intrinsic isotropic near-zero thermal expansion is discovered in borate crystal Zn4B6O13 with high transparency in the ultraviolet region. First-principles calculations demonstrate that the very low thermal expansion originates mainly from the invariability of the solid [B24O48] truncated octahedra that are fixed by the [Zn4O13] clusters in the ZBO structure.

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Держатели документа:
Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Funct Crystals & Laser Technol, Ctr Crystal R&D, Beijing 100190, Peoples R China.
Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
RAS, Lab Crystal Phys, Kirensky Inst Phys, SB, Krasnoyarsk 660036, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Cryogen, Beijing 100190, Peoples R China.
Chinese Acad Sci, Fujian Inst Res Struct Matter, Fuzhou 350002, Fujian, Peoples R China.
Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Beijing 100871, Peoples R China.
Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China.

Доп.точки доступа:
Jiang, Xingxing; Molokeev, M. S.; Молокеев, Максим Сергеевич; Gong, Pifu; Yang, Y.i.; Wang, Wei; Wang, Shuaihua; Wu, Shaofan; Wang, Yingxia; Huang, Rongjin; Li, Laifeng; Wu, Yicheng; Xing, Xianran; Lin, Zheshuai; Special Foundation of the Director of Technical Institute of Physics and Chemistry (TIPC); National Scientific Foundations of China [11474292, 51401224]; China "863" project [2015AA034203]
}
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Director configurations in nematic droplets with tilted surface anchoring / M. N. Krakhalev [et al.] // Liq. Cryst. - 2017. - Vol. 44, Is. 2. - P. 355-363, DOI 10.1080/02678292.2016.1205225. - Cited References:32. - This work was supported by Russian Foundation for Basic Research (RFBR) under Grants 15-02-06924 and 16-32-00164 and Siberian Branch of the Russian Academy of Sciences (SB RAS) under Complex Program [II.2P 0358-2015-0010], and V.S.S. acknowledges financial support from RFBR [16-32-60036]. . - ISSN 0267-8292. - ISSN 1366-5855

РУБ Chemistry, Multidisciplinary + Crystallography + Materials Science, Multidisciplinary
Рубрики:
DISPERSED LIQUID-CRYSTALS
   RIGIDLY FIXED POLES
   ELECTRIC-FIELD
   POLYMER
Кл.слова (ненормированные):
Polymer dispersed liquid crystal -- nematic droplet -- director -- configuration -- boundary conditions -- surface anchoring strength -- optical -- texture
Аннотация: The polymer dispersed nematic liquid crystal (LC) with the tilted surface anchoring has been studied. The droplet orientational structures with two point surface defects – boojums and the surface ring defect – are formed within the films. The director tilt angle α = 40° ± 4° at the droplet interface and LC surface anchoring strength Ws ~ 10–6 (J m−2) have been estimated. The bipolar axes within the studied droplets of oblate ellipsoidal form can be randomly oriented are oriented randomly relatively to the ellipsoid axes as opposed to the droplets with homeotropic and tangential anchoring.

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Держатели документа:
Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk, Russia.
Siberian Fed Univ, Krasnoyarsk, Russia.

Доп.точки доступа:
Krakhalev, M. N.; Крахалев, Михаил Николаевич; Prishchepa, O. O.; Прищепа, Оксана Олеговна; Sutormin, V. S.; Сутормин, Виталий Сергеевич; Zyryanov, V. Ya.; Зырянов, Виктор Яковлевич; Russian Foundation for Basic Research (RFBR) [15-02-06924, 16-32-00164]; Siberian Branch of the Russian Academy of Sciences (SB RAS) [II.2P 0358-2015-0010]; RFBR [16-32-60036]
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10.

Director reorientation induced by electrically controlled anchoring transition in cholesteric layer / V. S. Sutormin [et al.] // 14th Eur. Conf. Liq. Cryst. (ECLC) : conf. programme / чл. нац. орг. и прогр. ком. V. Ya. Zyryanov. - 2017. - Ст. O34. - P. 8. - Библиогр.: 4

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Доп.точки доступа:
Zyryanov, V. Ya. \чл. нац. орг. и прогр. ком.\; Зырянов, Виктор Яковлевич; Sutormin, V. S.; Сутормин, Виталий Сергеевич; Timofeev, I. V.; Тимофеев, Иван Владимирович; Krakhalev, M. N.; Крахалев, Михаил Николаевич; Prishchepa, O. O.; Прищепа, Оксана Олеговна; Zyryanov, V. Ya.; European Conference on Liquid Crystals(14 ; 2017 ; June ; 25-30 ; Moscow); Московский государственный университет им. М.В. Ломоносова
}
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