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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov S.V.
Заглавие : Dynamic Changes of Optical Characteristics of Resonant Domains in Metal Nanoparticle Aggregates under Pulsed Laser Fields
Место публикации : Applied Physics B: Lasers and Optics. - 2010. - Vol. 101. - С. 512
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov. S.V.
Заглавие : Dynamic changes of optical characteristics of resonant domains in metal nanoparticle aggregates under pulsed laser fields
Коллективы : International Conference on Coherent and Nonlinear Optics, International Conference on Lasers, Applications, and Technologies
Место публикации : Technical digest International conference ICONO/LAT 2010. - Казань, 2010. - Ст.ITuQ39
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Morozov E. V., Trukhan, Sergey N., Kozhevnikov, Ivan V., Peterson, Ivan V., Martyanov, Oleg N.
Заглавие : Dynamics of asphaltene aggregates under high-pressure CO2 revealed by pulsed-field gradient NMR
Колич.характеристики :12 с
Место публикации : Energy & Fuels. - 2023. - Vol. 37, Is. 22. - P.17215-17226. - ISSN 08870624 (ISSN), DOI 10.1021/acs.energyfuels.3c02862. - ISSN 15205029 (eISSN)
Примечания : Cited References: 90. - The present research was performed with the financial support of the Russian Science Foundation (project no. 21-13-00171, http://rscf.ru/project/21-13-00171/) using the equipment of the Krasnoyarsk Regional Center of Research Equipment of the Federal Research Center “Krasnoyarsk Science Center SB RAS”
Аннотация: The work demonstrates the results of the first experimental PFG NMR study in situ of the complex phase behavior of asphaltenes in the presence of high-pressure CO2. To perform the experiments, a series of sealed, thick-walled quartz capillaries were prepared with a mixture of CO2 and asphaltenes dissolved either in chloroform or benzene at different initial concentrations. Then, the temperature dependence of the diffusion coefficients of the asphaltene aggregates was measured for each sample after the mixture reached its equilibrium state, at which, in accordance with the solubility limit, only part of the initial asphaltenes remained dissolved. Despite quite low residual asphaltene concentrations in solution, experimental data clearly demonstrated the presence of aggregated structures (up to 70–80 wt %) attributed solely to nanoaggregates, with no signs of the presence of macroaggregates in the samples. Temperature dependencies of aggregate diffusivity clearly showed that the scenario, according to which the evolution of the asphaltene aggregates will develop, strongly depends on the initial asphaltene concentration, mass fraction of CO2 loaded into the system, and chemical nature of the solvent used. In particular, the most diluted asphaltene solution, expected to be the most resistive to the aggregation processes in a high-pressure CO2 environment, revealed the most pronounced aggregation-dependent translational dynamics as compared to those with a moderate initial asphaltene concentration. Contrarily, the concentrated asphaltene solution may not show drastic aggregation processes if the mass fraction of the CO2 loaded will not appear to be so high. Finally, the experimental results provide evidence that the temperature-triggered structural transformation of asphaltene aggregates due to the noncovalent bond breakup is not hindered under high-pressure CO2, but instead becomes more emphasized. The results obtained shed new light on asphaltene aggregate dynamics and brought new knowledge about the fundamental behavior of asphaltene in high-pressure CO2 conditions.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V., Semina P. N.
Заглавие : Effect of local environment in resonant domains of polydisperse plasmonic nanoparticle aggregates on optodynamic processes in pulsed laser fields
Коллективы : Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101), 3-9-5]
Место публикации : Chin. Phys. B: IOP Publishing, 2015. - Vol. 24, Is. 4. - Ст.047804. - ISSN 1674, DOI 10.1088/1674-1056/24/4/047804. - ISSN 17414199(eISSN)
Примечания : Cited References:25. - Project supported by the Russian Academy of Sciences (Grant Nos. 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101), and 3-9-5).
Предметные рубрики: METAL NANOPARTICLES
GOLD NANOPARTICLES
OPTICAL-PROPERTIES
Ключевые слова (''Своб.индексиров.''): nanoparticle--surface plasmon--colloid aggregate--optodynamics
Аннотация: Interactions of pulsed laser radiation with resonance domains of multiparticle colloidal aggregates having an increasingly complex local environment are studied via an optodynamic model. The model is applied to the simplest configurations, such as single particles, dimers, and trimers consisting of mono- and polydisperse Ag nanoparticles. We analyze how the local environment and the associated local field enhancement by surrounding particles affect the optodynamic processes in domains, including their photomodification and optical properties.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Isaev I. L., Semina P. N., Markel V. A., Karpov S. V.
Заглавие : Effects of size polydispersity on the extinction spectra of colloidal nanoparticle aggregates
Место публикации : Phys. Rev. B: American Physical Society, 2012. - Vol. 85, Is. 4. - Ст.045421. - P. - ISSN 1098-0121, DOI 10.1103/PhysRevB.85.045421
Примечания : Cited References: 41. - This work was supported by grants from the following foundations of the Russian Federation: Presidium of RAS, OFN RAS, and SB RAS.
Предметные рубрики: METAL FRACTAL CLUSTERS
OPTICAL-PROPERTIES
ABSORPTION
NONLINEARITIES
COMPOSITES
SCATTERING
PARTICLES
SPHERES
GRAINS
Аннотация: We investigate the effect of particle polydispersity on the optical extinction spectra of colloidal aggregates of spherical metallic (silver) nanoparticles, taking into account the realistic interparticle gaps caused by layers of stabilizing polymer adsorbed on the metal surface (adlayers). The spectra of computer-generated aggregates are computed using two different methods. The coupled-multipole method is used in the quasistatic approximation and the coupled-dipole method beyond the quasistatics. The latter approach is applicable if the interparticle gaps are sufficiently wide relative to the particle radii. Simulations are performed for two different particle size distribution functions (bimodal and Gaussian), varying the number of particles per aggregate, and different distribution functions of the interparticle gap width. The strong influence of the latter factor on the spectra is demonstrated and investigated in detail.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Markel V. A., Pustovit V. N., Karpov S. V., Obuschenko A. V., Gerasimov V. S., Isaev I. L.
Заглавие : Electromagnetic density of states and absorption of radiation by aggregates of nanospheres with multipole interactions
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2004. - Vol. 70, Is. 5. - Ст.54202. - ISSN 1098-0121, DOI 10.1103/PhysRevB.70.054202
Примечания : Cited References: 81
Предметные рубрики: DISCRETE-DIPOLE APPROXIMATION
ENHANCED RAMAN-SCATTERING
METAL FRACTAL CLUSTERS
OPTICAL-PROPERTIES
SELECTIVE PHOTOMODIFICATION
DISORDERED CLUSTERS
NUMERICAL-SIMULATION
SPECTRAL DEPENDENCE
PARTICULATE MATTER
LIGHT-SCATTERING
Ключевые слова (''Своб.индексиров.''): carbon--iron--palladium--silver--article--dipole--electromagnetic field--geometry--mathematical analysis--molecular interaction--nanoparticle--radiation absorption
Аннотация: We calculate the quasistatic electromagnetic density of states for aggregates of touching spheres, in particular, linear chains and computer-generated random fractal aggregates. Multipole moments with orders of up to L=64 are taken into account for random aggregates with the number of particles of up to N=100 and up to L=8000 for linear chains. Extensive comparisons with the dipole approximation and geometrical cluster renormalization method are performed. Extinction spectra are calculated for several metals and black carbon. Long wavelength electromagnetic properties of fractal aggregates are considered in details.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V.
Заглавие : Plasmonic nanoparticle aggregates in high-intensity laser fields: effect of pulse duration
Место публикации : Plasmonics: Springer, 2016. - Vol. 11, No. 2. - P.403-410. - ISSN 1557-1955, DOI 10.1007/s11468-015-0054-8
Примечания : Cited References: 20. - Authors are thankful to Prof. V.A. Markel (University of Pennsylvania) for supplying program codes with realization of coupled dipole method for polydisperse nanoparticle aggregates. This work was performed within the state contract of the RF Ministry of Education and Science for Siberian Federal University for scientific research in 2014 (Reference number 1792)
Предметные рубрики: METAL NANOPARTICLES
Ключевые слова (''Своб.индексиров.''): nanoparticle--surface plasmon--colloidal aggregate--optodynamics
Аннотация: We use an optodynamic model to study the interaction of pulsed laser radiation of different duration with mono- and polydisperse dimers and trimers of plasmonic nanoparticles as resonant domains of colloid Ag multiparticle aggregates. A comparative analysis of the influence of pulse duration on the kinetic characteristics of domains accompanied by the change in their local structure was carried out taking into account the intensity of incident radiation. The obtained results explain the reasons for laser photochromic reactions in materials containing colloidal aggregates of plasmonic nanoparticles.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gerasimov V. S., Rasskazov I. L., Karpov S. V.
Заглавие : Variations in extinction spectra of plasmonic nanoparticle aggregates upon deformation during deposition on planar dielectric substrate
Коллективы : "Days on diffraction", International conference, Санкт-Петербургское отделение Института математики им. В. А. Стеклова, Санкт-Петербургский государственный университет, Euler International Mathematical Institute, Российский фонд фундаментальных исследований
Место публикации : Annual Int. Conf. "Days on Diffraction". - 2015. - P.141-142
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Karpov S. V., Gerasimov V. S., Isaev I. L., Markel V. A.
Заглавие : Local anisotropy and giant enhancement of local electromagnetic fields in fractal aggregates of metal nanoparticles
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2005. - Vol. 72, Is. 20. - Ст.205425. - ISSN 1098-0121, DOI 10.1103/PhysRevB.72.205425
Примечания : Cited References: 56
Предметные рубрики: SMALL-PARTICLE COMPOSITES
DIFFUSION-LIMITED AGGREGATION
OPTICAL-PROPERTIES
SELECTIVE PHOTOMODIFICATION
NUMERICAL-SIMULATION
DISORDERED CLUSTERS
ABSORPTION-SPECTRUM
PARTICULATE MATTER
NONLINEAR OPTICS
LIGHT-SCATTERING
Аннотация: We have shown within quasistatic approximation that the giant fluctuations of a local electromagnetic field in random fractal aggregates of silver nanospheres are strongly correlated with a local anisotropy factor S which is defined in this paper. The latter is a purely geometrical parameter which characterizes the deviation of local environment of a given nanosphere in an aggregate from spherical symmetry. Therefore, it is possible to predict the sites with anomalously large local fields in an aggregate without explicitly solving the electromagnetic problem. We have also demonstrated that the average (over nanospheres) value of S does not depend noticeably on the fractal dimension D, except when D approaches the trivial limit D=3. In this case, as one can expect, the average local environment becomes spherically symmetrical and S approaches zero. This corresponds to the well-known fact that in trivial aggregates, fluctuations of local electromagnetic fields are much weaker than in fractal aggregates. Thus, we find that, within the quasistatics, the large-scale geometry does not have a significant impact on local electromagnetic responses in nanoaggregates in a wide range of fractal dimensions. However, this prediction is expected not to be correct in aggregates which are sufficiently large for the intermediate- and radiation-zone interaction of individual nanospheres to become important.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yakubailik E. K., Ganzhenko I. M., Balaev A. D., Butov, P. Yu.
Заглавие : Magnetic parameters of separation products and impurity aggregates in concentrates
Место публикации : J. Min. Sci. - 2017. - Vol. 53, Is. 6. - P.1133-1140. - ISSN 1062-7391, DOI 10.1134/S1062739117063233. - ISSN 1573-8736(eISSN)
Примечания : Cited References: 14
Ключевые слова (''Своб.индексиров.''): processing circuit--wet laboratory separation--concentrate impurity--magnetic characteristics
Аннотация: The changes in separation performance and magnetic characteristics of separation products is traced along the processing circuit of Abagur concentrator at a laboratory scale in order to determine the limit content of magnetite iron in impurity aggregates in the concentrate. The wet magnetic analysis is carried out in the field of H = 175 kA/m, and the magnetic characteristics are determined in the vibration magnetic detector in the field up to 800 kA/m. The concentrate impurity content is governed by the relative content of barren rock and ore aggregates removable in concentration at the given level of the technology.
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Morozov E. V., Martyanov O. N.
Заглавие : Reversibility of asphaltene aggregation as revealed by magnetic resonance imaging in situ
Место публикации : Energy Fuels: American Chemical Society, 2017. - Vol. 31, Is. 10. - P.10639-10647. - ISSN 08870624 (ISSN), DOI 10.1021/acs.energyfuels.7b01755
Примечания : Cited References: 56. - This research was performed on the equipment of Krasnoyarsk Regional Research Equipment Centre of Siberian Branch of Russian Academy of Sciences with the financial support of Russian Science Foundation (Project No. 15-19-00119).
Ключевые слова (''Своб.индексиров.''): aggregates--crude oil--flocculation--heavy oil production--magnetic resonance imaging--asphaltene aggregates--asphaltene aggregation--asphaltene precipitation--equilibrium compositions--flocculant concentrations--inhomogeneous distribution--mechanical stirring--multi-component systems--asphaltenes
Аннотация: Aggregation of asphaltenes followed by precipitation presents severe problems for existing technologies in the production, recovery, and processing of heavy oils. Better understanding of asphaltene behavior behind the processes of their precipitation and dissolution is vital to address this issue. While investigating the inhomogeneity of different oil systems, the reversibility of the asphaltene aggregation process initiated by flocculant in either asphaltene solution in toluene or crude heavy oil was revealed and investigated using magnetic resonance imaging methods. It was found that the inhomogeneous distribution of the flocculant initiates local spatial-selective asphaltene aggregation registered in a thin layer around the flocculant/oil sample interface. The local excess of flocculant concentration over the threshold of asphaltene precipitation onset is a driving force of this process. As the flocculant diffuses into the volume of the sample, a decrease of the asphaltene flocculated area is observed until it disappears when the equilibrium composition throughout the whole volume of the system is achieved. Depending on the overall flocculant concentration, the asphaltene aggregation may not be reversible and could be followed by subsequent precipitation of the asphaltene aggregates. The similarity of the phenomena observed for the model asphaltene solutions and crude heavy oil samples was established. Partial mechanical stirring of the multicomponent system comprising flocculant and oil or asphaltene solution does not prevent the formation of the local zones with increased concentration of asphaltene aggregates; those sizes evolve depending on the flocculant concentration. The results obtained in this work are consistent with the generally accepted concept of asphaltene precipitation reversibility depending on the system composition and are compatible with the observations obtained by other methods. The approach presented can provide deeper insight into the asphaltene precipitation reversibility issue and can facilitate the understanding of asphaltene behavior in heavy oils.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Morozov E. V., Yushmanov, Pavel, V, Martyanov, Oleg N.
Заглавие : Temperature-Triggered Rearrangement of Asphaltene Aggregates as Revealed by Pulsed-Field Gradient NMR
Коллективы : Russian Science FoundationRussian Science Foundation (RSF) [15-19-00119]
Место публикации : Energy Fuels. - 2019. - Vol. 33, Is. 8. - P.6934-6945. - ISSN 0887-0624, DOI 10.1021/acs.energyfuels.9b00600. - ISSN 1520-5029(eISSN)
Примечания : Cited References: 119. - This research was performed using the equipment of Krasnoyarsk Regional Research Equipment Centre of Siberian Branch of Russian Academy of Sciences with the financial support of Russian Science Foundation (Project No. 15-19-00119).
Предметные рубрики: CRITICAL NANOAGGREGATE CONCENTRATION
ELECTRON-SPIN-RESONANCE
Аннотация: The tendency of asphaltenes for aggregation followed by precipitation and deposition plays a crucial role in the petroleum industry since these processes present severe problems during the production, recovery, and processing of crude oils and fossil hydrocarbon feedstocks. The dynamics of oil asphaltene aggregates dissolved in chloroform at different concentrations varied in a wide range that was investigated at temperatures from 0 to 55 °C using the Pulsed-Field Gradient NMR technique. The components attributed to nanoaggregates and macroaggregates were successfully resolved, which allowed us to measure their diffusion coefficients. The diffusion coefficients for all types of aggregates grow as the asphaltene concentration decreases, whereas the partial weight of the aggregates increases with the increase of asphaltene concentration. The difference in diffusion behavior of the aggregates of different types was registered when passing the critical concentration range 10–20 g/L. The nano- and macroaggregates behave independently when the asphaltene concentration is higher than 20 g/L (concentrated regime), while below 20 g/L (semidiluted regime) the components related to the different types of aggregates cannot be properly resolved. It was found that regardless of the asphaltene concentration, the diffusion coefficients for nano- and macroaggregates demonstrate similar temperature behavior giving the straight lines in the Arrhenius coordinates which change their slopes when passing the temperature range 20–30 °C. The phenomenon evidences the thermally induced cleavage of noncovalent bonds with subsequent rearrangement of asphaltene aggregates that is observed for all concentration regimes covering the existence of asphaltene aggregates of all types. The data obtained are well consistent with the modern concept of asphaltene aggregate structure and fairly agree with the data obtained earlier. We believe these results will contribute essentially to a better understanding of the fundamental behavior of asphaltenes and their aggregates, providing a deep insight into aggregate transformation triggered by the temperature.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Markel V. A., Shalaev V. M., Poliakov E. Y., George T. F.
Заглавие : Numerical studies of second- and fourth-order correlation functions in cluster-cluster aggregates in application to optical scattering
Место публикации : Phys. Rev. E: AMERICAN PHYSICAL SOC, 1997. - Vol. 55, Is. 6. - P7313-7333. - ISSN 1063-651X, DOI 10.1103/PhysRevE.55.7313
Примечания : Cited References: 21
Предметные рубрики: DIFFUSION-LIMITED AGGREGATION
COLLOIDAL AGGREGATION
FRACTAL CLUSTERS
ANTICORRELATION
SIMULATIONS
Аннотация: Two- and four-point density correlation functions p(2)(r) and p(4)(r) are studied numerically and theoretically in computer-generated three-dimensional lattice cluster-cluster aggregates (CCA) with the number of particles N up to 20 000 in application to the light scattering problem. The ''pure'' aggregation algorithm is used, where subclusters of all possible sizes are allowed to collide. We find that large CCA clusters demonstrate pronounced multiscaling. In particular, the fractal dimension determined from the slope of p(2)(r) at small distances differs from that found from the dependence of the radius of gyration on the number of monomers (according to our data, 1.80 and 1.94, respectively). We also consider different functional forms for p(2) and their general properties and applicability. We find that the best fit to the numerical data is provided by the generalized exponential cutoff function with coefficients depending on N. The latter dependence is a manifestation of multiscaling. We propose some theoretical approaches for calculating p(4)(r), assuming p(2)(r) is known. In particular, we find the small-r asymptote for the p(4)(r) and verify it numerically. In addition, we find that p(4)(r) cannot be represented by a scaling dependence with a cutoff function, like p(2)(r) Instead, p(4)(r) is given by an expansion in terms of integer powers of r(2D-3), where D is the fractal dimension (approximate to 1.8 for CCA clusters).
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14.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V., Semina P. N.
Заглавие : Optodynamic and photochrome effects in composite media with aggregates of plasmonic nanoparticles in pulsed laser fields
Коллективы : International Conference on Lasers, Applications, and Technologies (LAT 2013) (2013 ; June ; 18-22; Moscow)
Место публикации : ICONO/LAT 2013 : Advance conference program. - 2013. - P.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V., Semina P. N.
Заглавие : Optodynamic phenomena in aggregates of polydisperse plasmonic nanoparticles
Коллективы : Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101)]; Ministry of Education and Science of Russian Federation [14.B37.21.0457]
Место публикации : Appl. Phys. B: Springer, 2014. - Vol. 115, Is. 4. - P.547-560. - ISSN 0946-2171, DOI 10.1007/s00340-013-5636-6. - ISSN 1432-0649
Примечания : Cited References: 48. - Authors are thankful to Prof. V. A. Markel (University of Pennsylvania) for supplying program codes for realization of the coupled dipole method for polydisperse metal nanoparticle aggregates. This research was supported by the Russian Academy of Sciences under the Grants 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101); Ministry of Education and Science of Russian Federation under Contract 14.B37.21.0457.
Предметные рубрики: SMALL-PARTICLE COMPOSITES
OPTICAL-PROPERTIES
NOBLE-METALS
SILVER
ELECTRON
LIQUID
GENERATION
DYNAMICS
FORCES
GOLD
Аннотация: We propose an optodynamical model of interaction of pulsed laser radiation with aggregates of spherical metallic nanoparticles embedded into host media. The model takes into account polydispersity of particles, pair interactions between the particles, dissipation of absorbed energy, heating and melting of the metallic core of particles and of their polymer adsorption layers, and heat exchange between electron and ion components of the particle material as well as heat exchange with the interparticle medium. Temperature dependence of the electron relaxation constant of the particle material and the effect of this dependence on interaction of nanoparticles with laser radiation are first taken into consideration. We study in detail light-induced processes in the simplest resonant domains of multiparticle aggregates consisting of two particles of an arbitrary size in aqueous medium. Optical interparticle forces are realized due to the light-induced dipole interaction. The dipole moment of each particle is calculated by the coupled dipole method (with correction for the effect of higher multipoles). We determined the role of various interrelated factors leading to photomodification of resonant domains and found an essential difference in the photomodification mechanisms between polydisperse and monodisperse nanostructures.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A. P., Karpov S. V.
Заглавие : Processes in resonant domains of metal nanoparticle aggregates and optical nonlinearity of aggregates in pulsed laser fields
Место публикации : Appl. Phys. B-Lasers Opt. - NEW YORK: SPRINGER, 2009. - Vol. 97, Is. 1. - С. 163-173. - SEP. - ISSN 0946-2171, DOI 10.1007/s00340-009-3592-y
Примечания : Cited Reference Count: 43. - Гранты: Authors are thankful to Prof. V. A. Markel ( University of Pennsylvania) for computation of multipole polarizability of silver nanoparticle bispheres, for the attention to this paper, fruitful discussions and great support. This research was supported by grants: 27.1 of the Presidium of RAS, 9.1 DPS RAS, 5 SB RAS, 3818.2008.3 and 6612.2006.3 of the President of RF ( SS RAS), DSP 2.1.1.1814, 05- 03- 32642 RFBR.Финансирующая организация: [27.1 of the Presidium of RAS]; [9.1 DPS RAS]; [5 SB RAS]; [3818.2008.3]; [6612.2006.3]
Предметные рубрики: SMALL-PARTICLE COMPOSITES
FRACTAL CLUSTERS
SELECTIVE PHOTOMODIFICATION
ABSORPTION-COEFFICIENTS
REFRACTIVE-INDEXES
SILVER
ENHANCEMENT
RESPONSES
GOLD
Ключевые слова (''Своб.индексиров.''): metal nanoparticles--nanosecond pulsed laser--nonlinear refractive index--optical nonlinearity--physical effects--pulsed-laser field--resonant domain--silver nanoparticles--simple physical models--aggregates--laser excitation--nanoparticles--nonlinear optics--organic polymers--pulsed laser applications--refractive index--silver
Аннотация: Optical nonlinearities in aggregates of nanoparticles formed in silver hydrosols (SHs) are studied under pico- and nanosecond pulsed laser excitation. The dependence of the nonlinear refractive index n (2) on the degree of hydrosol aggregation is studied experimentally at the wavelength lambda=1.064 mu m. It is found that n (2) changes sign when the degree of hydrosol aggregation is increased. Various physical effects occurring in resonant domains of the aggregates are analyzed using a simple physical model of two bound silver nanoparticles. The theory takes into account thermal, elastic, electrostatic, and light-induced effects. Experimental results are discussed in the context of this theory.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov S.V.
Заглавие : Processes in Resonant Domains of Metal Nanoparticle Aggregates and Optical Nonlinearity of Aggregates in Pulsed Laser Fields
Место публикации : arXiv: Cornell University, 2008. - Ст.0808.2355
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gerasimov V. S., Isaev I. L., Gavrilyuk A. P., Karpov S. V.
Заглавие : Processes underlying the laser photochromic effect in colloidal plasmonic nanoparticle aggregates*
Коллективы : Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Government of the Krasnoyarsk Territory [18-42-243023]; Krasnoyarsk Regional Fund of Science [18-42-243023]; RF Ministry of Science and Higher Education; Siberian Federal University for Scientific Research; Russian FederationRussian Federation [075-15-2019-676]
Место публикации : Chin. Phys. B. - 2020. - Vol. 29, Is. 3. - Ст.037802. - ISSN 1674-1056, DOI 10.1088/1674-1056/ab6551. - ISSN 1741-4199(eISSN)
Примечания : Cited References: 38. - Project funded by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science (Grant 18-42-243023), the RF Ministry of Science and Higher Education, and the State Contract with Siberian Federal University for Scientific Research. A.E. thanks the grant of the President of Russian Federation (agreement 075-15-2019-676).
Предметные рубрики: SELECTIVE PHOTOMODIFICATION
LIGHT
FORCES
OPTICS
Аннотация: We have studied the dynamic and static processes occurring in disordered multiparticle colloidal Ag aggregates with natural structure and affecting their plasmonic absorption spectra under pico- and nanosecond pulsed laser radiations, as well as the physical origin responsible for these processes. We have shown that depending on the duration of the laser pulse, the mechanisms of laser modification of such aggregates can be associated both with changes in the resonant properties of the particles due to their heating and melting (picosecond irradiation mode) and with the particle shifts in the resonant domains of the aggregates (nanosecond pulses) which depend on the wavelength, intensity, and polarization of the radiation. These mechanisms result in formation of a narrow dip in the plasmonic absorption spectrum of the aggregates near the laser radiation wavelength and affect the shape and position of the dip. The effect of polydispersity of nanoparticle aggregates on laser photochromic reaction has been studied.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V., Polyutov S. P.
Заглавие : Restructuring of plasmonic nanoparticle aggregates with arbitrary particle size distribution in pulsed laser fields
Место публикации : Chin. Phys. B: IOP, 2016. - Vol. 25, Is. 11. - Ст.117806. - ISSN 16741056 (ISSN), DOI 10.1088/1674-1056/25/11/117806
Примечания : Cited References: 47. - This work was performed within the state contract of the RF Ministry of Education and Science for Siberian Federal University for scientific research in 2016 (Reference number 1792) and SB RAS Program No II.2P (0358-2015-0010). Numerical computations were performed on the cluster MVS-1000 M of the Institute of computational modeling SB RAS.
Ключевые слова (''Своб.индексиров.''): optodynamics--nanoparticle--surface plasmon--laser radiation
Аннотация: We have studied processes of interaction of pulsed laser radiation with resonant groups of plasmonic nanoparticles (resonant domains) in large colloidal nanoparticle aggregates having different interparticle gaps and particle size distributions. These processes are responsible for the origin of nonlinear optical effects and photochromic reactions in multiparticle aggregates. To describe photo-induced transformations in resonant domains and alterations in their absorption spectra remaining after the pulse action, we introduce the factor of spectral photomodification. Based on calculation of changes in thermodynamic, mechanical, and optical characteristics of the domains, the histograms of the spectrum photomodification factor have been obtained for various interparticle gaps, an average particle size, and the degree of polydispersity. Variations in spectra have been analyzed depending on the intensity of laser radiation and various combinations of size characteristics of domains. The obtained results can be used to predict manifestation of photochromic effects in composite materials containing different plasmonic nanoparticle aggregates in pulsed laser fields. © 2016 Chinese Physical Society and IOP Publishing Ltd.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Karpov S. V., Gerasimov V. S., Isaev I. L., Markel V. A.
Заглавие : Spectroscopic studies of fractal aggregates of silver nanospheres undergoing local restructuring
Место публикации : J. Chem. Phys.: AMER INST PHYSICS, 2006. - Vol. 125, Is. 11. - Ст.111101. - ISSN 0021-9606, DOI 10.1063/1.2229202
Примечания : Cited References: 30
Предметные рубрики: ENHANCED RAMAN-SCATTERING
SMALL-PARTICLE COMPOSITES
OPTICAL-PROPERTIES
DISORDERED CLUSTERS
NONLINEAR OPTICS
LOCALIZATION
NANOPARTICLES
EIGENMODES
BOUNDS
Ключевые слова (''Своб.индексиров.''): large-scale fractal geometry--nonlinear optical responses--restructuring--silver nanospheres--aggregates--colloids--electromagnetic fields--fractals--nonlinear optics--sampling--spectroscopic analysis--silver
Аннотация: We present an experimental spectroscopic study of large random colloidal aggregates of silver nanoparticles undergoing local restructuring. We argue that such well-known phenomena as strong fluctuation of local electromagnetic fields, appearance of "hot spots" and enhancement of nonlinear optical responses depend on the local structure on the scales of several nanosphere diameters, rather than the large-scale fractal geometry of the sample. (c) 2006 American Institute of Physics.
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