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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrakovskii G. A., Kuzmin E. V., Aplesnin S. S.
Заглавие : Spin-wave spectrum and thermodynamic properties of antiferromagnet with diamagnetic dilution and fluctuating exchange interactions
Место публикации : Fiz. Tverd. Tela. - 1984. - Vol. 26, Is. 3. - P.765-772. - ISSN 0367-3294
Примечания : Cited References: 17
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Dimerization of antiferromagnetic chain with 4-spin interaction
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1996. - Vol. 38, Is. 6. - P1868-1877. - ISSN 0367-3294
Примечания : Cited References: 30
Предметные рубрики: SPIN-1/2 HEISENBERG-ANTIFERROMAGNET
COMPETING INTERACTIONS
MONTE-CARLO
THERMODYNAMIC PROPERTIES
SYSTEMS
CUGEO3
TEMPERATURE
NEUTRON
STATE
MODEL
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : APLESNIN S. S.
Заглавие : MAGNETIC-PROPERTIES OF A UNIAXIAL ANISOTROPIC ANTIFERROMAGNET WITH TRIANGULAR LATTICE
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1989. - Vol. 31, Is. 10. - P83-91. - ISSN 0367-3294
Примечания : Cited References: 12
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fedoseeva N. V., Gekht R. S., Velikanova T. A., Balaev A. D.
Заглавие : New intermediate phase in the spiral antiferromagnet cscucl3 induced by a strong magnetic-field
Место публикации : JETP Letters. - 1985. - Vol. 41, Is. 8. - P.406-410. - ISSN 0021-3640
Примечания : Cited References: 5
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Rudenko V. V.
Заглавие : Magnetic anisotropy of a manganese carbonate antiferromagnet
Место публикации : Russ. Phys. J.: SPRINGER, 2009. - Vol. 52, Is. 9. - P.990-991. - ISSN 1064-8887
Примечания : Cited References: 9
Предметные рубрики: S-IONS
Ключевые слова (''Своб.индексиров.''): magnetic anisotropy--crystalline field--electron paramagnetic resonance
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Boldyrev K. N., Stanislavchuk T. N., Sirenko A. A., Kamenskyi D., Bezmaternykh L. N., Popova M. N.
Заглавие : Bifurcations of coupled electron-phonon modes in an antiferromagnet subjected to a magnetic field
Место публикации : Phys. Rev. Lett.: American Physical Society, 2017. - Vol. 118, Is. 16. - Ст.167203. - ISSN 00319007 (ISSN), DOI 10.1103/PhysRevLett.118.167203
Примечания : Cited References: 26. - This research was supported by the Russian Scientific Foundation under Grant No. 14-12-01033, the President of Russian Federation (MK-3577.2017.2, K. N. B.), and the U.S. Department of Energy under Grant No. DE-FG02-07ER46382 (experiments at U4-IR beam line NSLS-BNL, T. N. S. and A. A. S.). The National Synchrotron Light Source is operated as a user facility for the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. Part of this work was supported by EMFL (Contract No. 26211). M. N. P. thanks B. Z. Malkin and A. V. Popov for helpful discussions.
Ключевые слова (''Своб.индексиров.''): antiferromagnetic materials--bifurcation (mathematics)--electron-phonon interactions--electrons--magnetic fields--magnetism--temperature--antiferromagnetic crystals--bifurcation points--electron phonon couplings--electronic excitation--external magnetic field--field independents--low temperatures--reflection spectra--phonons
Аннотация: We report on a new effect caused by the electron-phonon coupling in a stoichiometric rare-earth antiferromagnetic crystal subjected to an external magnetic field, namely, the appearance of a nonzero gap in the spectrum of electronic excitations in an arbitrarily small field. The effect was registered in the low-temperature far-infrared (terahertz) reflection spectra of an easy-axis antiferromagnet PrFe3(BO3)4 in magnetic fields Bext-c. Both paramagnetic and magnetically ordered phases (including a spin-flop one) were studied in magnetic fields up to 30 T, and two bifurcation points were observed. We show that the field behavior of the coupled modes can be successfully explained and modeled on the basis of the equation derived in the framework of the theory of coupled electron-phonon modes, with the same field-independent electron-phonon interaction constant |W|=14.8 cm-1. © 2017 American Physical Society.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Wu L. S., Nikitin S. E., Frontzek M., Kolesnikov A. I., Ehlers G., Lumsden M. D., Shaykhutdinov K. A., Guo, E. -J., Savici A. T., Gai Z., Sefat A. S., Podlesnyak A.
Заглавие : Magnetic ground state of the Ising-like antiferromagnet DyScO3
Коллективы : Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division
Место публикации : Phys. Rev. B: American Physical Society, 2017. - Vol. 96, Is. 14. - Ст.144407. - ISSN 2469-9950, DOI 10.1103/PhysRevB.96.144407. - ISSN 2469-9969(eISSN)
Примечания : Cited References:37. - We thank J. M. Sheng and Q. Zhang for the help with the neutron data refinement. We would like to thank A. Christianson, I. Zaliznyak, M. Mourigal, Z. T. Wang, and C. Batista for useful discussions. The research at the Spallation Neutron Source (ORNL) is supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). Research supported in part by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This work was partly supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division.
Предметные рубрики: THIN-FILMS
FERROELECTRICITY
VISUALIZATION
EXCITATIONS
Аннотация: We report on the low-temperature magnetic properties of the DyScO3 perovskite, which were characterized by means of single crystal and powder neutron scattering, and by magnetization measurements. Below TN = 3.15 K, Dy3+ moments form an antiferromagnetic structure with an easy axis of magnetization lying in the ab plane. The magnetic moments are inclined at an angle of ∼ +/- 28 degrees to the b axis. We show that the ground-state Kramers doublet of Dy3+ is made up of primarily |+/- 15/2 ⟩ eigenvectors and well separated by a crystal field from the first excited state at E1 = 24.9 meV. This leads to an extreme Ising single-ion anisotropy, M⊥/M∥∼ 0.05. The transverse magnetic fluctuations, which are proportional to M⊥2/M∥2, are suppressed, and only moment fluctuations along the local Ising direction are allowed. We also found that the Dy-Dy dipolar interactions along the crystallographic c axis are two to four times larger than in-plane interactions.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gnatchenko S. L., Kashur I. S., Kurnosov V. S., Piryatinskaya V. G., Malakhovskii A. V., Gudim I. A.
Заглавие : Transversal Zeeman effect in NdFe3(BO3)4 antiferromagnet
Коллективы : Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium, Институт физики им. Л.В. Киренского Сибирского отделения РАН
Место публикации : VI Euro-Asian Symposium "Trends in MAGnetism" (EASTMAG-2016): abstracts/ ed.: O. A. Maksimova, R. D. Ivantsov. - Krasnoyarsk: KIP RAS SB, 2016. - Ст.P6.13. - P.321. - ISBN 978-5-904603-06-9 (Шифр -478014040)
Примечания : References: 1
Ключевые слова (''Своб.индексиров.''): kramers doublet--splitting--effective field
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Prosnikov M. A., Smirnov A. N., Davydov, V. Yu, Sablina K. A., Pisarev R. V.
Заглавие : Lattice and magnetic dynamics of a quasi-one-dimensional chain antiferromagnet PbFeBO4
Коллективы : Russian Science Foundation [16-12-10456]
Место публикации : J. Phys.: Condens. Matter: IOP Publishing, 2017. - Vol. 29, Is. 2. - Ст.025808. - ISSN 0953-8984, DOI 10.1088/0953-8984/29/2/025808. - ISSN 1361-648X(eISSN)
Примечания : Cited References:32. - This research was supported by the Russian Science Foundation, grant No. 16-12-10456.
Предметные рубрики: LIGHT-SCATTERING
DIELECTRIC-PROPERTIES
RAMAN-SPECTROSCOPY
Ключевые слова (''Своб.индексиров.''): raman scattering--spin and phonon excitations--spin-phonon interaction--antiferromagnetism--magnetic symmetry analysis--two-magnon scattering
Аннотация: A group of recently synthesized orthorhombic Pnma crystals PbMBO4 (M = Cr, Mn, Fe) demonstrates a number of unusual structural and magnetic properties. We report on polarized Raman scattering study of the lattice and magnetic dynamics in single crystals of an antiferromagnet PbFeBO4 below and above T-N = 114 K. Polarization properties of the observed magnetic excitations below T-N as well as intense quasi-elastic scattering support the quasi-one-dimensional character of the magnetic structure of PbFeBO4. Frequency overlapping of magnetic excitations and low-frequency phonons in the range of 90-200 cm-1 leads to pronounced asymmetric anomalies thus confirming intrinsic coupling of magnetic and lattice subsystems. This conclusion is also supported by observation of anomalous temperature behaviour of higher frequency phonons in the vicinity of T-N. Experimental investigations are supported by relevant magnetic symmetry analysis which allows us to explain previously observed anomalous results.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Rasch JCE, Boehm M., Ritter C., Mutka H., Schefer J., Keller L., Abramova G. M., Cervellino A., Loffler J. F.
Заглавие : Magnetoelastic coupling in the triangular lattice antiferromagnet CuCrS2
Коллективы : Russian Academy of Science (RAS), Siberian Branch [06-1000013-9002]
Место публикации : Phys. Rev. B. - 2009. - Vol. 80, Is. 10. - Ст.104431. - ISSN 1098-0121, DOI 10.1103/PhysRevB.80.104431
Примечания : Cited References: 30. - We are grateful for support and allocated beam time at the Institut Laue-Langevin (D1A, IN3),Grenoble, France, the spallation neutron source SINQ (TriCS, DMC) and the SLS-MS beamline, both Paul Scherrer Insitut, Villigen, Switzerland. This work was supported by INTAS Grant No. 06-1000013-9002 of the Russian Academy of Science (RAS), Siberian Branch.
Предметные рубрики: NEUTRON POWDER DIFFRACTION
MAGNETIC-STRUCTURE
STRUCTURAL-PROPERTIES
PHASE-TRANSITION
SOLID OXYGEN
ALPHA-PHASES
BETA-PHASES
SELENIDES
SULFIDES
Аннотация: CuCrS2 is a triangular lattice Heisenberg antiferromagnet with a rhombohedral crystal structure. We report on neutron and synchrotron powder diffraction results which reveal a monoclinic lattice distortion at the magnetic transition and verify a magnetoelastic coupling. CuCrS2 is therefore an interesting material to study the influence of magnetism on the relief of geometrical frustration.
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Martynov S. N.
Заглавие : Phase diagram of the helical structure of a two-subsystem frustrated antiferromagnet
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2009. - Vol. 108, Is. 1. - P72-82. - ISSN 1063-7761, DOI 10.1134/S1063776109010105
Примечания : Cited References: 25
Предметные рубрики: GROUND SPIN-STATE
PYROCHLORE ANTIFERROMAGNET
TRIANGULAR-LATTICE
CLASSICAL-THEORY
MODEL
TRANSITION
Ключевые слова (''Своб.индексиров.''): antiferromagnetic materials--antiferromagnetism--free energy--magnetic devices--magnetic fields--magnetic structure--phase diagrams--vectors--antiferromagnet--antiferromagnetic--antiferromagnetic sublattices--comparative analysis--critical fields--external fields--field boundaries--first derivatives--first-order transitions--helical orderings--helical phase--helical structures--higher temperatures--incommensurate magnetic structures--isotropic exchanges--magnetic subsystems--magnetization jumps--mean-field approximations--minimum free energies--numerical minimizations--spatial displacements--temperature dependences--thermodynamic potentials--variational equations--wave vectors--phase transitions
Аннотация: The expansion of the thermodynamic potential for the two-subsystem antiferromagnet with frustrated intersubsystem isotropic exchange is obtained. It is demonstrated that this expansion contains the first derivatives with respect to the antiferromagnetic vectors of the subsystems, i.e., the Lifshitz invariant. The equation for the temperature-field boundary of the helical phase for the two-subsystem frustrated antiferromagnet is derived by linearizing the variational equations for the minimum free energy within the mean-field approximation. Relationships are obtained for the critical field at T = 0, the angle of canting of moments of the antiferromagnetic sublattices, and the temperature of spontaneous appearance of helical ordering in the absence of an external field. It is revealed that there is a second higher temperature of formation of the helical magnetic structure induced by the magnetic field with the wave vector of the helix nonmonotonically depending on the external field. The phase boundary of the helical phase and the temperature dependence of the orientation of moments of the magnetic subsystem with weak exchange interaction are determined using numerical minimization of the free energy. It is shown that the transition to the commensurate phase is a first-order transition with a small magnetization jump. A comparative analysis of models with different spatial displacements of ions in the subsystems along the direction of the vector of the helical structure is performed. A criterion is proposed for the choice of the direction of the vector of the incommensurate magnetic structure.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bondarenko I. N., Gekht R. S., Ponomarev V. I.
Заглавие : Magnetic transitions in layered triangular antiferromagnets
Место публикации : Phys. Lett. A: ELSEVIER SCIENCE BV, 1996. - Vol. 222, Is. 4. - P269-274. - ISSN 0375-9601, DOI 10.1016/0375-9601(96)00635-4
Примечания : Cited References: 22
Предметные рубрики: HEISENBERG-ANTIFERROMAGNET
PHASE-TRANSITION
VBR2
SYSTEMS
FIELD
VCL2
Ключевые слова (''Своб.индексиров.''): triangular antiferromagnets--quantum and thermal fluctuations--successive phase transitions--quantum and thermal fluctuations--successive phase transitions--triangular antiferromagnets
Аннотация: Magnetic states and phase transitions of the layered triangular antiferromagnets in an applied field are studied. It is shown that in compounds like VBr2 and VCl2 quantum effects change the ground state structure and cause successive phase transitions as the magnetic field increases. Coplanar structures of different spin configuration are realized far from the saturation field and a noncoplanar structure of umbrella-type configuration is realized near this field. The ground-state phase diagram is constructed, and a finite region of fields where the collinear phase is also possible is indicated.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Martynov S. N.
Заглавие : The incommensurate magnetic structure of a tetragonal antiferromagnet with antisymmetric exchange
Место публикации : J. Exp. Theor. Phys. - 2009. - Vol. 109, Is. 6. - P.979-988. - ISSN 1063-7761, DOI 10.1134/S1063776109120097
Примечания : Cited References: 34
Предметные рубрики: FLUCTUATION-INDUCED PHASE
FIELD-INDUCED GAP
COPPER METABORATE
WEAK FERROMAGNETISM
SOLITON LATTICE
SPIN-WAVES
CUB2O4
BA2CUGE2O7
CSCUCL3
CHAINS
Ключевые слова (''Своб.индексиров.''): anti-symmetric--antiferromagnetic sublattices--antiferromagnets--antisymmetric exchange--exchange bonds--ferromagnetic component--ferromagnetic moments--ginzburg-landau functional--incommensurate magnetic structures--mean field approximation--modulation vectors--polarization planes--polarization vectors--symmetry groups--antiferromagnetic materials--antiferromagnetism--crystal orientation--crystal symmetry--ferromagnetic materials--ferromagnetism--magnetic devices--magnetic structure--modulation--polarization--vector spaces--vectors--crystallography
Аннотация: Analysis of the incommensurate magnetic structure that emerges for two coexisting types of the antisymmetric Dzyaloshinski-Moriya exchange interaction (the weakly ferromagnetic component of vector D along the tetragonal axis and the helicoidal component distributed in the tetragonal plane) is carried out for the first time for a tetragonal antiferromagnet. The helicoidal component for each pair of interacting spins has a 2D distribution; its direction in the tetragonal plane depends on the direction of the exchange bond in each pair. The Lifshits invariant of the Ginzburg-Landau functional is obtained, which is responsible for the formation of an incommensurate magnetic structure for such a distribution. It is shown in the mean field approximation that the incommensurate magnetic structure that forms in this case is a nonlinear double helicoid with a modulation vector lying in the tetragonal plane and with a varying angle between the polarization planes of quasi-antiferromagnetic sublattices. The ground state of the magnet is degenerate in the orientation of the modulation vector in the tetragonal plane. The rate of variation in the orientations of moments in the polarization planes passing through the tetragonal axis is controlled by the angle between the directions of the moments and the tetragonal axis. The local weakly ferromagnetic moment remaining in the polarization plane varies in magnitude and sign. The relation between the orientations of the modulation and polarization vectors is derived for the cases of simple and inversion tetragonal axes in the space symmetry group of the crystal.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : The study of magnetic properties of the quasi-one-dimensianal spin-1/2 antiferromagnet by Monte-Carlo method
Место публикации : Phys. Low-Dimens. Struct.: V S V CO. LTD, 2000. - Vol. 07.08.2013. - P37-46. - ISSN 0204-3467
Примечания : Cited References: 15
Предметные рубрики: ONE-DIMENSIONAL ANTIFERROMAGNETS
SYSTEMS
CHAINS
CA2CUO3
Аннотация: The thermodynamic quantities, two- and four-spin correlation functions as well as the correlation radius for weakly coupled antiferromagnetic spin chains with S = 1/2 are calculated using the mean-field approximation for the interchain coupling (J(2)) for longitudinal and transverse spin components by quantum Monte Carlo method. Results for the staggered magnetization and Neel temperature are in agreement with general scaling arguments. The value of triplet DeltaS(z) =1 gp in the spectrum of excitations is estimated. The transverse staggered field was found to induce an additional maximum in the correlation radius of the four spin correlation function around T/J(1) approximate to [0.05 divided by 0.075), J(2)/J(1) 0.03.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : PETRAKOVSKII G. A., APLESNIN S. S., PETROV S. V., FEDOSEEVA N. V.
Заглавие : MAGNETIC-BEHAVIOR OF QUASIONE-DIMENSIONAL CSMNBR3 WITH TRIANGULAR SPIN-LATTICE
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1993. - Vol. 35, Is. 4. - P965-973. - ISSN 0367-3294
Примечания : Cited References: 13
Предметные рубрики: ANTIFERROMAGNET
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : New magnetic structural types in a stochastic easy-plane hexagonal-lattice antiferromagnet
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz. - 1991. - Vol. 100, Is. 6. - P.2068-2073. - ISSN 0044-4510
Примечания : Cited References: 8
Аннотация: By means of the numerical simulation new magnetic states, such as a domain structure antiferromagnet having the periodic and nonperiodic solutions in the spin transverse components and two spin-glass states in the chiral and spin order parameters, are found in a stochastic antiferromagnet with the competing couplings and easy-plane anisotropy. Two temperature transitions caused by the chiral and spin symmetry breaking and the magnetic field regions with the induced long-range chiral order are calculated.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ovchinnikov S. G.
Заглавие : Quasiparticles in strongly correlated electronic systems in cuprate oxides
Место публикации : Uspekhi Fiz. Nauk: MEZHDUNARODNAYA KNIGA, 1997. - Vol. 167, Is. 10. - P.1043-1068. - ISSN 0042-1294
Примечания : Cited References: 227
Предметные рубрики: T-J-MODEL
HIGH-TEMPERATURE SUPERCONDUCTORS
DIMENSIONAL HUBBARD-MODEL
QUASI-PARTICLE DISPERSION
HEISENBERG-ANTIFERROMAGNET SR2CUO2CL2
ANGLE-RESOLVED PHOTOEMISSION
CHARGE FLUCTUATION REGIME
SADDLE-POINT SINGULARITY
SINGLET-TRIPLET MODEL
LA-SR-CU
Аннотация: New experimental and theoretical results on the electronic structure and spectral properties of quasiparticles in cuprate oxides are reviewed. It is shown that the electronic structure transforms from antiferromagnetic insulators to optimally doped high-temperature superconductors as the doping level is varied. The experimental methods considered are primarily angular resolved photoelectron spectroscopy (ARPES), neutron scattering, and NMR. Two types of electronic structure calculations for data interpretation purposes are considered, namely, exact numerical methods for finite clusters (exact diagonalisation and the quantum Monte Carlo method) and approximate schemes for the infinite lattice. As a result, a coherent unified picture emerges, in which the magnetic polaron of a weakly doped antiferromagnetic lattice transforms into a system of Fermi particles dressed by short-range antiferromagnetic type spin fluctuations. In the region of weakly doped metal compositions, deviations from Fermi-liquid properties are seen, such as the failure of Luttinger's theorem, shadowy photoemission bands, and the spin pseudogap effect in spectral and thermodynamic measurements. The situation in the neighbourhood of the insulator-metal concentration transition is described as least understood.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Quantum spin liquid in the frustrated anisotropic Heisenberg antiferromagnet on a square lattice
Место публикации : Phys. Low-Dimens. Struct.: V S V CO. LTD, 1997. - Vol. 10. - P95-102. - ISSN 0204-3467
Примечания : Cited References: 13
Аннотация: Finite-temperature properties of the frustrated S = 1/2 Heisenberg model with the next-nearest-neighbor exchange (J(2) 0) and anisotropic exchange (Delta
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Troyanchuk I. O., Bushinsky M. V., Tereshko N. V., Lanovsky R. A., Sikolenko V. V., Ritter C., Orlov Yu. S., Ovchinnikov S. G.
Заглавие : Ferromagnet-antiferromagnet transition in layered perovskites of Sr3YCo4O10.5 type
Коллективы : Belarussian Foundation for Basic Research [F18R-159]; Russian Foundation Basic Research [18-52-00017 Bel_a, 16-02-00507, 18-52-00020]; Council on grants of the President of the Russian Federation [SP-1844.2016.1]
Место публикации : Mater. Res. Express. - 2019. - Vol. 6, Is. 2. - Ст.026105. - ISSN 2053-1591, DOI 10.1088/2053-1591/aaef21
Примечания : Cited References: 30. - This work was supported by the Belarussian Foundation for Basic Research (project F18R-159) and Russian Foundation Basic Research (contract no. 18-52-00020). Yu S Orlov and SG Ovchinnikov are grateful Russian Foundation Basic Research (contracts no. 18-52-00017 Bel_a, 16-02-00507) and Council on grants of the President of the Russian Federation (SP-1844.2016.1) for the support.
Предметные рубрики: SPIN
NANOWIRES
Ключевые слова (''Своб.индексиров.''): neutron diffraction--orbital ordering--spin state
Аннотация: Sr1−xYxCoO2.65 (x = 0.2) with layered perovskite structure was studied by neutron diffraction, synchrotron x-ray and magnetometry methods. It is shown that in the 90–375 K temperature range the crystal structure can be described by the monoclinic space group A2/m with the superstructure 4√2a p × 2√2a p × 4a p (with a p corresponding to the unit cell parameter of the primitive cell) while basic diffraction peaks are well indexed in the space group I4/mmm (2a p × 2a p × 4a p ) shows an almost standard magnetization. The basic magnetic structure is G-type antiferromagnetic with average magnetic moments of 2.7 μ B/Co and 1.7 μ B/Co in anion-deficient CoO4+γ and stoichiometric CoO6 layers, respectively. A ferromagnetic component of about 0.27 μ B/Co is determined from the magnetization measurements at 8 K. Sr0.8Y0.2CoO2.65 shows an almost standard magnetization versus temperature dependence whereas Sr0.75Y0.25CoO2.65 exhibits an antiferromagnet-ferromagnet transition accompanied by a structural transformation. There is practically no spontaneous magnetization in x = 0.3. The type of the magnetic structure and the high value of TN suggest that the Co3+ ions are in both structural layers predominantly in the low-spin (LS)/high-spin (HS) state mixture. It is proposed that the ferromagnetic component is due to the orbital ordering occurring at TN in the CoO5 pyramids and the concomitant appearance of ferromagnetic coupling between the Co3+(HS) ions located in these CoO5 pyramids in the anion-deficient CoO4+γ layer.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Rasch J.C.E., Boehm M., Ritter C., Mutka H., Schefer J., Keller L., Abramova G. M., Cervellino A., Leoffler J.F.
Заглавие : Magnetoelastic coupling in triangular lattice antiferromagnet CuCrS2
Место публикации : arXiv. - 2009. - Ст.cond-mat/0907.4850. - С. 1-6
Примечания : Библиогр.: 30
Аннотация: CuCrS2 is a triangular lattice Heisenberg antiferromagnet with a rhombohedral crystal structure. We report on neutron and synchrotron powder diffraction results which reveal a monoclinic lattice distortion at the magnetic transition and verify a magnetoelastic coupling. CuCrS2 is therefore an interesting material to study the influence of magnetism on the relief of geometrical frustration.
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