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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Гребенькова, Юлия Эрнестовна, Соколов, Алексей Эдуардович, Еремин, Евгений Владимирович, Эдельман, Ирина Самсоновна, Марущенко, Дмитрий Анатольевич, Зайковский В. И., Чичков В. И., Андреев Н. В., Муковский Я. М.
Заглавие : Намагниченность и магнитный круговой дихроизм поликристаллических пленок La0.7Sr0.3MnO3/YSZ
Место публикации : Физ. тверд. тела. - 2013. - Т. 55, Вып. 4. - С. 771-778
Примечания : Работа поддержана грантами РФФИ № 11-02-00972 и 12-02-92607
Аннотация: Исследованы магнитные и магнитооптические свойства, а также морфология поверхности и структура поликристаллических пленок La0.7Sr0.3MnO3 различной толщины. Показано, что поверхность пленок шероховатая с характерным линейным размером в плоскости ∼ 30 nm, кристаллиты c линейными размерами 10−20 nm случайно ориентированы в плоскости. Температурные и полевые зависимости намагниченности пленок свидетельствуют об их магнитной неоднородности. В спектрах магнитного кругового дихроизма наблюдается ряд полос, одна из которых при 2.4 eV объясняется вкладом электронов проводимости.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Соколов, Алексей Эдуардович, Овчинников, Сергей Геннадьевич, Заблуда, Владимир Николаевич, Кальсин А. М., Зубавичус Я. В.
Заглавие : Магнитный круговой дихроизм и природа ферромагнетизма в коллоидных наночастицах золота
Место публикации : Письма в Журн. эксперим. и теор. физ. - 2013. - Т. 97, Вып. 2. - С. 104-107. - DOI 10.7868/S0370274X13020070
Аннотация: Измерены спектры оптического поглощения и магнитного кругового дихроизма (МКД) в интервале длин волн 350-1150 нм для серии коллоидных растворов наночастиц Au со средним размером 6.0 нм с различной степенью хиральности тиолятного покрытия. Вид спектров поглощения и МКД свидетельствует о дипольном характере межзонных переходов 5d-6(sp)-орбиталей. Отсутствие зависимости (в пределах погрешности эксперимента) МКД от вида покрытия позволяет исключить гипотезу об орбитальной природе магнетизма. Делается вывод о преобладающей роли спиновой поляризации в формировании магнетизма наночастиц золота с тиолятным покрытием.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Соколов, Валерий Владимирович, Малаховский, Александр Валентинович, Гудим, Ирина Анатольевна
Заглавие : Магнитный круговой дихроизм и поглощение кристалла HoAl3(BO3)4 в области f-f перехода 5I8 → 5S2
Коллективы : "Новое в магнетизме и магнитных материалах", международная конференция, Научный совет по физике конденсированных сред РАН, МИРЭА - Российский технологический университет, Московский государственный университет им. М.В. Ломоносова, Магнитное общество России
Место публикации : Новое в магнетизме и магнитных материалах: сборник трудов XXIV международной конференции/ прогр. ком.: Р. С. Исхаков, С. Г. Овчинников [и др.]. - 2021. - Секция 12: Магнитооптика и фотомагнетизм. - Ст.12-60-63
Примечания : Библиогр.: 3
Аннотация: Работа посвящена изучению спектров поглощения и магнитного кругового дихроизма (МКД) кристалла HoAl3(BO3)4. С помощью спектров МКД определены Зеемановские расщепления линий поглощения. Зеемановские расщепления также вычислены теоретически в приближении волновых функций свободного иона.This work is devoted to the study of the absorption and magnetic circular dichroism (MCD) spectra of the HoAl3(BO3)4 crystal. The Zeeman splitting of the absorption lines was determined using the MCD spectra. Zeeman splittings were also calculated theoretically in the approximation of the wave functions of free ion.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Малаховский, Александр Валентинович, Гудим, Ирина Анатольевна, Качур И. С., Пирятинская В. Г.
Заглавие : Аномалии поведения магнитного линейного дихроизма и магнитоэлектрическое взаимодействие в HoFe3(BO3)4
Коллективы : "Новое в магнетизме и магнитных материалах", международная конференция, Научный совет по физике конденсированных сред РАН, МИРЭА - Российский технологический университет, Московский государственный университет им. М.В. Ломоносова, Магнитное общество России
Место публикации : Новое в магнетизме и магнитных материалах: сборник трудов XXIV международной конференции/ прогр. ком.: Р. С. Исхаков, С. Г. Овчинников [и др.]. - 2021. - Секция 13: Магнитоэлектрические явления. - Ст.13-30
Примечания : Библиогр.: 3
Аннотация: Исследован магнитный линейный дихроизм (МЛД) перехода 5I8→5F3 в базисной плоскости монокристалла HoFe3(BO3)4 при распространении света вдоль тригональной оси с при температуре 2K в функции от магнитного поля 0-65 кЭ, направленного вдоль с-оси. МЛД – чётная функция магнитных моментов. Однако было обнаружено, что дихроизм между поляризациями вдоль a и b осей в магнитном поле, параллельном тригональной оси c, не только существует в лёгкоосном состоянии кристалла, но и меняет знак при смене знака поля. Таким образом, магнитное поле H||c нарушает аксиальную симметрию магнитной структуры гольмия в изученных возбуждённых состояниях. Мы доказали существование спонтанной электрической поляризации в HoFe3(BO3)4 при 2 K и рассмотрели магнитоэлектрическое взаимодействие, как один из источников нарушения аксиальной симметрии и других особенностей локальных магнитных свойств гольмия.We studied spectra of magnetic linear dichroism (MLD) of 5I8→ 5F3 transition in the basal plane of the HoFe3(BO3)4 single crystal in the light propagated along the trigonal c axis at temperature 2 K as a function of magnetic field 0 – 65 kOe directed along c axis. MLD is an even function of magnetic moments. However it was found, that dichroism between polarizations along a and b axis in the magnetic field parallel to the trigonal c axis not only exists in the easy axis state of the crystal, but it changes sign with the changing of the field sign. Thus, magnetic field H||c violates the axial symmetry of the Ho magnetic structure in the studied excited states. We proved existence of a spontaneous electric polarization in HoFe3(BO3)4 at 2 K and considered magneto-electric interaction as one of the sources of violation of the axial symmetry and of other features of the local holmium magnetic properties.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yakushkin S. S., Balaev D. A., Dubrovskiy A. A., Semenov S. V., Knyazev Yu. V., Bayukov O. A., Kirillov V. L., Ivantsov R. D., Edelman I. S., Martyanov O. N.
Заглавие : ε-Fe2O3 nanoparticles embedded in silica xerogel – Magnetic metamaterial
Место публикации : Ceram. Int. - 2018. - Vol. 44, Is. 15. - P.17852-17857. - ISSN 02728842 (ISSN), DOI 10.1016/j.ceramint.2018.06.254
Примечания : Cited References: 31. - This work was supported by the Russian Science Foundation, project no. 17-12-01111.
Ключевые слова (''Своб.индексиров.''): ε-fe2o3 iron oxide nanoparticles--metamaterial--mossbauer spectroscopy--magnetic properties--magnetic circular dichroism
Аннотация: A novel method for synthesizing a new metamaterial based on ε-Fe2O3 nanoparticles immobilized in the xerogel matrix was proposed. Samples with different contents of ε-Fe2O3 nanoparticles dispersed in silica xerogel were synthesized by impregnation of as prepared hydrogel with iron (II) salts with the subsequent calcination. The structure and magnetic properties of the prepared composites were studied by transmission electron microscopy, X-ray diffraction, Mössbauer spectroscopy, and static magnetic measurements. The absence of other iron oxide polymorphs, controllable particle size distribution, and high ε-Fe2O3 nanoparticle concentration in combination with the weak interparticle magnetic interactions ensured the preservation of the unique magnetic properties of individual ε-Fe2O3 nanoparticles and allowed us to obtain a novel metamaterial. The high optical transparency and homogeneity of the prepared composites made it possible to detect the magnetic circular dichroism (MCD) of the magnetic silica xerogel, which is typical of the ε-Fe2O3-based systems.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Samardak, Alexander S., Ognev, Alexey, V, Kolesnikov, Alexander G., Stebliy, Maksim E., Samardak, Vadim Yu, Iliushin, Ilia G., Pervishko, Anastasiia A., Yudin, Dmitry, Platunov M. S., Ono, Teruo, Wilhelm, Fabrice, Rogalev, Andrey
Заглавие : XMCD and ab initio study of interface-engineered ultrathin Ru/Co/W/Ru films with perpendicular magnetic anisotropy and strong Dzyaloshinskii-Moriya interaction
Коллективы : Russian Ministry of Science and Higher Education [075-15-2021-607, 0657-2020-0013]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [19-32-60020]; Russian Federation President Scholarship for Young Scientists [SP-1640.2021.5]; Russian Science FoundationRussian Science Foundation (RSF) [21-42-00041]; Russian Ministry of Science and Higher Education
Место публикации : Phys. Chem. Chem. Phys. - 2022. - Vol. 24, Is. 14. - P.8225-8232. - ISSN 1463-9076, DOI 10.1039/d1cp05456b. - ISSN 1463-9084(eISSN)
Примечания : Cited References: 47. - A. V. O., I. G. I. and T. O. thank the Russian Ministry of Science and Higher Education for state support of scientific research conducted under the supervision of leading scientists in Russian institutions of higher education, scientific foundations and state research centers (Project No. 075-15-2021-607) in parts of sample preparation and its magnetic characterization. The micromagnetic simulations performed by M. E. S. were supported by the Russian Ministry of Science and Higher Education under the state task (0657-2020-0013). A. A. P. (ab initio calculations) acknowledges the support from the Russian Foundation for Basic Research (Project No. 19-32-60020) and the Russian Federation President Scholarship for Young Scientists (SP-1640.2021.5). The work of A. S. S. related to the experimental and analytical study of DMI and skyrmion bubbles was supported by the Russian Science Foundation (Project No. 21-42-00041). The authors acknowledge the use of computational resources of the Skoltech supercomputer Zhores47 to obtain the theoretical results presented in this paper. The authors thank ID12 beamline staff for their help during the XMCD experiment and gratefully acknowledge the provision of beamtime (Proposal MA-3661) by the ESRF. The research contribution of M. P. (XMCD anaysis) was partially funded by the Russian Ministry of Science and Higher Education via the budget project of SRF SKIF, Boreskov Institute of Catalysis
Предметные рубрики: TOTAL-ENERGY CALCULATIONS
CIRCULAR-DICHROISM
MOLECULAR-DYNAMICS
Аннотация: Understanding the nature of recently discovered spin–orbital induced phenomena and a definition of a general approach for “ferromagnet/heavy-metal” layered systems to enhance and manipulate spin–orbit coupling, spin–orbit torque, and the Dzyaloshinskii–Moriya interaction (DMI) assisted by atomic-scale interface engineering are essential for developing spintronics and spin-orbitronics. Here, we exploit X-ray magnetic circular dichroism (XMCD) spectroscopy at the L2,3-edges of 5d and 4d non-magnetic heavy metals (W and Ru, respectively) in ultrathin Ru/Co/W/Ru films to determine their induced magnetic moments due to the proximity to the ferromagnetic layer of Co. The deduced orbital and spin magnetic moments agree well with the theoretically predicted values, highlighting the drastic effect of constituting layers on the system's magnetic properties and the strong interfacial DMI in Ru/Co/W/Ru films. As a result, we demonstrate the ability to simultaneously control the strength of magnetic anisotropy and intermixing-enhanced DMI through the interface engineered inversion asymmetry in thin-film chiral ferromagnets, which are a potential host for stable magnetic skyrmions.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Platunov M. S., Gudim I. A., Ovchinnikova, Elena N., Kozlovskaya, Ksenia A., Wilhelm, Fabrice, Rogalev, Andrei, Hen, Amir, Ivanov, Vsevolod Y., Mukhin, Alexander A., Dmitrienko, Vladimir E.
Заглавие : X-ray Natural Circular Dichroism imaging of multiferroic crystals
Коллективы : Russian Science FoundationRussian Science Foundation (RSF) [19-72-00002, 16-12-10531]; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [19-52-12029, 19-02-00483]; Ministry of Science and Higher Education of the Russian Federation within the State assignment FSRC "Crystallography and Photonics" RAS
Место публикации : Crystals. - 2021. - Vol. 11, Is. 5. - Ст.531. - ISSN 2073-4352, DOI 10.3390/cryst11050531
Примечания : Cited References: 70. - This research was funded by the Russian Science Foundation (grant 19-72-00002). K.A.K. acknowledges support from the Russian Foundation for Basic Research (project no. 19-52-12029 and project no. 19-02-00483). V.E.D. was partly supported by the Ministry of Science and Higher Education of the Russian Federation within the State assignment FSRC "Crystallography and Photonics" RAS. V.Y.I. and A.A.M. were supported by the Russian Science Foundation [grant 16-12-10531]
Предметные рубрики: OPTICAL-ACTIVITY
MAGNETOELASTIC PROPERTIES
SINGLE-CRYSTAL
Аннотация: The polarizing spectroscopy techniques in visible range optics have been used since the beginning of the 20th century to study the anisotropy of crystals based on birefringence and optical activity phenomena. On the other hand, the phenomenon of X-ray optical activity has been demonstrated only relatively recently. It is a selective probe for the element-specific properties of individual atoms in non-centrosymmetric materials. We report the X-ray Natural Circular Dichroism (XNCD) imaging technique which enables spatially resolved mapping of X-ray optical activity in non-centrosymmetric materials. As an example, we present the results of combining micro-focusing X-ray optics with circularly polarized hard X-rays to make a map of enantiomorphous twinning in a multiferroic SmFe3(BO3)4 crystal. Our results demonstrate the utility and potential of polarization-contrast imaging with XNCD as a sensitive technique for multiferroic crystals where the local enantiomorphous properties are especially important. In perspective, this brings a novel high-performance method for the characterization of structural changes associated with phase transitions and identification of the size and spatial distribution of twin domains.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Rogalev A., Samoshkina Yu. E., Edelman I. S., Sokolov A. E., Ollefs K., Andreev N., Chichkov V. I.
Заглавие : X-ray and visible magnetic circular dichroism spectroscopy of Pr1-xSrxMnO3 thin films: comparative study
Коллективы : International Conference on Magnetism
Место публикации : 20th Int. Conf. on Magnetism (ICM-2015): book of abstracts. - 2015. - Ст.TU.E-P12
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Edelman I. S., Greben'kova Yu. E., Sokolov A. E., Molokeev M. S., Aleksandrovsky A. S., Chichkov V. I., Andreev N. V., Mukovskii Y.
Заглавие : Visible magnetic circular dichroism spectroscopy of the Pr0.8Sr0.2MnO3 and Pr0.6Sr0.4MnO3 thin films
Место публикации : AIP Adv.: American Institute of Physics, 2014. - Vol. 4, Is. 5. - Ст.057125. - ISSN 2158-3226, DOI 10.1063/1.4879818
Примечания : Cited References: 30. - The work was supported partly by the Russian Foundation for Basic Researches, grant No’s 14-02-01211, 12-02-00717-a and Grant of the Russian President No Sh-2886.2014.2
Предметные рубрики: MANGANITES
LA1-XSRXMNO3
PEROVSKITES
SPECTRA
Аннотация: Visiblemagnetic circular dichroism (MCD) in Pr1-xSrxMnO3 with x=0.2 and 0.4was investigated for the first time. Samples for the investigation – polycrystalline films with thickness from 20 to 150 nm were prepared with the dc magnetron sputtering. MCD spectra obtained in the energy interval 1–4 eV at temperatures 100–300 K consist of several maxima with different intensities: very strong one near 3.25–3.4 eV and a broad essentially weaker band near 2 eV. An additional maximum of opposite sign arises in the samples with x = 0.4MCD spectrum at 2.33 eV. Experimental spectra were decomposed to several Gaussian components, and their amplitudes temperature dependences were analyzed. In the case of x = 0.2, all four Gaussian components are characterized by the identical temperature dependence of their amplitudes. In the case of x = 0.4, maxima observed in different spectral intervals demonstrate different temperature dependences of their amplitudes. One more unexpected phenomenon is associated with the different MCD value change in different spectral intervals when coming from x = 0.2 to x = 0.4: high-energy maximum increases more than twice while low-energy maxima intensity stays at that, practically, unchanged.
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10.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Zabluda V.N, Sokolov A.E, Ovchinnikov S.G., Zubavichus Ya.V, Kalsin A.M.
Заглавие : Visible magnetic circular dichroism in gold nanoparticles
Коллективы : International Conference Functional Materials
Место публикации : International Conference Functional Materials (ICFM-2011): Book of abstracts : [3-8 Oct. 2011, Crimea, Ukraine]. - 2011. - С. 187
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11.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Samoshkina Yu. E., Edelman I. S., Sokolov A. E., Andreev N. V., Chichkov V. I.
Заглавие : Visible circular and linear magnetic dichroism in manganite thin films
Место публикации : Circular and Linear Dichroism/ ed. J. Wallace. - New York: Nova Science Publishers, 2015. - P.131-158. - (Lasers and electro-optics research and technology). - ISBN 978-1-63483-762-0
Примечания : Cited References: 45. - The work was supported partly by RFBR, grant № 14-02-01211 and Grant of President of Russian Federation No. NSh-2886.2014.2
Аннотация: Evolution of the magneto-optical spectra of the La0.7Sr0.3MnO3, Pr0.6Sr0.4MnO3 and Pr0.8Sr0.2MnO3 manganite films with the change in the Sr concentration has been studied in the visible and near infrared range. Magnetic circular dichroism (MCD) and magnetic linear dichroism (MLD) have been chosen for investigation as these effects are higher informative comparing to the Faraday and Kerr effects. The Sr concentration increase in the samples leads to a sequential shift of the gravity centers of the magneto-optical bands to lower energies, to a strong increase of the effects magnitude in the range of 2.5-3.6 eV, and to the appearance of the additional bands in the spectra of the films with metallic conductivity. Experimental spectra have been decomposed to several Gaussian and Lorentz contours, and their intensity temperature dependences have been analyzed. For the films with metallic conductivity, the different character of the temperature dependences of the different bands intensity has been found. Basing on the characteristic dependence of the magneto-optical bands intensity on temperature, Sr concentration, and films conductivity type, electron transitions responsible for the MCD and MLD spectra formation have been identified.
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12.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Ovchinnikov S. G., Platunov M. S., Kazak, N. V., Knyazev Yu. V., Bezmaternykh L. N., Rogalev A., Wilhelm F., Weschke E., Schierle E., Zubavichus Y. V.
Заглавие : Valence-specific magnetization of the ferrimagnetic oxyborate single crystals using soft and hard X-ray mag-netic circular dichroism under high magnetic fields
Коллективы : International Conference on Magnetism
Место публикации : 20th Int. Conf. on Magnetism (ICM-2015): book of abstracts. - 2015. - Ст.TU.H-P31
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pomogaev V., Avramov P. V., Kachin S., Pomogaeva A., Jalkanen K. J.
Заглавие : Thermo-dynamical contours of electronic-vibrational spectra simulated using the statistical quantum-mechanical methods
Место публикации : Theor. Chem. Acc. - NEW YORK: SPRINGER, 2011. - Vol. 130, is. 4-6. - С. 609-632. - DEC. - ISSN 1432-881X, DOI 10.1007/s00214-011-0936-6
Примечания : Cited Reference Count: 112. - Гранты: We would like to acknowledge scientific discussions with the following collaborators and friends: Daniel Chipman, Victor Ya. Artyukhov for common discussions concerning theoretical questions and methodology; John S. Tse and Dennis D. Klug for initial discussions concerning the properties of cyanoanthracene; and Yuriko Aoki for discussions of benzene and estradiol. We would also like to thank the following funding agencies and institutions for supporting this work during its various stages of development: Kyushu University, Japan; Steacie Institute for Molecular Sciences, Canada; University of Notre Dame, USA; Siberian Physical-Technical Institute, Russia; Siberian Federal University, Russia; Kirensky Institute of Physics, Russia. We would like to thank FAPESP for project 16782-2/2009 which allowed Prof. Jalkanen to visit LEVB at UniVaP for the period from June 2010 to May 2011 from the Quantum Protein (QuP) Center at the Technical University in Denmark during which time this work was completed.Финансирующая организация: Kyushu University, Japan; Steacie Institute for Molecular Sciences, Canada; University of Notre Dame, USA; Siberian Physical-Technical Institute, Russia; Siberian Federal University, Russia; Kirensky Institute of Physics, Russia
Предметные рубрики: DENSITY-FUNCTIONAL THEORY
INITIO MOLECULAR-DYNAMICS
CIRCULAR-DICHROISM SPECTRA
LASER-INDUCED FLUORESCENCE
NUCLEAR SHIELDING TENSORS
ALANINE N'-METHYLAMIDE
ALKALINE-EARTH DIMERS
ABSORPTION-SPECTRA
HYDRATED ELECTRON
AQUEOUS-SOLUTION
Ключевые слова (''Своб.индексиров.''): organic compounds--molecular dynamics--photophysical properties--electronic spectra--electronic spectra--molecular dynamics--organic compounds--photophysical properties
Аннотация: Three polycyclic organic molecules in various solvents focused on thermo-dynamical aspects were theoretically investigated using the recently developed statistical quantum mechanical/classical molecular dynamics method for simulating electronic-vibrational spectra. The absorption bands of estradiol, benzene, and cyanoanthracene have been simulated, and most notably, the increase in the spectral intensity for the lowest excited state transition as the temperature is increased observed experimentally is well reproduced. In addition, this method has been extended to treat luminescent processes also, and it is seen that the experimental emission spectrum of cyanoanthracene is also well described. The method still needs further refinement, but results to date, including those presented in this work, document clearly that our model is one which is able to treat the many complex effects that the environment have on electronic absorption and emission spectra.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Malakhovskii A. V., Morozova T. P.
Заглавие : Temperature dependence of the fine structure of the C and E absorption bands in RbMnF3 below the Neel temperature
Разночтения заглавия :авие SCOPUS: Temperature dependence of the fine structure of the C and E absorption bands in RbMnF3 below the neel temperature
Место публикации : Phys. Solid State: SPRINGER, 2006. - Vol. 48, Is. 2. - P283-290. - ISSN 1063-7834, DOI 10.1134/S1063783406020156
Примечания : Cited References: 24
Предметные рубрики: PEROVSKITE FLUORIDES
VIBRONIC SPECTRA
CRYSTALS
MNF2
INTENSITY
DICHROISM
STATES
Аннотация: The variation in the parameters (width, position, intensity) of the fine structure lines in the C[(6)A(1g) - (4)A(1g), E-4(g)((4)G)] and E[(6)A(1g) - E-4(g)(D-4)] bands in RbMnF3 with temperature is studied in the temperature range 10-70 K. In the C band, two narrow ( 6 cm(-1)) lines are are distinguished at distances of 77 and 80 cm(-1) from the exciton line at T
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15.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Sukhachev A. L., Malakhovskii A. V., Sokolov V. V., Zabluda V. N., Gudim I. A.
Заглавие : Temperature dependence of magnetic circular dichroism in DyFe3(BO3)4 and ErFe3(BO3)4 crystals : Abstract
Коллективы : "Functional Materials", International Conference , Taurida National V. I. Vernadsky University
Место публикации : Functional materials: Abstracts/ ed. V. N. Berzhansky. - Simferopol, 2013. - Ст.DQ1-4P/19. - P.207. - ISBN 978-966-491-465-6
Аннотация: Изучены спектры поглощения и магнитного кругового дихроизма и магнитооптическая активность f-f переходов в кристаллах DyFe3(BO3)4, ErFe3(BO3)4 и ErAl3(BO3)4 в функции от температуры. Проведено сравнение экспериментальных результатов с теорией. Обнаружено, что одни и те же переходы в изоструктурных кристаллах ErFe3(BO3)4 и ErAl3(BO3)4 имеют существенно разную магнитооптическую активность вплоть до различия в знаке. Это явление может быть объяснено предложенной авторами ранее теорией.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrov D. A., Ivantsov R. D., Zharkov S. M., Lin C.-R., Shu F.-R., Tseng Y.-T.
Заглавие : Synthesis, morphology, and visible magnetic circular dichroism of Ni-C nanoparticles
Место публикации : J. Sib. Fed. Univ. Math. Phys. - 2016. - Vol. 9, Is. 4. - P.481-484. - ISSN 1997-1397, DOI 10.17516/1997-1397-2016-9-4-481-484; Журн. СФУ. Сер. "Математика и физика"
Примечания : Библиогр.: 2. - This work was supported by the RFBR grant 14-02-01211 and MOST 102-2112-M-153-002-MY3.
Ключевые слова (''Своб.индексиров.''): mcd--nanoparticles--ni-c--tem--наночастицы--мкд--электронная микроскопия
Аннотация: Ni-C nanoparticles powder (NP) was synthesized using high-temperature pyrolysis of nickel nitrate in an organic solvent. The NP was characterized by transmission electron microscopy (TEM), energy dispersive x-ray spectroscopy (EDXS) and selected-area electron diffraction (SAED). Structural characterization of the samples confirmed the formation of small, medium and large Ni nanoparticles with face-centered cubic structure (fcc) and enlarged lattice parameter. Magnetic circular dichroism (MCD) of samples with different mean particle sizes showed a red shift with decrease of mean particle size. © Siberian Federal University. All rights reserved.Порошок наночастиц Ni-C был синтезирован с помощью высокотемпературного пиролиза нитрата никеля в органическом растворителе. Наночастицы были исследованы с помощью просвечивающей электронной микроскопии, энергодисперсионной рентгеновской спектроскопии и дифракции электронов выбранной зоны. Структурная характеризация образцов подтвердила образование маленьких, средних и больших наночастиц никеля с гранецентрированной кубической структурой и увеличенным параметром решётки. Магнитный круговой дихроизм образцов с различными средними размерами частиц показал красное смещение при уменьшении среднего размера частиц.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ivantsov R. D., Evsevskaya N., Saikova S., Linok E., Yurkin G. Yu., Edelman I. S.
Заглавие : Synthesis and characterization of Dy3Fe5O12 nanoparticles fabricated with the anion resin exchange precipitation method
Место публикации : Mater. Sci. Eng. B: Elsevier, 2017. - Vol. 226. - P.171-176. - ISSN 09215107 (ISSN), DOI 10.1016/j.mseb.2017.09.016
Примечания : Cited References: 49. - The work was supported partly by the Grant of the President of the Russian Federation – Russia no. NSh-7559.2016.2, and by the Russian Foundation for Basic Research – Russia (RFBR): grant. No. 16-33-00043.
Ключевые слова (''Своб.индексиров.''): dy3fe5o12 nanoparticles--anion resin exchange precipitation method--magnetic circular dichroism
Аннотация: Dysprosium-iron garnet (DyIG) nanoparticles were synthesized with the new modification of the anion resin exchange precipitation method. Fourier transform infrared spectroscopy, X-ray diffraction, and transmission electron microscopy showed nanoparticles to be of the garnet structure with an excellent crystallinity. Magnetic properties were studied by using QUANTUM Design MPMS-XL system and the visible magnetic circular dichroism (MCD). Nanoparticles magnetic properties were close to those of bulk DyIG crystals. Dependence of the nanoparticles magnetization (M) on the external magnetic field (H) is described by a narrow hysteresis loop in relatively low fields and the strong linear M increase with the further H increase. The visible MCD of DyIG was studied in this work for the first time. The MCD spectra consisted of several peaks associated with electron transitions in iron and dysprosium ions located in different spectral intervals. Dependences of the MCD peak intensities on temperature and magnetic field were studied.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Saykova, Diana, Saikova, Svetlana, Mikhlin, Yuri, Panteleeva, Marina, Ivantsov R. D., Belova E.
Заглавие : Synthesis and characterization of core-shell magnetic nanoparticles NiFe2O4@Au
Место публикации : Metals. - 2020. - Vol. 10, Is. 8. - Ст.1075. - ISSN 2075-4701(eISSN), DOI 10.3390/met10081075
Примечания : Cited References: 45
Предметные рубрики: NICKEL FERRITE NANOPARTICLES
GOLD NANOPARTICLES
OXIDATION
REDUCTION
Аннотация: In this study, NiFe2O4@Au core–shell nanoparticles were prepared by the direct reduction of gold on the magnetic surface using amino acid methionine as a reducer and a stabilizing agent simultaneously. The obtained nanoparticles after three steps of gold deposition had an average size of about 120 nm. The analysis of particles was performed by X-ray diffraction, transmission electron microscopy, X-ray photoelectron spectroscopy, and UV-Vis spectroscopy techniques. The results indicate successful synthesis of core–shell particles with the magnetic core, which consists of a few agglomerated nickel ferrite crystals with an average size 25.2 ± 2.0 nm, and the thick gold shell consists of fused Au0 nanoparticles (NPs). Magnetic properties of the obtained nanoparticles were examined with magnetic circular dichroism. It was shown that the magnetic behavior of NiFe2O4@Au NPs is typical for superparamagnetic NPs and corresponds to that for NiFe2O4 NPs without a gold shell. The results indicate the successful synthesis of core–shell particles with the magnetic nickel ferrite core and thick gold shell, and open the potential for the application of the investigated hybrid nanoparticles in hyperthermia, targeted drug delivery, magnetic resonance imaging, or cell separation. The developed synthesis strategy can be extended to other metal ferrites and iron oxides.
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19.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Petrov D. A.
Заглавие : Study of morphology, magnetic properties, and visible magnetic circular dichroism of Ni nanoparticles synthesized in SiO2 by ion implantation
Коллективы : Russian-French workshop on Nanosciences and Nanotechnologies, Российская академия наук, Сибирское отделение РАН, Институт неорганической химии им. А.В. Николаева Сибирского отделения РАН, Институт катализа им. Г.К. Борескова Сибирского отделения РАН, Институт физики полупроводников им. А.В. Ржанова Сибирского отделения РАН
Место публикации : The 7th Russian-French workshop on Nanosciences and Nanotechnologies: Program and abstract book/ ed. A. V. Okotrub. - Novosibirsk, 2013. - P.67. - ISBN 978-5-901688-29-8
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Edelman I. S., Petrov D. A., Ivantsov R. D., Zharkov S. M., Velikanov D. A., Gumarov G. G., Nuzhdin V. I., Valeev V. F., Stepanov A. L.
Заглавие : Study of morphology, magnetic properties, and visible magnetic circular dichroism of Ni nanoparticles synthesized in SiO2 by ion implantation
Место публикации : Physical Review B - Condensed Matter and Materials Physics. - 2013. - Vol. 87, Is. 11. - Ст.115435. - P. - ISSN 1098-0121, DOI 10.1103/PhysRevB.87.115435
Аннотация: A systematic study of ensembles of nickel nanoparticles fabricated by Ni+-ion implantation at a dose of (0.5-1.0)?1017 ions/cm2 in a thin near-surface layer of an amorphous SiO2 matrix by means of transmission electron microscopy (TEM), dc magnetic measurements, and magneto-optical technique is presented. TEM characterization of Ni nanoparticles proves the formation of isolated spherical nickel nanoparticles with diameters from 2 to 16 nm. The crystal structure and lattice constant of the nanoparticles correspond to face-centered-cubic Ni. The larger size nanoparticles are shown to have core-shell structure, which is unusual for the implantation conditions used. The shell of these nanoparticles consists of Ni, while the core has supposedly the composition coinciding with the matrix, i.e., SiO2. The core-shell nanoparticles in the investigated sample coexist with ordinary pure Ni nanoparticles, which strongly affects the magnetic and especially magneto-optic properties of the samples. For all three doses, the nanoparticles are in the superparamagnetic state at room temperature passing to the "frozen" state at lower temperatures. However, only the sample implanted with the lowest dose demonstrates the classic superparamagnetic behavior according to the shape of the experimental magnetization temperature dependencies for the zero-field-cooled (ZFC) and field-cooled regimes. This shape deviation from that characteristic of the pure superparamagnetic ensembles is ascribed mainly to the particle core-shell structure. The Ni nanoparticles' anisotropy constant estimated with the help of ZFC curves appears to exceed the bulk Ni anisotropy second constant approximately by two orders of magnitude. Magnetic circular dichroism (MCD) is characterized by spectral dependence modified strongly as compared to the MCD spectra of a continuous Ni film. In the spectral range 1.1-4.2 eV, the MCD spectrum consists of two broad maxima of opposite sign with the characteristics depending on the implantation dose and the measurement temperature. The MCD spectra analysis allows one to show that the higher-energy maximum (at 3.34-3.48 eV depending on the dose) is related to the surface plasmon resonance (SPR) excitation in pure Ni nanoparticles, while the lower-energy maximum (at 2.19-2.73 eV depending on the dose) should be associated with the SPR excitation in core-shell nanoparticles. В© 2013 American Physical Society.
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