Библиотека института физики им. Л.В. Киренского СО РАН

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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zou X., Wang X., Zhang H., Kang Y., Yang X., Zhang X., Molokeev M. S., Lei B.
Заглавие : A highly efficient and suitable spectral profile Cr3+-doped garnet near-infrared emitting phosphor for regulating photomorphogenesis of plants
Место публикации : Chem. Eng. J. - 2022. - Vol. 428. - Ст.132003. - ISSN 13858947 (ISSN), DOI 10.1016/j.cej.2021.132003
Примечания : Cited References: 46. - The work was supported from the National Natural Science Foundations of China (Nos. 21671070, 51802101), the Guangdong Basic and Applied Basic Research Foundation (No. 2021A1515012613), the Guangdong Provincial Science & Technology Project (Nos. 2020A1414010046, 2021A0505050006), the Guangzhou Science & Technology Project (No. 202007020005), the Natural Science Foundation of Guangdong Province (No. 2018A030310217), the Project of GDUPS (2018) for Prof. Bingfu LEI, and the Guangdong Provincial Special Fund for Modern Agriculture Industry Technology Innovation Teams (Nos. 2021KJ131 , 2021KJ122)
Аннотация: Far-red/phytochrome (PFR) plays a key role in photomorphogenesis of plants. However, how to obtain a near-infrared (NIR) emitting phosphor with high external quantum efficiency (EQE), suitable spectral profile, and low thermal quenching remains a huge challenge. Herein, a NIR phosphor, Gd2.4Lu0.6Ga4AlO12:Cr3+,H3BO3 (GLGA:Cr3+) was developed via regulating the crystal field environment and adding fluxes, which exhibits a peak maximum at 728 nm with a relatively narrow full-width at half maximum (FWHM) of 107 nm, matching well with the absorption band of PFR. Upon 450 nm excitation, the internal quantum efficiency (IQE) and EQE of the optimal phosphor are 90.3% and 32.0%, respectively. At 423 K, the integrated emission intensity of the investigated phosphor is about 75% of that at room temperature. Benefiting from the excellent optical performance, a NIR phosphor-converted light-emitting diode (pc-LED) was fabricated, which shows a NIR output power of 505.99 mW and photoelectric conversion efficiency of 11.24% at 300 mA. Moreover, plant growth experiments demonstrate that the biomass of pea seedlings is increased by 67.72% under supplementary NIR light irradiation. The findings of this research will motivate further research on new Cr3+-doped NIR phosphors for regulating photomorphogenesis of plants.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yelisseyev A., Lobanov S., Molokeev M. S., Zhang S., Pugachev A., Lin Z., Vedenyapin V., Kurus A., Khamoyam A., Isaenko L.
Заглавие : A New Nonlinear Optical Selenide Crystal AgLiGa2Se4 with Good Comprehensive Performance in Mid-Infrared Region
Место публикации : Adv. Opt. Mater. - 2021. - Vol. 9, Is. 5. - Ст.2001856. - ISSN 21951071 (ISSN), DOI 10.1002/adom.202001856
Примечания : Cited References: 32. - Crystal growth and investigation of physical properties were supported by Russian Science Foundation, Russia (#19‐12‐00085). Spectroscopic data were obtained at the Institute of Geology and Mineralogy, Siberian Branch of Russian Academy of Sciences, Russia; Ministry of Science and Higher Education, Russia (performed on a state assignment). The work on first‐principles calculations also supported by National Science Foundation in China (No.51872297) and Fujian Institute of Innovation (FJCXY18010201) in Chinese Academy of Sciences
Аннотация: Mid‐infrared (mid‐IR) nonlinear optical (NLO) crystals are indispensable for the mid‐IR lasers generation with tunable wavelengths from 3 to 20 µm. AgGaSe2 is a commercial mid‐IR NLO crystal with the highest figures of merit, but suffers low laser damage threshold (LDT). To achieve the balance of optical transmission, NLO effect, and LDT, it is proposed to molecularly modify the AgGaSe2 structure by introducing the [LiSe4] tetrahedra, and successfully grow large crystals of a new selenide AgLiGa2Se4. The replacement of half of the heavy Ag+ cations with light Li+ increases the band gap to 2.2 eV (vs. 1.7 eV in AgGaSe2). The LDT value in AgLiGa2Se4 increases five times compared to that in AgGaSe2, while keeping a relatively large NLO susceptibility of 26 pm V−1. Moreover, the thermal expansion coefficients in AgLiGa2Se4 are approximately two times lower in absolute value compared with AgGaSe2, which is beneficial to the large crystal growth. All these advantages would make AgLiGa2Se4 a new promising NLO crystal for mid‐IR laser applications.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Formation of a spin density wave in copper metaborate by a spin polaron
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2004. - Vol. 16, Is. 32. - P5907-5914. - ISSN 0953-8984, DOI 10.1088/0953-8984/16/32/023
Примечания : Cited References: 12
Предметные рубрики: SOLITON LATTICE
CUB2O4
Ключевые слова (''Своб.индексиров.''): absorption--correlation methods--electric fields--infrared radiation--magnetization--mathematical models--polarons--specific heat--intraband transition--optical conductivity--spin density waves--spin polaron--copper compounds
Аннотация: Formation of incommensurate three-dimensional magnetic order below T* similar to 10 K in CuB2O4 is explained on the basis of strong correlation between the holes and localized spins. The Kondo lattice model is analysed for the case where spin polarons are the elementary excitations. The origin of the low-temperature specific heat maximum at T similar to 5 K is associated with a displacement of the polaron band bottom. A set of anomalies in the temperature dependence of the conductivity, shift of the optical conductivity maximum in the range of energies 0.02-0.12 eV and decreasing of the infrared absorption intensity is predicted.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Kharkov A. M., Filipson G. Y.
Заглавие : Magnetic capacitance in variable-valence manganese sulfides
Место публикации : Phys. Status Solidi B. - 2020. - Vol. 257, Is. 5. - Ст.1900637. - ISSN 03701972 (ISSN), DOI 10.1002/pssb.201900637
Примечания : Cited References: 12. - This study was supported by the Russian Foundation for Basic Research No. 18-32-00079 mol_a. The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science No. 18-42-240001 r_a
Аннотация: The permittivity of TmxMn1–xS (0 < x < 0.15) solid solutions is measured in the frequency range of 102–106 Hz at temperatures of 300–500 K in magnetic fields of up to 12 kOe. The migration and relaxation conductivity contributions to the electric polarization are established. The relaxation time and activation energy are calculated using the Debye model. A decrease in the capacitance and relaxation time in a magnetic field is observed. The electron polarization relaxation channel provided by recombination of the electron–hole pairs is found using the infrared spectroscopy investigations.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : AVERYANOV E. M.
Заглавие : MIXING THE MOLECULAR EXCITATIONS IN MONOAXIAL LIQUID-CRYSTALS
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz.: MEZHDUNARODNAYA KNIGA, 1995. - Vol. 108, Is. 1. - P258-280. - ISSN 0044-4510
Примечания : Cited References: 60
Предметные рубрики: LOCAL FIELD
INFRARED DICHROISM
DISPERSIONS
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Udod L. V., Sitnikov M. N., Shestakov N. P.
Заглавие : Bi2(Sn0.95Cr0.05)2O7: Structure, IR spectra, and dielectric properties
Место публикации : Ceram. Int.: Elsevier, 2016. - Vol. 42, Is. 4. - P.5177-5183. - ISSN 02728842 (ISSN), DOI 10.1016/j.ceramint.2015.12.040
Примечания : Cited References: 45. - This work was supported by the Russian Foundation for Basic Research Projects no. 15-42-04099 r_siberia_a, Siberian Branch of Science and NAS of Belarus “Electronic and magnetic phase transitions in materials with magnetoelectric affect” and government work no. 114090470016.
Предметные рубрики: BISMUTH PYROSTANNATE
PYROCHLORE STRUCTURE
MAGNETIC-PROPERTIES
PARTIAL OXIDATION
HIGH-TEMPERATURE
X-RAY
Bi2Sn2O7
SUBSTITUTION
CATALYSTS
DIFFRACTION
Ключевые слова (''Своб.индексиров.''): bismuth pyrostannate--infrared absorption spectra--structural transition--permittivity--debye model
Аннотация: Infrared absorption spectra of the bismuth pyrostannate Bi2(Sn0.95Cr0.05)2O7 were investigated in the frequency range 350-1100 cm-1 at temperatures of 110-525 K. Four frequency regions with split absorption lines are distinguished. Softening of frequencies at the structural transitions was observed. The maxima of permittivity measured in the frequency range 1-200 kHz at temperatures 100-400 K were determined. It was found that the magnetic susceptibility changes its sign in the low-temperature region. The correlation between anomalies in the magnetic susceptibility, permittivity, and absorption line intensity was established. Softening of frequencies is explained by the variation in the coefficient of thermal expansion of the lattice. The temperature behavior of permittivity is described using the Debye model. © 2015 Elsevier Ltd and Techna Group S.r.l.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bikbaev R. G., Vetrov S. Ya., Timofeev I. V.
Заглавие : Transparent conductive oxides for the epsilon-near-zero Tamm plasmon polaritons
Место публикации : J. Opt. Soc. Am. B. - 2019. - Vol. 36, Is. 10. - P.2817-2823. - ISSN 07403224 (ISSN), DOI 10.1364/JOSAB.36.002817
Примечания : Cited References: 44. - The reported study was funded by RFBR according to the research project No 18-32-00053 and financial support RFBR and MOST according to the research project No 19-52-52006.
Аннотация: We demonstrate the possibility of using transparent conducting oxides [aluminum-doped zinc oxide (AZO), gallium-doped zinc oxide (GZO), indium tin oxide (ITO)] to form Tamm plasmon polaritons in the near-infrared spectral range where the permittivity of oxides is near zero. The spectral properties of the structures are investigated in the framework of the temporal coupled-mode theory and confirmed by the transfer matrix method. It is found that in the critical coupling conditions, the maximal Q-factor of a Tamm plasmon polariton is achieved when a photonic crystal is conjugated with the AZO film, while at the conjugation with the ITO films, the broadest spectral line is obtained. The sensitivity of the wavelength and spectral width of the Tamm plasmon polariton to changes in the oxide film thickness, bulk concentration of a dopant, and angle of incidence is demonstrated.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Solovyov L. A., Golovnev N. N., Molokeev M. S., Lesnikov M. K.
Заглавие : Bis(μ3-barbiturato−O,O,O′)-(μ2-aqua)- aqua-barium(II): crystal structure, spectroscopic and thermal properties
Место публикации : J. Coord. Chem.: Taylor & Francis, 2017. - Vol. 70, Is. 12. - P.1984-1993. - ISSN 00958972 (ISSN), DOI 10.1080/00958972.2017.1319943
Примечания : Cited References: 21
Ключевые слова (''Своб.индексиров.''): barbituric acid--barium--coordination compound--x-ray diffraction--infrared spectroscopy--thermal analysis
Аннотация: A polymeric coordination compound, [Ba(H2O) 2(Hba)2] (1) (H2ba – barbituric acid, C4H4N2O3), was obtained. The structure of 1 was solved using powder X-ray diffraction methods. The Ba2+ ion in 1 formed a three-capped trigonal prism. The BaO9 polyhedra, connected with each other by the edges and faces, formed a chain. Several 4- and 12-membered cycles due to the bridging μ2-H2O and bridging μ3-Hba– also formed implementing a 3-D polymer structure. The structures of 1 and other thiobarbiturate complexes were compared. The replacement of a S atom by an O atom in the heterocyclic ligand Htba− (thiobarbiturate ion) of the compound Ba(H2O)2(Htba)2 resulted in changes of the coordination number Ba(II) and supramolecular structure. The intermolecular hydrogen bonds O–H⋯O and N–H⋯O formed a 3-D net where pronounced 2-D layers of Hba– ions could be found. A new topological net in 1 was observed. The IR and thermal stability were investigated.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bulgakov E. N., Sadreev A. F.
Заглавие : Current-voltage characteristics of the resonant tunnelling double-barrier structure under time-periodical perturbation
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 1996. - Vol. 8, Is. 45. - P.8869-8887. - ISSN 0953-8984, DOI 10.1088/0953-8984/8/45/020
Примечания : Cited References: 38
Предметные рубрики: SEMICONDUCTOR DOUBLE-BARRIER
OSCILLATING QUANTUM-WELL
DEPENDENT TRANSPORT
INFRARED-RADIATION
TUNNELING TIMES
HETEROSTRUCTURES
TRANSMISSION
MODEL
FREQUENCIES
COHERENT
Аннотация: We consider a typical semiconductor resonant tunnelling GaAs/AlGaAs/GaAs nanostructure which forms a double-barrier potential with quasienergy levels corresponding to transition frequencies in the infrared and microwave regions. Two types of dynamical perturbation of the heterostructure in the form V-1(x, t) = V(1)x cos Omega t and V-2(t) = V-2 cos Omega t are considered. We analyse numerically a reconstruction of the electron transmission through the heterostructure and the current-voltage characteristics (IVC) under the influence of these dynamical perturbations. Both weak and strong perturbations are considered. We investigate the dependences of the transmission on the electron energy and the frequency of the external field with the main accent on the case where a frequency of the perturbation is tuned to a transition between quasienergies of the double-barrier structure. it is found that these resonant phenomena give rise to new peaks and dips in the IVC. In particular, it is shown that the dipole type of perturbation V-1(x, t) gives rise to a Rabi splitting of the transmission peaks and under certain conditions to a Rabi splining of the IVC peaks and dips. We demonstrate that dynamical perturbation may induce a direct current opposite to the direction of the applied voltage, and that this phenomenon takes the form of a sharp dip which has a resonant origin. It is observed that the dipole type of perturbation V-1(x, t) of laser radiation is more effective for tuning the IVC than the first perturbation V-2(t). Also absorption and emission of energy by an electron transmitted through the DBRTS are considered.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bulgakov E. N., Maksimov D. N.
Заглавие : Light enhancement by quasi-bound states in the continuum in dielectric arrays
Место публикации : Opt. Express: Optical Society of America, 2017. - Vol. 25, Is. 13. - P.14134-14147. - ISSN 10944087 (ISSN), DOI 10.1364/OE.25.014134
Примечания : Cited References: 85. - Ministry of Education and Science of Russian Federation (state contract N3.1845.2017/4.6) and RFBR grant 16-02-00314. We appreciate discussions with Almas F. Sadreev and Polina N. Semina.
Ключевые слова (''Своб.индексиров.''): optical constants--optics--asymptotic behaviors--circular cross-sections--dielectric elements--light enhancement--linear periodic arrays--near-infrared range--quasi-bound state--structural resonance--dielectric materials
Аннотация: The article reports on light enhancement by structural resonances in linear periodic arrays of identical dielectric elements. As the basic elements both subwavelength spheres and rods with circular cross section have been considered. In either case it has been demonstrated numerically that high-Q structural resonant modes originated from bound states in the continuum enable near-field amplitude enhancement by factor of 10–25 in the red-to-near infrared range in lossy silicon. The asymptotic behavior of the Q-factor with the number of elements in the array is explained theoretically by analyzing quasi-bound states propagation bands. © 2017 Optical Society of America.
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gabrienko A. A., Morozov E. V., Subramani V., Martyanov O. N., Kazarian S. G.
Заглавие : Chemical visualization of asphaltenes aggregation processes studied in situ with ATR-FTIR spectroscopic imaging and NMR imaging
Коллективы : Skolkovo Foundation; BP
Место публикации : J. Phys. Chem. C: American Chemical Society, 2015. - Vol. 119, Is. 5. - P.2646-2660. - ISSN 1932-7447, DOI 10.1021/jp511891f
Примечания : Cited References:78. - This research was performed under the UNIHEAT project. The authors wish to acknowledge the Skolkovo Foundation and BP for financial support. The authors thank BP for providing samples of crude oil
Предметные рубрики: MEXICAN CRUDE OILS
X-RAY-DIFFRACTION
INFRARED-SPECTROSCOPY
PETROLEUM ASPHALTENES
MOLECULAR-DYNAMICS
VARIABLE SELECTION
ORGANIC-SOLVENTS
LIGHT-SCATTERING
N-HEPTANE
NEAR-IR
Аннотация: Crude oil phase behavior and asphaltene precipitation have been studied by two complementary chemical imaging methods for the first time. ATR-FTIR spectroscopic imaging approach has revealed the chemical composition of agglomerated and precipitated asphaltenes upon dilution with a flocculant. Asphaltenes, containing oxygen and nitrogen heteroatomic functional groups, have been detected to be least stable. Aromatic abundant asphaltenes have been observed to have relatively high solubility in crude oil/heptane blends. NMR imaging approach, capable of imaging in the bulk of crude oil samples, has demonstrated that n-heptane causes aggregation which can lead to the stable suspension or to the sedimentation followed by the formation of deposits, depending on flocculant concentration. These processes have been monitored for small and large amounts of heptane added to crude oil. The data obtained by ATR-FTIR spectroscopic imaging and NMR imaging have been correlated to propose a possible link between the chemical structure of asphaltenes and a mechanism of the formation of deposits.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Golovnev N. N., Molokeev M. S., Sterkhova I. V., Lesnikov M. K., Atuchin V. V.
Заглавие : Coordination effects in hydrated manganese(II) 1,3-diethyl-2-thiobarbiturates and their thermal stability
Место публикации : Polyhedron: Elsevier, 2017. - Vol. 134. - P.120-125. - ISSN 02775387 (ISSN), DOI 10.1016/j.poly.2017.06.002
Примечания : Cited References: 25
Ключевые слова (''Своб.индексиров.''): 1,3-diethyl-2-thiobarbituric acid--complexes--x-ray diffraction--infrared spectroscopy--manganese(ii)
Аннотация: Three new complexes of 1,3-diethyl-thiobarbituric acid (HDetba), barbiturate-bridged 2D Mn(II) polymer [Mn(H2O)2(Detba)2] (1), trinuclear [Mn3(H2O)10(Detba)6] (2) and discrete molecular [Mn(H2O)4(Detba)2]·H2O (3) are synthesized and structurally characterized by the X-ray single crystal technique. In 1–3, the Detba− ions are coordinated to Mn(II) only through O atoms with manganese ions in the octahedral environment. In 1, the Mn(II) ion is coordinated by four μ2 bridge Detba− ions and two terminal H2O molecules. In 2, the Mn1 ion is coordinated by three terminal H2O molecules, two terminal and one μ2 bridge Detba− ion, and Mn2 is connected with two μ2-Detba− ions and four H2O molecules. In 3, the Mn(II) ion is coordinated by two terminal Detba− ions and four terminal H2O molecules. There are intermolecular hydrogen bonds O–H⋯O, O–H⋯S in the structures of 1–3 which form the 3D networks. Structure 2 is stabilized by the π–π interaction. The compounds thermal decomposition comprises dehydration steps and the organic ligand oxidation.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Golovnev N. N., Molokeev M. S., Sterkhova I. V., Lesnikov M. K.
Заглавие : Crystallographic, thermal and spectroscopic characterization of the anhydrous thiourea−barbituric acid and thiourea−2-thiobarbituric acid co-crystals
Место публикации : J. Mol. Struct. - 2019. - Vol. 1176. - P.865-870. - ISSN 00222860 (ISSN) , DOI 10.1016/j.molstruc.2018.09.035
Примечания : Cited References: 28
Ключевые слова (''Своб.индексиров.''): barbituric acid--2-thiobarbituric acid--thiourea--x-ray diffraction--infrared spectroscopy
Аннотация: Thiourea (Tu) crystallizes with barbituric acid (H2ba) and 2-thiobarbituric (H2tba) in the aqueous solution to yield co-crystals H2ba∙Tu (1) and H2tba∙Tu (2). Powder of 1 was also obtained from individual compounds via kneading with H2O. The structure of compounds was solved by the X-ray single crystal diffraction technique. In 1–2, NH⋯O, NH⋯S, CH⋯S and CH⋯O hydrogen bonds form the different 3D nets. In structure 1, centrosymmetric dimers of H2ba and Tu molecules are formed by two NH⋯O and NH⋯S hydrogen bonds, respectively. These dimers alternate in one-dimensional tapes. In compound 2, the same molecules are not bound by hydrogen bonds. Here, infinite chains are formed consisting of alternating molecules of H2tba and Tu. In these chains, each of the molecules is connected to the other by two NH⋯S hydrogen bonds. The compounds have been characterized by powder XRD, TG-DSC, and FT-IR.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Deich L. I.
Заглавие : Absorption of light by glasses in the far infrared
Место публикации : Jetp Lett. - 1992. - Vol. 56, Is. 10. - P.492-495. - ISSN 0021-3640
Примечания : Cited References: 9
Предметные рубрики: STATES
Аннотация: An explanation is proposed for the deviation from the Debye shape of the absorption curve of glasses in the far infrared.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Deich L. I.
Заглавие : Far-infrared attenuation in glasses
Разночтения заглавия :авие SCOPUS: Far-infrared attenuation in glasses
Место публикации : Phys. Rev. B. - 1994. - Vol. 49, Is. 1. - P.109-113. - ISSN 0163-1829, DOI 10.1103/PhysRevB.49.109
Примечания : Cited References: 29
Предметные рубрики: VITREOUS SILICA
TEMPERATURE
MODEL
LOCALIZATION
ABSORPTION
SOLIDS
STATES
Аннотация: The influence of quasilocal vibrations on the far-infrared spectra of glasses is investigated under the supposition that the quasilocal vibrations are directly inactive in the attenuation. It is shown that taking into account phonon-quasilocal-vibration coupling and both medium- and short-range structure of the inhomogeneities of a photon-phonon coupling parameter can give rise to an attenuation curve similar to one observed for a-SiO2 and related materials.
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16.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Deich L. I.
Заглавие : On far-infrared attenuation in glasses
Место публикации : Phonon scattering in condensed matter: proceedings: Springer Verlag, 1993. - Vol. 112. - P.233-234. - (Springer series in solid-state sciences). - ISBN 0171-1873. - ISBN 3-540-56395-4
Примечания : Cited References: 0
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lyu, Kuangnan, Liu, Gaochao, Molokeev M. S., Xia, Zhiguo
Заглавие : Double-site occupation triggered broadband and tunable NIR-I and NIR-II luminescence in AlNbO4:Cr3+ phosphors
Место публикации : Adv. Phys. Res. - 2023. - Vol. 2, Is. 4. - Ст.2200056. - ISSN 27511200 (eISSN), DOI 10.1002/apxr.202200056
Примечания : Cited References: 38. - This research was supported by the International Cooperation Project of the National Key Research and Development Program of China (2021YFB3500400 and 2021YFE0105700), National Natural Science Foundations of China (Grant No. 51972118), Guangzhou Science & Technology Project (202007020005), the State Key Laboratory of Luminescent Materials and Devices (Skllmd-2022-02), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01×137). This work was also funded by RFBR according to the research project No. 19-52-80003
Аннотация: Near-infrared (NIR) phosphor-converted light-emitting diodes (pc-LEDs) are desired for optoelectronic and biomedical applications, while the development of target broadband NIR phosphors still remains a significant challenge. Herein, a kind of Cr3+-doped AlNbO4 phosphors with a broad NIR emission ranging from 650 to 1400 nm under 450 nm excitation are reported. A giant red-shift emission peak from 866 to 1020 nm together with broadened full width at half-maximum of 320 nm is achieved simply by varying the doped Cr3+ concentrations. Structural and spectroscopy analysis demonstrate that a concentration-dependent site-occupation of Cr3+ emitters in different Al3+ sites is responsible for the tunable NIR luminescence. The as-fabricated NIR pc-LED based on optimized AlNbO4:Cr3+ phosphor exhibits great potential in night-vision applications. This work provides a novel design principle on the Cr3+-doped AlNbO4 phosphor with tunable broadband luminescence from NIR-I to NIR-II, and these materials can be employed in NIR spectroscopy applications.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gel'mukhanov F., Odelius M., Polyutov S. P., Fohlisch A., Kimberg V.
Заглавие : Dynamics of resonant x-ray and Auger scattering
Место публикации : Rev. Mod. Phys. - 2021. - Vol. 93, Is. 3. - Ст.035001. - ISSN 00346861 (ISSN), DOI 10.1103/RevModPhys.93.035001
Примечания : Cited References: 467. - The reported study was funded by the Russian Foundation for Basic Research (RFBR) (Project No. 19-29-12015) and partly supported by the Ministry of Science and Higher Education of the Russian Federation (Project No. FSRZ-2020-0008). M. O. acknowledges funding from the European Union’s Horizon 2020 research and innovation program under Marie Skłodowska-Curie Grant Agreement No. 860553, the Carl Tryggers Foundation (Contract No. CTS18:285), and the Swedish Energy Agency (Contract No. 2017-006797). Funding is acknowledged from the European Research Council through ERC-ADG-2014 (Advanced Investigator Grant No. 669531 EDAX) at the University of Potsdam within the Horizon 2020 EU Framework Programme for Research and Innovation. Support from the Helmholtz Association, in particular, the Helmholtz Virtual Institute 419 “Dynamic Pathways in Multidimensional Landscapes” and the Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, is acknowledged. Support from the Swedish Research Council (Grants No. 2019-03470 and No. 2015-03781) is also acknowledged
Аннотация: An overview of both experimental and theoretical results in the field of resonant scattering of tunable soft and hard x-ray radiation is presented, with a main focus on the closely related processes of resonant inelastic x-ray scattering (RIXS) and resonant Auger scattering (RAS). The review starts with an overview of fundamental dynamical aspects of RIXS illustrated for different systems. A detailed analysis of case studies with increasing complexity, considering both gas-phase and condensed matter (liquids and solids) applications, is given. In the review, the most important achievements in investigations of coupled electron-nuclear dynamics and structural aspects in studies of liquids and solids over the last two decades are outlined. To give a perspective on the insights from RIXS and RAS, the x-ray results are discussed against the background of complementary experimental techniques like vibrational infrared absorption and Raman spectroscopy, as well as small-angle x-ray and neutron scattering. Finally, recent achievements in time-resolved studies based on x-ray free-electron lasers are described.
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19.

Вид документа : Статья из журнала
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Автор(ы) : Ivantsov R. D., Lin C. -R., Chen Y. -Z., Ivanova O. S., Altunin R. R., Knyazev Yu. V., Molokeev M. S., Zharkov S. M., Shestakov N. P., Sukhachev A. L., Edelman I. S.
Заглавие : Effect of surfactants on the structure, phase composition, and magnetic properties of FexSy nanoparticles synthesized by thermal decomposition
Место публикации : Nanobiotechnol. Rep. - 2022. - Vol. 17, Is. 3. - P.336-344. - ISSN 26351676 (ISSN), DOI 10.1134/S2635167622030089
Примечания : Cited References: 27. - This study was supported by the Russian Foundation for Basic Research with Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science, the research project no. 19-42-240005: “Features of the Electronic Structure, Magnetic Properties, and Optical Excitations in Nanocrystals of Multifunctional Magnetic Chalcogenides Fe3S4 and FeSe” and the Russian Foundation for Basic Research and the Ministry of Science and Technology of Taiwan, joint projects nos. 19-52-52002 and 109-2112-M-153-003 and 108-2923-M-153-001-MY3The electron-microscopy study was carried out at the Laboratory of Electron Microscopy of the Center for Collective Use of the Siberian Federal University within the state assignment of the Ministry of Science and Higher Education of the Russian Federation (research code FSRZ-2020-0011). The magnetic measurements were carried out on a vibrating sample magnetometer at the Krasnoyarsk Regional Center for Collective Use, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences
Аннотация: The effect of surfactants on the structure, morphology, and magnetic properties of FexSy iron-sulfide nanoparticles synthesized by thermal decomposition is studied. Oleylamine, hexadecylamine, and octadecylamine are used as surfactants. It is established by X-ray and electron-diffraction analysis combined with Mossbauer spectroscopy that, in samples 1 and 2 prepared using oleylamine and hexadecylamine, respectively, the Fe3S4 greigite phase dominates, with an inverse spinel structure isostructural to the iron oxide Fe3O4 magnetite with minor Fe9S11 impurities. Deviations in the distribution of iron cations over the tetrahedral and octahedral sites relative to the bulk greigite crystals are observed. The nanoparticles synthesized using octadecylamine (sample 3) are found to be multiphase with a greigite fraction of ~20%. In all three cases, as showed the results of transmission electron microscopy and Fourier transform infrared spectroscopy together with thermogravimetry analysis, the magnetic nanoparticles have an organic shell chemically bonded to their magnetic core, which prevents the agglomeration of the particles. This shell is much more massive in samples 2 and 3. The magnetization values for samples 1 and 2 are similar to those of greigite nanoparticles reported in publications, while the magnetization of sample 3 is several times lower, in accordance with the greigite fraction in it. The combination of fairly high magnetization with a massive organic shell allows one to consider hexadecylamine to be a promising surfactant for the synthesis of iron-sulfide nanoparticles protected from external impact and agglomeration.
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20.

Вид документа : Статья из журнала
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Автор(ы) : Stepin E. A., Sushko E. S., Vnukova N. G., Churilov G. N., Rogova A. V., Tomilin F. N., Kudryasheva N. S.
Заглавие : Effects of endohedral Gd-containing fullerenols with a different number of oxygen substituents on bacterial bioluminescence
Колич.характеристики :19 с
Место публикации : Int. J. Mol. Sci. - 2024. - Vol. 25, Is. 2. - Ст.708. - ISSN 16616596 (ISSN), DOI 10.3390/ijms25020708. - ISSN 14220067 (eISSN)
Примечания : Cited References: 102. - This research was funded by the State Assignment of the Ministry of Science and Higher Education of the Russian Federation, project No. 0287-2021-0020, and partly supported by the Russian Science Foundation No. 23-26-10018, Krasnoyarsk Regional Science Foundation
Аннотация: Gadolinium (Gd)-containing fullerenols are perspective agents for magnetic resonance imaging and cancer research. They combine the unique paramagnetic properties of Gd with solubility in water, low toxicity and antiradical activity of fullerenols. We compared the bioeffects of two Gd-containing fullerenols with a different number of oxygen groups—20 and 42: Gd@C82O20H14 and Gd@C82O42H32. The bioluminescent bacteria-based assay was applied to monitor the toxicity of fullerenols, bioluminescence was applied as a signal physiological parameter, and bacterial enzyme-based assay was used to evaluate the fullerenol effects on enzymatic intracellular processes. Chemiluminescence luminol assay was applied to monitor the content of reactive oxygen species (ROS) in bacterial and enzymatic media. It was shown that Gd@C82O42H32 and Gd@C82O20H14 inhibited bacterial bioluminescence at 10?1 and 10?2 gL?1, respectively, revealing a lower toxicity of Gd@C82O42H32. Low-concentration (10?3–10?1 gL?1) bacterial bioluminescence activation by Gd@C82O42H32 was observed, while this activation was not found under exposure to Gd@C82O20H14. Additional carboxyl groups in the structure of Gd@C82O42H32 were determined by infrared spectroscopy and confirmed by quantum chemical calculations. The groups were supposed to endow Gd@C82O42H32 with higher penetration ability through the cellular membrane, activation ability, lower toxicity, balancing of the ROS content in the bacterial suspensions, and lower aggregation in aqueous media.
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