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    Морозов, Евгений Владимирович.
    Применение ЯМР томографии для исследования межфазных границ в системах коллоидного кремнезема / Е. В. Морозов, О. В. Шабанова, О. В. Фалалеев // Конденсир. среды и межфаз. границы. - 2012. - Т.14. № 1. - С. 60-69 . - ISSN 1606-867X
   Перевод заглавия: NMR imaging application for interfaces investigation in the colloid silica
Аннотация: В работе представлены результаты ЯМР томографических исследований золей коллоидного кремнезема, полученных из силикатов щелочных металлов кислотным выщелачиванием. Исследована динамика времен ядерной спин-решеточной и спин-спиновой релаксации в процессе гелеобразования, а также визуализировано пространственное распределение протекающих процессов. Рассмотрена методологическая сторона проблемы обеспечения контраста на ЯМР томограммах модельных коллоидных систем при золь-гель переходе. Экспериментально продемонстрирована актуальность разработки методологии исследования межфазных границ с помощью нового для данного направления метода.
The NMR Imaging investigation results of colloid silica obtained from alkali metals silicates by acidic leaching are presented. The dynamic of nuclear spin-lattice and spin-spin relaxation times was studied during the sol-gel transfer processes and the spatial distribution of occurred processes was visualized. The methodological direction of problem associated with contrast supply on the NMR Images was examined using model colloids samples during sol-gel transfer. It was demonstrated experimentally that the development of interfaces investigation methodology seems to be very important for advance of NMR Imaging to this field of research.

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Держатели документа:
Институт физики им. Л.В. Киренского СО РАН

Доп.точки доступа:
Шабанова, О. В.; Фалалеев, Олег Владимирович; Falaleev, O.V.; Morozov, E. V.
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Ignatchenko, V. A.
Wave spectrum of multilayers with finite thicknesses of interfaces / V. A. Ignatchenko, Y. I. Mankov, A. A. Maradudin // Phys. Rev. B. - 2000. - Vol. 62, Is. 3. - P. 2181-2184, DOI 10.1103/PhysRevB.62.2181. - Cited References: 24 . - ISSN 0163-1829

РУБ Physics, Condensed Matter
Рубрики:
SPIN
EXCITATIONS
MEDIA
Аннотация: To describe a multilayer structure with arbitrary thicknesses of the interfaces between layers, we introduce a model in which the dependence of a material parameter along the axis of such a superlattice is described by a Jacobian elliptic sine function. Depending on the value of the modulus kappa of the elliptic function, the model describes the limiting cases of multilayers with sharp interfaces (kappa=1, d/l=0, where d is the thickness of the interface, l is the period of the superlattice) and of sinusoidal superlattices (kappa=0, d/l=1/4), as Well as all intermediate situations. We investigate the wave spectrum in such a superlattice. The dependences of the widths of the gaps in the spectrum at the boundaries of ail odd Brillouin zones on the ratio d/l are found. It is shown that the thicknesses of the interfaces can be determined if the experimental value of the relation between the widths of the first gap Delta v(1) and any other gap Delta v(n) is known.

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Держатели документа:
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA
ИФ СО РАН

Доп.точки доступа:
Mankov, Y. I.; Maradudin, A. A.; Игнатченко, Вальтер Алексеевич
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    Understanding the energy barriers of the reversible ion exchange process in CsPbBr1.5Cl1.5@Y2O3:Eu3+ macroporous composites and their application in anti-counterfeiting codes / M. Li, Y. Zhao, S. Zhang [et al.] // ACS Appl. Mater. Interfaces. - 2021. - Vol. 13, Is. 50. - P. 60362-60372, DOI 10.1021/acsami.1c18030. - Cited References: 49. - This work is financially jointly supported by the Guangzhou Science & Technology Project (202007020005), NSFC (Grant No. 51772104), the Fundamental Research Funds for the Central Universities (2020ZYGXZR096), Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137), and RFBR according to the research project No. 19-52-80003 . - ISSN 1944-8244
   Перевод заглавия: Понимание энергетических барьеров процесса обратимого ионного обмена в макропористых композитах CsPbBr1.5Cl1.5@Y2O3: Eu3 + и их применение в кодах защиты от подделок
Кл.слова (ненормированные):
mixed-halide CsPbX3NCs -- macroporous Y2O3:Eu3+ -- energy barriers -- photoinduced ion exchange -- anti-counterfeiting codes
Аннотация: The photoinduced reversible ion exchanges in mixed halide perovskites and the resulting luminescent variations make them promising for constructing anti-counterfeiting patterns; however, its understanding in an interfacial view is lacking. In this work, nominal CsPbBr1.5Cl1.5 (CPBC) nanocrystals (NCs) were introduced into macroporous Y2O3:Eu3+ (MYE) to realize emission color variations from red emission of MYE to green emission of halide NCs. The large surface area of MYE helps the formation of Y–Cl/Br bonds which induces fluctuation in the halide composition, while water and intrinsic halogen defects have also been proved to be essential in the reversible ion segregation process. The PL variations of several samples with different pore sizes were investigated upon irradiation of light with different photon energies and excitation power at certain temperatures. According to combined results of density functional theory calculation, the research reveals the presence of two energy barriers that would be overcome correspondingly by the excitation photon and the concentration difference in the ion exchange and recovery process. A photochromic anti-counterfeiting quick response (QR) code was constructed facilely with the perovskite composites. This work provides a deeper understanding from the interfacial aspect and also proposes a feasible strategy to realize reversible PL variation for anti-counterfeiting applications.

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State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, South China University of Technology, Guangzhou, 510641, China
Department of Chemistry, City University of Hong Kong, Kowloon, 999077, Hong Kong
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 680021, Russian Federation
Siberian Federal University, Krasnoyarsk, 680021, Russian Federation
Research and Development Department, Kemerovo State University, Kemerovo, 650061, Russian Federation

Доп.точки доступа:
Li, M.; Zhao, Y.; Zhang, S.; Yang, R.; Qiu, W.; Wang, P.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Ye, S.
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    Two-dimensional-layered perovskite ALaTa2O7:Bi3+ (A = K and Na) phosphors with versatile structures and tunable photoluminescence / G. J. Zhou [et al.] // ACS Appl. Mater. Interfaces. - 2018. - Vol. 10, Is. 29. - P. 24648-24655, DOI 10.1021/acsami.8b08129. - Cited References: 48. - The authors acknowledge the support from the National Natural Science Foundation of China (Nos. 51722202, 91622125, and 51572023) and the Natural Science Foundations of Beijing (2172036) and RFBR (17-52-53031). . - ISSN 1944-8244
   Перевод заглавия: 2D-слоистые перовскитоподобные люминофоры ALaTa2O7:Bi3+ (A = K and Na) с разнообразными структурами и управляемой люминесценцией.

РУБ Nanoscience & Nanotechnology + Materials Science, Multidisciplinary
Рубрики:
GENERALIZED GRADIENT APPROXIMATION
YELLOW-EMITTING PHOSPHOR
Кл.слова (ненормированные):
2D-layered perovskite -- Bi3+ emission -- ion exchange -- photoluminescence tuning -- white light LEDs
Аннотация: Topological chemical reaction methods are indispensable for fabricating new materials or optimizing their functional properties, which is particularly important for two-dimensional (2D)-layered compounds with versatile structures. Herein, we demonstrate a low-temperature (∼350 °C) ion exchange approach to prefabricate metastable phosphors ALa1–xTa2O7:xBi3+ (A = K and Na) with RbLa1–xTa2O7:xBi3+ serving as precursors. The as-prepared ALa0.98Ta2O7:0.02 Bi3+ (A = Rb, K, and Na) share the same Dion–Jacobson type 2D-layered perovskite phase, and photoluminescence analyses show that ALa0.98Ta2O7:0.02 Bi3+ (A = Rb, K, and Na) phosphors exhibit broad emission bands peaking at 540, 550, and 510 nm, respectively, which are attributed to the nonradiative transition of Bi3+ from excited state 3P1 or 3P0 to ground state 1S0. The various Bi3+ local environments at the crystallographic sites enable the different distributions of emission and excitation spectra, and the photoluminescence tuning of ALa0.98Ta2O7:0.02 Bi3+ (A = Rb, K, and Na) phosphors are realized through alkali metal ion exchange. Notably, the combination of superior trivalent bismuth emission and low-temperature ion exchange synthesis leads to a novel yellow-emitting K(La0.98Bi0.02)Ta2O7 phosphor which is successfully applied in a white LED device based on a commercially available 365 nm LED chip. Our realizable cases of this low-temperature ion exchange strategy could promote exploration into metastable phosphors with intriguing properties.

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Держатели документа:
Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing Municipal Key Lab New Energy Mat & Techno, Beijing 100083, Peoples R China.
Chinese Acad Sci, Tech Inst Phys & Chem, Beijing 100190, Peoples R China.
Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
SB RAS, KSC, Fed Res Ctr, Kirensky Inst Phys,Lab Crystal Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.

Доп.точки доступа:
Zhou, Guojun; Jiang, Xingxing; Zhao, Jing; Molokeev, M. S.; Молокеев, Максим Сергеевич; Lin, Zheshuai; Liu, Quanlin; Xia, Zhiguo
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Theoretical investigation of the interfaces and mechanisms of induced spin polarization of 1D narrow zigzag graphene- and h-BN nanoribbons on a SrO-terminated LSMO(001) surface / P. Avramov [et al.] // J. Phys. Chem. A. - 2017. - Vol. 121, Is. 3. - P. 680-689, DOI 10.1021/acs.jpca.6b09696. - Cited References:74. - We acknowledge the Siberian Supercomputer Center (SSCC) of SB RAS, Novosibirsk; the Joint Supercomputer Center of RAS, Moscow; and the ICC of Novosibirsk State University for providing the computing resources. P.B.S. acknowledges the financial support of the Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NUST MISiS (No. K2-2015-033). The Russian Science Foundation (Grant No 14-13-00139) supported the work of the Russian team. The Japanese Science Foundation (JSPS KAKENHI, Grant No 16H3875) supported the work of the Japanese team. . - ISSN 1089-5639

РУБ Chemistry, Physical + Physics, Atomic, Molecular & Chemical
Рубрики:
HEXAGONAL BORON-NITRIDE
AUGMENTED-WAVE METHOD
GIANT MAGNETORESISTANCE
Аннотация: The structure of the interfaces and the mechanisms of induced spin polarization of 1D infinite and finite narrow graphene- and h-BN zigzag nanoribbons placed on a SrO-terminated La1-xSrxMnO3 (LSMO) (001) surface were studied using density functional theory (DFT) electronic structure calculations. It was found that the pi-conjugated nanofragments are bonded to the LSMO(001) surface by weak disperse interactions. The types of coordination of the fragments, the strength of bonding, and the rate of spin polarization depend upon the nature of the fragments. Infinite and finite graphene narrow zigzag nanoribbons are characterized by the lift of the spin degeneracy and strong spin polarization caused by interface-induced structural asymmetry and oxygen-mediated indirect exchange interactions with Mn ions of LSMO support. Spin polarization changes the semiconducting nature of infinite graphene nanoribbons to half-metallic state with visible spin-up density of states at the Fermi level. The h-BN nanoribbon binding energy is weaker than graphene nanoribbon ones with noticeably shorter interlayer distance. The asymmetry effect and indirect exchange interactions cause spin polarization of h-BN nanoribbon as well with formation of embedded states inside the band gap. The results show a possibility to use one-atom thick nanofragments to design LSMO-based heterostructures for spintronic nanodevices with h-BN as an inert spacer to develop different potential barriers.

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Держатели документа:
Kyungpook Natl Univ, Dept Chem, 80 Daehak Ro, Daegu 41566, South Korea.
Kyungpook Natl Univ, Green Nano Mat Res Ctr, 80 Daehak Ro, Daegu 41566, South Korea.
Siberian Fed Univ, 79 Svobodniy Pr, Krasnoyarsk 660041, Russia.
LV Kirensky Inst Phys SB RAS, 50-38 Akademgorodok, Krasnoyarsk 660036, Russia.
Natl Inst Quantum & Radiol Sci & Technol QST, Naka, Ibaraki 3191106, Japan.
Natl Univ Sci & Technol MISiS, Moscow 119049, Russia.

Доп.точки доступа:
Avramov, P. V.; Аврамов, Павел Вениаминович; Kuzubov, A. A.; Кузубов, Александр Александрович; Kuklin, A. V.; Куклин, Артем Валентинович; Lee, H.; Kovaleva, E. A.; Ковалева, Евгения Андреевна; Sakai, S.; Entani, S.; Naramoto, H.; Sorokin, P. B.; Ministry of Education and Science of the Russian Federation [K2-2015-033]; Russian Science Foundation [14-13-00139]; Japanese Science Foundation (JSPS KAKENHI) [16H3875]
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Theoretical investigation of magnetic properties in interfaces of magnetic nanoparticles and amorphous carbons / S. -J. Sun [et al.] // J. Magn. Magn. Mater. - 2017. - Vol. 432. - P. 102-105, DOI 10.1016/j.jmmm.2017.02.001. - Cited References: 21. - We would like to thank the Ministry of Science and Technology, Taiwan, for the Grant No. MOST 104-2112-M-390-001 and 104-2923-M-390-001-MY3 (Shih-Jye Sun). The work is supported also by the President of Russia program of the leading scientific schools, Grant NSh-7559.2016.2. . - ISSN 0304-8853
Кл.слова (ненормированные):
Antiferroelectricity -- Antiferromagnetism -- Ferromagnetism -- Molecular dynamics -- Nanomagnetics -- Nanoparticles -- Spin waves -- Antiferro-magnetic interactions -- Antiferromagnetics -- Kondo interactions -- Magnetic nano-particles -- Molecular dynamics simulations -- Spinwave excitation -- Theoretical investigations -- Theoretical modeling -- Amorphous carbon
Аннотация: Based on the experimental finding of the exchange bias in amorphous carbon samples with embedded Co nanoparticles and on the graphited character of the amorphous carbon interface confirmed by molecular dynamics simulations we have proposed the interface of graphited carbon to be antiferromagnetic. A theoretical model, which comprises the Kondo interactions in the interfaces of Co nanoparticles and the induced antiferromagnetic interactions in the graphited carbons, is employed to evaluate the ferromagnetism of the interfaces of Co nanoparticles. We have shown that the ferromagnetism of interfaces of Co nanoparticles will be enhanced by the increase of antiferromagnetic interaction as well as the increase of electron density in the graphited carbons. In particular, we found that the antiferromagnetic interactions in graphited carbons will change the spin-wave excitation in interfaces of Co nanoparticles from the quasiacoustic mode to the quasioptical one. © 2017 Elsevier B.V.

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Держатели документа:
Department of Applied Physics, National University of Kaohsiung, Kaohsiung, Taiwan
Department of Applied Physics, National Pingtung University, Pingtung, Taiwan
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Sun, S.-J.; Hsu, Hua-Shu; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Chen, G.-L.
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Avramov, P. V.
The role of interfaces in determination of electronic properties of complex silicon nanoclusters / P. V. Avramov // Workshop "Trends in Nanomechanics and Nanoengineering" : book of abstracts / предс. сем. K. S. Aleksandrov ; зам. предс. сем.: G. S. Patrin, S. G. Ovchinnikov ; чл. лок. ком.: N. N. Kosyrev, A. S. Fedorov [et al]. - 2009. - P. 11

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Доп.точки доступа:
Aleksandrov, K. S. \предс. сем.\; Александров, Кирилл Сергеевич; Patrin, G. S. \зам. предс. сем.\; Патрин, Геннадий Семёнович; Ovchinnikov, S. G. \зам. предс. сем.\; Овчинников, Сергей Геннадьевич; Kosyrev, N. N. \чл. лок. ком.\; Косырев, Николай Николаевич; Fedorov, A. S. \чл. лок. ком.\; Федоров, Александр Семенович; Аврамов, Павел Вениаминович; "Trends in Nanomechanics and Nanoengineering", workshop(2009 ; Aug. ; 24-28 ; Krasnoyarsk); Сибирский федеральный университет; Институт физики им. Л.В. Киренского Сибирского отделения РАН
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The effect of paramagnetic impurities in normal metal on the critical current in a network of S-N-S Josephson junctions in bulk Y3/4Lu1/4Ba2Cu3O7+BaPb(1-x)Fe(x)O(3)composites / D. A. Balaev [et al.] // Supercond. Sci. Technol. - 2003. - Vol. 16, Is. 1. - P. 60-64, DOI 10.1088/0953-2048/16/1/311. - Cited References: 41 . - ISSN 0953-2048

РУБ Physics, Applied + Physics, Condensed Matter
Рубрики:
CURRENT-VOLTAGE CHARACTERISTICS
   WEAK LINKS
   RESISTIVE PROPERTIES
   MAGNETIC-IMPURITIES
   EXCHANGE FIELD
   SNS JUNCTIONS
   F-S
   COMPOSITES
   SUPERCONDUCTOR
   SCATTERING
Кл.слова (ненормированные):
Critical currents -- Interfaces (materials) -- Josephson junction devices -- Paramagnetism -- Transport properties -- Non-superconducting ingredient -- Paramagnetic impurities -- Superconductor normal metal superconductor -- Oxide superconductors
Аннотация: Bulk Y3/4Lu1/4Ba2Cu3O7 + BaPb1-xFexO3 composites representing a model of a network of superconductor-normal metal-superconductor (SNS) Josephson junctions with paramagnetic impurities (Fe) in the N layers have been prepared. The transport properties of the composites have been studied. An exponential decay of the critical current with increasing Fe content in the non-superconducting ingredient of the composite has been observed. Such a behaviour is accounted for in terms of the de Gennes proximity effect theory.

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Держатели документа:
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН

Доп.точки доступа:
Balaev, D. A.; Балаев, Дмитрий Александрович; Ospishchev, S. V.; Petrov, M. I.; Петров, Михаил Иванович; Aleksandrov, K. S.; Александров, Кирилл Сергеевич
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The direct exchange mechanism of induced spin polarization of low-dimensional π-conjugated carbon- and h-BN fragments at LSMO(001) MnO-terminated interfaces / A. V. Kuklin [et al.] // J. Magn. Magn. Mater. - 2017. - Vol. 440: EURO-Asian Symposium on Trends in Magnetism (EASTMAG) (AUG 15-19, 2016, Siberian Fed Univ, Krasnoyarsk, RUSSIA). - P. 23-29, DOI 10.1016/j.jmmm.2016.12.096. - Cited References:70. - We acknowledge the Siberian Supercomputer Center (SSCC) of SB RAS, Novosibirsk; the Joint Supercomputer Center of RAS, Moscow and the ICC of Novosibirsk State University for providing the computing resources. Russian Science Foundation (Grant No 14-13-00139) supported the work of Russian team. . - ISSN 0304-8853. - ISSN 1873-4766

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
HEXAGONAL BORON-NITRIDE
   THIN-FILMS
   GIANT MAGNETORESISTANCE
   METALLIC
Кл.слова (ненормированные):
Graphene nanoribbons -- DFT -- LSMO thin films -- Induced spin polarization -- h-BN nanoribbons -- Half-metal
Аннотация: Induced spin polarization of π-conjugated carbon and h-BN low dimensional fragments at the interfaces formed by deposition of pentacene molecule and narrow zigzag graphene and h-BN nanoribbons on MnO2-terminated LSMO(001) thin film was studied using GGA PBE+U PAW D3-corrected approach. Induced spin polarization of π-conjugated low-dimensional fragments is caused by direct exchange with Mn ions of LSMO(001) MnO-derived surface. Due to direct exchange, the pentacene molecule changes its diamagnetic narrow-band gap semiconducting nature to the ferromagnetic semiconducting state with 0.15 eV energy shift between spin-up and spin-down valence bands and total magnetic moment of 0.11 μB. Direct exchange converts graphene nanoribbon to 100% spin-polarized half-metal with large amplitude of spin-up electronic density at the Fermi level. The direct exchange narrows the h-BN nanoribbon band gap from 4.04 to 1.72 eV in spin-up channel and converts the h-BN ribbon semiconducting diamagnetic nature to a semiconducting magnetic one. The electronic structure calculations demonstrate a possibility to control the spin properties of low-dimensional π-conjugated carbon and h-BN fragments by direct exchange with MnO-derived LSMO(001) surface for spin-related applications.

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Доп.точки доступа:
Kuklin, A. V.; Kuzubov, A. A.; Кузубов, Александр Александрович; Kovaleva, E. A.; Ковалева, Евгения Андреевна; Lee, Hyosun; Sorokin, Pavel B.; Sakai, Seiji; Entani, Shiro; Naramoto, Hiroshi; Avramov, P. V.; Аврамов, Павел Вениаминович; Russian Science Foundation [14-13-00139]; Euro-Asian Symposium "Trends in MAGnetism"(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); "Trends in MAGnetism", Euro-Asian Symposium(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); Институт физики им. Л.В. Киренского Сибирского отделения РАН
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10.

    Superconductivity on interfaces of nonsuperconducting granules La2CuO4 and La1.56Sr0.44CuO4 / A. A. Bykov [et al.] // J. Supercond. Nov. Magn. - 2018. - Vol. 31, Is. 12. - P. 3867–3874, DOI 10.1007/s10948-018-4668-x. - Cited References: 19. - The authors are grateful to D.A. Balaev for fruitful discussions, and I.V. Nemtsev for electronic microscope measurements in the center for shared use, KSC SB RAS. The work is supported by the Russian Science Foundation (project No. 17-72-10067). . - ISSN 1557-1939
   Перевод заглавия: Сверхпроводимость на интерфейсах несверхпроводящих гранул La2CuO4 и La1.56Sr0.44CuO4
Кл.слова (ненормированные):
Magnetic properties -- Superconductivity -- Oxide superconductors -- Grain boundaries -- LCO -- LSCO -- Josephson media
Аннотация: Composite materials fabricated by annealing of nonsuperconducting ceramics La2CuO4 and La1.56Sr0.44CuO4 at 910 °C during various time are investigated. Areas of superconducting La1.85Sr0.15CuO4 phase arises at boundaries of contacting nonsuperconducting granules. The volume fraction of the superconducting phase increases with increasing annealing time. A model describing the magnetic and transport properties of the samples at low magnetic fields is constructed. The magnetotransport characteristics of obtained samples at low magnetic fields (∼ 100 Oe) are defined by weak links network formed by superconducting areas. At high fields, behavior of the system is defined by a magnetization of the disconnected superconducting islands. The average size of the superconducting areas has been estimated from an extended critical state model.

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Petersburg Nuclear Physics Institute named by B.P. Konstantinov of National Research Centre “Kurchatov Institute”, Gatchina, 1, mkr., Orlova roshcha, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Bykov, A. A.; Terent'ev, K. Yu.; Терентьев, Константин Юрьевич; Gokhfeld, D. M.; Гохфельд, Денис Михайлович; Savitskaya, N. E.; Popkov, S. I.; Попков, Сергей Иванович; Petrov, M. I.; Петров, Михаил Иванович
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