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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Change in the polarizability of MBBA molecules upon the nematic-isotropic liquid transition and physical consequences
Место публикации : Phys. Solid State. - 2013. - Vol. 55, Is. 10. - P.2136-2141. - ISSN 1063-7834, DOI 10.1134/S106378341310003X
Аннотация: The Lorentz tensor components Lj and the polarizability tensor components ?j of 4-methoxyben-zylidene-4?-butylaniline (MBBA) liquid crystal molecules in nematic and isotropic phases have been determined experimentally. The quadratic dependences of the mean value ?(S) and anisotropy ??(S) of the polarizability in the nematic phase on the orientational order parameter S of molecules have been established. Within the phenomenological approach, the dependences ?(S) and ??(S) have been derived, and their features for MBBA and other known objects have been interpreted. The relation of the dependences ?(S) and ??(S) to the features of the nematic-isotropic liquid phase transition has been found. В© 2013 Pleiades Publishing, Ltd.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Change in the polarizability of molecules at the phase transitions isotropic liquid -nematic - smectic-A - crystal-B in liquid crystal 4О.8
Коллективы : European Conference on Liquid Crystals, Московский государственный университет им. М.В. Ломоносова
Место публикации : 14th Eur. Conf. Liq. Cryst. (ECLC): conf. programme/ чл. нац. орг. и прогр. ком. V. Ya. Zyryanov. - 2017. - Ст.P3. - Poster
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Change in the spectrum of the polarizability density of molecules at the smectic-A - crystal-B phase transition
Коллективы : European Conference on Liquid Crystals, Московский государственный университет им. М.В. Ломоносова
Место публикации : 14th Eur. Conf. Liq. Cryst. (ECLC): conf. programme/ чл. нац. орг. и прогр. ком. V. Ya. Zyryanov. - 2017. - Ст.P4. - Poster
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Influence of nematic and smectic orders on polarizability of molecules of ethyl-p-(4-ethoxybenzylideneamino-)alpha-methyl cinnamate liquid crystals
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2013. - Vol. 55, Is. 11. - P.2391-2396. - ISSN 1063-7834, DOI 10.1134/S1063783413110048
Примечания : Cited References: 16
Предметные рубрики: TRANSITION
MBBA
Аннотация: Experimental values of the polarizability tensor gamma components of molecules of ethyl-p-(4-ethoxybenzylideneamino-)alpha-methyl cinnamate liquid crystals in the nematic and smectic A phases have been obtained. Quadratic dependences of the longitudinal, gamma (l) , and transverse, gamma (t) , components, the mean value , and anisotropy Delta gamma in both phases have been established as functions of the orientational order parameter S of molecules in a maximally wide range of S. The nematic-smectic A phase transition with a continuous variation of S manifests itself as kinks in the linear dependences of , Delta gamma, and gamma (l) on S (2) and does not influence the dependence gamma (t) (S (2)). The observed dependences have been derived in the framework of the theory of the nematic-smectic A phase transition. The factors responsible for different influences of the orientational and positional orderings of molecules on the polarizability parameters have been determined.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Local-field anisotropy in cholesteric liquid crystals
Коллективы : Presidium of the Russian Academy of Sciences; Siberian Branch, Russian Academy of Sciences
Место публикации : JETP Letters. - 2009. - Vol. 89, Is. 7. - P.324-327. - ISSN 0021-3640, DOI 10.1134/S0021364009070030
Примечания : Cited References: 12. - This work was supported by the Presidium of the Russian Academy of Sciences ( Basic Research Program, project no. 27.1) and by the Siberian Branch, Russian Academy of Sciences ( Interdisciplinary Basic Research Program, project no. 5).
Предметные рубрики: ORDER
POLARIZABILITY
Аннотация: The first experimental values of the Lorentz tensor components L (j) for the cholesteric and smectic A phases of derivatives of cholesterol have been obtained using the dispersion of the refractive indices in the visible range. The temperature dependence of the components L (j) has been determined; it is invariant with respect to the cholesteric-smectic A phase transition. The effect of the isotropization of the Lorentz and local field tensors with decreasing anisotropy of the molecular polarizability has been revealed.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Long-Range Orientational Order, Local-Field Anisotropy, and Mean Molecular Polarizability in Liquid Crystals
Разночтения заглавия :авие SCOPUS: Long-range orientational order, local-field anisotropy, and mean molecular polarizability in liquid crystals
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2009. - Vol. 108, Is. 1. - P176-186. - ISSN 1063-7761, DOI 10.1134/S106377610901021X
Примечания : Cited References: 35
Предметные рубрики: REFRACTIVE-INDEXES
OPTICAL ANISOTROPY
Ключевые слова (''Своб.индексиров.''): anisotropy--crystal symmetry--crystals--electric fields--light sources--liquid crystals--liquids--molecules--tensors--biaxial liquid crystals--calamitic--discotic--discotic liquid crystals--experimental datum--field models--lorentz--mesoscopic--molecular polarizability--orientational orders--phase state--nematic liquid crystals
Аннотация: The problems on the relation of the mean effective molecular polarizability (gamma) over bar to the long-range orientational order of molecules (the optical anisotropy of the medium) in uniaxial and biaxial liquid crystals, the local anisotropy on mesoscopic scales, and the anisotropy of the Lorentz tensor L and the local-field tensor f are formulated and solved. It is demonstrated that the presence of the long-range orientational order of molecules in liquid crystals imposes limitations from below on the molecular polarizability (gamma) over bar, which differs for uniaxial and biaxial liquid crystals. The relation between the local anisotropy and the molecular polarizability (gamma) over bar is investigated for calamitic and discotic uniaxial liquid crystals consisting of lath- and disk-shaped molecules. These liquid crystals with identical macroscopic symmetry differ in the local anisotropy and the relationships between the components L(parallel to) L(perpendicular to,) f(parallel to) f(perpendicular to) (calamitic) and L(parallel to) L(perpendicular to,) f(parallel to) f(perpendicular to) (discotic) for an electric field oriented parallel and perpendicular to the director. The limitations from below and above on the molecular polarizability (gamma) over bar due to the anisotropy of the tensors L and f are established for liquid crystals of both types. These limitations indicate that the molecular polarizability (gamma) over bar depends on the phase state and the temperature. The factors responsible for the nonphysical consequences of the local-field models based on the approximation (gamma) over bar = const are revealed. The theoretical inferences are confirmed by the experimental data for a number of calamitic nematic liquid crystals with different values of birefringence and the discotic liquid crystal Col(ho).
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Mean polarizability of molecules and anisotropy of the Lorentz tensor upon a nematic-smectic a phase transition: Their behavior in a homologous series
Место публикации : Russ. J. Phys. Chem. A: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 86, Is. 5. - P.720-728. - ISSN 0036-0244, DOI 10.1134/S0036024412050044
Примечания : Cited References: 37
Предметные рубрики: CHOLESTERIC LIQUID-CRYSTALS
REFRACTIVE-INDEX DATA
A PHASE
MESOMORPHIC PROPERTIES
ORIENTATIONAL ORDER
OPTICAL ANISOTROPY
LOCAL-FIELD
POLYMORPHISM
TEMPERATURE
A-monotone
Alkyl chain
Experimental values
Homologous series
Homologues
Limiting values
Lorentz
Mesophases
Molecular core
Molecular polarizabilities
Nematic
Orientational order parameters
Polarizabilities
Polarizability density
Quadratic dependence
A-monotone
Smectic
Smectic phase
Smectic phasis
Smectic-A phasis
Ключевые слова (''Своб.индексиров.''): molecular polarizability--anisotropy--phase transition--nematic--smectic--homologues
Аннотация: Experimental values of the mean polarizability of molecules, (gamma) over bar, and components of the Lorentz tensor, L-j, in the nematic and smectic A phases are obtained for a homologous series of n-alkyl-p-(4-ethoxybenzylideneamino)-alpha-methylcinnamates. Dependences of the (gamma) over bar and L-j values on the mesophase temperature, the orientational order parameter S of molecules, and the number n in the homologous series are revealed. The quadratic dependence of (gamma) over bar (S) in the nematic and smectic phases is established that is invariant with respect to the nematic-smectic A transition. Polarizability densities of the molecular core and the alkyl chain are found from the monotone decreasing dependence (gamma) over bar (n)/v (where v is volume per one molecule) in the smectic phase. The presence (or absence) of the odd-even alternation of L-j(n) in the nematic (smectic) phase is shown. A monotone decrease in the Lorentz tensor anisotropy L with an increase in n is revealed in the smectic phase, and limiting values L-j(n - infinity) are determined.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : New features of a smectic-A-crystal-B phase transition in a homologous series of liquid crystals
Место публикации : JETP Letters. - 2014. - Vol. 99, Is. 3. - P.158-163. - ISSN 0021-3640, DOI 10.1134/S0021364014030047. - ISSN 1090-6487
Примечания : Cited References: 21
Предметные рубрики: POLARIZABILITY
POLYMORPHISM
ANISOTROPY
MOLECULES
BEHAVIOR
Аннотация: The components L j of the Lorentz tensor and the polarizability density of molecules G in the smectic-A and crystalline-B phases have been determined for homologues of the series of alkyl-p-(4-alkoxybenzylideneamino-)cinnamates. The quantity L j (G) in both phases is a linear (quadratic) function of the orientational order parameter of molecules S, which is invariant (noninvariant) with respect to the A-B transition, which is manifested in the form of jumps δL j and δG and enhancement of the G(S) dependence. An increase in the length of terminal molecular chains and weakening of interlayer correlation of molecules are accompanied by strengthening of the A-B transition of the first order and G(S) dependences in both phases together with an increase in δL j and δG. Change δG and dependence G(S) in the B phase are related to change in the conformation (flattening) of aromatic molecular cores.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Nonlinear coupling between the mean polarizability (gamma)over-bar of molecules and the local-field anisotropy in a liquid crystal and change of the "(gamma)over-bar = const" paradigm
Разночтения заглавия :авие SCOPUS: Nonlinear coupling between the mean polarizability gamma ̄ of molecules and the local-field anisotropy in a liquid crystal and change of the "gammā = const" paradigm; авие SCOPUS: Nonlinear coupling between the mean polarizability gamma ? of molecules and the local-field anisotropy in a liquid crystal and change of the "gamma = const" paradigm
Место публикации : JETP Letters. - 2008. - Vol. 87, Is. 5. - P.258-261. - ISSN 0021-3640, DOI 10.1134/S002136400805007X; \b JETP Letters. - 2008. - Vol. 87, Is. 5. - P.258-261. - Вариант Sopus
Примечания : Cited References: 14
Предметные рубрики: REFRACTIVE-INDEXES
ORDER
Аннотация: The nonlinear relation between the mean effective polarizability (gamma) over bar of molecules and the local-field anisotropy in uniaxial liquid crystals is demonstrated. Stringent constraints on (gamma) over bar from below, indicative of the dependence of on the liquid-crystal state and the change of the "(gamma) over bar = const" paradigm, are established. The theoretical results are confirmed by experiments with nematic liquid crystals having high and low birefringences.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Orientational order and polarizability of molecules in a nematic liquid crystal
Место публикации : Phys. Solid State. - 2014. - Vol. 56, Is. 5. - P.1058-1063. - ISSN 1063-7834, DOI 10.1134/S1063783414050035
Примечания : Cited References: 17
Предметные рубрики: NORMAL-BUTYLANILINE MBBA
INTERNAL-ROTATION
TRANSITION
PHASE
Аннотация: The influence of the orientational order of molecules in a nematic liquid crystal on the mean value ?? and anisotropy ?? of the molecular polarizability has been studied in the framework of the molecular statistical approach with allowance for the perturbation of the electronic structure of molecules due to the change in the conformation of their aromatic core and intermolecular interactions. Experimental dependences of ?? and ?? on the molecular orientational order parameter S have been derived, and their specific features for the known objects have been explained. The possibility of separating the contributions of opposite signs to the dependence ??(S) due to the change in the conformation of molecules and intermolecular interactions has been shown using nematic MBBA as an example. © 2014 Pleiades Publishing, Ltd.
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