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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gluck M., Kolovsky A. R., Korsch H. J.
Заглавие : A quantum cable car for Wannier-Stark ladders
Место публикации : Phys. Lett. A. - 2000. - Vol. 276, Is. 1-4. - P.167-174. - ISSN 0375-9601, DOI 10.1016/S0375-9601(00)00656-3
Примечания : Cited References: 13
Предметные рубрики: DYNAMIC LOCALIZATION
BLOCH PARTICLE
AC FIELDS
DC
STATES
STATISTICS
LIFETIME
Ключевые слова (''Своб.индексиров.''): wannier-stark ladder--induced transitions--induced transitions--wannier-stark ladder--article--energy--oscillation--quantum mechanics--time--transport kinetics
Аннотация: This Letter studies the dynamics of transitions between the levels of a Wannier-Stark ladder induced by a resonant periodic driving. The analysis of the problem is done in terms of resonance quasienergy states, which take into account the metastable character of the Wannier-Stark states. It is shown that the periodic driving creates from a localized Wannier-Stark state an extended Bloch-like state with a spatial length varying in time as similar to t(1/2). Such a state can find applications in the field of atomic optics because it generates a coherent pulsed atomic beam. (C) 2000 Elsevier Science B.V. All rights reserved.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volova, Tatiana G., Demidenko, Aleksey V., Murueva, Anastasiya V., Dudaev, Alexey E., Nemtsev I. V., Shishatskaya, Ekaterina I.
Заглавие : Biodegradable polyhydroxyalkanoates formed by 3- and 4-hydroxybutyrate monomers to produce nanomembranes suitable for drug delivery and cell culture
Колич.характеристики :23 с
Место публикации : Technologies. - 2023. - Vol. 11, Is. 4. - Ст.106. - ISSN 22277080 (eISSN), DOI 10.3390/technologies11040106
Примечания : Cited References: 116. - his research was funded by State Assignment of the Ministry of Science and Higher Education of the Russian Federation (project No. 0287-2021-0025)
Аннотация: Biodegradable polyhydroxyalkanoates, biopolymers of microbiological origin, formed by 3- and 4-hydroxybutyrate monomers P(3HB-co-4HB), were used to obtain nanomembranes loaded with drugs as cell carriers by electrospinning. Resorbable non-woven membranes from P(3HB-co-4HB) loaded with ceftazidime, doripinem, and actovegin have been obtained. The loading of membranes with drugs differently affected the size of fibers and the structure of membranes, and in all cases increased the hydrophilicity of the surface. The release of drugs in vitro was gradual, which corresponded to the Higuchi and Korsmeyer-Peppas models. Antibiotic-loaded membranes showed antibacterial activity against S. aureus and E. coli, in which growth inhibition zones were 41.7 ± 1.1 and 38.6 ± 1.7 mm for ceftazidime and doripinem, respectively. The study of the biological activity of membranes in the NIH 3T3 mouse fibroblast culture based on the results of DAPI and FITC staining of cells, as well as the MTT test, did not reveal a negative effect despite the presence of antibiotics in them. Samples containing actovegin exhibit a stimulating effect on fibroblasts. Biodegradable polyhydroxyalkanoates formed by 3-hydroxybutyrate and 4-hydroxybutyrate monomers provide electrospinning non-woven membranes suitable for long-term delivery of drugs and cultivation of eukaryotic cells, and are promising for the treatment of wound defects complicated by infection.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Murueva A. V., Dudaev A. E., Shishatskaya E. I., Ghorabe F. D. E., Nemtsev I. V., Lukyanenko A. V., Volova T. G.
Заглавие : Biodegradable polymer casting films for drug delivery and cell culture
Колич.характеристики :20 с
Место публикации : Giant. - 2024. - Vol. 19. - Ст.100314. - ISSN 26665425 (eISSN), DOI 10.1016/j.giant.2024.100314
Примечания : Cited References: 112. - The study was funded by State Assignment of the Ministry of Science and Higher Education of the Russian Federation (project No. FWES-2021–0025)
Аннотация: In this work, for the first time, films were obtained based on biodegradable polyhydroxyalkanoates (PHAs) - a copolymer of 3-hydroxybutyrate-co-3-hydroxyvalerate P(3HB-co-3HV) and a copolymer of 3-hydroxybutyrate-co-4-hydroxybutyrate P(3HB-co-4HB), containing drugs of different chemical structure and action - antibiotics (ceftazidime, doripenem), antiseptic (chlorhexidine) and tissue regeneration stimulator (Actovegin) for drug delivery and cell culture. Using SEM, AFM and measuring the contact angles of water wetting, it is shown how PHAs composition and loading of films of P(3HB-co-3HV) and P(3HB-co-4HB) with drugs affect the porosity, roughness indicators and adhesive properties of the surface. The constructed films are a depot form of drug, the release of which in vitro is realized for a long time, without burst releases, corresponds to Korsmeyer-Peppas and Higuchi models with diffusion character. Films loaded with antibiotics have pronounced antibacterial activity and suppress the development of pathogens S. aureus and E. coli, without a pronounced negative effect on the adhesion and proliferation of epidermal cells. In the cultures of human keratinocytes HaCaT it was shown that the presence of actovegin, as well as ceftazidime in the films, exhibits a stimulating effect, increasing their number. The results demonstrate the suitability of the depot-films for cellular technologies and are promising for the reconstruction of tissues complicated by infection.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Barinov G. I., Babkin Y. V.
Заглавие : Influence of high-pressure thermal-treatment on the phase compound and phase-transformation kinetics of a system magnetite-wustite
Место публикации : Izvestiya vysshikh uchebnykh zavedenii Fizika. - 1990. - Vol. 33, Is. 5. - P.95-96. - ISSN 0021-3411; \b Russian Physics Journal; \b Известия высших учебных заведений. Физика
Примечания : Cited References: 4
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Chzhan A. V., Podorozhnyak S. A., Rudenko R. Yu.
Заглавие : Influence of solid acidity on growth kinetics, structure and magnetic properties of CoP films during chemical deposition
Коллективы : Российская академия наук, Уральское отделение РАН, Институт физики металлов им. М. Н. Михеева Уральского отделения РАН, Уральский федеральный университет им. первого Президента России Б.Н. Ельцина, Российский фонд фундаментальных исследований, Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium
Место публикации : Euro-asian symposium "Trends in magnetism" (EASTMAG-2019): Book of abstracts/ чл. конс. ком.: S. G. Ovchinnikov, N. V. Volkov [et al.] ; чл. прогр. ком. D. M. Dzebisashvili [et al.]. - 2019. - Vol. 2. - Ст.J.P38. - P.254-255. - ISBN 978-5-9500855-7-4 (Шифр В33/E12-125657784)
Примечания : Cited References: 3
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Chzhan A. V., Podorozhnyak S. A., Patrin G. S., Rudenko R. Yu., Onufrienok V. V.
Заглавие : Influence of solution acidity on growth kinetics, structure and magnetic properties of Co-P films, obtained by chemical deposition
Коллективы : Euro-Asian Symposium "Trends in MAGnetism"
Место публикации : J. Phys. Conf. Ser. - 2019. - Vol. 1389, Is. 1. - Ст.012116. - ISSN 1742-6588, DOI 10.1088/1742-6596/1389/1/012116. - ISSN 1742-6596 (eISSN)
Примечания : Cited References: 21
Аннотация: The results of studies of the effect of solution acidity on the growth kinetics, structure and magnetic properties of Co-P films obtained by chemical deposition are presented. It was shown that the growth of Co-P films in the low pH region occurs mainly due to the growth of crystallite sizes, and in the high pH region, due to an increase in the nucleation rate. From the analysis of the chemical equilibrium of redox reactions, taking into account the balance of citrate and hydroxyl complexes of Co, a qualitative explanation of the features of the change in the rate and nature of the deposition of Co atoms from pH is proposed.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lamonova K.V., Zhitlukhina E.S., Babkin R.Y., Orel S.M., Pashkevich Y.G., Ovchinnikov S. G.
Заглавие : Intermediate-spin state of a 3D ion in the octahedral environment and generalization of the Tanabe - Sugano diagrams
Место публикации : The Journal of Physical Chemistry A (Dynamics, Kinetics, Environmental Chemistry, Spectroscopy, Structure, Theory): American Chemical Society, 2011. - Т. 115, № 46. - С. 13596-13604. - ISSN 1089-5639, DOI 10.1021/jp2071265. - ISSN 1520-5215(eissn)
РИНЦ
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zharkov S. M., Altunin R. R., Yumashev V. V., Moiseenko E. T., Belousov O. V., Solovyov L. A., Volochaev M. N., Zeer G. M.
Заглавие : Kinetic study of a solid-state reaction in Ag/Al multilayer thin films by in situ electron diffraction and simultaneous thermal analysis
Коллективы : Russian Science Foundation, RussiaRussian Science Foundation (RSF) [181300 080]
Место публикации : J. Alloys Compd. - 2021. - Vol. 871. - Ст.159474. - ISSN 0925-8388, DOI 10.1016/j.jallcom.2021.159474. - ISSN 1873-4669(eISSN)
Примечания : Cited References: 47. - This work was supported by the Russian Science Foundation, Russia under grant #181300 080
Предметные рубрики: STRUCTURAL PHASE-TRANSFORMATIONS
COMMITTEE RECOMMENDATIONS
ICTAC KINETICS
Аннотация: A solid-state reaction process in Ag/Al multilayer thin films has been investigated by the methods of in situ electron diffraction, simultaneous thermal analysis, transmission electron microscopy and X-ray diffraction with the aim of studying the phase formation kinetics of intermetallic compounds. The sequence of the phase transformations in the solid-state reaction has been established: Ag+Al→(Ag)+(Al)→(Ag)+δ-Ag2Al→μ-Ag3Al. The process of the solid-state interaction has been shown to consist of two steps; each of them is described by a kinetic model of the nth order reactions with autocatalysis. The kinetic parameters of the autocatalytic process of the phase formation for δ-Ag2Al and µ-Ag3Al, have been determined, in particular, their apparent activation energy: 126 kJ/mol and 106 kJ/mol, respectively.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Azarapin N. O., Khritokhin N. A., Atuchin V. V., Gubin A. A., Molokeev M. S., Mukherjee S., Andreev O. V.
Заглавие : Kinetics and mechanism of BaLaCuS3 oxidation
Место публикации : Crystals. - 2023. - Vol. 13, Is. 6. - Ст.903. - ISSN 20734352 (eISSN), DOI 10.3390/cryst13060903
Примечания : Cited References: 65. - The work was partially carried out using the resources of the Research Resource Center “Natural Resources Management and Physico-Chemical Research” (Tyumen University) with financial support from the Ministry of Science and Higher Education of the Russian Federation (contract No. 05.594.21.0019., Unique identification number RFMEFI59420X0019). M.S. Molokeev was supported by the Tyumen Oblast Government, as part of the West-Siberian Interregional Science and Education Center’s project No. 89-DON (3)The authors would like to thank the staff of the Engineering Center of the Tyumen State University (special Alexej V. Matigorov) for their help in carrying out physical and chemical tests
Аннотация: The oxidation reactions of BaLaCuS3 in the artificial air atmosphere were studied at different heating rates in the temperature range of 50–1200 °C. The oxidation stages were determined by DSC-TG, XRD and IR–vis methods. The kinetic characteristics of the proceeding reactions were obtained with the use of the Kissinger model in a linearized form. Compound BaLaCuS3 was stable in the air up to 280 °C. Upon further heating up to 1200 °C, this complex sulfide underwent three main oxidation stages. The first stage is the formation of BaSO4 and CuLaS2. The second stage is the oxidation of CuLaS2 to La2O2SO4 and copper oxides. The third stage is the destruction of La2O2SO4. The final result of the high-temperature treatment in the artificial air atmosphere was a mixture of barium sulfate, copper (II) oxide and La2CuO4. The mechanism and stages of BaLaCuS3 oxidation and further interactions of the components were discussed.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : BABKIN E. V., CHARYEV A. A., DROBOTENKO V. V., VYSHINSKAYA L. I.
Заглавие : KINETICS OF METAL-INSULATOR PHASE-TRANSITION IN VO2-N FILMS
Место публикации : Solid State Commun.: PERGAMON-ELSEVIER SCIENCE LTD, 1988. - Vol. 65, Is. 4. - P241-243. - ISSN 0038-1098, DOI 10.1016/0038-1098(88)90778-8
Примечания : Cited References: 6
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Slyusareva E. A., Sizykh A. G., Gerasimova M. A., Slabko V. V., Myslivets S. A.
Заглавие : Laser photolysis of fluorone dyes in a chitosan matrix
Место публикации : Quantum Electron.: Turpion LTD, 2012. - Vol. 42, Is. 8. - P.687-692. - ISSN 1063-7818, DOI 10.1070/QE2012v042n08ABEH014860
Примечания : Cited References: 32
Предметные рубрики: POLY(VINYL ALCOHOL) MATRIX
XANTHENE DYES
ROSE-BENGAL
FLUORESCENCE PROPERTIES
DELAYED FLUORESCENCE
ORGANIC-MOLECULES
TRIPLET-STATE
EXCITATION
ABSORPTION
PHOSPHORESCENCE
Ключевые слова (''Своб.индексиров.''): laser photolysis--fluorescein--dibromofluorescein--eosin y--erythrosin b--rose bengal--chitosan--photobleaching kinetics--two-step absorption
Аннотация: Kinetics of laser-induced photobleaching of fluorone dyes (fluorescein, dibromofluorescein, eosin Y, erythrosin B, Rose Bengal) is studied in a chitosan matrix. For all dyes the bleaching kinetics at the intensities of laser radiation 0.7 — 11.9 W cm-2 demonstrates quasi-monomolecular behaviour. The results are analysed using a kinetic model, based on the four-level (S0, S1, T1, Tn) scheme of the dye with chemically active triplet states taken into account. It is shown that the rate constants of the chemical reaction involving higher triplet states in the dyes studied amount to (3.9 — 18.6) × 106 s-1 and exceed the analogous values for the reaction involving the first lower triplet states by nine orders of magnitude. The rate of reaction involving the first triplet states appeared to be higher by one — two orders of magnitude than that in the case of higher triplet states involved because of low population of the latter. The possible mechanism of dye bleaching with participation of chitosan that consists in reduction of the dye to the leuco form by transfer of hydrogen from the chitosan matrix is discussed.
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12.

Вид документа : Однотомное издание
Шифр издания :
Заглавие : Lasers and applications . Vol. III : Ligth-induced kinetics. Education
Выходные данные : Красноярск, 1991
Колич.характеристики :219 с
Коллективы : International school of lasers and applications (March 17-23,1989; Sayanogorsk)
Примечания : Refs. at the and of the paps. :
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Potylitsyna, Arina R., Mishakov, Ilya, V, Bauman, Yury, I, Kibis, Lidia S., Shubin, Yury, V, Volochaev M. N., Melgunov, Maxim S., Vedyagin, Aleksey A.
Заглавие : Metal dusting as a key route to produce functionalized carbon nanofibers
Коллективы : Ministry of Science and Higher Education of the Russian Federation [AAAA-A21-121011390054-1, 0239-2021-0010, 121031700315-2]
Место публикации : React. Kinet. Mech. Catal. - 2022. - Vol. 135, Is. 3. - P.1387-1404. - ISSN 1878-5190, DOI 10.1007/s11144-022-02169-y. - ISSN 1878-5204(eISSN)
Примечания : Cited References: 65. - This work was supported by the Ministry of Science and Higher Education of the Russian Federation (Project numbers AAAA-A21-121011390054-1 (ID: 0239-2021-0010) and 121031700315-2)
Предметные рубрики: CHLORINATED HYDROCARBONS
NI-CU
DECOMPOSITION
NANOTUBES
CATALYST
Аннотация: The present paper reports a new method of producing N-doped carbon nanofibers via metal dusting of a ternary NiMoW alloy in the atmosphere containing C2HCl3 and CH3CN vapors at 600 °C. The initial alloy was prepared by a co-precipitation technique. The carbon deposition was monitored gravimetrically. The early stages of the metal dusting process were studied in detail using scanning and transmission electron microscopies. It was established that the rapid disintegration of the microdispersed NiMoW alloy with the formation of nanosized particles catalyzing the growth of carbon filaments occurs within the first 5 min of the reaction. The presence of C2HCl3 vapors in the reaction medium was shown to be the urgent condition to provide efficient metal dusting. The effect of the CH3CN concentration in the trichloroethylene-containing reaction mixture on the carbon deposition is investigated. As observed, the CH3CN content noticeable affects the carbon yield (after 2 h of reaction). The dome-shaped dependence of carbon yield reaches its maximal value of ~ 200 g/g(cat) at a CH3CN concentration of 33 vol%. According to X-ray photoelectron spectroscopy, the obtained carbon filaments are functionalized with Cl (0.1–1.2 wt%), O (3–6 wt%), and N (0.5–1.3 wt%). The prepared carbon filaments possess a segmented secondary structure, which is typical for carbon nanomaterials derived via catalytic decomposition of chlorine-substituted hydrocarbons. Low-temperature nitrogen adsorption measurement revealed that the specific surface area of the N-containing samples varies in a range from 370 to 550 m2/g.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Anshits A. G., Bayukov O. A., Anshits N. N., Pletnev O. N., Rabchevskii E. V., Vereshchagin S. N., Kondratenko E. V.
Заглавие : Nature of the active sites of ferrospheres in the oxidative condensation of methane
Коллективы : Russian Science Foundation [4-13-00289], Russian Congress on Catalysis (2; 2014 ; Oct. ; 2–5; Samara)
Место публикации : Kinet. Catal.: MAIK Nauka-Interperiodica / Springer, 2015. - Vol. 56, Is. 4. - P.523-531. - ISSN 0023, DOI 10.1134/S0023158415040023. - ISSN 16083210(eISSN)
Примечания : Cited References:37. - This work was supported by the Russian Science Foundation (grant no. 14-13-00289).
Предметные рубрики: GLASS CRYSTAL CATALYSTS
HIGH-TEMPERATURE
MOSSBAUER
MAGNETITES
MICROSPHERES
SELECTIVITY
CONVERSION
FERRITES
ASHES
IRON
Ключевые слова (''Своб.индексиров.''): oxidative condensation of methane--ferrospheres--iron spinel--mossbauer spectroscopy--structural defects
Аннотация: The catalytic properties of ferrospheres containing 76–97 wt % Fe2O3 in the oxidative condensation of methane were compared with their phase composition and the distribution of iron cations over the crystallographic positions of iron-containing phases in a steady state. It was established that the reaction route of methane oxidation changed at a Fe2O3 content of 89 wt %. Deep oxidation was the main reaction route on ferrospheres with a Fe2O3 content of 88.8 wt %. At a Fe2O3 content of ≥89 wt %, the yield of C2 hydrocarbons sharply increased and the contribution of deep oxidation decreased. The yield of C2 hydrocarbons correlated with the amount of defects in the structure of iron spinel, which are iron ions with the tetrahedral cation of Ca2+ and the octahedral cation vacancy among the nearest neighbors.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vereshchagin S. N., Solov'ev L. A., Rabchevskii E. V., Dudnikov V. A., Ovchinnikov S. G., Anshits A. G.
Заглавие : New method for regulating the activity of ABO3 perovskite catalysts
Коллективы : Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools [NSh-2886.2014.2]
Место публикации : Kinet. Catal.: MAIK Nauka-Interperiodica / Springer, 2015. - Vol. 56, Is. 5. - P.640-645. - ISSN 0023, DOI 10.1134/S0023158415040199. - ISSN 16083210(eISSN)
Примечания : Cited References:23. - This work was supported in part by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (grant no. NSh-2886.2014.2).
Предметные рубрики: MEMBRANE REACTORS
METHANE COMBUSTION
OXIDATION
OXIDES
OXYGEN
PERFORMANCE
FEATURES
PHASES
CO
Ключевые слова (''Своб.индексиров.''): perovskite--cobalt--methane--deep oxidation--oxidative condensation
Аннотация: A new possibility of changing the activity and selectivity of perovskite catalysts in the oxidative conversion of methane was demonstrated using the Sr x Gd1–x CoO3–δ (0.5 x 0.9) compounds as an example. It was established that, at the same chemical composition, the disordering of Sr2+/Gd3+ ions over the A positions of the crystal structure led to a significant increase in activity in the deep oxidation reaction of CH4, as compared with the samples with an ordered distribution of cations.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhigalov V. S., Myagkov V. G., Bayukov O. A., Bykova L. E., Bondarenko G. N., Matsynin A. A.
Заглавие : Phase transformations in Mn/Fe(001) films: Structural and magnetic investigations
Коллективы : Russian Foundation for Basic Research [07-03-00190]; Ministry of Education and Science of the Russian Federation [2.1.1/4399]
Место публикации : JETP Letters. - 2009. - Vol. 89, Is. 12. - P.621-625. - ISSN 0021-3640, DOI 10.1134/S0021364009120066
Примечания : Cited References: 36. - This work was supported by the Russian Foundation for Basic Research (project no. 07-03-00190) and by the Ministry of Education and Science of the Russian Federation (project no. 2.1.1/4399, program " Development of the Scientific Potentiality of Higher Education" in 2009- 2010).
Предметные рубрики: HIGH-TEMPERATURE SYNTHESIS
SOLID-STATE SYNTHESIS
FE-MN
THIN-FILMS
MARTENSITIC TRANSFORMATIONS
KINETICS
ALLOY
Аннотация: The solid-phase synthesis in epitaxial Mn/Fe(001) bilayer film systems with 24 at % of Mn has been shown to start at a temperature of 220A degrees C with the formation of a gamma-austenite lattice and the Mn and Fe films react completely under annealing to 600A degrees C. In the sample cooling process after annealing below 220A degrees C, the gamma austenite undergoes a martensitic transformation to an oriented a(100) martensite. When the annealing temperature is increased above 600A degrees C, Mn atoms migrate from the gamma-lattice, which becomes unstable, and the film is partially again transformed to the epitaxial Fe(001) layer. The solid-phase synthesis in Mn/Fe(001) bilayer nanofilms and multilayers is assumingly determined by the inverse epsilon - gamma martensitic transformation in the Mn-Fe system. The existence of a new low-temperature (similar to 220A degrees C) structure transition in the Mn-Fe system with a high iron content is assumed.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : PATRIN G. S., VOLKOV N. V., PETRAKOVSKII G. A.
Заглавие : PHOTOMAGNETIC EFFECT KINETICS IN ALPHA-FE2O3 - GA CRYSTALS
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1994. - Vol. 36, Is. 5. - P1385-1391. - ISSN 0367-3294
Примечания : Cited References: 10
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A. P., Isaev I. L., Gerasimov V. S., Karpov S. V.
Заглавие : Physical principles of the formation of a nanoparticle electric double layer in metal hydrosols
Место публикации : Colloid Polym. Sci. - 2020. - Vol. 298, Is. 1. - P.1-7. - ISSN 0303-402X, DOI 10.1007/s00396-019-04573-8. - ISSN 1435-1536 (eISSN)
Примечания : Cited References: 25. - The reported research was funded by the Russian Foundation for Basic Research and the government of the Krasnoyarsk territory, Krasnoyarsk Regional Fund of Science, grant No 18-42-243023, the RF Ministry of Education and Science, the State contract with Siberian Federal University for scientific research in 2017–2019.
Аннотация: The Brownian dynamics method is employed to study the formation of an electrical double layer (EDL) on the metal nanoparticle (NP) surface in hydrosols during adsorption of electrolyte ions from the interparticle medium. Also studied is the charge accumulation by NPs in the Stern layer. To simulate the process of the formation of EDL, we took into account the effect of image forces and specific adsorption, dissipative and random forces, and the degree of hydration of adsorbed ions on the EDL structure. The employed model makes it possible to determine the charge of NPs and the structure of EDL. For the first time, the charge of both the diffuse part of EDL and the dense Stern layer has been determined. A decrease in the electrolyte concentration (below c ˂ 0.1 mol/l) has been found to result in dramatic changes in the formation of the Stern layer.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fedorov A. S., Fedorov D. A., Kuzubov A. A., Avramov P. V., Nishimura Y., Irle S., Witek H. A.
Заглавие : Relative Isomer Abundance of Fullerenes and Carbon Nanotubes Correlates with Kinetic Stability
Разночтения заглавия :авие SCOPUS: Relative isomer abundance of fullerenes and carbon nanotubes correlates with kinetic stability
Место публикации : Phys. Rev. Lett.: AMER PHYSICAL SOC, 2011. - Vol. 107, Is. 17. - Ст.175506. - ISSN 0031-9007, DOI 10.1103/PhysRevLett.107.175506
Примечания : Cited References: 29. - S. I, P. V. A, and A. S. F gratefully acknowledge generous hospitality during their visits to Krasnoyarsk (S. I) and Fukui Institute for Fundamental Chemistry in Kyoto and Nagoya University (P. V. A and A. S. F) under support of the joint JSPS-RFBR travel grant 09-02-92107. This work was partially supported by National Science Council (grants NSC96-2113-M009-022-MY3 and NSC96-2113-M009-011-MY3) and Ministry of Education of Taiwan (MOE-ATU project), as well as by the JAEA Research fellowship (P. V. A). We thank the Institute of Computer Modeling (Siberian Division of RAS) and the Joint Supercomputer Center RAS for opportunity to use cluster computers for performing all calculations.
Предметные рубрики: CHEMICAL MOLECULAR-DYNAMICS
C-60
BUCKMINSTERFULLERENE
MECHANISM
ROAD
Ключевые слова (''Своб.индексиров.''): carbon nanostructures--kinetic factors--kinetic stability--thermal vibration--carbon nanotubes--fullerenes--isomers--kinetics
Аннотация: A methodology to evaluate the kinetic stability of carbon nanostructures is presented based on the assumption of the independent and random nature of thermal vibrations. The kinetic stability is directly correlated to the cleavage probability for the weakest bond of a given nanostructure. The application of the presented method to fullerenes and carbon nanotubes yields clear correlation to their experimentally observed relative isomer abundances. The general and simple formulation of the method ensures its applicability to other nanostructures for which formation is controlled by kinetic factors.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Chen M., Nong S., Zhao Y., Riaz M. S., Xiao Y., Molokeev M. S., Huang F.
Заглавие : Renewable P-type zeolite for superior absorption of heavy metals: Isotherms, kinetics, and mechanism
Место публикации : Sci. Total Environ. - 2020. - Vol. 726. - Ст.138535. - ISSN 00489697 (ISSN), DOI 10.1016/j.scitotenv.2020.138535
Примечания : Cited References: 47. - This work was supported by the National Key Research and Development Program of China (Grant No. 2016YFB0901600 ); National Science Foundation of China (Grant No. 21871008 ); Science and Technology Commission of Shanghai Municipality (Grant No. 14520722000 ) and China Postdoctoral Science Foundation [Grant No. 8206300161 ]. Thank Shuying Nong for her experimental assistance
Аннотация: Zeolite is a characteristic material for removing heavy metals exhibiting by low tolerance quantities. It is particularly desirable although challenging to cultivate an unmodified and reusable zeolite for eradicating heavy metals with great capacity. Herein, we sought out and firstly synthesized the uniform octahedral zeolite Na6Al6Si10O32·12H2O for heavy metal ions trap, proven extraordinarily effective decontamination of M2+ (Pb2+, Cd2+, Cu2+, and Zn2+). The maximum capacities of Pb2+, Cd2+, Cu2+, and Zn2+ were 649, 210, 90 and 88 mg/g, and the distribution coefficients (Kd) was ~108 mL/g for Pb2+ which emphasized the superior effectiveness of Na6Al6Si10O32·12H2O contrasted with other zeolites. Rapid adsorption was observed that Pb2+ concentration (7.5 ppm) was reduced to 0.6 ppb in 2 min. The removal mechanism was ascribed to the ion exchange and hydroxyl groups thereby affording high adsorption capacity. We also investigated the heavy metal removal of zeolite 13X and 4A for comparison and concluded the determining factor affecting absorption capacity. The removal rate of Pb remained at 97% even after five regeneration recycles. The zeolite was therefore promising for practical water purification and industrialization.
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