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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mikhaleva E. A., Flerov I. N., Gorev M. V., Molokeev M. S., Cherepakhin A. V., Kartashev A. V., Mikhashenok N. V., Sablina K. A.
Заглавие : Caloric characteristics of PbTiO3 in the temperature range of the ferroelectric phase transition
Место публикации : Phys. Solid State: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 54, Is. 9. - P.1832-1840. - ISSN 1063-7834, DOI 10.1134/S1063783412090181
Примечания : Cited References: 31. - This study was supported by the Russian Foundation for Basic Research (project no. 12-08-00079) and the Council on Grants from the President of the Russian Federation for Support of Leading Scientific Schools of the Russian Federation (grant no. NSh-4828.2012.2).
Предметные рубрики: SINGLE-CRYSTALS
LEAD TITANATE
DIELECTRIC PROPERTIES
SOLID-SOLUTIONS
PRESSURE
PEROVSKITES
DEPENDENCE
BEHAVIOR
HEAT
Аннотация: The heat capacity and thermal expansion of the PbTiO3 ceramic sample have been measured in the temperature range 80–970 K. The electrocaloric and barocaloric efficiencies of lead titanate in the ferroelectric phase transition range have been investigated by analyzing the experimental data in terms of the thermodynamic theory of phase transitions, the electrical equation of state P(T, E), the Pippard equation, and the S(T, p) diagram.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zaitsev A. I., Aleksandrovsky A. S., Kozhukhov A. S., Pokrovsky L. D., Atuchin V. V.
Заглавие : Growth, optical and microstructural properties of PbB4O7 plate crystals
Коллективы : SB RAS [28.14, 43.14]; President of the Russian Federation for the support of leading scientific schools [SS-4828.2012.2]; PSB RAS [2.5.2]; Ministry of Education and Science of the Russian Federation
Место публикации : Opt. Mater.: Elsevier Science, 2014. - Vol. 37. - P.298–301. - ISSN 0925-3467, DOI 10.1016/j.optmat.2014.06.012. - ISSN 1873-1252
Примечания : Cited References: 42. - This study is supported by SB RAS via Projects 28.14 and 43.14, and the Grant of the President of the Russian Federation for the support of leading scientific schools SS-4828.2012.2 and by PSB RAS, Grant 2.5.2. V.V.A. gratefully acknowledge the Ministry of Education and Science of the Russian Federation for financial support
Предметные рубрики: LEAD TETRABORATE
SINGLE-CRYSTAL
SUSCEPTIBILITIES
ANISOTROPY
STRONTIUM
SURFACES
RAMAN
Ключевые слова (''Своб.индексиров.''): pbb4o7--czochralski growth--facet--rheed--afm
Аннотация: Centimeter-sized optical quality plate-like PbB4O7 crystals have been grown by Czochralski method. The fundamental absorption edge has been found at 237 nm (corresponding bandgap 5.75 eV) with the distinct sideband protruding up to 300 nm. The crystals are well faceted with the (100), (010) and (101) planes, (100) surfaces being mostly developed. The etching in diluted nitric acid (5 wt.%) at the temperature of 90 °C have been used to reveal the defect structure and remove melt residuals. The (100) surface shows the presence of etching pits and twin boundaries. The Kikuchi line pattern and developed microrelief with the roughness of ~8 nm have been observed by RHEED and AFM, respectively.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lykhin A. O., Novikova G. V., Kuzubov A. A., Staloverova N. A., Sarmatova N. I., Varganov S. A., Krasnov P. O.
Заглавие : A complex of ceftriaxone with Pb(II): synthesis, characterization, and antibacterial activity study
Коллективы : RFBR [14-03-31, 170 MOJI_a]
Место публикации : J. Coord. Chem.: Taylor & Francis, 2014. - Vol. 67, Is. 16. - З2783-2794. - ISSN 0095-8972, DOI 10.1080/00958972.2014.938065. - ISSN 1029-0389
Примечания : Cited References: 48. - The reported study was supported by RFBR, research project No. 14-03-31, 170 MOJI_a and Krasnoyarsk regional fund for supporting scientific and technological activities. We thank the Center for Equipment Joint Use of the Siberian Federal University. We are grateful to the HPC Research Departments of Siberian Federal University and Moscow University Supercomputing Center (SKIF MSU "Chebyshev") for the access to the high-performance computer clusters.
Предметные рубрики: BETA-LACTAM ANTIBIOTICS
TERNARY COMPLEX
METAL-COMPLEXES
BASIS-SETS
3 DECADES
RESISTANCE
COPPER(II)
CEPHALOSPORINS
EVOLUTION
1ST-ROW
Ключевые слова (''Своб.индексиров.''): ceftriaxone lead(ii) complex--dft--ir spectroscopy--tga--antibacterial screening
Аннотация: A Pb(II) complex with ceftriaxone (H2Ceftria) antibiotic was synthesized by reaction of ceftriaxone disodium salt (hemi)heptahydrate with lead nitrate in water–ethanol medium. The complex was characterized on the basis of complexometric titration, spectrophotometric and thermogravimetric analyses, capillary electrophoresis, IR, Raman and UV–vis spectroscopies, and density functional theory calculations. Pb(II) is five-coordinate with distorted square pyramidal geometry. The coordination of Ceftria2− to Pb(II) occurs through N and O of the triazine, lactam carbonyl, carboxylate, and amine groups. The antibacterial activity study showed that Klebsiella pneumoniae is resistant to [Pb(Ceftria)]·3H2O. The antibacterial activity of [Pb(Ceftria)]·3H2O against Staphylococcus aureus is reduced compared with ceftriaxone. In contrast, the antibacterial activity of [Pb(Ceftria)]·3H2O against Escherichia coli is 28% higher than that of ceftriaxone antibiotic.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aleksandrov K. S., Zamkov A. V., Zaitsev A. I., Turchin P. P., Sysoev A. M., Parfenov A. A.
Заглавие : Acoustical and acoustooptical properties of lead tetraborate single crystals
Место публикации : Phys. Solid State. - 2004. - Vol. 46, Is. 9. - P.1637-1638. - ISSN 1063-7834, DOI 10.1134/1.1799178
Примечания : Cited References: 6
Предметные рубрики: STRONTIUM
Аннотация: The velocities of bulk acoustic waves and the acoustooptical Q factors M-2 are measured. The results of these measurements are used for calculating the photoelastic coefficients of a lead tetraborate single crystal. (C) 2004 MAIK "Nauka/Interperiodica".
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Raevski I. P., Molokeev M. S., Misyul S. V., Eremin E. V., Blazhevich A. V., Kubrin S. P., Sarychev D. A., Titov V. V., Chen H., Chou, C. -C., Raevskaya S. I., Malitskaya M. A.
Заглавие : Studies of ferroelectric and magnetic phase transitions in multiferroic PbFe0.5Ta0.5O3
Коллективы : International Conference of Piezoresponse Force Microscopy and Nanoscale Phenomena in Polar Materials , Russian Foundation for Basic Research (RFBR) [12-08-00887_a, 14-02-90438_Ucr_a], Ministry of education and science of Russian Federation [2132, 2014/174], Southern Federal University [213.01-2014/012-VG], Research Committee of the University of Macau under Research & Development Grant for Chair Professor
Место публикации : Ferroelectrics: Taylor & Francis, 2015. - Vol. 475, Is. 1: Special Issue: Proceedings of International Conference of Piezoresponse Force Microscopy and Nanoscale Phenomena in Polar Materials (PFM-2014) Part I of III. - P.52-60. - ISSN 0015, DOI 10.1080/00150193.2015.995009. - ISSN 15635112(eISSN)
Примечания : Cited References:26. - This study is partially supported by the Russian Foundation for Basic Research (RFBR) project (projects 12-08-00887_a and 14-02-90438_Ucr_a), Ministry of education and science of Russian Federation (research project 2132, task 2014/174), Southern Federal University grant 213.01-2014/012-VG and Research Committee of the University of Macau under Research & Development Grant for Chair Professor.
Предметные рубрики: NEUTRON POWDER DIFFRACTION
Pb(Fe1/2Ta1/2)O-3
Ключевые слова (''Своб.индексиров.''): lead iron tantalate--multiferroic--ferroelectric--lattice parameters--phase transition
Аннотация: X-ray, magnetic, and Mossbauer studies of a PbFe0.5Ta0.5O3 powder have been carried out. For the first time temperature dependence of the unit cell parameters was obtained. Antiferromagnetic Neel temperature T-N approximate to 180K was determined using the results of Mossbauer studies. In the vicinity of T-N an anomaly in the temperature dependence of the monoclinic angle beta was revealed in PFT. This anomaly seems to be due to the magnetoelectric coupling.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Golovnev N. N., Molokeev M. S., Golovneva I. I.
Заглавие : The crystal structure of lead(II) 1,3-diethyl-2-thiobarbiturate
Место публикации : Russ. J. Coord. Chem.: MAIK Nauka-Interperiodica / Springer, 2015. - Vol. 41, Is. 5. - P.300-304. - ISSN 1070, DOI 10.1134/S1070328415050012. - ISSN 16083318(eISSN)
Примечания : Cited References:25
Предметные рубрики: HYDROGEN-BOND
COMPLEXES
ACID
2-THIOBARBITURATE
DIFFRACTION
SERIES
Аннотация: The complex [Pb2(DETBA)4] n (I), where HDETBA is 1,3-diethyl-2-thiobarbituric acid (C8H12N2O2S), was obtained and structurally characterized by X-ray diffraction (CIF file CCDC no. 1031501). The crystals of complex I are trigonal: a = 12.9503(3), c = 32.077(1) Å, V = 4658.9(3) Å3, space group R3¯ , Z = 9. One of the crystallographically independent lead ions, Pb(1)2+, is coordinated in an octahedral fashion by six DETBA− ions through the O atoms. The other ion, Pb(2)2+, is coordinated to six DETBA− ions through three O atoms and three S atoms making up a trigonal prism. The polyhedra Pb(1)O6 and Pb(2)O6 are united through bridging DETBA− ions into infinite layers. The ligands are linked by neither intermolecular hydrogen bonds nor π-π interactions.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mikhlin Y., Vorobyev S., Romanchenko A., Karasev S., Karacharov A., Zharkov S. M.
Заглавие : Ultrafine particles derived from mineral processing: A case study of the Pb-Zn sulfide ore with emphasis on lead-bearing colloids
Место публикации : Chemosphere: Elsevier, 2016. - Vol. 147. - P.60-66. - ISSN 00456535 (ISSN), DOI 10.1016/j.chemosphere.2015.12.096
Примечания : Cited References: 47. - This research was supported by the Russian Science Foundation, Grant No. 14-17-00280.
Предметные рубрики: GALENA DISSOLUTION
METALLIC COPPER
NANOPARTICLES
SOIL
ENVIRONMENT
SEPARATION
TRANSPORT
FLOTATION
WATER
SIZE
Ключевые слова (''Своб.индексиров.''): lead sulfide--lead-zinc ore--lead sulfide--ultrafine particles--aquatic nanoparticles
Аннотация: Although mining and mineral processing industry is a vast source of heavy metal pollutants, the formation and behavior of micrometer- and nanometer-sized particles and their aqueous colloids entered the environment from the technological media has received insufficient attention to date. Here, the yield and characteristics of ultrafine mineral entities produced by routine grinding of the Pb-Zn sulfide ore (Gorevskoe ore deposit, Russia) were studied using laser diffraction analysis (LDA), dynamic light scattering (DLS) and zeta potential measurement, microscopy, X-ray photoelectron spectroscopy, with most attention given to toxic lead species. It was revealed, in particular, that the fraction of particles less that 1 ?m in the ground ore typical reaches 0.4 vol. %. The aquatic particles in supernatants were micrometer size aggregates with increased content of zinc, sulfur, calcium as compared with the bulk ore concentrations. The hydrodynamic diameter of the colloidal species decreased with time, with their zeta potentials remaining about -12 mV. The colloids produced from galena were composed of 20-50 nm PbS nanoparticles associated with lead sulfate and thiosulfate, while the surface oxidation products at precipitated galena were largely lead oxyhydroxides. The size and zeta potential of the lead-bearing colloids decreased with time down to about 100 nm and from -15 mV to -30 mV, respectively. And, conversely, lead sulfide nanoparticles were mobilized before the aggregates during redispersion of the precipitates in fresh portions of water. The potential environmental impact of the metal-bearing colloids, which is due to the large-scale production and relative stability, is discussed. © 2015 Elsevier Ltd.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Balaev D. A., Popkov S. I., Semenov S. V., Bykov A. A., Sabitova E. I., Dubrovskiy A. A., Shaikhutdinov K. A., Petrov M. I.
Заглавие : Contributions from Inter-grain Boundaries to the Magneto-resistive Effect in Polycrystalline High-T (C) Superconductors. The Underlying Reason of Different Behavior for YBCO and BSCCO Systems
Разночтения заглавия :авие SCOPUS: Contributions from inter-grain boundaries to the magneto-resistive effect in polycrystalline high-TC superconductors. the underlying reason of different behavior for YBCO and BSCCO systems
Место публикации : J. Supercond. Nov. Magn: SPRINGER, 2011. - Vol. 24, Is. 7. - P2129-2136. - ISSN 1557-1939, DOI 10.1007/s10948-011-1166-9
Примечания : Cited References: 30. - This work is supported by program N5 of RAS, project N7.
Предметные рубрики: HIGH-TEMPERATURE SUPERCONDUCTORS
PHASE-SLIP
TRANSPORT-PROPERTIES
TRANSITION
FIELD
COMPOSITES
BULK
TAPES
YBA2CU3O7-DELTA
DISSIPATION
Ключевые слова (''Своб.индексиров.''): bscco--ybco--intergrain boundaries--magnetoresistance--bscco--intergrain boundaries--magnetoresistance--ybco--bscco--bscco system--comparative studies--high tc superconductors--high-field--inter-grain--irreversibility lines--magneto-resistive effect--polycrystalline--resistive transition--standard measurements--weak pinning--ybco--bismuth--electric resistance--grain boundaries--high temperature superconductors--lead--magnetic fields--magnetoelectronics--magnetoresistance--magnetos--superconductivity--yttrium barium copper oxides--semiconductor metal boundaries
Аннотация: In order to clarify the mechanisms in charge of broadening of resistive transition R(T) in magnetic fields of bismuth-based polycrystalline high-T (C) superconductor (HTSC), a comparative study of Bi1.8Pb0.3Sr1.9Ca2Cu3O (x) (BSCCO) and YBa2Cu3O7-delta (YBCO) have been performed. Magnetoresistive effects and irreversibility line obtained from magnetic measurements have been studied. It was established that (1) for YBCO, the smooth part of R(T) dependence unambiguously corresponds to dissipation in the intergrain boundaries for arbitrary magnetic fields; (2) for polycrystalline BSCCO, the smooth part of R(T) dependences correspond to dissipation within intergrain boundary subsystem in the field range H 10(2) Oe only, while standard measurements of R(T) dependences in magnetic field range H 10(2) Oe reflect the dissipation processes occurring both in intergrain boundary and HTSC grain subsystems; (3) for the high-field range, the contribution from intergrain boundaries of BSCCO can be distinguished from magnetoresistance R(H) dependences obtained at high enough current density on textured samples. It is proposed that various magneto-resistive properties of these classical HTSC systems are due comparatively weak pinning in BSCCO.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shaykhutdinov K. A., Balaev D. A., Semenov S. V., Popkov S. I., Dubrovskiy A. A., Sapronova N. V., Volkov N. V.
Заглавие : Relaxation of low-temperature magnetoresistance and magnetization of polycrystalline (La0.5Eu0.5)(0.7)Pb0.3MnO3
Разночтения заглавия :авие SCOPUS: Relaxation of low-temperature magnetoresistance and magnetization of polycrystalline (La 0.5Eu 0.5) 0.7Pb 0.3MnO 3
Место публикации : J. Phys. D. - 2011. - Vol. 44, Is. 25. - Ст.255001. - ISSN 0022-3727, DOI 10.1088/0022-3727/44/25/255001
Примечания : Cited References: 34. - This work was partially supported by the Lavrentyev Competition of the Young Scientist's Projects of the Siberian Branch of the Russian Academy of Sciences, Project No 12. The authors are grateful to A D Balaev and V M Sosnin for useful discussions on the results.
Предметные рубрики: INSULATOR-METAL TRANSITION
GRANULAR FILMS
NANOPARTICLES
PR0.7CA0.3MNO3
PERCOLATION
MANGANITES
Ключевые слова (''Своб.индексиров.''): antiferromagnetic boundaries--characteristic value--ferromagnetic domains--ferromagnetic metal--lanthanum manganites--logarithmic law--low temperatures--magneto-resistive effect--polycrystalline--relative orientation--relaxation of magnetization--temperature fluctuation--time evolutions--time interval--tunnel magnetoresistance--antiferromagnetism--electric resistance--europium--ferromagnetic materials--ferromagnetism--grain boundaries--grain size and shape--lanthanum compounds--lead--magnetic domains--magnetic moments--magnetoelectronics--magnetoresistance--manganese oxide--magnetization
Аннотация: Hysteresis and relaxation of magnetoresistance and magnetization of substituted (La0.5Eu0.5)(0.7)Pb0.3MnO3 lanthanum manganite in a low-temperature region ( 40 K) are investigated. It is shown that at these temperature features of the magnetoresistive effect are determined mainly by spin-dependent tunnelling of carriers via insulating grain boundaries. As was demonstrated previously, the grain boundaries may be antiferromagnetically ordered. Therefore, relaxation of magnetization and resistance is determined by the processes of relative orientation of the magnetic moments of ferromagnetic domains neighbouring the antiferromagnetic boundary of ferromagnetic domains under the action of temperature fluctuations. It is shown that relaxation follows the logarithmic law within the time interval t similar to 10(2)-3x10(3) s. A comparison between time evolutions of the magnetic moment and resistance shows that magnetoresistance and magnetization are related as delta R
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shaykhutdinov K. A., Popkov S. I., Semenov S. V., Balaev D. A., Dubrovskiy A. A., Sablina K. A., Sapronova N. V., Volkov N. V.
Заглавие : Low-temperature resistance and magnetoresistance hysteresis in polycrystalline (La0.5Eu0.5)(0.7)Pb0.3MnO3
Разночтения заглавия :авие SCOPUS: Low-temperature resistance and magnetoresistance hysteresis in polycrystalline (La0.5Eu0.5)0.7Pb 0.3MnO3
Место публикации : J. Appl. Phys.: AMER INST PHYSICS, 2011. - Vol. 109, Is. 5. - Ст.53711. - ISSN 0021-8979, DOI 10.1063/1.3559303
Примечания : Cited References: 20. - This study was partially supported by the Russian Foundation for Basic Research, Project No. 08-02-00259a and the Lavrentyev Competition of the Young Scientists' Projects of the Siberian Branch of the Russian Academy of Sciences, Project No. 12.
Предметные рубрики: RESISTIVITY MINIMUM
MANGANITES
FILMS
Ключевые слова (''Своб.индексиров.''): antiferromagnets--electrical resistances--ferromagnets--field dependence--inter-grain--lanthanum manganites--low temperatures--low-temperature resistance--polycrystalline--temperature dependence--tunnel contacts--antiferromagnetic materials--europium--ferromagnetic materials--ferromagnetism--hysteresis--lead--magnetic field effects--magnetoelectronics--magnetoresistance--magnets--manganese oxide--paramagnetism--superconducting materials--electric resistance
Аннотация: The behavior of temperature dependences of electrical resistance and magnetoresistance of polycrystalline substituted lanthanum manganite (La0.5Eu0.5)(0.7)Pb0.3MnO3 at low temperatures was thoroughly studied. A broad hysteresis was found in the field dependences of electrical resistance in the low-temperature region. Above 40 K, no hysteresis feature was observed. The temperature T = 40 K corresponds to the temperature of minimum electrical resistance and the temperature T-N to the antiferromagnet-paramagnet phase transition of the material of the intergrain boundaries. In this work we propose a model which explains the observed features of the rho(T) and rho(H) curves at temperatures below T-N by the formation of a network of ferromagnet-antiferromagnet-ferromagnet tunnel contacts. (C) 2011 American Institute of Physics. [doi:10.1063/1.3559303]
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gokhfeld D. M., Balaev D. A., Petrov M. I., Popkov S. I., Shaykhutdinov K. A., Val'kov V. V.
Заглавие : Magnetization asymmetry of type-II superconductors in high magnetic fields
Место публикации : J. Appl. Phys.: AMER INST PHYSICS, 2011. - Vol. 109, Is. 3. - Ст.33904. - ISSN 0021-8979, DOI 10.1063/1.3544038
Примечания : Cited References: 23. - D. M. Gokhfeld is thankful to S. A. Satzuk and Yu. S. Gokhfeld for discussions. The work is supported by Project No. 7 of RAS Program "Quantum physics of condensed matter," Federal Target Program " Research and scientific-pedagogical cadres of Innovative Russia" and Grant No. 13 of Lavrentyev competition of young researchers of SB RAS.
Предметные рубрики: HIGH-TEMPERATURE SUPERCONDUCTORS
CRITICAL-STATE MODEL
CRITICAL-CURRENT DENSITIES
SURFACE-BARRIER
TRANSPORT
Ключевые слова (''Своб.индексиров.''): field distribution--high magnetic fields--inhomogeneous distribution--magnetization loops--pinning forces--thermal equilibriums--type ii superconductors--lead--magnetic fields--superconducting materials--superconductivity--magnetization
Аннотация: Inhomogeneous distribution of the pinning force in superconductor results in a magnetization asymmetry. A model considering the field distribution in superconductor was developed and symmetric and asymmetric magnetization loops of porous and textured Bi1.8Pb0.3Sr1.9Ca2Cu3Ox were fitted. It is found that the thermal equilibrium magnetization realizes in crystals smaller than some size depending on temperature and magnetic field. (C) 2011 American Institute of Physics. [doi:10.1063/1.3544038]
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shaykhutdinov K. A., Popkov S. I., Balaev D. A., Semenov S. V., Bykov A. A., Dubrovskiy A. A., Sapronova N. V., Volkov N. V.
Заглавие : Non-linear current-voltage characteristics of (La0.5Eu0.5)(0.7)Pb0.3MnO3 single crystals: Possible manifestation of the internal heating of charge carriers
Коллективы :
Разночтения заглавия :авие SCOPUS: Non-linear currentvoltage characteristics of (La0.5Eu 0.5)0.7Pb0.3MnO3 single crystals: Possible manifestation of the internal heating of chargecarriers
Место публикации : Physica B: ELSEVIER SCIENCE BV, 2010. - Vol. 405, Is. 24. - P4961-4965. - ISSN 0921-4526, DOI 10.1016/j.physb.2010.09.043
Примечания : Cited References: 19. - The authors are grateful to A.N. Lavrov for useful discussions on the results. This study was partially supported by the Russian Foundation for Basic Research, Project no. 08-02-00259a and the Lavrent'ev Young Scientists' Competition of the Siberian Branch of the Russian Academy of Sciences. Project no. 12.
Предметные рубрики: INSULATOR-METAL TRANSITION
PR0.7CA0.3MNO3
MANGANITES
Ключевые слова (''Своб.индексиров.''): manganites--negative differential resistance--cvc--cvc--manganites--negative differential resistance--applied electric field--charge ordering--current switching--cvc--dielectric regions--experimental data--internal heating--lanthanum manganites--metal-dielectric transition--negative differential resistances--non equilibrium--non-linear--sample heating--temperature evolution--transport currents--electric fields--electron gas--europium--heating--lanthanum--lead--manganites--negative resistance--phase separation--single crystals--thermal conductivity--manganese oxide
Аннотация: Temperature evolution of the current-voltage characteristics (CVCs) of a single-crystal lanthanum manganite (La0.5Eu0.5)(0.7)Pb0.3MnO3 is investigated in a wide (up to 1 A) range of instrumental currents. Effects of a transport current and an applied electric field on the resistance of the material are studied in view of possible implementation of the charge ordering break in dielectric regions occurring due to phase separation in manganites. A negative differential resistance portion observed in the CVCs suggests the presence of a current switching effect. Below the temperature of the metal-dielectric transition in (La0.5Eu0.5)(0.7)Pb0.3MnO3, the hysteresis is observed in the CVC. The detailed analysis of the internal sample heating on the basis of experimental data on thermal conductivity showed, however, that these CVC features can be explained within the concept of non-equilibrium heating of electron gas. (C) 2010 Elsevier B.V. All rights reserved.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Eremin E. V., Sablina K. A., Sapronova N. V.
Заглавие : Dielectric properties of a mixed-valence Pb3Mn7O15 manganese oxide
Коллективы :
Разночтения заглавия :авие SCOPUS: Dielectric properties of a mixed-valence Pb3Mn7O 15 manganese oxide
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2010. - Vol. 22, Is. 37. - Ст.375901. - ISSN 0953-8984, DOI 10.1088/0953-8984/22/37/375901
Примечания : Cited References: 14. - This study was supported by the Russian Foundation for Basic Research 'Siberia', project No. 09-02-98003, and the Siberian Branch of the Russian Academy of Sciences, integration project No. 101.
Ключевые слова (''Своб.индексиров.''): cation--lead--manganese derivative--oxide--article--chemical model--chemistry--crystallization--electric conductivity--electronics--methodology--temperature--cations--crystallization--electric conductivity--electronics--lead--manganese compounds--models, chemical--oxides--temperature--ac electric field--analysis of resistivity--carrier hopping--charge ordering--complex dielectric constant--crystal site--debye models--dielectric constants--dielectric spectra--frequency windows--lattice sites--low frequency--manganese ions--mixed valence--mixed valence state--relaxation behaviors--temperature range--electric fields--manganese--manganese oxide--permittivity--single crystals--crystal symmetry
Аннотация: We investigated the low-frequency dielectric properties of a Pb3Mn7O15 single crystal with manganese ions in the mixed-valence state (Mn3+/Mn4+). Dielectric relaxation was found in the frequency window from 20 to 100 kHz in the temperature range 110-180 K. The dielectric spectra of the crystal were analyzed using a Debye model. Estimations made within the model and analysis of resistivity data suggest that the relaxation behavior of the dielectric constant is related to polaronic charge carrier hopping. Around 250 K, charge ordering occurs in the crystal when the Mn3+ and Mn4+ ions are arranged in a specific order among the crystal sites. With a decrease in temperature, an ac electric field can induce a charge hop between the equivalent lattice sites available, related to crystal symmetry. This hopping is equivalent to the reorientation of an electric dipole that yields Debye-type behavior of the complex dielectric constant. The observed anisotropy in the behavior of the dielectric properties and resistivity can be attributed to a pronounced two-dimensional character of the crystal structure.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Balaev D. A., Popkov S. I., Semenov S. V., Bykov A. A., Shaykhutdinov K. A., Gokhfeld D. M., Petrov M. I.
Заглавие : Magnetoresistance hysteresis of bulk textured Bi1.8Pb0.3Sr1.9Ca2Cu3Ox + Ag ceramics and its anisotropy
Коллективы :
Место публикации : Physica C. - 2010. - Vol. 470, Is. 1. - P.61-67. - ISSN 0921-4534, DOI 10.1016/j.physc.2009.10.007
Примечания : Cited References: 24. - Authors thanks to I.L. Belozerova for help in preparation of textured ceramics. This work was supported by program N5 of RAS, project N7, and in part in frames of young scientist projects of Siberian Federal University, project N6.
Предметные рубрики: CRITICAL-CURRENT ANISOTROPY
HIGH-TEMPERATURE SUPERCONDUCTOR
CRITICAL-CURRENT DENSITY
MAGNETIC HYSTERESIS
TAPES
FLUX
YBA2CU3O7-DELTA
FIELD
Ключевые слова (''Своб.индексиров.''): magnetoresistance--anisotropy--scaling--magnetization--bi2223--bscco--anisotropy--bi2223--bscco--magnetization--magnetoresistance--scaling--bi-2223--bscco--external fields--granular superconductors--magnetic induction--parameters characterizing--anisotropy--calcium--ceramic materials--crystallites--electric resistance--hysteresis--lead--magnetic moments--magnetoelectronics--magnetoresistance--nanocrystalline alloys--silver--superconducting materials--superconductivity--magnetic field effects
Аннотация: Magnetoresistance of bulk textured Bi1.8Pb0.3Sr1.9Ca2Cu3Ox + Ag ceramics has been studied in the magnetic fields applied parallel and perpendicular to a-b planes of Bi2223 crystallites. Besides well known anisotropy of magnetoresistance of textured superconductors (R-H parallel to c RH parallel to a-b), anisotropic hysteresis of R(H) dependences was investigated. Parameters characterizing hysteretic R(H) curves differ for the cases H parallel to c and H parallel to a-b. This behavior is explained within the model of a granular superconductor where the total magnetic induction in the intercrystallite boundaries is superposition of the external field and the magnetic field induced by dipole magnetic moments of neighbor crystallites. (C) 2009 Elsevier B.V. All rights reserved.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Sablina K. A., Eremin E. V., Boni P., Shah V. R., Flerov I. N., Kartashev A., Rasch JCE, Boehm M., Schefer J.
Заглавие : Heat capacity of a mixed-valence manganese oxide Pb(3)Mn(7)O(15)
Коллективы :
Разночтения заглавия :авие SCOPUS: Heat capacity of a mixed-valence manganese oxide Pb3Mn 7O15
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2008. - Vol. 20, Is. 44. - Ст.445214. - ISSN 0953-8984, DOI 10.1088/0953-8984/20/44/445214
Примечания : Cited References: 11. - This study was supported by the INTAS (project No 061000013-9002), the Division of Physical Sciences of RAS, program `Spin-dependent Effects in Solids and Spintronics' (project No. 2.4.2 of SB RAS), the President of the Russian Federation, grant for Support of Leading Scientific Schools (project No. NSh-1011.2008.2), KRSF-RFBR `Enisey2007', project No. 07-02-96801-a, and the Siberian Branch of RAS, Integration project No. 3.7.
Ключевые слова (''Своб.индексиров.''): antiferromagnetism--crystallography--entropy--lead alloys--magnetic materials--magnetism--manganese--manganese compounds--powders--single crystals--specific heat--spin dynamics--antiferromagnetic orders--charge localizations--entropy losses--excess heat capacities--experimental datums--heat capacities--magnetic contributions--magnetic orders--magnetic states--magnetic subsystems--magnetic transitions--manganese oxides--nonmagnetic--spin systems--temperature curves--temperature dependences--temperature intervals--temperature ranges--manganese alloys
Аннотация: We present the results of a heat capacity study of Pb(3)Mn(7)O(15) single crystals with approximately equal concentrations of Mn(3+) and Mn(4+) ions. In the temperature interval between 210 and 260 K, an excess heat capacity of nonmagnetic origin, most likely associated with the process of charge localization, has been observed. Also, three pronounced anomalies corresponding to the changes in a magnetic subsystem of the crystal have been observed in the temperature dependence of the heat capacity. A broad hump near 150 K is related to the formation of a short-range magnetic order. This process of short-range ordering is rather prominent, considering the appreciable value of the entropy loss accompanying the change in the magnetic state. A clear lambda-shaped peak at 70 K marks the onset of a long-range antiferromagnetic order. Another anomalous contribution to the heat capacity of magnetic origin has been revealed at temperatures below 20 K. This contribution is associated with a magnetic transition of an unknown nature, which is also clearly evident in magnetization versus temperature curves. The total magnetic contribution to the entropy deduced from the actual experimental data over the entire temperature range is much smaller than is expected for a completely ordered Mn spin system in the crystal. We suggest several possible reasons that may account for this `missing' entropy.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrov M. I., Belozerova I. L., Shaikhutdinov K. A., Balaev D. A., Dubrovskii A. A., Popkov S. I., Vasil'ev A. D., Mart'yanov O. N.
Заглавие : Preparation, microstructure, magnetic and transport properties of bulk textured Bi(1.8)Pb(0.3)Sr(1.9)Ca(2)Cu(3)O(x) and Bi(1.8)Pb(0.3)Sr(1.9)Ca(2)Cu(3)O(x)+Agceramics
Коллективы :
Разночтения заглавия :авие SCOPUS: Preparation, microstructure, magnetic and transport properties of bulk textured Bi1.8Pb0.3Sr1.9Ca2Cu 3Ox and Bi1.8Pb0.3Sr 1.9Ca2Cu3Ox+Ag ceramics
Место публикации : Supercond. Sci. Technol.: IOP PUBLISHING LTD, 2008. - Vol. 21, Is. 10. - Ст.105019. - ISSN 0953-2048, DOI 10.1088/0953-2048/21/10/105019
Примечания : Cited References: 22. - This work is supported by program of RAS 'Quantum macrophysics' No. 3.4 and integration project of SB RAS No. 3.4 and in part by Krasnoyarsk Regional Scientific Foundation (KRSF), Grants 17G057, 18G148 and 18G011. DAB and AAD acknowledge the Russian Science Support Foundation.
Предметные рубрики: HIGH-TEMPERATURE SUPERCONDUCTORS
CRITICAL-CURRENT DENSITY
BI-2223 TAPES
BI2223
SILVER
DISCS
(BI
Ключевые слова (''Своб.индексиров.''): building materials--calcium--copper--crystallites--diamagnetic materials--lead--lead alloys--magnetic anisotropy--magnetic properties--nanocrystalline alloys--silver--textures--transport properties--bi-2223--bulk samples--degree of textures--diamagnetic responses--liquid mediums--magnetic and transport properties--magnetic measurements--room temperatures--ceramic materials
Аннотация: A new method of preparation of bulk textured Bi2223 ceramics and Bi2223 + Ag composites, based on room temperature pressing of foamed precursor (Bi2223, Bi2223 + Ag) in a liquid medium, is proposed. SEM and XRD data prove a high degree of texture of the bulk samples obtained. Magnetic measurements performed in directions H parallel to c-axis and H parallel to a-b-planes of Bi2223 crystallites demonstrates anisotropy of magnetization confirming the texture of the ceramics. The materials obtained possess large diamagnetic response in the direction H parallel to a-b-planes of Bi2223 crystallites at both 77.4 and 4.2 K.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Balaev D. A., Shaihutdinov K. A., Popkov S. I., Gokhfeld D. M., Petrov M. I.
Заглавие : Magnetoresistive effect in bulk composites 1-2-3 YBCO+CuO and 1-2-3 YBCO+BaPb(1-x)SnxO(3) and their application as magnetic field sensors at 77 K
Разночтения заглавия :авие SCOPUS: Magnetoresistive effect in bulk composites 1-2-3 YBCO + CuO and 1-2-3 YBCO + BaPb1-xSnxO3 and their application as magnetic field sensors at 77 K
Место публикации : Supercond. Sci. Technol.: IOP PUBLISHING LTD, 2004. - Vol. 17, Is. 1. - P175-181. - ISSN 0953-2048, DOI 10.1088/0953-2048/17/1/031
Примечания : Cited References: 27
Предметные рубрики: PHASE-SLIP
SUPERCONDUCTOR
TEMPERATURE
YBA2CU3O7-DELTA
TRANSITION
Ключевые слова (''Своб.индексиров.''): ceramic materials--composite materials--critical current density (superconductivity)--high temperature operations--high temperature superconductors--lead compounds--magnetoresistance--sensors--yttrium barium copper oxides--high temperature superconductor ceramics--magnetic field sensors--magnetoresistive effect--transport current density--oxide superconductors
Аннотация: We have studied the magnetoresistive effect in bulk 1-2-3 YBCO + CuO and 1-2-3 YBCO + BaPb1-xSnxO3 composites prepared using the fast backing technique. We have found that the composites exhibit large magnetoresistance in low magnetic fields ( 100 Oe) for a broad temperature range. We have studied the experimental dependences of resistivity versus magnetic field at various transport current densities. The high-T-C superconductor (HTSC) based composites exhibit a much higher sensitivity to weak magnetic fields at liquid nitrogen temperature, compared to that for pure HTSC ceramics. This effect is attractive for practical applications and the composite materials can be used as active elements in magnetic field sensor devices.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gorev M. V., Flerov I. N., Bondarev V. S., Sciau P.
Заглавие : Heat capacity study of relaxor PbMg1/3Nb2/3O3 in a wide temperature range
Разночтения заглавия :авие SCOPUS: Heat capacity study of relaxor PbMg1/3Nb2/3O 3 in a wide temperature range
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2003. - Vol. 96, Is. 3. - P531-537. - ISSN 1063-7761, DOI 10.1134/1.1567427
Примечания : Cited References: 21
Предметные рубрики: DIFFUSE PHASE-TRANSITION
FERROELECTRICS
Ключевые слова (''Своб.индексиров.''): differential scanning calorimetry--mathematical models--phonons--random processes--specific heat--spectrum analysis--thermal effects--bond-random field models--wide temperature intervals--lead compounds
Аннотация: Heat capacity of the PbMg1/3Nb2/3O3 compound is measured using the methods of adiabatic and differential scanning calorimetry in the temperature range 80-750 K. Two blurred anomalies on the C-p(T) dependence are observed in wide temperature intervals of 200- 400 K and 500-700 K. The results of studies are discussed together with data on the structure and phonon spectrum in the framework of spherical random bond-random field model. (C) 2003 MAIK "Nauka/Interperiodica".
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gorev M., Bondarev V., Sciau P., Savariault J. M.
Заглавие : Heat capacity study of relaxors BaTi0.65Zr0.35O3 and BaTi0.60Zr0.40O3
Разночтения заглавия :авие SCOPUS: Heat capacity study of relaxors BaTi0.65Zr0.35O 3 and BaTi0.60Zr0.40O3
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2006. - Vol. 18, Is. 17. - P.4407-4416. - ISSN 0953-8984, DOI 10.1088/0953-8984/18/17/026
Примечания : Cited References: 21
Предметные рубрики: CERAMICS
BA(TI1-XZRX)O-3
BATIO3
Ключевые слова (''Своб.индексиров.''): calorimetry--composition--data reduction--lead compounds--mathematical models--permittivity--specific heat--adiabatic calorimetry--burns temperature--diffuse anomalies--barium compounds
Аннотация: The heat capacity of two relaxors BaTi(1-x)ZrxO(3) (x = 0.35, 0.40) was measured using adiabatic calorimetry in the temperature range 100-360 K. The Cp(T) dependence of both compositions is characterized by the presence of two diffuse anomalies near the Burns temperature T-d and the temperature of the maximum in permittivity T-m in the temperature ranges 250-350 K and 120 200 K. The anomalous heat capacity near T-d was analysed taking into account the distribution of Zr concentration in nanoregions leading to the distribution of their transition temperatures into the polar phase. Excess heat capacity near Tm was discussed in the framework of the spherical random bond-random field model. The results are compared with the data obtained by the same procedures for PbMg1/3Nb2/3O3 studied experimentally earlier.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Sobol A. A., Shukshin V. E., Zaitsev A. I.
Заглавие : Raman spectroscopy of crystalline, glassy, and molten states of lead diborate
Место публикации : Opt. Spectrosc: Maik Nauka-Interperiodica Publishing, 2016. - Vol. 121, Is. 6. - P.810-818. - ISSN 0030400X (ISSN), DOI 10.1134/S0030400X16120249
Примечания : Cited References: 30. - This work was performed with financial support from RFBR, research project no. 13-02-00707.
Ключевые слова (''Своб.индексиров.''): boron--crystalline materials--raman scattering--single crystals--internal vibration--molten state--oxygen complexes--phonon lines--polarized raman spectra--glass
Аннотация: Polarized Raman spectra of single crystals of lead diborate, PbB4O7 (PBO), are studied in detail at 300 K. The TO-, LO-, and IO-phonon lines of the A1, A2, B1, and B2 symmetries in the Raman spectra of this compound are assigned. Changes in the Raman spectra of the internal vibrations of boron–oxygen complexes upon transition from the crystalline to the glassy and the molten states of PBO are observed. On the basis of the obtained results, the regularities in the formation of boron–oxygen complexes in glasses, melts, and crystals of the PbO · 2B2O3, SrO · 2B2O3, and Li2O · 2B2O3. diborate compositions are analyzed. © 2016, Pleiades Publishing, Ltd.
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